间接测量中重放射性核中子俘获截面——替代比率法

s过程中的放射性核素中子俘获截面对天体核合成和核素丰度有重大影响, 在直接测量异常困难的情况下, 替代比率法是获得放射性核素中子俘获截面数据的一种间接新方法。 简单介绍了替代比率法理论, 并简要论述了用替代比率法推导中重核区放射性核素中子俘获截面的可行性。 The radioactive nuclei neutron capture cross section is very important to nuclearsynthesis and nuclide abundance in s process, but it is difficult to be measured directly because of the target production. A new method, surrogate ratio method which is developed from surrogate method, could be used to determine the cross section of radioactive nuclei neutron capture. In this paper, the surrogate ratio method was introduced and the feasibility was discussed to deduce the desired neutron capture cross sections with surrogate ratio method.     

替代反应法测量锕系核(n,f)和(n,xn)截面

对于某些中子反应截面,在直接测量上存在困难。为了获得那些对核能发展极其重要的核数据,人们提出替代反应法,即利用带电粒子代替中子进行反应,从而实现中子反应截面间接测量的方法。现有替代反应一般采用非弹激发、转移等周边反应,涉及的角动量远比中子反应的大,需要理论修正,这造成了一定的困难。有鉴于此,提出利用轻带电离子的俘获反应作为替代反应,其复合核自旋与中子反应的相当,有效避免了自旋修正的困难。根据这个思路,采用236U的（α,f）和（α,2n）反应作为替代反应,成功提取了239Pu的（n,f）和（n,2n）反应截面,与ENDFB7评价库数据在误差范围内符合较好,表明了替代反应法的优越性,可以在核数据测量中推广应用。There are always difficulties in the direct measurement of reactions induced by neutron, in order to obtain the neutron induced nuclear reaction data which are extremely important for nuclear power development, the surrogate reaction method, which uses charged particles instead of neutron, was proposed. The existing surrogate reaction method generally chooses peripheral reaction as the surrogate reaction, such as inelastic scattering excitation or transfer reaction. As a result, the angular momentum involved is always far larger than the neutron induced reaction, which causes difficulties in the theoretical calculation. Because of this, we proposed to use light-ion capture reaction as the surrogate reaction, the compound nuclei spin is similar with that of the neutron induced reaction, so that the difficulties in spin correction can be effectively avoided. Based on this idea, the 239Pu(n, f) and (n, 2n) reaction cross sections were successfully extracted using 236U(α,f) and (α,2n) reactions as the surrogate reaction. The results coincide well with the data of ENDFB7 within the error range, which shows that the surrogate reaction method has its own superiority, and it can be applied in the measurement of nuclear data.     

88Y(n,2n)反应截面研究

本工作用相同复合系统的核反应替代法获得了入射中子能量在10.3MeV到17.4MeV区间不稳定靶核⁸⁸Y(n,2n)核反应截面,并把该结果同我们的理论计算结果及Prestwood等人的实验和理论计算结果进行了比较,比较结果表明这种替代测量法值得研究.     

14MeV中子(n,T)与(n,3He)反应截面的系统学研究

本文研究14MeV中子(n,T)和(n,³He)反应截面的系统学特性。在考虑奇偶效应的基础上,给出了截面的系统学公式,σ_u,q=(A^1/3+1)²aexp[β(N-Z+δ)/A]。用最小二乘法拟合得到奇偶核的经验参数对(n,T)反应,α,β分别为327.602,9.592和-24.495,-14.038。对(n,³He)反应,α,β分别为0.918和-11.340。利用这套参数计算的截面与实验值符合较好。此外,文中还讨论了反应的Ω值效应以及可能的反应机制。 关键词：     

基于(p,γ)-(γ,p)平衡近似的快质子俘获过程模型及其应用

在(p,γ)-(γ,p)平衡近似下,本文建立了简化的快质子俘获(rp)过程模型, 讨论了天体物理条件输入量 (即质子辐照时间、质子数密度及温度) 对rp过程的影响. 结合中国科学院近代物理研究所等时性质谱仪 (IMS) 上的最新实验数据, 本文进而分析了新测的缺中子原子核质量对rp过程的影响; 发现利用新测的⁴¹Ti质量, A=41处的丰度相较之前的计算结果增大了两个数量级, 而计算的相对丰度误差减小了近两个量级. 关键词： 快质子俘获过程 γ)-(γ,p)平衡')" href="#">(p,γ)-(γ,p)平衡 原子核质量 缺中子原子核     

14MeV中子引起的185Re(n,2n)184g,mRe和191Ir(n,2n)190Ir的核反应截面测量

利用活化方法测量了1?4MeV中子引起的¹⁸⁵Re(n,2n)^184gRe,¹⁸⁵Re(n,2n)^184mRe和¹⁹¹Ir(n,2n)¹⁹⁰Ir核反应的截面.中子能量E_n=(14.7±0.2)MeV时的实验结果分别为:(1817±85)mb,(390±18)mb和(2038±82)mb.并利用HFTT程序计算了中子能量在7—18MeV范围内的截面值,给出了其中两个核反应的激发函数曲线.     

一维贫铀/聚乙烯交替系统中D-T中子诱发的~(232)Th(n,γ)反应率的测定与分析

开展了钍样品装置内钍核参数的积分中子学基础研究.参考混合堆概念设计搭建了内部放置了钍样品的一维贫铀/聚乙烯交替系统装置,采用加速器D-T中子源模拟聚变堆芯,利用前期开发的离线伽马测量方法测定了不同位置、不同中子谱情况下的232Th(n,γ)反应率,不确定度约为5%.结果显示,聚乙烯对14.1 MeV中子的慢化作用可有效提升钍俘获率,且贫铀对钍俘获率也有显著提升作用.实验结果与主流核数据库计算结果的对比显示,ENDF/B-VI.6和JENDL-3.3数据库的计算值比实验值平均约大6%,而较新的ENDF/B-VII.0数据库的计算值比实验值平均约大4%.因此,相比于之前数据库的钍核数据,ENDF/B-VII.0的计算值与实验结果匹配得较好,可作为相关概念设计的推荐核数据库.     

50,40,46的(n,p)(n,α)和58Ni的(n,2n)(n,p)反应截面的测量

本文叙述了从13.50MeV到14.81MeV中子能区用活化法相对²⁷Al(n,α²⁴Na的反应截面,对⁵⁰Ti(n,α)⁴⁷Ca、⁴⁸Ti(n,p)⁴⁸Sc、⁴⁶Ti(n,p)⁴⁶Sc、⁵⁸Ni(n,2n)⁵⁷Ni、⁵⁸Ni(n,p)^58m+gCo五个反应截面的测量.并将所得的结果和其他作者的结果进行了比较.     

181Hf(n,γ)182Hf反应截面测量

在中国原子能科学研究院重水研究堆上用活化法对反应堆中子引起的181Hf (n,γ)182Hf反应截面进行了测量. 反应堆中样品照射位置的热中子与超热中子的通量比值约为10. 照射后样品中的182Hf/180Hf和 181Hf/180Hf的原子数比值是用热电离质谱测量的. 本工作以180Hf (n,γ)181Hf反应截面(14.80±0.60 b)为标准，测得的反应堆中子引起的181Hf (n,γ)182Hf反应截面值为80.0±5.6 b.     

100Mo(n2n)99Mo,96Mo(n,p)96Nb和92Mo(n,α)89m+gZr反应截面测量

本文报告了在E_n=13.40—14.79MeV中子能区用活化法以²⁷Al(n,α)²⁴Na截面为中子注量标准测行的¹⁰⁰Mo(n2n)⁹⁹Mo,⁹⁶Mo(n,p)⁹⁶Nb和⁹²Mo(n,α)^89m+gZr的反应截面,中子能量是用铌锆截面比法测定的.文中将实验测量值与理论计算值进行了比较,还对上述三个反应的截面进行了编评,给出了推荐的激发曲线.     

Excited states of 96Nb from the 96Zr(p,nγ)96Nb reaction

The γ-ray spectra of the ⁹⁶Zi(p, nγ)⁹⁶Nb reaction have been measured with Ge(Li) detectors at different bombarding proton energies between 1.3 and 5.1 MeV. γγ coincidences were observed at E_p = 4.7 and 5.0 MeV. On the basis of experimental results a level scheme of ⁹⁶Nb was deduced, and γ-threshold energies and γ-branching ratios were determined. Computed Hauser-Feshbach (p, n′) cross sections have been compared with experimental data obtained from the γ-ray measurements, and level spins and parities have been determined. The energies of ⁹⁶Nb levels were calculated on the basis of the parabolic rule, derived from the cluster-vibration model. The Racah multipole decomposition method was used also for the theoretical interpretation of several ⁹⁶Nb multiplet states.     

Study of (d, α) reactions on 94Zr and 96Zr

The nuclear structure of ⁹²Y and ⁹⁴Y has been investigated by the (d, α) reaction on ⁹⁴Zr and ⁹⁶Zr with 11.5 MeV deuterons. Some new levels have been seen in ⁹²Y and ⁹⁴Y. The angular distributions for these levels have been measured. A zero-range DWBA analysis has been carried out for these distributions and spin-parity assignments have been made for the new levels.     

Experimental and shell-model studies of the reactions 91Zr(d,p)92Zr and 90Zr(t,p)92Zr

The results of high-resolution studies of the ⁹¹Zr(d, p) reaction at E_d = 12 MeV and the ⁹⁰Zr(t, p) reaction at E_t = 11.85 MeV are presented. Absolute cross sections have been measured for both reactions and (d, p) spectroscopic factors determined. A comparison of these results with earlier data has been made, and although many of the previous assignments have been confirmed, many new features concerning the structure of ⁹²Zr have been discovered. Shell-model calculations have been performed for ⁹¹Zr and ⁹²Zr using a neutron space which includes the $\text{2}\text{d}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}$, $\text{3}\text{s}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}$, $\text{2}\text{d}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}$, $\text{1}\text{g}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}$ and $\text{1}\text{h}{}_{\mathrm{<mtext>11</mtext><mtext>2</mtext>}}$ orbits and a proton space comprising the $\text{1}\text{g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}$ and $\text{2}\text{p}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}$ orbits. Realistic proton-neutron and neutron-neutron interactions based on the Sussex matrix elements were used in the calculations. Spectroscopic factors have been calculated for the ⁹⁰Zr(d, p) and ⁹¹Zr(d, p) reactions and cross sections calculated for the ⁹⁰Zr(t, p) reaction. In general, good agreement between the theoretical and the experimental results has been obtained.     

中子与56Fe反应的理论计算

应用光学模型、核内级联模型、激子模型（含改进的Iwamoto-Harada模型）、统一的Hauser-Feshbach理论以及扭曲波玻恩近似理论,对入射能量在20 MeV以下中子与56Fe非弹性散射反应的γ产生截面、分立能级截面和总的非弹性散射截面进行计算,并与最新实验数据以及来自ENDF/B-VII、JEFF-3.1和JENDL-4库的评价数据进行比较和分析。结果显示,理论计算结果与实验数据符合较好,并且对于有些激发态的非弹性散射截面我们的计算结果优于ENDF/B-VII,JEFF-3.1和JENDL-4库的评价结果。The gamma production, level production and total inelastic scattering cross sections are calculated at incident neutron energy below 20 MeV. The optical model, the intra-nuclear cascade model, the exciton model (including improved Iwamoto-Harada model), the uni ed Hauser-Feshbach theory and the distorted wave Born approximation theory are used. Theoretical calculated results are compared with the recent experimental data and other evaluated data from ENDF/B-VII, JEFF-3.1, and JENDL-4. It is found that our calculated results agree with the experimental data and the calculated results for some level cross sections are more consistent with the related experimental data than the results from ENDF/B-VII, JEFF-3.1, and JENDL-4 data base.     

Low-lying levels of 92Nb from the 92Zr(3He,t) and 92Zr(3He,p2nγ) reactions

The structure of ⁹²Nb has been investigated using the 33.8 MeV ⁹²Zr(³He, t) and (³He, p2nγ) reactions. Several previously unobserved levels, including several belonging to the $\text{π(}\text{g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)ν(}\text{g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)}{}^{\mathrm{?1}}$ multiplet, are reported. The results are discussed in terms of the shell model.     

^106,110Pd （p,nγ）^106,110 Ag reactions at Ep = 6.0 - 7.7 MeV

This paper reports that the experimental excitation functions of reaction （p,n） are measured for ^106pd and ^110pd at proton energy Ep = 6.1 - 7.5 MeV and Ep = 6.0 - 7.7 MeV respectively. The off-resonance excitation functions were compared with calculation values of the statistical model. A new formula used to estimate the peak cross section of isobaric analogue resonance was tested and it was found that calculation values agree reasonably well with the present data within experimental error, which confirms that the excitation strength of isobaric analogue state in （p,n） reaction not only depends on its spin, but also proportionally increases with the projectile proton spatial transmission Tp and the spectroscopic factor S for reaction （d,p） on the same target.     

Single electron capture in collisions of N^q＋ （q = 5, 6, 7） ions with helium

Close-coupling calculations are carried out for cross sections of the single electron capture in collisions of N^q+ (q = 5, 6, 7) ions with helium atoms in the collision velocity range from 0.3 a.u. to 1.8 a.u. The relative importances of the single ionization (SI) to the single capture (SC) are investigated for the N^q+ (q = 5, 6, 7) projectiles, respectively. The SI/SC cross section ratio for the N⁷⁺ projectile obtained from our calculations is in excellent agreement with the experimental data. The ratio curves also show us distinct behaviours when the charge of the projectile is different. The partial electron capture cross sections for different projectiles indicate that the electron on the target He atom tends to be captured by the projectile into its lower orbital of the outer shell with the decreasing projectile charge.     

3He(4He)与H2分子碰撞的同位素效应研究

用公认精确度较高的密耦近似方法计算了入射能量E=05eV时惰性气体原子³He(⁴He)与H₂分子替代碰撞体系的转动激发碰撞截面.通过分析³He(⁴He)-H₂碰撞体系分波截面和微分截面的差异,总结出在氦原子的同位素替代情形下³He(⁴He)-H₂碰撞体系分波截面和微分截面随分波数增加和同位素原子质量改变的变化规律. 关键词： 散射截面 密耦方法 同位素替代 散射角