A～130过渡区核的高自旋态研究

评述了Ａ～１３０过渡区Ｉ、Ｘｅ、Ｃｓ和Ｂａ核的高自旋核结构研究．在这些核中观测到的极为丰富的核结构现象,如质子中子转排竞争、形状共存、带终结、带交叉延迟、Ｓｉｇｎａｔｕｒｅ反转和八极关联等与这些核的价质子、价中子都位于ｈ１１／２支壳及这些核易产生γ形变有关. The studies of high spins states of A ～130 transitional I,Xe,Cs and Ba nuclei are reviewed. The variety of nuclear structure, such as proton neutron alignment competition, shape coexistance, band termination, crossing delay, signature inversion, octupole correlation, etc. observed in these nuclei is closely related to that both the valence proton and neutron of these nuclei are located in the h 11/2 subsell and the nuclei are soft against the γ deformation.     

SD配对壳模型对质量数A~130区原子核的形状渡越研究(英文)

利用SD配对壳模型研究了质量数A~130区原子核的低激发态性质。为了减少参数,模型采用了等强度对力,取质子和中子对力强度等同近似,而非同类核子间的四极-四极相互作用强度取为同类核子间四极-四极相互作用强度的两倍。计算结果显示,模型的振动-转动和振动-γ不稳定运动的形状渡越特征与相互作用玻色子模型对应的形状相变特征基本吻合,从而说明SD配对壳模型是壳模型的一种合理近似。The SD-pair shell model is applied to analyze the evolution of low-lying states of even-even nuclei in A~130 mass region. In the model, the pairing and the quadrupole-quadrupole interactions are taken into account. The results show that there are clear signatures of the crossover from vibrational to rotational or from vibrational to the γ-soft shape phase.     

Quasiparticle structure of superheavy nuclei in α-decay chains of ~(285)Fl and ~(291,293)Lv

Two mean-field potentials, Woods-Saxon and Skyrme based potentials, are used to calculate the energies of low-lying one-quasiparticle states. The spectra of the low-lying states and the α-decay spectra of nuclei belonging to the α-decay chains of ~(285)Fl and ~(291,293)Lv are calculated and compared with the available experimental data. Dependence of the splitting of the pseudospin doublets and of the energies of the unique parity neutron one-quasiparticle states on the mean field potential are discussed. As shown, the α-decay spectra could be different in the α-decay chain and at the direct production of the nucleus in a fusion reaction.     

Lifetimes of Excited Levels in ^131Ce

The fusion-evaporation reaction ^116Sn (^19F, p3n)^131 Ce at projectile energy of 95 MeV is used to populate high spin states in ^131Ce. The de-exciting γ-rays are detected in γ-γ coincidence measurement with Compton-suppressed BGO-HPGe detectors. Level lifetimes of ^131 Ce were determined by using the Doppler shift attenuation method.The experimental results indicate that collectivity of ^131 Ce is reduced relative to that of ^130Ce and it follows that deformation decreases with increase of the neutron number on the basis of systematic comparison of transition quadrupole moments for the light cerium isotopes.     

122~125Sn中子谱因子的实验研究

多个Sn同位素位于慢速中子俘获（s-）过程路径上,其中子谱因子可用于计算ASn（n,γ） A+1Sn直接辐射俘获的天体物理反应率,并可研究Sn同位素对s-过程核合成的贡献。本工作在中国原子能科学研究院HI-13串列加速器Q3D磁谱仪上,对实验室系下8°~66°范围内的122,124Sn（d,p）和（p,d）单中子转移反应角分布进行了测量。利用DWBA理论计算了转移反应角分布,并提取了122-125Sn的基态以及123,125Sn第一激发态的中子谱因子。其中,122Sn和124Sn的基态中子谱因子是首次从实验上获得。由于本工作成功鉴别开了123,125Sn的基态和第一激发态的效应,因此给出的谱因子比前人的结果更可信。Several Tin isotopes are on the path of slow neutron capture (s-) process, and the direct components of (n, γ) reactions can be derived from their neutron spectroscopic factors. In the present work, the angular distributions of 122,124Sn(p, d) and (d, p) reactions are obtained using the high-precision Q3D magnetic spectrograph in Beijing HI-13 tandem accelerator in China Institute of Atomic Energy. The distorted-wave Born approximation (DWBA) calculations are performed to extract the neutron spectroscopic factors of the ground state of 122-125Sn and the first excited state of 123,125Sn. The neutron spectroscopic factors of the ground state of 122Sn and 124Sn are firstly obtained in this work. As the events of the ground state and first excited state of 123,125Sn can be distinguished clearly by our experiment, the neutron spectroscopic factories of 123,125Sn are more reliable.     

中子注量率波动修正因子及其应用

在中子核反应研究中,尤其是在利用活化法进行中子核反应截面测量研究时,需要准确测量样品辐照的中子注量。监督反应标准截面法简便可行,在一些核反应截面测量研究中经常用来定量样品辐照的中子注量。在利用监督片核反应剩余核的放射性活度计算平均中子注量率时,中子注量率波动修正因子是一个很重要的参数。对中子注量率波动修正因子进行了详细阐述,通过理论推导给出了中子注量率波动修正因子的定义,从实际应用出发讨论了中子注量率波动修正因子的使用条件和监督反应的选择原则。Incident neutron flux has to be measured accurately in the neutron reaction study especially in the neutron reaction cross-section measurement with activation method. Average neutron flux in the irradiated sample is usually determined by the monitor reaction with reference cross-section values. However, the average incident neutron flux, based on the radioactivity of the residual nuclei produced in the monitor reaction, is dependent upon the neutron flux fluctuation. In the procedure of the average neutron flux calculation, the correction factor for the neutron flux fluctuation plays a key role. In this paper, definition of the neutron flux fluctuation correction factor is inferred heoretically. The selection principles of the monitor reaction and the utilization of the correction factor have been discussed.     

Low—Lying States of the A^＋B^—A^＋B^— Coulomb systems in Two—Dimensional Quantum Dots

The features of the low-lying spectra of four-body A B-A B- systems have been dedudced based on symmetry,Using the method of few-body physics,we calculate the energy spectra of A B-A B- systems in a harmonic quantum dot.We find tha t the biexcition in a two-dimensional quantum dot may have other bound excited states and the quantum mechanical symmetry plays a crucial role in determining the energy levels and structures of the low-lying the quantum mechanical symmetry plays a crucial role in determining the energy levels and structures of the low-lying states.     

Description of spectrum and electromagnetic transitions in ~(94)Mo through the proton-neutron interacting boson model

We investigated the properties of low-lying states in ~(94)Mo within the framework of the proton-neutron interacting boson model(IBM-2), with special focus on the characteristics of mixed-symmetry states. We calculated level energies and M1 and E2 transition strengths. The IBM-2 results agree with the available quantitative and qualitative experimental data on ~(94)Mo. The properties of mixed-symmetry states can be well described by IBM-2 given that the energy of the d proton boson is different from that of the neutron boson, especially for the transition of B(M1, 4_2~+→ 4_1~+).     

丰中子锰同位素的壳模型计算

利用球形壳模型和投影壳模型两种方法对Z≤28,N=40附近pf壳的丰中子核素的结构进行了一系列的研究。以丰中子的锰同位素为例讨论了对奇奇核58,60Mn的两种壳模型计算结果。结果显示,两种理论方法都很好地再现了58,60Mn实验上观测到的从低激发到高自旋态的能级。在对这两个同位素由中子g_9/2轨道闯入所产生的负宇称转动带进行描述时,两种理论计算也得到了一致的结果。通过对比,阐明了两种壳模型方法及其采用的有效相互作用在该丰中子核区的适用性,特别强调了中子g_9/2轨道的激发对于pf壳Z≤28丰中子核素结构的重要性。Recently,we have carried out a series of studies on the structures of pf shell neutron-rich nuclei around N=40 using the spherical shell model and the projected shell model respectively.As an example,these two types of shell model calculations for the neutron-rich odd-odd isotopes 58,60Mn are discussed in this paper.The results show that both the calculations reproduce the observed experimental energy levels from the lowexcitation states to the high-spin ones in 58,60Mn.Consistent results are also obtained by these two theoretical calculations when describing the negative-parity rotational band derived from the intruder neutron g_9/2 orbital in both isotopes.Through comparison,we show the applicability of these two shell model methods and the adopted effective interactions in the present neutron-rich mass region.The significance of the excitations from neutron g_9/2 orbital to the structures of the neutron-rich nuclei in pf shell with Z≤28 are especially emphasized in this paper.     

缺中子核素101In低位同核异能态的首次观测

在兰州重离子加速器冷却储存环（HIRFL-CSR）上,用初级束流112Sn35+轰击了靶厚约10 mm的Be靶,产生了101In的基态和低位同核异能态。这些实验产生的碎片每25 s经过放射性束流线RIBLL2的筛选后注入到实验环CSRe中,利用飞行时间探测器测量离子在CSRe中的回旋周期。在此次实验中,磁场晃动会导致离子在环内的循环周期发生改变,传统的离子鉴别方法难以完成大部分离子的鉴别。通过发展和运用单次注入离子鉴别这一新的离子鉴别方法,有效地消除了磁场晃动对于离子鉴别的影响,并清楚地将101In基态和低位同核异能态鉴别出来,从而首次在实验中观测到101In的低位同核异能态。实验得到的激发能与理论外推值在112 keV的误差范围内一致,其低位同核异能态的寿命大于200 μs。Isochronous mass spectrometry has been applied to 112Sn projectile fragments at the HIRFL-CSR facility in Lanzhou. To produce short-lived nuclei of interest, we used projectile fragmentation of 112Sn35+ primary beams in a~10 mm thick 9Be production target. The fragments were selected and analyzed by RIBLL2 and injected into the experimental storage ring(CSRe) every 25 s. To measure revolution times of stored ions,we used a Time-Of-Flight detector installed in CSRe. A new particle identification method was developed to distinguish ions on the measured revolution time spectrum for each injection. Based on this method, the shifts of the revolution time due to instable dipole magnet fields can be corrected and the ground and isomeric states of 101In have been well-resolved. The measured excitation energy is consistent with the theoretical value in the error range of 112 keV. The lifetime of the isomeric states of 101In is more than 200 μs.     

Probing Shell Correction at High Spin by Neutron Emission of Doubly Magic Nuclei 208Pb and 132Sn

Shell effects in particle emission for two doubly magic nuclei ^132Sn and ^208pb were studied in the framework of Smoluchowski equation taking into account temperature and spin-dependent shell correction. It is shown that the shelle ffects in the emission of pre-scission neutrons are sensitive to the spin dependence of the shell correction at a moderate excitation energy. Therefore, we propose to use neutron multiplicity as an observable to probe the shell correction at high spins.     

香港大学在束伽玛谱学研究与新一代伽玛探测器阵列(英文)

探索原子核的壳层演化,验证奇特核的幻数结构是香港大学核物理研究的重要方向。目前,科研团队利用在束伽玛谱学技术已经研究了30Ne的N=20幻数消失和78Ni（Z=28,N=50）附近原子核的双幻数结构,而即将开展的53,56Ca在束伽玛谱学实验会对新幻数N=34的定量研究,以及到N=40核的壳层演化提供重要的数据。下一步的研究目标是探索100Sn（N=Z=50）的奇特结构,特别是研究它的第一个2+激发态与其邻近原子核的低激发态性质。100Sn处于质子滴线以及核天体快质子俘获路径上,因此,它的幻数结构及其临近原子核单粒子性能研究将会极大增强对核力和核合成机制的认识。为了进一步提高物理实验统计,香港大学在数量上增加了30% NaI（Tl）晶体从而全面升级了DALI2伽玛探测阵列。此外,为了探索远离稳定线核区的新物理,开展更高精度在束伽玛谱学实验,香港大学与中国科学院近代物理研究所、中国原子能科学研究院计划合作研制基于溴化镧晶体的新一代伽玛探测器阵列。这套阵列主要在兰州重离子加速器（HIRFL）和将来建成的强流重离子加速器（HIAF）等大科学装置上开展实验,从而在奇特核研究方面取得大量重要的成果,促进科研人员全面认识、理解核力以及天体核合成过程。Exploring the evolution of shell closures and examining the magicity of extremely exotic nuclei are the main research interests of HKU (University of Hong Kong) experimental nuclear physics group. The group has employed in-beam gamma-ray spectroscopy technique to investigate the vanishing of N=20 magicity in 30Ne (N=20) and the strong magicity in nuclei around 78Ni (Z=28, N=50). The approved future's experiment on spectroscopy of 53,56Ca, proposed by HKU, will give quantitative information for the "magic index" of N=34 and shell evolution toward N=40. The next goal is to investigate the structure of 100Sn (N=Z=50), particularly the energy of the first 2+ state, and the low-lying states in the neighboring nuclei. 100Sn lies on the proton drip-line and on the astrophysical rp-process path. Characterizing the magicity of 100Sn and the nature of single-particle states in its neighboring nuclei is therefore essential to the fundamental understanding of nuclear forces and nucleo-synthesis. To significantly increase the data statistics for our physics goals, HKU group has prepared the upgrade of gamma-ray spectrometer DALI2 with 30% more NaI(Tl) detectors integrated into a new array configuration. On the other hand, next significant insights into the structure of nuclei would require new gamma-ray detection array capable for higher precision gamma-ray spectroscopy. HKU group in collaboration with IMP and CIAE therefore proposes to construct a new-generation gamma-ray detection array based on the novel scintillator LaBr₃(Ce) to explore the new physics in nuclei far from the valley of stability. Utilizing the radioactive beams at the Chinese large-scale facilities such as the Heavy Ion Research Facility in Lanzhou (HIRFL) in IMP and the future's High Intensity heavy-ion Accelerator Facility (HIAF), this novel LaBr₃(Ce) array would lead to a significant boost to the frontiers of exotic-nuclei research, which will guide scientists towards the comprehensive and even beyond-traditional understanding of nuclear forces and nucleosynthesis.     

Interaction of 11 MeV neutrons with Y

Differential cross section for scattering of 11 MeV neutrons by ⁸⁹Y were measured using the Ohio University beam swinger time-of-flight facility. Measurements were taken in the angular range between 15° and 145°. Empirical optical model parameters have been obtained from the measured elastic scattering data. Deformation parameters were obtained for low-lying excited states using these optical-model parameters in a DWBA collective formalism. A comparison with deformation parameters in neighboring even-even nuclei ⁸⁸Sr and ⁹⁰Zr is presented. The weak-coupling model is used to describe neutron scattering to low-lying states in ⁸⁹Y.     

∧超核中单粒子谱的自旋及赝自旋对称性研究(英文)

原子核中单粒子谱的自旋和赝自旋对称性对核结构的研究具有重要意义。本文基于相对论平均场理论,以132Sn,_∧133Sn,及_2∧134Sn为例,研究了∧超核中单∧谱和单中子谱的自旋和赝自旋对称性。研究发现,单∧谱的自旋对称性保持得相当好,与实验观测一致;而其赝自旋对称性只是近似保持,与核子谱的情况类似。此外,还研究了∧超子对中子谱的杂质效应,发现∧超子使中子谱的自旋对称性变差,赝自旋对称性变好。Spin and pseudospin symmetries in the single-particle spectra of atomic nuclei are of great significance for the study of nuclear structure. In this work, taking 132Sn, _∧133Sn, and _2∧134Sn as examples, the spin and pseudospin symmetries in ∧ hypernuclei are studied by using the relativistic mean-field model. For the single-∧ spectra, results show that the spin symmetry maintains well while the pseudospin symmetry is approximately conserved. Besides, as impurities, the ∧ hyperons worsen the spin symmetry of single-neutron spectra while improve the pseudospin symmetry.     

Isospin Dependence in Nuclear Multifragmentation Within Site Percolation and Nucleation Pictures

The isospin dependence, recently observed in Sn + Sn reactions at 40 MeV/nucleon, is discussed within the framework of two simple nuclear multifragmentation models, namely the site percolation and the nucleation-evaporation models. It is shown that both the models are able to discriminate between ¹¹²Sn+ ¹¹²Sn and ¹²⁴Sn+ ¹²⁴Sn reactions. The nucleation-evaporation model succeeds to reproduce nicely the experimental data, but the site percolation model fails in doing that, even if the cluster noncompactive effect is taken into account. The calculations indicate that the data are originated mainly from a single source.     

2,6-双(三甲基锡)-4,8-双(2-乙基己氧基)苯并[1,2-b∶4,5-b']二噻吩的合成与多核NMR研究

以苯并[1,2-b∶4,5-b´]二噻吩-4,8-二酮为原料合成了一种聚合物太阳能电池材料的单体2,6-双(三甲基锡)-4,8-双(2-乙基己氧基)苯并[1,2-b∶4,5-b´]二噻吩. 通过多核1D和2D NMR技术（包括1D ¹H、¹³C、¹¹⁹Sn、¹¹⁷Sn NMR、DEPT、选择性1D TOCSY及2D¹H-¹H COSY、gHSQC、gHMBC）表征了目标分子结构,完成了 ¹H、¹³C、¹¹⁹Sn 与¹¹⁷Sn NMR化学位移归属,并探讨了该化合物的NMR谱线特征.