The dependence of the Fe <Emphasis Type="Italic">K</Emphasis><Subscript><Emphasis Type="BoldItalic">α</Emphasis></Subscript> yield on the chirp of the femtosecond exciting laser pulse

The hard X-ray yield generated with femtosecond laser pulses is studied for differently chirped irradiating laser pulses. The radiation of a Ti:sapphire CPA laser system (29 fs, 750 μJ, 1 kHz) is focused onto an iron containing solid state target producing incoherent hard X-ray radiation, Bremsstrahlung as well as target-specific K_α and K_β lines. The hard X-ray yield has been optimized by introducing negative and positive group delay dispersion (GDD) and third order dispersion (TOD) to the femtosecond laser pulse. The K_α yield could be enhanced by a factor of 1.7 and reached 1.9×10⁸ Fe K_α photons/s in 4π with the laser pulse positively chirped, and 1.5×10⁸ Fe K_α photons/s with the pulse negatively chirped. When the pulse energy is lowered to about 400 μJ the yield maximum at negative chirp vanishes and only the maximum at positive chirp remains. We explain this behavior with an increased electron temperature caused by the induced GDD and TOD in the pulse. PACS 42.65.Re; 52.38.Ph; 52.50.Jm     

K<Subscript><Emphasis Type="Italic">α</Emphasis></Subscript> x-ray emission characterization of 100 Hz, 15 mJ femtosecond laser system with high contrast ratio

We report K _α x-ray production with a high energy (110 mJ per pulse at 800 nm before compression/15 mJ at 400 nm after compression), high repetition rate (100 Hz), and high pulse contrast (better than 10⁻⁹ at 400 nm) laser system. To develop laser-based x-ray sources for biomedical imaging requires to use high-energy and high-power ultrafast laser system where compression is achieved under vacuum. Using this type of laser system, we demonstrate long-term stability of the x-ray yield, conversion efficiency higher than 1.5×10⁻⁵ with a Mo target, and the x-ray spot size close to the optical focal spot. This high-repetition K _α x-ray source can be very useful for x-ray phase-contrast imaging. S. Fourmaux and C. Serbanescu contributed equally to this work.     

Femtosecond hard X-ray plasma sources with a kilohertz repetition rate

Laser-driven plasma sources of femtosecond hard X-ray pulses have found widespread application in ultrafast X-ray diffraction. The recent development of plasma sources working at kilohertz repetition rates has allowed for diffraction experiments with strongly improved sensitivity, now revealing subtle fully reversible changes of the geometry of crystal lattices. We provide a brief review of this development and present a novel plasma source with an optimized mechanical and optical design, providing a high flux of several 10¹⁰ photons/s at the Cu-Kα energy of 8.04 keV and a pulse duration of ≤300 fs. First experiments, including the generation of Debye–Scherrer diffraction patterns from Si powder, demonstrate the high performance of this source.     

A comparative study of the ionic keV X-ray line emission from plasma produced by the femtosecond,picosecond and nanosecond duration laser pulses

We report here an experimental study of the ionic keV X-ray line emission from magnesium plasma produced by laser pulses of three widely different pulse durations (FWHM) of 45 fs, 25 ps and 3 ns, at a constant laser fluence of ∼1.5 × 10⁴ J cm^− 2. It is observed that the X-ray yield of the resonance lines from the higher ionization states such as H- and He-like ions decreases on decreasing the laser pulse duration, even though the peak laser intensities of 3.5 × 10¹⁷ W cm^− 2 for the 45 fs pulses and 6.2 × 10¹⁴ W cm^− 2 for the 25 ps pulses are much higher than 5 × 10¹² W cm^− 2 for the 3 ns laser pulse. The results were explained in terms of the ionization equilibrium time for different ionization states in the heated plasma. The study can be useful to make optimum choice of the laser pulse duration to produce short pulse intense X-ray line emission from the plasma and to get the knowledge of the degree of ionization in the plasma.     

XUV generation from plasma produced by a XeCl excimer laser on a Cu target

Summary We present a detailed study of XUV and soft X-ray emission from Cu plasma produced by an excimer laser at intensitiesI _L≦8·10¹¹ W/cm². The XeCl excimer laser (ψ≈308 nm) delivers pulses with energyE _L≈2.3 J, temporal durationt _L≈100 ns and brightnessB≧10¹⁴ W/cm² sr. We recorded a spectral conversion efficiency η=0.5% eV⁻¹ forI _L=4·10¹¹W/cm² in the aluminium window at 73eV with a harder X-ray tail around ≈400eV. We also measured the dependence of X-ray signal on laser intensity and viewing angle. Experimental results have been compared with some analytical laser-plasma interaction models.     

Efficient high-repetition-rate fs-laser based X-ray source

The generation of [_Fe]K line radiation has been studied on a compact, ultrashort, laser based hard X-ray source, particularly suited for high-repetition-rate laser systems (1 to >10 kHz). Sub-millijoule, 25 fs Ti:sapphire laser pulses are applied to generate hard X-ray radiation on a commercially available ferric audio cassette tape target. Spectroscopic investigations reveal strong iron K emission in addition to a weak bremsstrahlung continuum. Under single exposure and single pulse conditions the X-ray yield is low. Energy conversion efficiencies of about _K=2×10^-7 are observed. Prepulse and multiple shot exposure techniques, both successfully used with high energy/low repetition rate systems, are investigated for these low energy/high repetition rate conditions. Depending on the applied pulse energy and intensity, the X-ray yield can be enhanced by more than three orders of magnitude. Photon fluxes exceeding 2×10⁹Kphotons/s are generated with the presented tape target yielding conversion efficiencies of nearly _K=10^-5. PACS 42.65.-k; 52.38.Ph; 52.50.Jm     

Enhanced soft X-ray emission from carbon nanofibers irradiated with ultra-short laser pulses

A comparative experimental study of the X-ray emission in the water-window spectral region has been performed using carbon nanofibers (CNFs) of different sizes and graphite plate targets, irradiated with ultra-short (Ti:sapphire) laser pulses. More than an order of magnitude enhancement in the X-ray yield is observed from CNFs of 60-nm diameter with respect to graphite targets. The X-ray emission from CNFs of 160-nm diameter was also high. The integrated X-ray yield of these carbon-based targets scales with the laser intensity (I _L) as I_L ^{~ 1.3-1.4}I_{\mathrm{L}}^{\sim 1.3-1.4} in the intensity range of 4×10¹⁶–4×10¹⁷ W/cm². The effect of the laser pulse duration on the X-ray emission from the CNFs was also studied by varying the pulse duration from 45 fs up to 3 ps at a constant fluence of 2×10⁴ J/cm². The optimum laser pulse duration for maximum X-ray emission increases with the diameter of the CNFs used. The results are explained from physical considerations of heating and hydrodynamic expansion of the CNF plasma in which resonance field enhancement takes place while passing through two times the critical density. The results add to the efforts towards achieving an efficient low-cost water-window X-ray source for microscopy.     

Femtosecond laser plasma in CaF<Subscript>2</Subscript> crystal microchannel and effective generation of characteristic X-ray radiation

The dependence of the characteristic X-ray radiation yield from CaF₂ crystal on the formed microchannel depth under highly intensive (I ∼ 3 × 10¹⁵ W/cm²) laser pulses with different contrast was obtained. The maximum of the characteristic X-ray radiation yield at these experimental conditions corresponded to the microchannel depth of 30–50 μm. The efficiency of the laser radiation conversion to the characteristic X-ray radiation increased from 6 × 10⁻⁸ for the surface up to 10⁻⁷ in the microchannel. The dependence of the characteristic X-ray radiation yield on the viewing angle showed that the source of X-ray radiation was located near the surface inside the microchannel.     

Spatial characteristics of Kα radiation from weakly relativistic laser plasmas

The spatial dependence of K _α emission generated from laser-produced hot electrons is investigated experimentally and theoretically. In addition, the conversion efficiency of K _α production as a function of laser intensity is measured and compared with modeling results. We use the terawatt Ti:sapphire laser at MPQ and vary the peak intensity from 10¹⁵ to 10¹⁸ W/cm² with a pulse duration of 200 fs. A solid Cu target is placed at various positions in the laser focus, which allows one to vary the intensity but keep the total energy on the target constant. When the target is near best focus, the FWHM of the K _α emission, measured using a knife-edge, is considerably larger than the FWHM of the laser intensity. In measuring the efficiency of K _α production using the fundamental wavelength of the laser, a clear maximum of K _α emission is observed at a position away from best focus, where the peak intensity is down by more than an order of magnitude from the value at best focus. When the second harmonic of the laser is used, the K _α emission is peaked near best focus. The K _α emission from layer targets is used to obtain an estimate of the temperature of the hot electrons. Modeling of K _α production, using a Monte Carlo electron/photon transport code, shows the relationship between incident electron energy and the emitted K _α emission. Efficient K _α generation from the low-intensity wings of the laser pulse contributes to the large spot size of the K _α emission. The lower electron temperatures that are expected for the second harmonic explain the differences in the location of maximum K _α emission for the two wavelengths. We discuss the use of K _α emission in photoionizing inner-shell electrons with the goal of achieving X-ray lasing at short wavelengths. Received: 6 April 1999 / Revised version: 31 May 1999 / Published online: 11 August 1999     

Mechanically driven millimeter source of nanosecond X-ray pulses

The emission of nanosecond pulses of ≈20 keV photons having a total energy of GeVs which are generated by peeling millimeter wide strips of pressure sensitive adhesive (PSA) tape in a partial pressure of air (≈10⁻³ Torr) is demonstrated. The X-ray spectrum is similar to that obtained by peeling much wider bands of PSA, implying that the characteristic length for the sequence of processes that govern this phenomenon is less than 1 mm. These experiments demonstrate that MEMS-type X-ray generators are technologically feasible.     

Growth velocity and the topography of Ni-Zn binary alloy electrodeposits

We show that the electrodeposition of Ni-Zn alloys at the lowest growth velocities, v < 0.5μm/s, exclusively proceeds from an abnormal co-deposition phenomenon. The growth process in this v region greatly depends on the initial [Co²⁺] concentration of the film deposition bath. A theoretical approach of this process including the role of the saturation surface roughness of the alloy, , leads to an estimation of the transport properties of the ad-atoms involved during the deposit formation. Their surface diffusion coefficient varying between 1.76×10^-10 and 2.40×10^-8 cm^-2/s exhibits a minimal value, D _s = 2.10×10^-10 cm^-2/s located between v = 0.17 and 0.35μm/s. The spatial scaling analysis of the local roughness, σ, examined according to the power-law σ≈L ^α reveals that the resulting roughness exponents concurs with the Kardar-Parisi-Zhang dynamics including the restricted surface diffusion. Two main v regions leads to different fractal textural features of the alloy film surface. Below 0.10 μm/s, the roughness exponent obtained is α≈ 0.6, depicting a limited ad-atom mobility. Over v = 0.30μm/s, this exponent stabilises at α≈ 0.82, indicating an increase of the surface diffusion. Received 16 August 2000 and Received in final form 20 June 2001     

Muon catalyzed fusion and muon to 3He transfer in solid T2 studied by X-ray and neutron detection

X-ray and neutron measurements were carried out for muon catalyzed fusion and related phenomena in solid T₂. The X-ray originated from the μ^- to α sticking in muon catalyzed fusion; t + t + μ ^- → (μ ^- α) + 2n was measured for the first time, yielding K _α X-ray intensity of (μα) atom and the intensity ratio of K _β to K _α . Utilizing the phenomena of ³He accumulation in solid T₂, the X-ray in the μ^- transfer process from (tμ) to ³He was detected, providing a formation rate and radiative decay branching-ratio of (t ³Heμ) molecule. From fusion neutron measurements, estimated values were obtained for (ttμ) molecular formation rate as well as sticking probability ω_t in ttμ fusion. A possible new insight in t + t fusion reaction process at a low energy limit is also obtained. This revised version was published online in August 2006 with corrections to the Cover Date.     

超短脉冲强激光与固体靶相互作用中Kα射线的实验研究

在相对论激光强度下，对p偏振30 fs激光与固体Cu靶相互作用中产生的Kα射线进行了实验研究.采用刀边成像技术和单光子计数X射线CCD相结合的探测装置，在单发激光脉冲打靶时同时得到X射线源的尺寸、能谱以及Kα光子的转换效率等多种信息.实验结果与Reich等人的理论计算结果有明显的差异，Kα光子的能量转换效率在激光功率密度为1.6×10¹⁸W/cm²的条件下达到最大值7.08×10^-6/sr.根据这一结果并结合蒙特卡罗程序，推断出在这一聚焦光强下激光能量转换为前向超热电子的效率约为10%.     

An incoherent sub-picosecond X-ray source for time-resolved X-ray-diffraction experiments

Ultrashort bursts of K _α X-ray radiation were generated from fs-laser-produced plasmas. A complete experimental characterization of the X-ray source in terms of spectral, spatial, and temporal properties was performed. The pulse width of the K _α burst is shorter than 250 fs. The time-resolved evolution of a shock wave launched by a synchronized laser pulse in InSb was investigated. The transient change of the rocking curve yields detailed information on the structural changes. Received: 29 June 2000 / Published online: 22 November 2000     

超强激光与Ar团簇相互作用中X射线的研究

本文主要研究了超强超短激光与Ar团簇相互作用过程中X射线能谱、K壳层光子产额、能量转换效率以及激光对比度对X射线光子产额的影响.实验中得到K壳层的光子产额约为1× 10¹¹/发,能量转换效率约为2.8× 10^-5．同时观测到较强预脉冲离化团簇会导致预电离,产生膨胀等离子体,然而主脉冲与膨胀的等离子体相互作用的强度较未膨胀时降低了,从而导致K壳层光子产额降低,而使用高对比度的激光能增加X射线光子产额.     

Characteristics of a multi-keV monochromatic point x-ray source based on vacuum diode with laser-produced plasma as cathode

Temporal, spatial and spectral characteristics of a multi-keV monochromatic point x-ray source based on vacuum diode with laser-produced plasma as cathode are presented. Electrons from a laser-produced aluminium plasma were accelerated towards a conical point tip titanium anode to generate K-shell x-ray radiation. Approximately 10₁₀ photons/pulse were generated in x-ray pulses of ∼18 to ∼28 ns duration from a source of ∼300 μm diameter, athυ = 4.51 keV (K _α emission of titanium), with a brightness of ∼10²⁰ photons/cm²/s/sr. This was sufficient to record single-shot x-ray radiographs of physical objects on a DEF-5 x-ray film kept at a distance of up to ∼10 cm.     

Nonlinear refraction of silver nanowires from nanosecond to femtosecond laser excitation

In order to investigate the effect of pulse width and solvent on the nonlinear properties of metal nanostructures, silver nanowires were fabricated in a direct current electric field (DCEF) using a solid-state ionic method and characterized by transmission electron microscopy (TEM) and X-ray diffraction (XRD). The nonlinear refractive index (γ) of silver nanowires suspended in ethanol was measured using the Z-scan technique and laser radiation of various (femto-, pico-, and nanosecond) pulse durations. Experimental results indicated that silver nanowires have obvious positive refractive nonlinearities and γ (the Kerr-induced self-focusing) increases as the pulse duration increases from 7.4×10⁻⁸ cm²/GW at 110 fs to 1.6×10⁻⁴ cm²/GW at 8 ns, due to the additional influence of the atomic reorientational Kerr effect in the case of longer pulses. Due to the solvent dependence of the nonlinear behavior of the silver nanowires, the nonlinear absorption and refraction of silver nanowires suspended in de-ionized water are smaller than those of silver samples suspended in ethanol. The thermal nonlinearities are insignificant in our experimental conditions.     

A diode-pumped, frequency-doubled, tunable single-mode quasi-continuous-wave Yb:YAG laser emitting 70 W peak power at 515 nm

An efficient pumping scheme for a quasi-continuous-wave diode-pumped Yb:YAG laser is presented. Single-mode operation and fine wavelength tuning are assured by the use of a rubidium titanyl phosphate (RTP) Fabry–Perot étalon. When frequency doubled, the 200–420 μs duration pulses reach a peak power of 70 W at a wavelength of 515 nm. The TEM₀₀ beam is nearly diffraction limited with an M ² factor of 1.06 at full power. The tuning range spans from 512 to 520 nm and the pulse to pulse frequency stability is on the order of ±10 MHz. Laboratoire Aimé Cotton is associated with Université Paris Sud 11.     

Multifilamentation of femtosecond laser pulses propagating in?turbulent air near the ground

The propagation of femtosecond laser pulses in turbulent air near the ground is analyzed. Confining to a power regime distinctly above the critical power for self-focusing, i.e. P≈100P _cr, and concentrating on initial peak intensities around 2.5×10¹¹W/cm², the onset and early evolution of multiple filaments are addressed. Making use of the turbulence phase-screen method, numerical simulations of the pulse propagation indicate that turbulence fields with spatial scales below 6 mm are able to induce the onset of multifilamentation. An analytical linear plane wave perturbation model of the underlying modulation instability of the pulse front is introduced in support of the computational results. By this means, insight into the amplification of an initial perturbation of the pulse front from the point of view of the spatial frequency domain is given.     

Fast electron energy deposition in aluminium foils: Resistive vs. drag heating

The high current electron beam losses have been studied experimentally with 0.7 J, 40 fs, 6 10¹⁹ Wcm^-2 laser pulses interacting with Al foils of thicknesses 10-200 μm. The fast electron beam characteristics and the foil temperature were measured by recording the intensity of the electromagnetic emission from the foils rear side at two different wavelengths in the optical domain, ≈407 nm (the second harmonic of the laser light) and ≈500 nm. The experimentally observed fast electron distribution contains two components: one relativistic tail made of very energetic (T _h ^tail ≈ 10 MeV) and highly collimated (7° ± 3°) electrons, carrying a small amount of energy (less than 1% of the laser energy), and another, the bulk of the accelerated electrons, containing lower-energy (T _h ^bulk=500 ± 100 keV) more divergent electrons (35 ± 5°), which transports about 35% of the laser energy. The relativistic component manifests itself by the coherent 2ω₀ emission due to the modulation of the electron density in the interaction zone. The bulk component induces a strong target heating producing measurable yields of thermal emission from the foils rear side. Our data and modeling demonstrate two mechanisms of fast electron energy deposition: resistive heating due to the neutralizing return current and collisions of fast electrons with plasma electrons. The resistive mechanism is more important at shallow target depths, representing an heating rate of 100 eV per Joule of laser energy at 15 μm. Beyond that depth, because of the beam divergence, the incident current goes under 10¹² Acm^-2 and the collisional heating becomes more important than the resistive heating. The heating rate is of only 1.5 eV per Joule at 50 μm depth.