Behavior of aluminum near an ultimate theoretical strength in experiments with femtosecond laser pulses

The dynamics of the motion of the free surface of micron and submicron films under the action of a compression pulse excited in the process of femtosecond laser heating of the surface layer of a target has been investigated by femtosecond interferometric microscopy. The relation between the velocity of the shock wave and the particle velocity behind its front indicates the shock compression to 9–13 GPa is elastic in this duration range. This is also confirmed by the small (≤1 ps) time of an increase in the parameters in the shock wave. Shear stresses reached in this process are close to their estimated ultimate values for aluminum. The spall strength determined at a strain rate of 10⁹ s⁻¹ and a spall thickness of 250–300 nm is larger than half the ultimate strength of aluminum.     

Surfing and generation of cosmic rays in relativistic shock waves

We consider the problem of cosmic-ray generation through the surfing acceleration of charged particles in relativistic magnetosonic shock waves (the branch of fast magnetic sound) propagating in magnetized space plasmas. The dependence of the particle surfing acceleration efficiency on the angle θ _Bn between the normal to the shock front plane and the magnetic field vector in the plasma upstream of the shock is analyzed in detail. We show that for angles satisfying the condition χ = βΓ tan θ _Bn ⩾ 1, where β = U/c, Γ = (1 − β)^{2 −1/2}, U is the shock velocity, and c is the speed of light, the particles can theoretically be accelerated through surfing for an unlimited time and can gain an unlimited energy. For angles satisfying the condition χ < 1, the kinetic energy ℰ of the particles is limited by ℰ = 2mc ²χ²/(1 − χ²) (m is the particle rest mass). Our main conclusion is that the generation of cosmic rays through the surfing acceleration of particles in the front of a relativistic shock wave for Γ ≫ 1 is also efficient when the angle θ _Bn is very small, i.e., it differs significantly from a right angle. Estimates for the energies of particles accelerated through surfing in relativistic jets are provided.     

Determination of absorption cross sections for oxygen molecules in the Schumann-Runge band region at high temperatures

We have measured the absorption cross sections of oxygen molecules in oxygen and in an oxygen-argon mixture heated by a shock wave, in the wavelength range 190–250 nm at temperatures of 1500–7000 K, for thermal equilibrium conditions behind the shock wave front. Analysis of the absorption cross sections obtained allowed us to select a data set that adequately describes the absorption characteristics of the electronic transition X³Σ _g ⁻ → B³Σ _u ⁻ for the oxygen molecule. In order to approximate the temperature dependence of these cross sections at a temperature of 1500–4500 K, we chose the function σ(λ, T) = σ₀(λ)(1 − exp (−θ/T)) exp (− n*θ/T) where θ₀ = 1.4·10⁻¹⁷, 1.4·10⁻¹⁷, 1.2·10^{− 17}, and 1.3·10⁻¹⁷ cm², n* = 3.1, 4.1, 5.6, and 7.47 for wavelengths 190, 210, 230, and 250 nm, respectively; θ = 2240 K is the characteristic temperature of the O₂ molecules. The approximation error was 19–25% and did not exceed the experimental error. __________ Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 73, No. 1, pp. 13–17, January–February, 2006.     

Effects of the diffusive acceleration of particles by shock waves in the primordial matter of the solar system

The effects of the shock wave diffusive acceleration of particles are considered in the case of formation of isotopic relations of the anomalous Xe-HL component of xenon in relic grains of nanodiamonds in chondrites. It is shown that this component could be formed and captured simultaneously with the nanodiamond synthesis in the conditions of the explosive shock wave propagation from supernova outbursts. The specificity of isotopic composition of Xe-HL is due to the high hardness of the spectrum of nuclear-active particles at the shock wave front and its enrichment with heavy isotopes. The spallogenic nature of both the anomalous and normal components of xenon is ascertained, and the role of the subsequent evolutionary processes in the change of their isotopic systems is shown. Experimental evidence of the formation of the power law spectrum of particles with the spectral index γ ∼ 1 by the supersonic turbulence during the carbon-detonation supernova SnIa explosion is obtained; this perhaps opens new perspectives in studying the problem of the origin of cosmic rays. It is shown that at the stage of free expansion of the explosive shock wave, the degree of compression of the matter at the wave front was σ = 31 (the corresponding Mach number M ∼ 97); this led to a 31-fold increase of the magnetic field as well as of the maximum energy of accelerated particles, so that even the energy of protons reached ∼ 3 × 10¹⁵ eV, i.e., the “knee” region.     

Influence of local dispersion on transient processes accompanying the generation of rf radiation by an electromagnetic shock wave

Transient processes accompanying the conversion of a video pulse into a radio pulse in a nonlinear transmission line having hysteretic properties are studied. It is established that the transition process leading to the establishment of “steady-state” (close in amplitude) oscillations has a minimum when the electromagnetic shock wave front is phase-matched with the wave excited by it at a frequency near the minimum local dispersion of the group velocity. Zh. Tekh. Fiz. 68, 89–95 (January 1998)     

Properties of shock-compressed liquid krypton at pressures of up to 90 GPa

The following quantities of shock-compressed liquid krypton are measured behind a plane shock front at pressures up to 90 GPa: compressibility up to densities of 7 g/cm³, brightness (color) temperatures of 6000–24000 K, and electrical conductivities of 40–60000 (Ω·m)⁻¹. X-t diagram methods are used to estimate sound speeds of up to 5.5 km/s at pressures of 30–75 GPa. The optical absorption coefficients in the violet and red (30–300 cm⁻¹) are measured at pressures of 20–90 GPa from the rise in brightness of the shock front luminosity. The optical reflection coefficient of the shock front (∼13%) at a pressure of 76.1 GPa is measured for the first time. Zh. éksp. Teor. Fiz. 116, 551–562 (August 1999)     

Electron kinetics in collisionless shock waves

We study the kinetic model of the formation of the energy spectrum of nonthermal electrons near the front of a quasilongitudinal, supercritical, collisionless shock wave. Nonresonant interactions of the electrons and the fluctuations generated by kinetic instabilities of the ions in the transition region inside the shock front play the main role in the heating and preacceleration of electrons. We calculate the electron energy spectrum in the vicinity of the shock wave and show that the heating and preacceleration of electrons occur on a scale of the order of several hundred ion inertial lengths in the vicinity of the viscous discontinuity. Although the electron distribution function is significantly nonequilibrium near the shock front, its low-energy part can be approximated by a Maxwellian distribution. The effective electron temperature T _eff ² behind the front, obtained in this manner, increases with the Mach number of the shock wave slower than it would if it followed the Hugoniot adiabat. We determine the condition under which the electron heating is ineffective but the electrons are effectively accelerated to high energies. The high-energy asymptotic behavior of the distribution function is that of a power law, with the exponent determined by the total compression ratio of the plasma, as in the case of acceleration by the first-order Fermi mechanism. The model is used to describe the case (important for applications) of acceleration of electrons by shock waves with large total Mach numbers, with the structure of these waves modified by the nonlinear interaction of nonthermal ions and consisting of an extended prefront with a smooth variation of the macroscopic parameters and a viscous discontinuity in speed with a moderate value of the Mach number. Zh. éksp. Teor. Fiz. 115, 846–864 (March 1999)     

Influence of temperature and strain on the amplitude-dependent internal friction of high-purity aluminum

The dislocation amplitude-dependent friction (ADIF) of high-purity (99.999%) polycrystalline aluminum is investigated in the temperature range 7–300K at vibrational strain amplitudes of 10⁻⁷–10⁻⁴ for samples in the annealed and deformed (by quasistatic, shock, and ultrasonic loading) states. The ADIF is a multistage effect in the indicated temperature and vibration amplitude ranges. Analysis of the amplitude-temperature spectra of the ADIF permits separation of components attributable to: interaction between dislocations, the interaction of dislocations with pinning points, and pure dislocation relaxation (the interaction of dislocations with the Peierls relief). ADIF is observed to depend nonmonotonically on the initial quasistatic strain determined by strain hardening and recovery processes. Fiz. Tverd. Tela (St. Petersburg) 40, 1839–1844 (October 1998)     

Near IR laser light visualizators using nonlinear GaSe and other layered crystallites

Two methods of preparation of the devices for visualization of pulsed and continuous near-IR (near infrared) are described and the results of conversion of pulsed and continuous IR (800–1360 nm) laser radiation into the visible range of spectra (400–680 nm) by using a transparent substrate covered with the particles (including nanoparticles) of effective nonlinear materials of GaSe _x S_{1 − x} (0.2 ≤ x ≤ 0.8) are presented. Converted light can be detected in transmission or reflection geometry as a visible spot corresponding to the real size of the incident laser beam. Developed device structures can be used for checking if the laser is working or not, for optical adjustment, for visualization of distribution of laser radiation over the cross of the beam and for investigation of the content of the laser radiation. Low energy (power density) limit for visualization of the IR laser pulses with 2–3 ps duration for these device structures are: between 4.6–2.1 μJ (3 × 10⁻⁴−1 × 10⁻⁴ W/cm²) at 1200 nm; between 8.4–2.6 μJ (4.7 × 10⁻⁴−1.5 × 10⁻⁴ W/cm²) at 1300 nm; between 14.4–8.1 μJ (8.2 × 10⁻⁴–4.6 × 10⁻⁴ W/cm²) at 1360 nm. Threshold damage density is more than 10 MW/cm² at λ = 1060 nm, pulse duration τ = 35 ps. The results are compared with commercially existing laser light visualizators.     

Model of pulsed electric discharge expansion in dense gas taking into account electron and radiative thermal conductivities. II. Energy balance and equation

Using an ionization sensor, it was found that weakly ionized plasma with an ionization degree larger than 10⁻⁶ is formed under exposure to UV radiation of a high-current pulsed electric discharge in gas (air, nitrogen, xenon, and krypton) at atmospheric pressure at a distance of ∼1.2–2.5 cm from the discharge boundary. It was shown that the structure of such discharge includes, in addition to the discharge channel, a dense shell and a shock wave, also a region of weakly ionized and excited gas before the shock wave front. The mechanism of discharge expansion in dense gas is ionization and heating of gas involved in the discharge due to absorption of the UV energy flux from the discharge channel and the flux of the thermal energy transferred from the discharge channel to the discharge shell due to electron thermal conductivity.     

Decay of an electronic vortex of a collisionless shock wave as a possible mechanism of a “Coulomb explosion”

A new mechanism of a “Coulomb explosion,” where ions are accelerated by the electric field separating charges at the magnetic Debye radius r _B∼B/4πen _e, is proposed on the basis of a nonquasineutral model of electronic vortices in a magnetic field. It is shown by means of numerical calculations that in the process of acceleration of the ions a collisionless shock wave, whose front has an effective width of the order of δ∼r _B, determined by the breakdown of quasineutrality, is formed in a time of the order of ω _pi ⁻¹ , where ω_pi is the ion plasma frequency. The origin of such explosive dynamics is the formation of “holes” in the electron density at characteristic times of the order of ω _pe ⁻¹ (ω_pe is the electronic plasma frequency) as a result of the generation of electronic vorticity by the Weibel instability of an electromagnetic wave. Calculations for a laser pulse with intensity J∼6×10¹⁸ W/cm² show that the ions expand in the radial direction with velocities up to 3.5×10⁸ cm/s. Pis’ma Zh. éksp. Teor. Fiz. 70, No. 10, 669–674 (25 November 1999)     

Kinetics of the photoconductivity and absorption in the D −(A +) bands in doped silicon

The photoconductivity (PC) spectra and the induced absorption of background radiation in the energy range 10–40 meV are investigated in weakly compensated B-, Ga-, and As-doped silicon at 4.2 K. It is shown that dips corresponding to the photoionization of long-lived excited states of B and As are observed in the PC spectra on the D ⁻(A ⁺) bands. It is found that the frequency dependence of the PC spectra corresponds to excitation relaxation times of the order of 10⁻⁴ s for the states in the D ⁻ (A ⁺) bands. It is established that in electric fields E>100 V/cm the PC decreases sharply, while the induced absorption of the background radiation changes very little. This confirms the conclusion that the excitation of the D ⁻ (A ⁺) itself makes the main contribution to the PC. Pis’ma Zh. éksp. Teor. Fiz. 66, No. 4, 224–227 (25 August 1997)     

Mixing of excitonic states containing light and heavy holes in an isolated GaAs/AlGaAs quantum well in a magnetic field

The Zeeman splitting of the ground states 1s(hh) and 1s(lh) of excitons with heavy and light holes, respectively, in a 15-nm isolated Al_0.3Ga_0.7As/GaAs quantum well in magnetic fields of up to 20 T is investigated according to the photoluminescence excitation spectra in the Faraday geometry (σ⁺− σ⁻ components). The observed anomalous pattern of nonlinear Zeeman splitting and the nonmonotonic behavior of the effective hole g factor are interpreted in terms of the strong mixing of the magnetoexcitonic states containing light and heavy holes. Pis'ma Zh. éksp. Teor. Fiz. 64, No. 1, 52–56 (10 July 1996)     

Electronic and electronic-vibrational phenomena in the new organic conductor ϰ-(ET)2[Hg(SCN)2Cl] with a metal-insulator transition

The reflection spectra and optical conductivity spectra of the new organic conductor ϰ-(ET)₂[Hg(SCN)₂Cl] with a metal-insulator transition in the spectral regions 700–5500 and 9000–40 000 cm⁻¹ have been studied in polarized light at 300 K. A comparisonis made between the spectra obtained and the corresponding spectra of related isostructural conductors based on the ET molecule, and also the properties of the crystal structure of the investigated compounds. An electronic transition between the ET molecules of the dimer (ET) ₂ ⁺ in the spectral region 700–5500 cm⁻¹ has been identified, as have the features of the electronic-vibrational structure arising as a consequence of the interaction of this transition with the completely symmetric intramolecular vibrations of the ET molecule. It is found that the conductor with the stronger dimer interaction between the ET molecules has the higher the transition temperature. Fiz. Tverd. Tela (St. Petersburg) 39, 1313–1319 (August 1997)     

Weak e+e− lines from internal pair conversion observed in collisions of 238U with heavy nuclei

We present the results of a Doppler-shift correction to the measured e⁺e⁻–sum-energy spectra obtained from e⁺e⁻–coincidence measurements in ²³⁸U +²⁰⁶Pb and ²³⁸U +¹⁸¹Ta collisions at beam energies close to the Coulomb barrier, using an improved experimental setup at the double-Orange spectrometer of GSI. Internal-Pair-Conversion (IPC) e⁺e⁻ pairs from discrete nuclear transitions of a moving emitter have been observed following Coulomb excitation of the 1.844 MeV (E1) transition in ²⁰⁶Pb and neutron transfer to the 1.770 MeV (M1) transition in ²⁰⁷Pb. In the collision system ²³⁸U +¹⁸¹Ta, IPC transitions were observed from the Ta-like as well as from the U-like nuclei. In all systems the Doppler-shift corrected e⁺e⁻–sum-energy spectra show weak lines at the energies expected from the corresponding γ–ray spectra with cross sections being consistent with the measured excitation cross sections of the γ lines and the theoretically predicted IPC coefficients. No other than IPC e⁺e⁻–sum-energy lines were found in the measured spectra. The transfer cross sections show a strong dependence on the distance of closest approach (R_min), thus signaling also a strong dependence on the bombarding energy close to the Coulomb barrier. Received: 22 July 1997 / Revised version: 15 October 1997     

Thermal stability and impedance spectroscopy studies of (Cu, Ni) substituted Bi4V2O11 ceramics

Polycrystalline samples of the oxygen ion conductor Bi₂V_0.9Cu_0.1−xNi_xO_5.35 with various contents of nickel (0 ≤ × ≤ 0.1) were investigated. The X-ray powder diffraction revealed the tetragonal structure of all compositions. DTA curves exhibit effects due to phase transition, one endothermic effect during heating and one exothermic one during cooling. The impedance of the ceramics with Pt electrodes was measured in the frequency range 10⁻¹–10⁷ Hz at constant temperatures between 350 and 920 K. The conductivity was determined by nonlinear least-squares analysis of the impedance spectra. Separation of the total resistance into grain interior and grain boundary components was feasible at temperatures below 580 K. The transition temperatures observed in DTA coincide with those observed in conductivity measurements. A phase transition, involving a reordering process of the oxygen ions is considered to be responsible for this phenomenon. The frequency dependent part of the intragrain conductivity was modeled by a constant phase admittance. The effective hopping rate was estimated by comparing the frequency dependent part and the dc limit of the intragrain conductivity. Paper presented at the 4th Euroconference on Solid State Ionics, Renvyle, Galway, Ireland, Sept. 13–19, 1997.     

Spectral components that form UV absorption spectrum of Ce3+ and Ce(IV) valence states in matrix of photothermorefractive glasses

We have measured the UV absorption spectra of photothermorefractive glasses of the system Na₂O-ZnO-Al₂O₃-NaF-SiO₂ doped by cerium oxide in the range of (2.8–5.0) × 10⁴ cm⁻¹ (360–200 nm). The spectra have been processed by the method of dispersion analysis based on the analytical convolution model for the complex dielectric function of glasses. We show that the absorption band centered at 3.3 × 10⁴ cm⁻¹ (∼303 nm) that is attributed to the transition 2F _5/2 → 5d in the Ce³⁺ ion, is an envelope of three spectral components. The broad absorption range (3.5–4.7) × 10⁴ cm⁻¹ (200–270 nm) that is commonly interpreted as a charge transfer band of the Ce(IV) valence state, is an envelope of at least three spectral components.     

Application of abrupt cut-off models in the analysis of the capacitance spectra of conjugated polymer devices

In this paper, a detailed study of the capacitance spectra obtained from Au/doped-polyaniline/Al structures in the frequency domain (0.05 Hz–10 MHz), and at different temperatures (150–340 K) is carried out. The capacitance spectra behavior in semiconductors can be appropriately described by using abrupt cut-off models, since they assume that the electronic gap states that can follow the ac modulation have response times varying rapidly with a certain abscissa, which is dependent on both temperature and frequency. Two models based on the abrupt cut-off concept, formerly developed to describe inorganic semiconductor devices, have been used to analyze the capacitance spectra of devices based on doped polyaniline (PANI), which is a well-known polymeric semiconductor with innumerous potential technological applications. The application of these models allowed the determination of significant parameters, such as Debye length (≈20 nm), position of bulk Fermi level (≈320 meV) and associated density of states (≈2×10¹⁸ eV⁻¹ cm⁻³), width of the space charge region (≈70 nm), built-in potential (≈780 meV), and the gap states’ distribution.     

Twisted lines and small-scale structures in generation spectra of Yb-doped media excited by focused radiation of LiF:F 2 + color center laser

Spectral lines of Yb lasing in 1.03–1.05 μm region structured by 50–200 μm spots were found at focusing a pulsed LiF:F₂⁺ color center laser of 0.5–5.0 GW/cm² intensity on highly doped Yb:YAG or Yb:glass plates in a resonator. Small spots at the spectrograph located ≈ 1 m apart from the resonator indicated a “sub-diffraction” directivity of Yb generation, 1–2 orders better than the diffraction limit 10⁻³–10⁻² rad determined by the pumped volume dimensions. Observed features of Yb emission are explained assuming off-axis oscillations in Yb laser on phase-synchronized photons due to a strong spatial-angular selection of radiation in the resonator. Propagation of near diffraction free beams at angles to the axis built at the spectrograph slit for every 10–15 ns pulse of Yb generation a magnified “image” of a structure of generating channels in the active medium. This image projection brought a corresponding structure of spots in Yb spectra. It was found that channels may be formed due to a high-frequency spatial modulation (micrometers scale) of the refractive index profile in samples caused by the oscillating amplitude of thermoelastic stresses in the pumped medium. Obtained data demonstrate a possibility to study (with high spatial and temporal resolution) non-equilibrium stales of materials in small volumes using laser radiation emerging from these objects. This study results evidence for the novel concept of the spatial distribution of electromagnetic field of a photon: not in the form of a “travelling” wave but in the form of a wave with maxima and nodes located at fixed positions along the photon propagation direction.     

2p3/2?13x?1?3x?13d?1 X-ray satellites spectra in the Lα1 region of 4d transition elements

The X-ray satellite spectra arising due to 2p _3/2 ⁻¹3x ⁻¹−3x ⁻¹3d ⁻¹ (x ≡ s, p, d) transition array, in elements with Z = 40 to 48, have been calculated, using available Hartree-Fock-Slater (HFS) data on 1s ⁻¹−2p ⁻¹ 3x ⁻ and 2p _3/2 ⁻¹−3x ⁻¹,3x ⁻¹ Auger transition energies. The relative intensities of all the possible transitions have been estimated by considering cross — sections for the Auger transitions simultaneous to a hole creation and then distributing statistically the total cross sections for initial two hole states 2p _3/2 ⁻¹−3x ⁻¹ amongst various allowed transitions from these initial states to 3x ⁻¹ 3d ⁻¹ final states by Coster-Kronig (CK) and shake off processes. In both these processes initial single hole creation is the prime phenomenon. Each transition has been assumed to give rise to a Gaussian line and the overall spectrum has been computed as the sum of these Gaussian curves. The calculated spectra have been compared with the measured satellite energies in Lα₁ spectra. Their intense peaks have been identified as the observed satellite lines. The peaks in the theoretical satellite spectra were identified as the experimentally reported satellites α₃, α₄ and α₅, which lie on the high-energy side of the Lα₁ dipole line.