D+CD4→CD3+D2反应的量子含时动力学研究

运用半刚体振动转子靶(semirigid vibrating rotor target)模型,利用含时波包法(TDWP method),对反应D+CD4→CD3+D2进行了量子含时动力学研究与计算.反应几率随平动能的变化图象,呈现出显著的量子共振特性.并通过对v=0时,j=0,1,2的反应几率以及j=0时,v=0,1的反应几率的计算,对该反应的空间效应进行了研究与分析.     

D+CD4→CD3+D2反应的四维量子散射计算

运用约化维数量子动力学理论 ,利用含时波包法 ,对反应D +CD4 →CD3+D2 进行了四维量子散射计算 .将反应多原子CD4 看作双原子D—CD3,反应D +CD4 →CD3+D2 看作单原子 双原子反应 ,把体系的反应简化为四维散射问题 .波函数的传播采用分裂算符法 ,为避免格点边界处含时波函数的边界反射 ,采用了光学吸收势法 ,在格点边界处引入光学势 ,消除边界反射 .根据CD4 分子的C3v对称性 ,选取了Jordan和Gilbert提出的半经验势能面 .计算结果表明 ,反应概率随平动能的变化图像 ,呈现出显著的量子共振特性 ,这是很多提取反应的共同特征 .而不同振动态下的反应概率随平动能的变化表明 ,随振动量子数的增大 ,反应概率有明显提高 ,且反应阈能明显降低 ,这说明反应分子的振动能对分子的碰撞反应有重要贡献 .而对基态和第一振动激发态时散射截面的计算 ,也证明了这一结论 .同时 ,还分别通过计算量子数j,k ,m对反应概率的影响 ,对该反应的空间取向效应进行了研究 ,并与H +CH4→CH3+H2 反应进行了比较 .     

D+和D0介子的φXl+υ遍举分支比上限的测定

利用北京谱仪(BES)在北京正负电子对撞机(BEPC)e+e-质心系能量为4.03GeV处采集的积分亮度为22.3pb-1的数据,从D介子的5个非轻子衰变模式中共选出2471±218组tagD+X(X可能是γ或π0或π±)和7629±251组tagD0X介子样本. 在这些样本中没有找到D+→φe+υ,φK-π+e+υ,和D0→φK-e+υ,φK-μ+υ的衰变事例,测定在90髎置信度下分支比的上限分别为B(D+→φe+υ)<1.38髎,B(D+→φK-π+e+υ)<2.01髎,B(D0→φK-e+υ)<0.53髎,和B(D0→φK-μ+υ)<0.53髎.     

Measurement of the D0, D+ and Ds+ meson lifetimes at √s = 10.58 GeV

We have measured the lifetimes of the D⁰, D⁺ and D_s⁺ mesons with data from the CLEO detector. We find τ_D⁰ = (5.0 ± 0.7 ± 0.4) × 10⁻¹³s, τ_D⁺ = (11.4 ± 1.6 ± 0.7) × 10⁻¹³s and τ_Ds⁺ = (4.7 ± 2.2 ± 0.5) × 10⁻¹³s, giving lifetime ratios τ_D⁺/τ_D⁰ = 2.3 ± 0.5 and τ_Ds⁺/τ_D⁰ = 0.9 ± 0.5.     

氘氢混合气体的高频离子源中H2D+与D+2的比例实测研究

分子离子H2D+在天体物理和天体化学研究中有重要意义,但在实验研究中不可避免混入D+2从而对实验结果产生影响.本文采取产物对比与分析的方法,将离子源中两种离子的比例实际测量出来,从而能较为准确地研究H2D+的结构和性质.将实验测量的结果与理论推算进行比较,得到了相对较好的结果.本文所采用的方法将对类似的研究提供有益的借鉴和启发.     

Stereodynamics study of reactions N(~2D)+HD→NH+D and ND+H

The product polarizations of the title reactions are investigated by employing the quasi-classical trajectory (QCT) method. The four generalized polarization-dependent differential cross-sections (PDDCSs) $({2\pi } / \sigma )(\d\sigma _{00} / \d\omega _t )$, $({2\pi } / \sigma )(\d\sigma _{20} / \d\omega _t )$, $({2\pi } / \sigma )(\d\sigma _{22 + } / \d\omega _t )$, and $({2\pi } / \sigma )(\d\sigma _{21 - } / \d\omega _t )$ are calculated in the centre-of-mass frame. The distribution of the angle between ${{\bm k}}$ and ${{\bm j^\prime }}$, $P(\theta _r )$, the distribution of the dihedral angle denoting ${{\bm k}}${--}$\bm k^\prime $--$\bm j^\prime $ correlation, $P(\phi _r )$, as well as the angular distribution of product rotational vectors in the form of polar plots $P(\theta _r ,\phi _r )$ are calculated. The isotope effect is also revealed and primarily attributed to the difference in mass factor between the two title reactions.     

用联合D0和D+单双标记测定分支比的方法

报道了用“联合D0 和D+单双标记”测定衰变分支比的方法 .基于北京谱仪 (BES)在北京正负电子对撞机 (BEPC)质心系能量s =4 .0 3GeV处获取的数据 ,利用联合D0 和D+单双标记的方法 ,可以测定D0 和D+介子单举和遍举衰变分支比 .作为该方法的应用举例 ,利用BES实验组发表的数据 ,在 90 %置信度的情况下 ,测得D+→e+ν衰变过程分支比的上限为Br(D+→e+ν) <1 .6% .此上限值与BES曾发表的结果一致 .     

Final state interaction effects in the B + → D + K 0 decay

The exclusive decay of B ⁺ → D ⁺ K ⁰ is calculated by the QCD factorization method (QCDF) and final state interaction (FSI). First, the B ⁺ → D ⁺ K ⁰ decay is calculated via QCDF method. The result that is found by using the QCDF method is less than the experimental result. So FSI is considered to solve the B ⁺ → D ⁺ K ⁰ decay. For this decay, the D _s ⁺ π⁰, D _s ⁺ *ρ⁰, D _s ⁺ *? via the exchange of \(\bar K^0\) , \(\bar K^{0*} \) , D ^?, and D ^?* mesons are chosen for the intermediate states. The above intermediate states are calculated by using the QCDF method. In the FSI effects, the results of our calculations depend on η as the phenomenological parameter. The range of this parameter is selected from 2 to 2.4. It is found that if η = 2.4 is selected, the numbers of the branching ratio are placed in the experimental range. The experimental branching ratio of this decay is less than 2.9 × 10^?6 and our results calculated by QCDF and FSI are (0.16 ± 0.04) × 10^?6 and (2.8 ± 0.09) × 10^?6, respectively.     

Isotope effect and Coriolis coupling effect forthe Li + H(D)Cl → LiCl + H(D) reaction

A time-dependent quantum wave packet method is used to investigate the dynamics of the Li + H(D)Cl reaction based on a new potential energy surface(J. Chem. Phys. 146 164305(2017)). The reaction probabilities of the Coriolis coupled(CC) and centrifugal sudden(CS) calculations, the integral cross sections, the reaction rate constants are obtained. The rate constants of the Li + HCl reaction are within the error bounds at low temperature. A comparison of the CC and CS results reveals that the Coriolis coupling plays an important role in the Li + H(D)Cl reaction. The CC cross sections are larger than the CS results within the entire energy range, demonstrating that the Coriolis coupling effect can more effectively promote the Li + DCl reaction than the Li + HCl reaction. It is found that the isotope effect has a great influence on the title reaction.     

A coupled-channel treatment of Cabibbo-angle favoured (D,D s + )→VP decays

We have performed a two-channel calculation of Cabibbo-angle favoured decays,D _s ⁺ →VP. We find a satisfactory fit toS _s ⁺ →φπ ⁺,ρ ⁰ π ⁺ andK ⁺ \(\bar K^{ * 0} \) data from ARGUS and E-691. We have also studied Cabbibo-angle favouredD→VP decays in a coupled channel formalism. We coupleD→K ^*π,K _? and \(\bar K^0 \phi \) channels inI=1/2 state, andK ^*π andK _? channels inI=3/2 state. We leave the two channels, \(\bar K^0 \omega \) and \(\bar K^{ * 0} \eta \) out of our unitarization scheme. Particular attention is paid to the role of the weak annihilation term in these decays.     

D+DBr反应的态-态动力学研究

在0—2.0 eV的碰撞能范围内采用含时量子波包方法和二阶分裂算符传播子对初始量子态为(v_0=0,j_0=0)的D+DBr反应进行了态分辨理论水平上的动力学计算.计算了抽取反应通道D+DBr→Br+D_2和置换反应通道D'+DBr→D+D'Br的反应概率、积分截面、微分截面、产物的振动和转动分布以及速率常数等动力学性质,并与相应的理论和实验结果进行了比较.结果表明:计算的速率常数与实验结果十分符合.微分截面的结果表明:对于抽取反应,前向的剥离反应机制在反应过程中占据主导地位;对于置换反应,头碰头的反弹机制占据主导地位.     

D+HS反应的含时量子动力学研究

利用含时波包方法对D+HS交换和抽取通道进行量子动力学研究,动力学计算中所采用的势能面由高精度从头算能量点构建.在平动能0.0～2.0 eV区间内计算了反应物初始振转基态时的总反应几率和积分反应截面,并且计算了初始振动激发态对积分反应截面的影响.所有动力学计算均考虑了科里奥利耦合效应.在低平动能时抽取通道在反应中占主导地位,而交换通道在高平动能时占主导地位.在整个所研究的平能能区间内,反应物HS的振动激发对抽取和交换通道反应都有增强作用.     

4+2D维Einstein–Maxwell量子宇宙

利用推广的Hartle-Hawking假设,研究了4+2D维Einstein-Maxwell量子宇宙,计算了微超空间波函数的近似解.发现当D≤2时存在与观测宇宙相符合的暴胀解.     

Inclusive decays χ b0,2 → ψD \bar D + X and duality relation

The three-body decays χ _b0,2 → J/ ψc $\bar c$ and the decays x _bJ → J/ ψD $\bar D$ related to them are studied. The differential widths with respect to these decays are calculated analytically, and their total widths are evaluated numerically. The duality relation between these decays and the two-body decays x _b0,2 → J/ ψ(c $\bar c$ ) is verified. The possibility of observing these decays at the LHC and Tevatron colliders is discussed.     

Reaction mechanism of D + ND→N + D_2 and its state-to-state quantum dynamics

The quantum state-to-state calculations of the D + ND→N + D_2 reaction are performed on a potential energy surface of 4 A' state. The state-resolved integral and differential cross sections and product state distributions are calculated and discussed. It is found that the rotational distribution, rather than the vibrational distribution, of the product has an obvious inversion. Due to the fact that it is a small-impact-parameter collision, its product D_2 is mainly dominated by rebound mechanism, which can lead to backward scattering at low collision energy. As the collision energy increases, the forward scattering and sideward scattering begin to appear. In addition, the backward collision is also found to happen at high collision energy, through which we can know that both the rebound mechanism and stripping mechanism exist at high collision energy.     

e+e-对撞中ψ(3770)非D(D)衰变的实验寻找

评述了以往与ψ(3770)非D(D)衰变相关的实验测量与研究,详细讨论了三种寻找非D(D)衰变的实验方法,即遍举、半单举和单举方法.这些方法对于在实验上寻找ψ(3770)非D(D)衰变具有启示和示范作用,有助于加深人们对粲夸克偶素态衰变动力学机制的理解.     

HD2+,H3+和D3+与固体相互作用和三体尾流效应

从分子离子H3 及其氘化同位素分子离子D3 和HD2 与超薄固体膜相互作用发生库仑爆炸为基础,分析讨论了H3 ,D3 和HD2 三种分子离子的形成机理,根据产物能谱分布,利用库仑爆炸技术确定了同位素分子离子HD2 的结构形式,给出具体核间距数值.并确定在实验中不存在线状结构的HD2 .提出一种三原子分子离子和固体相互作用中尾流效应的处理方式,通过和实验结果做比较发现这是一种非常理想的处理三体尾流效应的模式,并用之进一步确认了HD2 的结构形状.文章对H3 ,D3 和HD2 三种分子离子的实验结果做了对比和讨论.