KTiOPO4, KTiOAsO4, and KNbO3 crystals for mid-infrared femtosecond optical parametric amplifiers: analysis and comparison

We have designed a simple mid-IR femtosecond OPA seeded by a white-light continuum and delivering very stable, largely tunable and energetic output pulses. This OPA requires fewer than 200 7J of 120-fs Ti:sapphire pump pulses as energy. This system allowed us to experimentally compare the performances of potassium crystals (KTP, KTA, and KNbO₃) for the generation of up to 100-fs Fourier-transform-limited pulses tunable in 1-4.6 7m mid-IR wavelengths.     

Femtosecond ultraviolet pulses generated using noncollinear optical parametric amplification and sum frequency mixing

We demonstrate the generation of ultraviolet 33-fs pulses with a shot-to-shot energy fluctuation of less than 3% using sum frequency mixing of visible pulses of a noncollinear optical parametric amplifier with sub-40-fs pulses of a 1-kHz Ti:sapphire-amplified system. The pulses are transform-limited (ΔνΔτ=0.36) and tunable in the range from 315 nm to 355 nm with energy above 1 μJ (2.6 μJ at 330 nm). Received: 21 July 2000 / Published online: 8 November 2000     

Structural changes in fused silica after exposure to focused femtosecond laser pulses

Using in situ Raman scattering in a confocal microscopy setup, we have observed changes in the network structure of fused silica after modifying regions inside the glass with tightly focused 800-nm 130-fs laser pulses at fluences of 5-200 J cm(-2). The Raman spectra show a large increase in the peaks at 490 and 605cm(-1), owing to 4- and 3-membered ring structures in the silica network, indicating that densification occurs after exposure to the femtosecond laser pulses. The results are consistent with the formation of a localized plasma by the laser pulse and a subsequent microexplosion inside the glass.     

Ablation and ultrafast dynamics of zinc selenide under femtosecond laser irradiation

The ablation in zinc selenide (ZnSe) crystal is studied by using 150-fs, 800-nm laser system. The images of the ablation pit measured by scanning electronic microscope (SEM) show no thermal stress and melting dynamics. The threshold fluence is measured to be 0.7 J/cm2. The ultrafast ablation dynamics is studied by using pump and probe method. The result suggests that optical breakdown and ultrafast melting take place in ZnSe irradiated under femtosecond laser pulses.     

Pulse characteristics of an optical parametric oscillator pumped by sub-30-fs light pulses

We obtained nearly transform-limited light pulses of 34 fs near 1.2 microm by pumping an optical parametric oscillator with a 2-mm-long KTP crystal by 26-fs pulses from a Ti:sapphire laser. The average power of the pulses that were obtained was greater than 50 mW, at an 80-MHz repetition rate. Attempts to downscale the pulse duration by decreasing the pump-pulse duration revealed remarkable limitations of the attainable pulse length for sub-30-fs pump pulses, in accordance with a recent theoretical study [J. Opt. Soc. Am. B 17, 741 (2000)].     

Continuous-wave mode-locked Ti:sapphire laser focusable to 5 x 10(13) W/cm(2)

Generation of sub-10-fs pulses with an average power of 1 W and a peak of 1.5 MW from a Kerr-lens mode-locked mirror-dispersion-controlled Ti:sapphire laser is demonstrated. A specially designed lens triplet focuses the output of this compact all-solid-state source to a peak intensity in excess of 5x10(13) W/cm (2) . Nonperturbative nonlinear optics is now becoming feasible by use of the output of a cw mode-locked laser.     

Self-starting five optical cycle pulse generation in Cr<Superscript>4+</Superscript>:YAG laser

We report stable self-starting near-transform-limited 26-fs pulses at 250-mW output power from a Kerr-lens mode-locked (KLM) Cr⁴⁺:YAG laser using chirped mirrors in combination with prisms. The highest output power achieved in KLM regime was 600 mW at 55-fs pulse duration. The experimental results agree well with the results of theoretical analysis with respect to KLM self-starting ability and stability against continuous-wave and multi-pulse operation. Parameter ranges for stable transform-limited KLM pulses as well as the shortest achievable pulse durations are established. Using an InGaAs-InP semiconductor saturable absorber mirror we could obtain self-starting 57-fs pulses at the average output power of 200 mW. Two-photon absorption was found to be the main mechanism favoring the multiple-pulse operation. Received: 2 May 2002 / Revised version: 16 July 2002 / Published online: 8 January 2003 RID="*" ID="*"Corresponding author. Fax: +43-1/58801-38799, E-mail: sorokina@tuwien.ac.at     

High-order harmonics from solid targets as a probe for high-density plasmas

The interaction of 100-fs Ti:sapphire laser pulses with thin foil targets was experimentally investigated at intensities exceeding 10(18) W/cm(2). High harmonics were observed in transmission through an overdense plasma in the direction of the incident beam. From the cutoff frequency of the harmonics an electron density of 1 x 10(24) cm(-3) is inferred, indicating a compression of the plasma by the ponderomotive force of the laser pulse.     

Guing of intense femtosecond pulses in preformed plasma channels

We report guiding of sub-100-fs pulses at intensities up to 5x10(15) W/cm (2) over a distance of 1 cm in a preformed plasma channel. The width of the guided pulse was shortened, which we attribute to ionization-induced refraction at the channel entrance. A pulse energy throughput of 30% in the lowest-order was measured.     

Generation of high-energy broadband femtosecond deep-ultraviolet pulses by highly nondegenerate noncollinear four-wave mixing in a thin transparent solid

We present a simple and efficient technique for the generation of ultrashort deep-ultraviolet pulses based on four-wave mixing of noncollinear laser pulses in a thin solid. Sub-30-fs pulses (Fourier-limit of 13 fs) centered at 270 nm, with energies up to 6 μJ, were obtained by mixing the fundamental and the second harmonic of a Ti:sapphire amplifier in fused silica. Temporal characterization was performed with a dispersionless self-diffraction FROG setup. Spectra as broad as 20 nm were also obtained that can in principle support sub-4-fs deep-ultraviolet pulses.The results are well described by two-dimensional numerical simulations.     

Femtosecond diode-pumped Nd:glass laser with more than 1 W of average output power

We have demonstrated 175-fs pulses with 1 W and 300-fs pulses with 1.2 W of average output power at a pulse repetition rate of 117 MHz from a Nd:phosphate (Schott LG 760) glass laser pumped by a 1-cm-wide, 20-W diode laser bar. Stable soliton mode locking was achieved by use of an intracavity semiconductor saturable absorber mirror. We obtained more than 2 W of average power without mode locking. Using cylindrical cavity mirrors, we adapted the laser mode inside the Nd:glass to the highly elliptical pump beam in both dimensions (tangential and sagittal axes) while maintaining a nearly ideal circular TEM(00) output beam with M(2) approximately 1.2 . Overpumping the laser mode in the tangential plane and efficient unidirectional heat removal in the sagittal plane using a 0.8-mm thin Nd:glass also contributed to the good output-beam quality.     

Two-color pump-probe ionization spectroscopy of gaseous water enhanced by preliminary impulsive Raman excitation

We use sub-10-fs pulses at 400 nm and 15-fs pulses at 800 nm to ionize water molecules and their isotopomers HDO and D₂O in a pump–probe scheme. Pulses are generated via spectral broadening of 25-fs pulses of a 1-kHz Ti:sapphire amplifier system by self-phase modulation in a noble-gas-filled hollow waveguide and subsequent compression using chirped mirrors. At this time scale vibronic excitation of the first bending mode of water in the electronic ground state by impulsive Raman scattering is possible (e.g. the fundamental bending mode of H₂O: t_vib=20 fs). The effect of this pre-excitation on the ionization rate is shown. Received: 14 May 2001 / Revised version: 24 August 2001 / Published online: 19 September 2001     

Efficient noncollinear parametric amplification of weak femtosecond pulses in the visible and near-infrared spectral range

We report measurement of efficient amplification of weak femtosecond supercontinuum seed pulses by use of a noncollinear optical parametric process in BBO crystal pumped with 150-fs pulses from a frequency-doubled regenerative-amplified Ti:sapphire laser at 390nm . The highest amplification factor, 10(8) , was achieved for 3x10(-16)J energy seed pulses at wavelength of 560nm.     

Microjoule supercontinuum generation by stretched megawatt femtosecond laser pulses in a large-mode-area photonic-crystal fiber

Microjoule supercontinuum generation is demonstrated using a large-mode-area photonic-crystal fiber (PCF) pumped by an amplified stretched-pulse output of a mode-locked Cr:forsterite laser. A PCF with a mode area of 380 μm² is employed to transform 300-fs Cr:forsterite laser pulses with a peak-power of a few megawatts into a supercontinuum radiation with a spectrum spanning from 700 to 1800 nm and a total energy of 1.15 μJ.     

Generation of high-energy, sub-20-fs pulses in the deep ultraviolet by using spectral broadening during filamentation in argon

Generation of sub-20-fs UV pulses with more than 300 μJ energy at 268 nm is reported. First, the UV pulses are produced by successive second-harmonic and third-harmonic (TH) generation of 805 nm pulses of a 1 kHz Ti:sapphire laser amplifier. The spectral broadening of TH pulses is realized in a filament, generated in argon. The produced pulses are compressed in a simple double-pass prism-pair compressor. Starting from 100 fs pulses, we achieve a fivefold pulse shortening.     

Characterization of sub-10-fs pulse focusing with high-numerical-aperture microscope objectives

Dispersion precompensation with a prism sequence and a third-order dispersion mirror resulted in negligible broadening of sub-10-fs pulses at subwavelength spot sizes when the pulses were focused with microscope objectives and moderate apertures. At larger apertures, lens chromaticity and spherical aberration led to an effective pulse broadening of up to 1.3x , depending on the aperture size and the detector position. The data suggest that intensities exceeding 10(14) W/cm(2) can be produced directly from femtosecond pulse oscillators.     

Generation of the fourth harmonic of a femtosecond Ti:sapphire laser

A high-repetition-rate femtosecond laser system operating, for the first time to our knowledge, in the spectral region near 200 nm is described. Frequency quadrupling of a mode-locked Ti:sapphire laser results in maximum average powers of 6 mW (165-fs pulses) and 15 mW (340-fs pulses) at 82 MHz. The shortest wavelength achieved is 193.7 nm.     

High-order harmonic generation by nonlinear reflection of an intense high-contrast laser pulse on a plasma

We demonstrate the use of a plasma mirror to obtain 60-fs 10-TW laser pulses with a temporal contrast of 10(8) on a nanosecond time scale and 10(6) on a picosecond time scale, and we use these high-contrast pulses to generate high harmonics by nonlinear reflection on a plasma with a steep electronic density gradient. Well-collimated harmonics up to 20th order are observed for a laser intensity of approximately equal to 3 x 10(17) W/cm2, whereas no harmonics are obtained without the plasma mirror.     

Generation of relativistic intensity pulses at a kilohertz repetition rate

By using adaptive optics to correct the wave-front distortion of a 21-fs, 0.7-mJ, 1-kHz laser, we are able to focus the pulses to a 1-mum spot with an f/1 off-axis parabolic mirror. The peak intensity at the focal position is 1.5x10(18) W/cm(2) , which is to the authors' knowledge the first demonstration of generating relativistic intensity at a kilohertz repetition rate.     

All-solid-state generation of 100-kHz tunable mid-infrared 50-fs pulses in type I and type II AgGaS(2)

We report the operation of an all-solid-state system for the generation of tunable mid-infrared sub-50-fs pulses. A Ti:sapphire regenerative amplifier, pumped by 10 W of power from 532-nm, diode-pumped, frequency-doubled Nd:YVO(4) lasers, produced 4-muJ energy, sub-50-fs pulses at 800 nm with a 100-kHz repetition rate. This output was used to drive a beta-BaB(2)O(4) optical parametric amplifier followed by a difference-frequency generator based on a AgGaS(2) crystal. Continuous tuning of ultrafast pulses from 2.4m to longer than 12mum was obtained. A performance comparison of difference-frequency generation in type I and type II phase-matched AgGaS(2) is reported.