Nuclear structure studies on halo nuclei by direct reactions with radioactive beams

The investigation of direct reactions with exotic beams in inverse kinematics gives access to a wide field of nuclear structure studies in the region far off stability. The basic concept and the methods involved are briefly discussed. The present contribution will focus on the investigation of light neutron-rich halo nuclei. Such nuclei reveal a new type of nuclear structure, namely an extended neutron distribution surrounding a nuclear core. An overview on this phenomenon, and on the various methods which gave first evidence and qualitative confirmation of our present picture of halo nuclei, is given. To obtain more quantitative information on the radial shape of halo nuclei, elastic proton scattering on neutron-rich light nuclei at intermediate energies was recently investigated for the first time. This method is demonstrated to be an effective means for studying the nuclear matter distributions of such nuclei. The results on the nuclear matter radii of ⁶He and ⁸He, the deduced nuclear matter density distributions, and the significance of the data on the halo structure is discussed. The present data allow also a sensitive test of theoretical model calculations on the structure of neutron-rich helium isotopes. A few examples are presented. The investigation of few-nucleon transfer reactions in inverse kinematics may provide new and complementary information on nuclear structure, as well as astrophysical questions. The physics motivation and the experimental concept for such experiments, to be performed due to momentum matching reasons at low incident energies around 5–20 MeV/u at the new generation low energy radioactive beam facilities SPIRAL, PIAFE, etc., is briefly discussed.     

Possibilities of producing superheavy nuclei in multinucleon transfer reactions based on radioactive targets

The multinucleon transfer(MNT) process has been proposed as a promising approach to produce neutronrich superheavy nuclei(SHN).MNT reactions based on the radioactive targets ~(249)Cf,~(254)Es,and ~(257)Fm are investigated within the framework of the improved version of a dinuclear system(DNS-sysu) model.The MNT reaction~(238)U+~(238)U was studied extensively as a promising candidate for producing SHN.However,based on the calculated cross-sections,it was found that there is little possibility to produce SHN in the reaction ~(238)U+~(238)U.In turn,the production of SHN in reactions with radioactive targets is likely.     

Fission experiments with secondary beams

Nuclear fission from excitation energies around 11 MeV was studied at GSI, Darmstadt for 76 neutron-deficient actinides and pre-actinides by use of relativistic secondary beams. The characteristics of multimodal fission of nuclei around ²²⁶Th are systematically investigated and related to the influence of shell effects on the potential-energy and on the level density between saddle point and scission. A systematic view on the large number of elemental yields measured gave rise to a new interpretation of the enhanced production of even elements in nuclear fission and allowed for a new understanding of pair breaking in fission.     

Sub and near barrier fusion of neutron rich heavy nuclei – studies with radioactive ion beams

The availability of accelerated fission fragments at HRIBF allows us to study fusion reactions where one of the reactants is a short-lived exotic nucleus. Most interesting in this respect are entrance channels involving neutron-rich target and projectile – where enhanced survival probability of the compound system may allow the synthesis of heavier system. Much depends though on the dynamic evolution of the captured nuclei into a compound nucleus and the ensuing competition between fission and evaporation residue decay modes. Our studies of fusion between heavy neutron-rich nuclei are aimed at acquiring data that will lead to the understanding and eventually the ability to predict the probabilities for these different processes.     

Detection of modulated molecular beams with electron bombardment detectors

By means of refinements in the modulated molecular beam technique the signal-to-noise ratio can be greatly improved, and differential cross-sections, for collision of molecuies of the same species, can be measured. This was accomplished by combining beam modulation and phase sensitive detection with very sharp turning on the front end of the lock-in-amplifier and long integration times on the output. In addition, the signal-to-noise ratio of the Ar-Ar system as a function of integration time was investigated using two different types of electron bombardment detectors an Aberth ion-source and a quadrupole mass filter. With an integration time of 40 min the estimated upper limit to the signal-to-noise ratio is 1500 to 1 for the Aberth ion-source. Using quadrupole mass filter with an integration time of 60 min the estimated upper limit to the signal-to-noise ratio is 5 × 10⁴ to 1. For chemical kinetics studies this ratio may be two orders of magnitude higher. Measurements were carried out at the Purdue University, Lafayette, Indiana, USA.     

Nuclear physics with RI Beam Factory

Research activities of nuclear physics at Radioactive Isotope Beam Factory over 10 years are reviewed and future directions are also discussed. Conceptual ideas in designing the facility as well as experimental devices are introduced. Special emphasis is given to highlighted results obtained at RIBF.     

Reactions with fast radioactive beams of neutron-rich nuclei

The neutron dripline has presently been reached only for the lightest nuclei up to the element oxygen. In this region of light neutron-rich nuclei, scattering experiments are feasible even for dripline nuclei by utilizing high-energy secondary beams produced by fragmentation. In the present article, reactions of high-energy radioactive beams will be exemplified using recent experimental results mainly derived from measurements of breakup reactions performed at the LAND and FRS facilities at GSI and at the S800 spectrometer at the NSCL. Nuclear and electromagnetically induced reactions allow probing different aspects of nuclear structure at the limits of stability related to the neutron-proton asymmetry and the weak binding close to the dripline. Properties of the valence-neutron wave functions are studied in the one-neutron knockout reaction, revealing the changes of shell structure when going from the beta-stability line to more asymmetric loosely bound neutron-rich systems. The vanishing of the N = 8 shell gap for neutron-rich systems like ¹¹Li and ¹²Be, or the new closed N = 14, 16 shells for the oxygen isotopes are examples. The continuum of weakly bound nuclei and halo states can be studied by inelastic scattering. The dipole response, for instance, is found to change dramatically when going away from the valley of stability. A redistribution of the dipole strength towards lower excitation energies is observed for neutron-rich nuclei, which partly might be due to a new collective excitation mode related to the neutron-proton asymmetry. Halo nuclei, in particular, show strong dipole transitions to the continuum at the threshold, being directly related to the ground-state properties of the projectile. Finally, an outlook on future experimental prospects is given.     

Elastic scattering and reactions of light exotic beams

The present work provides a literature survey of elastic scattering of exotic nuclei from ⁶He to ¹⁷F. It presents a set of definitions that allow different analyses to be put into a common language. A calculational approach is proposed that yields consistent results across different beams and targets so that conclusions concerning the influence of virtual and real breakup as well as transfer couplings on the elastic scattering may be drawn. Calculations of elastic scattering around the Coulomb barrier are emphasised, employing a Pb target whose large Z allows the interplay between nuclear and Coulomb forces to be exploited to maximise possible effects arising from proton or neutron haloes or skins. A series of test calculations is performed and where possible compared to data, demonstrating that there are instances where coupling to transfer channels can have a large effect on the elastic scattering angular distributions. By careful choice of target/beam combination, different aspects of the coupling effects may be emphasised.     

Photofission for the production of radioactive beams: Experimental data from an on-line measurement

A PARRNe 1 experiment (Production d'Atomes Radioactifs Riches en Neutrons) aimed at the production of neutron-rich radioactive noble gases produced by photofission has been performed at CERN. The LEP Pre-Injector (LPI) has been used to deliver a 50 MeV electron beam. The results obtained show clearly that the use of an electron beam to produce neutron-rich fission fragments for futur RNB facilities is an option that should not be neglected. Received: 20 July 2001 / Accepted: 5 June 2002 / Published online: 19 November 2002 RID="a" ID="a"e-mail: ibrahim@ipno.in2p3.fr Communicated by D. Guerreau     

Synthesis and decay properties of superheavy atoms in nuclear reactions induced by stable and radioactive ion beams

This talk consists of two parts. The first one presents the results of investigations performed in 1998-2000 in Dubna on the synthesis of superheavy nuclei in reactions induced by ⁴⁸Ca ions. The radioactive decay properties of the nuclei, indicating a considerable increase in the α-decay and spontaneous fission half-lives of the isotopes of elements 110-116 when approaching the closed neutron shell at N = 184, are given. In the second part the possible ways of advancing into the region of more neutron-rich nuclei, using stable and radioactive ion beams, are discussed. Since so far no intense radioactive ion beams are available, some experiments with stable beams are considered as a test for the suggested ideas. Received: 1 May 2001 / Accepted: 4 December 2001     

First results from laser spectroscopy on bunched radioactive beams from the JYFL ion-beam cooler

A new RFQ ion-beam cooler and buncher, installed after the mass-separating magnet of the ion guide isotope separator, IGISOL, JYFL, has dramatically increased the scope of on-line laser spectroscopy at this facility. The device, operated in a bunching mode, has permitted new measurements on short-lived radionuclei in the Ti, Zr and Hf chains at a sensitivity two orders of magnitude greater than that previously achieved. The device has also opened new prospects for laser-based nuclear spectroscopy at the facility, particularly collinear resonance ionisation spectroscopy. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"e-mail: pc@mags.ph.man.ac.uk     

Experimental nuclear astrophysics with radioactive ion beams

Reactions involving unstable nuclei play an important role in many astrophysical sites. Radioactive ion beams provide a unique tool to investigate the structure of such unstable nuclei as well as the cross sections for many reactions of astrophysical relevance. This paper provides a brief survey of some recent results in experimental nuclear astrophysics with Radioactive Ion Beams, particularly for processes which take place during explosive hydrogen burning in novae and X-ray bursts. Some prospects for future studies at next generation facilities are also briefly discussed.     

Shell effects and pairing correlations in fission investigated with radioactive beams

The secondary-beam facility at GSI allows to produce a large variety of exotic nuclei at relativistic energies. This technique offers a unique oportunity to investigate systematically fission in inverse kinematics. In the present experiment, the fission properties of more than 70 different actinides and preactinides were investigated at low excitation energy. The elemental yields and kinetic energies of the fission residues present new signatures of shell structure and pairing correlations. Received: 1 May 2001 / Accepted: 4 December 2001     

ISOL beams of hafnium isotopes and isomers

The production of ISOL beams of hafnium is described. Radioactive Hf isotopes were produced at ISOLDE by 1.4 GeV proton-induced spallation in Ta and W foils. Chemical evaporation in form of HfF₄ and mass separation in the molecular sideband HfF₃⁺ after electron impact ionization provided intense and pure beams. Beams of ^158-185Hf and short-lived isomers down to 1.1 s ^177mHf were observed, but the method could be extended to reach even more exotic isotopes: down to about ¹⁵⁴Hf (N=82) on the neutron-deficient side and up to neutron-rich ¹⁸⁸Hf.     

(Im-)possible ISOL beams

Refractory elements, i.e. elements with very high melting point and low vapor pressure, cannot be released in atomic form from an ISOL target. Therefore most of these elements are presently not available as ISOL beams. However, when reactive gases are introduced into the target, they may form volatile compounds with the refractory elements, allowing for an easier transport to the ion source. Particularly useful are high-temperature stable fluorides and oxides. By these chemical evaporation methods so far ISOL beams of the refractory elements C, Zr, Hf and Ta have been produced. We discuss how ISOL beams of B, Ti, Nb, Mo, Tc, Ru, W, Re, Os and Ir could be produced in a similar way.     

Integrated target-ion source unit for on-line production of radioactive short-lived isotopes

A new version of integrated target-ion source unit (ionising target) has been developed for the on-line production of radioactive single-charged ions. The target is able to withstand temperatures up to 2500 ^°C and acts also as an ion source of the surface and laser ionisation. Off-line and on-line experiments with the ionising target, housing tantalum foils as a target material, have been carried out at the IRIS (Investigation of Radioactive Isotopes on Synchrocyclotron) facility. The off-line surface ionisation efficiency measured for stable atoms of Li, Rb and Cs was correspondingly 6% , 40% and 55% at the target temperature of 2000 ^°C and 3-10% for atoms of rare-earth elements Sm, Eu, Tm and Yb at a temperature of 2200 ^°C. The off-line measured values of the ionisation efficiency for stable Gd and Eu atoms by the laser beam ionisation inside the target were 1% and 7%, respectively. The radioactive beam intensities of neutron-deficient rare-earth nuclides from Eu to Lu produced by the integrated target-ion source unit have been measured at a temperature of 2500 ^°C. The results of the integrated target-ion source unit use for on-line laser resonance ionisation spectroscopy study of neutron-deficient Gd isotopes have been also presented.     

Physical preseparation: A powerful new method for transactinide chemists

In recent years, the concept of physical preseparation of single atoms was introduced into the field of transactinide chemistry. In this approach, the transactinide element of interest is isolated in a physical recoil separator and then extracted from this machine. The beam as well as the unwanted reaction products are strongly suppressed, allowing for the investigation of new chemical systems that were not accessible before. The most important aspects of the technique are discussed and the advantages for chemistry experiments with transactinides are presented, using some of the chemical studies that were performed with preseparated isotopes as examples.     

Potential and limitations of nucleon transfer experiments with radioactive beams at REX-ISOLDE

As a tool for studying the structure of nuclei far off stability the technique of γ-ray spectroscopy after low-energy single-nucleon transfer reactions with radioactive nuclear beams in inverse kinematics was investigated. Modules of the MINIBALL germanium array and a thin position-sensitive parallel plate avalanche counter (PPAC) to be employed in future experiments at REX-ISOLDE were used in a test experiment performed with a stable ³⁶S beam on deuteron and ⁹Be targets. It is demonstrated that the Doppler broadening of γ lines detected by the MINIBALL modules is considerably reduced by exploiting their segmentation, and that for beam intensities up to 10⁶ particles/s the PPAC positioned around zero degrees with respect to the beam axis allows not only to significantly reduce the γ background by requiring coincidences with the transfer products but also to control the beam and its intensity by single particle counting. The predicted large neutron pickup cross-sections of neutron-rich light nuclei on ²H and ⁹Be targets at REX-ISOLDE energies of 2.2 MeV ^. A are confirmed. Received: 9 October 2000 / Accepted: 28 January 2001     

Production of low- and high-energy radioactive-ion beams by fragmentation

The physics opportunities made possible by beams of rare isotopes are among the richest available in nuclear science. The rare-isotope accelerator (RIA) now under development is an innovative accelerator that will define the state of the art for all such facilities. A novel aspect of the RIA project is the conversion of the most intense high-energy heavy-ion beams into both fast and reaccelerated exotic beams. Along with target fragmentation in next-generation high-power ISOL targets, RIA will use projectile fragmentation in a high-energy separator/gas-filled ion collector system to provide an extensive range of thermalized ions for reacceleration. In addition, a second high-energy separator will provide the same or larger range of ions for high-energy experiments. A brief overview of the RIA accelerator concept, the layout of the facility, and production techniques will be given along with information on the present R&D efforts in gaseous-ion collection. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"e-mail: morrissey@nscl.msu.edu