Nuclear structure of <Superscript>76</Superscript>Ge from proton-neutron interacting boson model calculations

The properties of low-lying states in ⁷⁶Ge, especially the characteristics of the mixed-symmetry states, have been investigated within the neutron-proton interacting boson model (IBM-2). By considering the relative energy of d proton boson to be different from that of neutron boson, the low-lying positive parity levels and M1, E2 transition strengths have been calculated. The IBM-2 calculated results are in good agreement with the experimental data. Particularly, the mixed-symmetry states have been reproduced quite well. The calculation and systematic analysis demonstrated that the collective character of ⁷⁶Ge lies closest to the SU*_πv(3), with some possible O_πv(6) dynamic symmetry in IBM-2 viewpoint.     

Shape coexistence close to N=50 in the neutron-rich isotope ~(80)Ge investigated by IBM-2

The properties of the low-lying states,especially the relevant shape coexistence in~(80)Ge,close to one of most neutron-rich doubly magic nuclei at N=50 and Z=28,have been investigated within the framework of the proton-neutron interacting model(IBM-2).Based on the fact that the relative energy of the d neutron boson is different from that of the proton boson,the calculated energy levels of low-lying states and E2 transition strengths can reproduce the experimental data very well.Particularly,the first excited state 0_2~+,which is intimately related to the shape coexistence phenomenon,is reproduced quite nicely.Theρ~2(E0,0_2~+→0_1~+)transition strength is also predicted.The experimental data and theoretical results indicate that both collective spherical andγ-soft vibration structures coexist in~(80)Ge.     

A study of the (3He,n) reaction on isotopes of tin

The (³He, n) reaction has been studied on^{112,116,118,120,124}Sn at 25.4 MeV. Angular distributions were measured over the range 0°–25° and the results compared with predictions of zero-range DWBA calculations. In addition to the around-state transitions, L = 0 transitions were also observed to low-lying states in every case. Simple two component wave functions, as well as those obtained from a more sophisticated pairing model, are compared with the data in order to explain the appearance of the anomalously low-lying excited 0⁺ states observed. L = 2 transitions were observed to low-lying 2⁺ states, but the strength of these transitions was much less than expected from the systematics of (t, p) results for N = 50 nuclei.     

Excited state geometry optimisation using Fock-space multi-reference coupled cluster method

The Fock-space multi-reference coupled cluster method is used for the geometry optimisation of the low-lying excited states of the molecules. Molecular geometries of the carbon monohydride cation (CH)⁺, water (H₂O), ozone (O₃) and formaldehyde (HCHO) in their low-lying excited states are optimised. Excited state gradients are calculated using finite field multi-reference coupled cluster method. We compare our results with other theoretical and/or experimental results, wherever available.     

States of 12ΛC formed in the reaction 12C(K−, π−)

States of ¹²_ΛC formed in the (K^?, π^?) reaction have been studied for momentum transfers up to 260 MeV/c, using an incident K^? beam of 800 MeV/c momentum. The angular distributions for the g.s. and for a peak at 11 meV have been measured between 0° and 19° in the laboratory. Limits on the splitting of the 11 MeV peak and on the formation of low-lying excited states are given.     

Electronic states of the CeO molecule: Absorption,emission, and laser spectroscopy

The electronic spectrum of the CeO molecule is characterized by the existence of many 0-0 bands resulting from transitions between various Ω components of excited states and the 16 lower Ω states which arise from the lowest configuration… (4f)(6s). Classical studies of rotational structure of absorption and emission spectra have been extended, and argon-ion and tunable dye (coumarin 460, rhodamine 6G, rhodamine 101) lasers have been used to excite known transitions in bands which had previously been rotationally analyzed. The resulting fluorescence spectra have been used to establish the relative energies of the lower states. By tuning the lasers to excite analyzed transitions from different known electronic states it has been possible to determine the energies of 16 low-lying states, to assign quantum numbers to 14 with certainty, and to suggest assignments for the other 2. The resulting energy level diagram of lower states is discussed and shown to correlate well with the 4f6s configuration of the Ce²⁺ ion. From the energies of the low-lying states, those of the higher excited states are calculated and in some cases new values of vibrational and rotational constants are derived.     

Electronic states and spectroscopic properties of MgH in absence and presence of spin–orbit coupling − a configuration interaction study

Electronic spectrum of astrophysically important molecule magnesium hydride (MgH) has been studied using configuration interaction methodology excluding and including spin–orbit coupling. Potential energy curves of several spin-independent (Λ?S) electronic states have been constructed and spectroscopic constants of low-lying bound Λ?S states within 8.2 eV of term energy are reported in the first stage of calculations. The X²Σ⁺ is identified as the ground state in the Λ?S level. In the subsequent stage, the spin–orbit interaction has been incorporated and its effects on the potential energy curves and spectroscopic features of different electronic states of the species have been investigated. The X²Σ⁺_1/2 is identified as the spin–orbit (Ω) ground state of the species. Transition moments of several dipole-allowed transitions are computed in both the stages and radiative lifetimes of the corresponding excited states are computed. Electric dipole moments (µ) for a number of low-lying bound Λ?S states as well as several low-lying Ω-states are also calculated in the present study.     

Study of low-lying levels in 47Ca with the 48Ca(d, t)47Ca reaction

Angular distributions of cross sections [α(θ)] and vector analyzing powers [iT₁₁(γ)] have been measured for seven low-lying states or groups of states excited by the ⁴⁸Ca($\text{d}$, t)⁴⁷Ca reaction with 13.5 MeV deuterons and analyzed by the DWBA. On the basis of comparison of vector analyzing powers with DWBA calculations, spin-parity assignments have been made or confirmed for several states. Spectroscopic factors have been extracted. Angular distributions for weak states at 3.30 and 3.57 MeV excitation in ⁴⁷Ca could not be reproduced by DWBA calculations. Investigations of compound nucleus and multi-step contributions to the cross sections and analyzing powers for these states have been made by means of Hauser-Feshbach and CCBA calculations. Optical model parameters were obtained from analysis of 13.5 MeV deuteron elastic scattering cross sections and analyzing powers.     

Ab initio study of ground and low-lying excited states of MgLi and MgLi+ molecules with valence full configuration interaction and MRCI method

The ground and low-lying excited states of MgLi and MgLi⁺ molecules have been investigated. The potential energy curves and the permanent and transition dipole moments of the MgLi and MgLi⁺ molecules are determined making use of the multi-reference configuration interaction and valence full configuration interaction with large basis sets. The core–valence correlation and scalar relativistic correction are also taken into account with aug-cc-pCVQZ basis set and the third-order Douglas–Kroll Hamiltonian approximation, respectively. The transition dipole moments are used to evaluate the radiative lifetimes of the vibrational levels for the low-lying excited states of the MgLi and MgLi⁺ molecules. The derived spectroscopic constants of the ground and low-lying excited states are in good agreement with available experimental and theoretical works.     

对力对希土原子核性质的影响

本文利用粒子数守恒方法分析对力对希土区变形偶偶核的各种性质的影响,其中包括低内部激发态(E≤2MeV)的激发机构、有关的β衰变和奇偶质量差等。为进行这些分析,本文先确定希土变形核内的单粒子能级。分析表明:适当改变参数μ和к以后的Nilsson能极,在考虑对力影响后,能较好地解释奇A核的低内部激发谱的自旋和宇称,并能近似地解释其能级间隔。参数μ,к,和η是由奇A核的实验能谱来确定的。在希土转动区中,к～0.067—0.072,η～4—4.6.     

A high resolution spectroscopic study of rhodium monochloride

Rhodium monochloride has been observed and characterized spectroscopically for the first time. The RhCl molecules were produced in a laser vaporization molecular beam source by the reaction of a laser vaporized rhodium plasma with CCl₄ doped in helium, and laser-induced fluorescence and dispersed fluorescence were used to study 15 of the strongest bands spanning the 535-415 nm region. Twelve of these bands were studied at high resolution using a cw ring dye laser. Two low-lying states separated by 140 cm⁻¹ have been observed. The ground state has Ω = 2 and is attributed to a ³Π_i state resulting from a δ⁴π³σ¹ electronic configuration. The other low-lying state has Ω = 3 and is attributed to a ³Δ_i state resulting from a δ³π⁴σ¹ electronic configuration. Excited states with Ω values ranging from 1 to 4 have been observed. Dispersed fluorescence from these excited levels has been used to identify a large number of low-lying electronic states within an energy range of 5200 cm⁻¹ and has also been used to determine a ground state vibrational frequency of ∼348 cm⁻¹. Λ-doublings have been observed in all the transitions studied at high resolution.     

The low-energy level structure and the electromagnetic properties of191Ir and193Ir

TheM 1 andE 2 reduced transition probabilities in¹⁹¹Ir and¹⁹⁹Ir have been calculated on the weak particle-core coupling model. The static moments of the ground state and the first three low-lying excited states have been computed. The theoretical values are in good agreement with the experimental results, in particular, the existing discrepancy between the theoretical and the experimental value for the magnetic moment of the first excited 5/2⁺ state, in both these nuclei, has been removed. The predicted sign of the quadrupole moment of the 2⁺ state in the neighbouring even-even nuclei is consistent with the results reported for Platinum nuclei. The level structure of both these nuclei has been calculated assuming the particle-core interaction to be dipole-dipole and quadrupole-quadrupole type.     

Level structure of the doubly odd nucleus 112In from the (p,nγ) reaction

Properties of the levels in ¹¹²In have been studied with the reaction ¹¹²Cd(p, nγ)¹¹²In. The level scheme of ¹¹²In below 1300 keV was constructed from the γ-ray excitation functions and γγ coincidences. In ¹¹²In, 22 excited states were observed and spins and parities of 8 excited states were newly assigned or restricted by comparing the measured angular distributions and linear polarizations of the deexciting γ-rays as well as the excitation functions of the residual levels with the predictions of the statistical compound nucleus model. Possible configurations of the low-lying levels are discussed in terms of their decay properties and the systematics of the excited states in the neighbouring doubly odd In isotopes.     

High-Resolution Survey of the Visible Spectrum of NiF by Fourier Transform Spectroscopy

High-resolution spectra of NiF have been recorded in emission by Fourier transform spectroscopy using a very stable discharge source. The 0-0 bands of 14 electronic transitions have been studied, 6 of them for the first time. This work confirms the presence of 5 low-lying spin components X²Π_3/2, [0.25]²Σ⁺, [0.83]A²Δ_5/2, [1.5]B²Σ⁺, and [2.2]A²Δ_3/2 as known from previous laser-induced fluorescence experiments. Eight electronic states are now identified in the 18 000-24 000 cm⁻¹ range above the ground X²Π_3/2 state. Electronic assignments for these excited states are not always obvious because of violations of the selection rules and unusual fine structure parameters. We think that some of the upper states are spin components of quartet states. In such a congested spectrum, high-resolution spectra are best analyzed in conjunction with an energy level diagram constructed mainly by dispersed low resolution laser-induced fluorescence.     

55Mn(n,n'γ) cross-section studies for En = 1.0–3.6 MeV

Absolute ⁵⁵Mn(n, n′γ) γ-ray production cross sections have been measured for 19 transitions from levels up to and including the 2429 keV state in ⁵⁵Mn over the energy range E_n = 1.0–3.6 MeV. Angular distributions were also measured for 6 of the transitions. Branching ratios were extracted and total inelastic neutron cross sections were inferred for these ⁵⁵Mn excited states. The measured and inferred cross sections are compared with calculated cross sections using the statistical compound nucleus theory.     

Investigation of22Na excited states

Fourteen²¹Ne(p, γ)²²Na resonances have been observed in the rangeE _p =300–1,300 keV. Theγ-decay of all these resonances has been investigated by means of a 38 cm³ Ge(Li) detector. Energies and branching ratios of several bound states have been determined. TheQ-value was determined as 6,738.5±1.7 keV. Lifetimes of seven states were determined with the Doppler-shift attenuation method. The observed upper limit (τ _m ≦4 fs) of the lifetime for the 4,071 keV state, regarded as the analogue of the third excited state in²²Ne, and the transition observed from this state to the 1,528 keV state do not support the proposed rotational band structure of the²²Na low-lying states.     

Collective states in 48V

The low-lying positive parity states of ⁴⁸V have been studied in the framework of deformed configuration mixing model calculations based on projected Hartree-Fock theory, within the full fp shell space. The modified Kuo-Brown effective interaction has been used. The calculated spectrum and the electromagnetic properties of these states are in good agreement with the experiment. The calculation predicts an excited low-lying collective K = 2⁺ band in the spectrum of ⁴⁸V and accounts for the observed breakdown of the “signature” selection rule arising in the shell-model calculation within the ($\text{f}\text{7}\text{2}\text{)}{}^{\mathrm{nd}}$ space. It does not favour a 5⁺ assignment to the observed 1.099 MeV level. Two sets of proton and neutron effective charges (i) e_p = 1.32e and e_n = 0.89e and (ii) Kuo and Osnes charges e_p = 1.25e and e_n = 0.47e were employed. The observed decay properties appear to favour the latter charges. Our model also explains in a semiquantitative way the observed K-value, moment of inertia parameter and the intrinsic quadrupole moment of the K = 1^?1 rotational band.     

Coulomb excitation of the odd-odd isotopes 106, 108In

The low-lying states in the odd-odd and unstable isotopes ^{106, 108}In have been Coulomb excited from the ground state and the first excited isomeric state at the REX-ISOLDE facility at CERN. With the additional data provided here the $ \pi$ g _9/2 ^-1 ? $ \nu$ d _5/2 and $ \pi$ g _9/2 ^-1 ? $ \nu$ g _7/2 multiplets have been re-analyzed and are modified compared to previous results. The observed $ \gamma$ -ray de-excitation patterns were interpreted within a shell model calculation based on a realistic effective interaction. The agreement between theory and experiment is satisfactory and the calculations reproduce the observed differences in the excitation pattern of the two isotopes. The calculations exclude a 6⁺ ground state in ¹⁰⁶In . This is in agreement with the conclusions drawn using other techniques. Furthermore, based on the experimental results, it is also concluded that the ordering of the isomeric and ground state in ¹⁰⁸In is inverted compared to the shell model prediction. Limits on B(E2) values have been extracted where possible. A previously unknown low-lying state at 367keV in ¹⁰⁶In is also reported.