Levels in182W populated in the decay of182Ta

Theγ-rays emitted in theβ-decay of¹⁸²Ta have been reinvestigated with improved statistics in attempting to clarify the reported new levels at 1460.41, 1592.98, 1620.36, 1712.29 and 1762.91 keV in¹⁸²W observed in theβ-decay of¹⁸²Ta. The present study demonstrated that the fifteen newγ-rays, which were used to support the existence of the five new levels, are not relevant to theγ-decay of¹⁸²Ta. Therefore the five new levels are not populated in this decay. Additionally, theγ-ray with an energy of 1035.6 keV (0 ₂ ⁺ →2 ₁ ⁺ ) deexciting theβ-band head in¹⁸²W is observed for the first time in the present decay study and the previous tentative placement of the 351.0 keVγ-ray in the level scheme is confirmed by the present coincidence measurements.     

Ground state properties and β-decay half-lives near 132Sn in a self-consistent theory

The level scheme of⁹⁵Tc has been investigated with Ge(Li)-detectors by observing the γ-rays after the decay of 1.65 h⁹⁵Ru. The energies and intensities of theγtransitions were extracted fromγ-singles andγγ-coincidence spectra. In the decay of⁹⁵Ru 88γ-transitions were observed; a scheme of⁹⁵Tc with 25 levels is proposed into which 86 transitions could be accomodated. Spin and parity assignments were made from log (ft) values andγ-ray branching ratios. The level structure of⁹⁵Tc is compared with that of the other odd Tc isotopes.     

Nuclear resonance fluorescence in94Mo,95Mo and96Mo

Using gaseous sources of Tc₂O₇ containing the radioactive isotopes⁹⁴Tc,⁹⁵Tc and⁹⁶Tc, levels at 871.0keV (⁹⁴Mo), 765.8, 820.6, 947.8, 1074.0keV (⁹⁵Mo) and 778.3keV (⁹⁶Mo) have been excited. From the effective cross sections for nuclear resonance scattering and from the lifetimes of the 947.8, 1074.0 and 778.3keV levels known from Coulomb excitation experiments the profiles of theγ-lines have been determined. A broadening of theγ-lines due to Coulomb explosion of the molecules has been observed. Making use of the line profiles, lifetimes ofΤ=(6.4±1.0) ps andΤ=(0.90 ± 0.20) ps have been determined for the 765.8 and 820.6keV levels, respectively. The angular distribution of the resonantly scattered radiation yields an amplitude ratioδ for the mixed M1 E2 765.8keV transition ofδ=0.14 _?0.009 ^+0.08 . TheB(E2) from a Coulomb excitation experiment and the lifetimeΤ from the present experiment yield ¦δ¦=0.07±0.01 for the 820.6keV transition.     

Electron capture ratios in206Bi

The level scheme of⁹⁷Tc has been investigated by observing theγ-rays following the decay of 2.9-d⁹⁷Ru.γ-singles andγγ-coincidence measurements were carried out with Ge(Li)-detectors. The time difference of coincident γ-rays was measured as a third parameter. From the coincidence events, the intensities ofγγ-cascades were extracted. The⁹⁷Ru decay gives rise to 18γ-lines which could be fitted into a level scheme of⁹⁷Tc consisting of 9 levels. Spin and parity assignments of the levels were made from log(ft) values andγ-ray branching ratios. Discrepancies concerning the energy of the first 3/2^? state and the existence of a 946 keV level are discussed.     

The beta decay of90g Tc and90m Tc

The level structure of⁹⁰Mo is investigated via the beta decay of^90g Tc and^90m Tc whose half-lives are measured to be 8.7±0.2 and 49.2±0.4 s, respectively. The decay properties are studied by means of beta and gamma spectroscopy techniques. The level structure of⁹⁰Mo populated in the decays of both isomers is proposed with deducedJ ^π values. Theβ-decay energies for^90g Tc and^90m Tc are 8.8±0.3 and 9.3±0.3 MeV, respectively. The structure is discussed in terms of the shell model.     

An investigation of short-lived isomers in the nuclei90,92Nb,99Mo,98,100,101Tc and101Ru

Short-lived isomers in the nuclei^90,92Nb,⁹⁹Mo,^98,100,101Tc and¹⁰¹Ru populated in photonuclear reactions were studied by pulsed beam techniques. Energy and half-life of theγ-rays deexciting the isomeric levels were measured by recording energy-time spectra. The delayedγ-rays andK X-rays were detected by means of an intrinsic Ge-detector of high resolution. From the measured intensity ratios internal conversion coefficients were determined. The multipolarities of the isomeric transitions could be deduced in most cases. A classification of the observed isomers has been tried on the basis of the obtained experimental results and most recent literature data.     

Kernspektroskopische Untersuchungen zu den Termschemata der Kerne56Fe und56Co

Gamma-gamma directional correlations have been investigated for several cascades in⁵⁶Fe formed in the decay of⁵⁶Mn or⁵⁶Co. A combination of NaI(Tl) and Ge(Li) detectors was used for the experiments. It was established that a level at 3601 keV is populated in the decay of⁵⁶Co. Spins given in the paranthesis were assigned to levels at the following energies: 2658(2), 2960(2), 3123(4), 3370(2), 3445(3), 3601(2), 3856(3), 4049(3), 4100(4), 4120(3), 4298(4), 4395(3) and 4459 keV (3,4). Multipole mixing ratios were determined forγ transitions of the following energies: 978, 1038, 1175, 1360, 1772, 1811, 1964, 2015, 2035, 2113, 2213, 2523, 2599, 3010, 3202, 3254, 3273, 3451 and 3548 keV. Theγ-rays from the decay of⁵⁶Co of energies 674.7 and 2657.4 keV have been observed for the first time, and the presence of several other weakγ-rays in the⁵⁶Fe decay has been confirmed. Nine angular correlations in the decay of⁵⁶Ni have been investigated. The spin sequence 4, 3, 2, 0, 1 was unambiguously determined for the levels at 0, 158.2, 970.1, 1450.7 and 1720.0 keV. The multipolarity of theγ-rays of energies 158.2, 749.9 and 811.9 keV was determined as almost pure M1. The results are discussed within the framework of recent shell model calculations.     

The decay of62Zn

Energies and relative intensities of 31γ-transitions from the decay of⁶²Zn have been measured using an anti-Compton spectrometer. Gamma-gamma coincidence measurements were performed. Besides the levels of⁶²Cu for which the population in the decay of⁶²Zn was known, also levels at 644.82, 698.32, 1221.5 and 1525.9 keV in⁶²Cu are found to be populated. The previously proposedβ-feeding of⁶²Cu levels at 1142.5 and 1280.8 keV is ruled out.     

The decay scheme of the 3-s Isomer of100Nb and the properties of levels in100Mo

Theβ ^? decay of the longer-lived isomer in¹⁰⁰Nb has been studied at the fission-product separator JOSEF. Measurements ofγ-ray singles spectra, ofγ-γ coincidences and ofγ-γ angular correlations have been performed. A value oft _1/2=2.99(11)s has been determined for the isomer which probably hasI ^π=4⁺ or 5⁺. A scheme of the levels of¹⁰⁰Mo which are populated in the decay of this isomer has been established. Information on the spins of several states of¹⁰⁰Mo has been obtained. Thus,I=0 levels have been identified at 1,505, 2,038 and 2,087 keV. The mixing ratios have been determined for the 2₂ ⁺→2₁ ⁺ and 2₃ ⁺→2₁ ⁺ transitions. The results provide evidence for a vibrational structure of¹⁰⁰Mo with separate bands based on the ground state and on the first excited 0⁺ level.     

The decay of93g Ru,93m Ru,91g Mo,91m Mo,91g Tc and91m Tc

Decay studies on a number of short-lived odd nuclei in theN=50 region are described. The 59.6-s ⁹³Ru ground state decay was studied in detail for the first time; in these experiments the 10.8-s activity^93m Ru was discovered. The⁹¹Tc activities were also observed for the first time. The ground state and an isomeric state of this nucleus decay with nearby equal half-lives (3.14 and 3.3-min). The activities^91g Mo (16.6-min) and^95m Mo (65.1-s) have been reinvestigated. A number ofγ-rays, previously erroneously assigned to the⁹¹Mo activities, could be eliminated. A strong similarity is noted for the decay schemes of theN=49 isotones^91m Mo and^93m Ru. The energy of the 1/2^? isomeric state in⁹³Ru and theB(M4)-value of the isomeric transition fit well into the systematics of the previously knownN=49 isotones.     

Measurements on117mSn

By combination of a differential and an integral measurement of perturbed angular correlations the sign and the magnitude of theg-factor of the 158.6 keV level in¹¹⁷Sn which is populated and depopulated by a 156.0 keV (M4)-158.6 keV (M1)-γ-γ-cascade was determined to beg=+ 0.45 _?0.30 ^+0.15 . An investigation of its halflife yieldedT _1/2=0.279 ± 0.009 nsec. The total conversion coefficient of theM4-transition was found to be 46.3 ± 1.8.     

Levels of195Au from the decays of195g Hg and195m Hg

The levels of¹⁹⁵Au were analyzed by observingγ-singles andγγ-coincidences following the¹⁹⁵Hg decay. Nine new lines are found which require two new levels at 778 and 946 keV. An interpretation of the level scheme is given on the basis of the de Shalit core-excitation model. A qualitative understanding of all levels up to 1 MeV excitation energy is obtained.     

Properties of electromagnetic transitions from high-spin states in94Mo

The multipole mixing ratios of transitions from 6⁺ and 8⁺ states in⁹⁴Mo, following the decay of⁹⁴Tc, have been measured by means ofγγ angular correlations. The spin of the 2423.4 keV state, being important for the interpretation ofγ cascades feeding this level, has been firmly established as 6⁺ by a method in which the angular correlation data are utilized in a non-conventional way. Furthermore, properties of electromagnetic transitions in⁹⁴Mo have been calculated in the shell model framework and are compared with the corresponding experimental quantities.     

β + ratio andβ-delayedγ-decay of146Eu

The positron decay of¹⁴⁶Eu was investigated, firstly to derive for the allowed transition to the 2046 keV state in¹⁴⁶Sm the electron capture to positron decay ratio. The experimental valueEC/β ⁺=43.7(42) is found to be in agreement within the respective error intervals with the ones calculated from the formalism of allowed decay using the recentQ-values of¹⁴⁶Eu. Further on, theγ-decay properties of¹⁴⁶Eu have been reinvestigated with emphasis on implied modifications of the hitherto accepted decay scheme: 42 new levels and 33 newγ-transitions were placed in the revised level scheme, 12 of the previously reported levels were deleted. The level distribution of¹⁴⁶Sm is discussed within a statistical model. The indication for a non-statisticalβ-strength function is observed.     

A high-resolution spectroscopic study of the gamma radiation from the decay of96Nb

The decay of 24h⁹⁶Nb has been studied with a Ge(Li) spectrometer and with a Ge(Li)-NaI(Tl) coincidence spectrometer. A total of 27 gamma-ray transitions were observed, their energies and intensities measured. All but one of these have been incorporated into the level scheme of⁹⁶Mo. The level at 1,625.9 keV reported recently in (n _th, γ) work on⁹⁵Nb has also been observed through the decay of⁹⁶Nb. No experimental evidence has been found for previously proposed levels at 2,657 and 2,791 keV in⁹⁶Mo.     

On the observability of enhancement effects in isochromat spectroscopic investigations of Pd and Rh

We have investigated theγ-rays from the decay of 46-min⁵¹Mn produced by the⁵⁰Cr (d, n) reaction. Twelveγ-rays were observed. Theseγ-rays have been incorporated into a level scheme of⁵¹Cr with levels at 0, 749.1, 1164.4, 1353.3, 1557.4, 1899.4, 2001.4, 2312.5 and 2829.7 keV. Branching ratios, logft values, and j^π assignments are discussed for these levels. The lifetime of the 749.1 keV level was measured to be T_1/2=7.6 ± 0.3 ns by utilizing the⁵¹V(p, n γ ⁵¹Cr reaction produced by a 3.8 MeV pulsed proton beam. The 749 keV,E2 transition is hindered by a factor of 34 compared to the Weisskopf estimate.     

γγ-Winkelkorrelationsmessungen an155Gd

Two Ge(Li) detectors were used to investigateγ transitions in¹⁵⁵Gd produced by the decay of¹⁵⁵Eu. Relative intensities were determined for the weak lines at 18.8, 26.5, 58.0, and 86.0 keV. Angular correlations for fourγ cascades were measured. As results, the mixing ratios of the 45.3 and 86.5 keVγ lines were determined, and it was shown that the sign of the mixing ratio is positive for theγ line at 18.8 keV and negative for the line at 60.0 keV. Spins 5/2 and 3/2 for the 86.5 and 105.3 keV levels, respectively, are consistent with the data, and spin 5/2 for the 105.3 keV level is inconsistent with it.     

Theβ + decay of the new isotope86Mo and the first observation of86m Nb

Theβ ⁺ decay of⁸⁶Mo has been firstly investigated by means ofβγ spectroscopy. The⁸⁶Mo nuclei were produced by fusion-evaporation reactions of⁵⁴ Fe (³⁵Cl, 1 p2n) and⁵⁸Ni (³²S,2p 2n) at beam energies of 103 and 120 MeV, respectively. Threeγ rays of 47.3, 49.8 and 187.0 keV were unambiguously identified to follow theβ ⁺ decay of⁸⁶Mo by results ofXγ andβγ coincidence and cross-bombardment. A half life and a maximumβ ⁺-ray energy of⁸⁶Mo were determined to be 19.6±1.1 s and 3.9±0.4 MeV, respectively. A decay scheme of⁸⁶Mo is proposed in this article. Furthermore, a decay of⁸⁶Nb has been studied using the same combinations of projectiles and targets, and a newβ-decaying isomer^86m Nb was observed with a half life of 56.3±8.3 s.