封离式He-N$lt;sub$gt;2$lt;/sub$gt;-CO$lt;sub$gt;2$lt;/sub$gt;激光器横模特性的测量与分析

利用激光光束分析仪,实时在线测量了一根He-N₂-CO₂封离式激光管的横模分布特性,得到了激光模式随放电电流的变化关系.实验表明该激光器在最佳工作电流时,容易形成低阶模运转,但很难获得基模运转,通过改善对称性以及加快冷却水流速可以获得基模运转.通过激光动力学过程分析了模式变化的形成原因,为大功率激光器模式控制与改善提供了一定的理论和实验借鉴. 关键词： 2激光')" href="#">CO₂激光 横模 激光模式分析 光束质量     

An experimental study of self-focusing and self-defocusing of a TEA CO2 laser pulse in CDF3

We observed self-focusing and self-defocusing of a TEA CO₂ laser pulse in CDF₃ vapor under different conditions. The experimental parameters we varied are the pressure inside the interaction cell, the frequency of the laser, the energy and the temporal length of the pulse. We have shown that it is possible to pass from self-focusing to self-defocusing by only increasing the intensity of the laser pulse. We propose a physical model that can explain these experimental results. This model is different from that used to explain the selffocusing of a CO₂ laser in SF₆.     

Surface evolution and laser damage resistance of CO2 laser irradiated area of fused silica

A 10.6 μm CO₂ laser has been reported to effectively mitigate the laser damage growth of fused silica. Two zones of the laser irradiated area are defined in this work: the distorted zone and the laser affected zone. The parameters of the two zones are studied at different CO₂ laser beam sizes, irradiation times, and powers by microscopy, profilometry, and photoelastic method. The results show that the diameter of laser affected zone is almost completely determined by the laser beam size and the distorted zone is associated with the mitigation range of CO₂ laser beam. The diameter and depth of the distorted zone increase as the laser power and irradiation time increase. The depth grows exponentially depending on the irradiation time. The maximum residual stress discrepancy is located near the boundary of the laser affected zone. The laser damage resistance test results show that the distorted zone and the laser affected zone have a better damage resistance than the original substrate.     

Laser micro-processing of amorphous and partially crystalline Cu45Zr48Al7 alloy

This paper presents a microstructural study of laser micro-processed high-purity Cu₄₅Zr₄₈Al₇ alloys prepared by arc melting and Cu-mould casting. Microprocessing of the Cu₄₅Zr₄₈Al₇ alloy was performed using a Rofin DC-015 diffusion-cooled CO₂ slab laser system with 10.6-μm wavelength. The laser was defocused to a spot size of 0.2 mm on the sample surface. The laser parameters were set to give 300- and 350-W peak power, 30% duty cycle and a 3000-Hz laser pulse repetition frequency (PRF). About 100-micrometer-wide channels were scribed on the surfaces of disk-shaped amorphous and partially crystalline samples at traverse speeds of 500 and 5000 mm/min. These channels were analysed using scanning electron microscopy (SEM) and 2D stylus profilometry. The metallographic study and profile of these processed regions are discussed in terms of the applied laser processing parameters. The SEM micrographs showed that striation marks developed at the edge and inside these regions as a result of the laser processing. The results from this work showed that microscale features can be produced on the surface of amorphous Cu–Zr–Al alloys by CO₂ laser processing.     

A note on tunneling in the presence of a superintense laser field

The influence of a superintense laser field on the transmission probability of a charged particle through a potential barrier is discussed. It is shown that the effect of the intense laser field is to weaken the potential barrier in such a way that its height decreases exponentially with the laser field. The implications to the ferro — to para - electric phase transition in BaTiO₃ under an intense CO₂ - laser field is also discussed.     

Effect of CO2 laser irradiation on the transport properties of La0.67Ba0.33MnO3 thin film

The effect of CO₂ laser irradiation on La_0.67Ba_0.33MnO₃ epitaxial thin film was investigated. Epitaxial thin films grown by pulsed laser deposition were irradiated by a CO₂ laser in air for 10-60 s. It is shown that after CO₂ laser irradiation treatment, the crystallinity of the film is strongly enhanced. It is found that a dramatic decrease in the resistivity of the CO₂-laser-irradiated film is accompanied by a remarkable increase in its insulator-metal transition temperature and the temperature coefficient of resistance. This significant improvement of its structure and properties is achieved in several dozens of seconds and surpasses that observed in films annealed in an oxygen atmosphere at 900 ^°C for 12 h, suggesting that CO₂ laser irradiation is a new and effective tool to optimize CMR manganites for bolometric applications.     

中远红外双波段激光器增益介质匹配

对中远红外双波段激光器中DF和CO2两种增益介质的匹配进行了研究。根据对DF和CO2两种增益介质分布的理论分析,发现DF相比于CO2介质增益峰值位置更靠前,激活区长度更短,据此设计加工了一台双波段激光器,使CO2气体注入孔位置可调,通过D2和CO2注入孔位置的差别来实现两种介质增益峰值位置的匹配。实验证明了这种设计是有效的,并确定了激光器共同光轴的最佳位置位于D2气注入孔下游3 mm,CO2注入孔下游33 mm处,此处双波段激光的输出功率均接近最大值。     

Two-photon pumping of random lasers by picosecond and nanosecond lasers

We experimentally demonstrated two-photon pumping of random lasers using picosecond and nanosecond pump lasers. The picosecond laser pumping experiment was performed with 400 ps laser pulses at 770 nm, and the gain media was a Coumarin 480D dye solution doped with TiO₂ nanoparticles. Onset of laser action was observed at a pump laser pulse energy below 500 μJ. The nanosecond laser pumping experiment was performed with 7 ns laser pulses at 1064 nm, and the gain media was a Rhodamine 640 dye solution doped with TiO₂ nanoparticles. Onset of laser action was observed at a pump laser energy ∼18 mJ. Our results suggest that there exists an optimal pulse duration of the pumping laser in two-photon pumped random lasing that leads to minimum photodamage of the gain media and still keeps a high pumping efficiency. PACS 33.50.Dq; 42.55.Mv; 42.55.Zz     

Influences of CO2 laser annealing on mechanical and laser-induced damage properties of ZrO2 thin films

Zirconium dioxide (ZrO₂) thin films were deposited on BK7 glass substrates by the electron beam evaporation method. A continuous wave CO₂ laser was used to anneal the ZrO₂ thin films to investigate whether beneficial changes could be produced. After annealing at different laser scanning speeds by CO₂ laser, weak absorption of the coatings was measured by the surface thermal lensing (STL) technique, and then laser-induced damage threshold (LIDT) was also determined. It was found that the weak absorption decreased first, while the laser scanning speed is below some value, then increased. The LIDT of the ZrO₂ coatings decreased greatly when the laser scanning speeds were below some value. A Nomarski microscope was employed to map the damage morphology, and it was found that the damage behavior was defect-initiated both for annealed and as-deposited samples. The influences of post-deposition CO₂ laser annealing on the structural and mechanical properties of the films have also been investigated by X-ray diffraction and ZYGO interferometer. It was found that the microstructure of the ZrO₂ films did not change. The residual stress in ZrO₂ films showed a tendency from tensile to compressive after CO₂ laser annealing, and the variation quantity of the residual stress increased with decreasing laser scanning speed. The residual stress may be mitigated to some extent at proper treatment parameters.     

Transient molecular absorptions induced by the absorption of CO2 laser radiation

Laser-induced molecular absorptions are reported for the species SF₆, CF₃I, and CF₃Br. Induced absorptions are observed at frequencies ～ 40 cm^-1 lower than that of a CO₂ TEA laser which is used to vibrationally excite the molecules in a low pressure cell. The dependence of the effect on pump laser intensity indicates that the species that exhibit the induced absorption have absorbed more than one laser photon. Applications of this phenomenon with respect to laser induced isotope separation are discussed.     

High power 4.65 μm single-wavelength laser by second-harmonic generation of pulsed TEA CO2 laser in AgGaSe2 and ZnGeP2

A high power 4.65 ??m single-wavelength laser by second-harmonic generation (SHG) of TEA CO₂ laser pulses in silver gallium selenide (AgGaSe₂) and zinc germanium phosphide (ZnGeP₂) crystals is reported. Experimental results show that the average output power of SHG laser is not only restricted by the damage threshold of the nonlinear crystals, but also limited by the irradiated power of fundamental-wave laser depending on the operating repetition-rate. It is found that ZnGeP₂ can withstand higher 9.3 ??m laser irradiation intensity than AgGaSe₂. As a result, using a parallel array stacked by seven ZnGeP₂ crystals, an average power of 20.3 W 4.65 ??m laser is obtained at 250 Hz. To the best of our knowledge, it is the highest output power for SHG of CO₂ laser by far.     

Nanoparticles produced by laser ablation of solids in liquid environment

A review of results on nanoparticles formation is presented under laser ablation of Ag, Au, and Ti solids targets in liquid environments (H₂O, C₂H₅OH, C₂H₄Cl₂, etc.). X-ray diffractometry (XRD), UV-Vis optical transmission spectrometry, and high-resolution transmission electron microscopy (HRTEM) characterise the nanoparticles. The morphology of nanoparticles is studied as a function of both laser fluence and nature of the liquid. The evidence of an intermediate phase of Au-Ag alloy is presented under exposure of a mixture of individual nanoparticles to laser radiation. Self-influence of the beam of a femtosecond laser is discussed under the ablation of the Ag target in liquids under Ti:sapphire laser. The factors are discussed that determine the distribution function of particle size under laser ablation. The influence of laser parameters as well as the nature on the liquid on the properties of nanoparticles is elucidated. PACS 42.62.-b; 61.46.+w; 78.66.-w     

Laser-induced desorption of polyatomic molecules with a CO2 laser

Laser-induced thermal desorption (LITD) has been increasingly employed as a tool for investigating surface processes. In LITD, a pulsed laser beam that is focused onto a surface induces a rapid temperature rise that causes desorption. In spite of the success enjoyed by the CO₂ laser in studies of diatomic molecules, its use with polyatomic molecules is shown to be severely limited by laser-induced dissociation. In desorption experiments with CH₃OH, HCOOH, CH₃NH₂ and NH₃ dissociation occurs only when the laser frequency coincides with an infrared absorption band of the molecule. Fragmentation may take place either on the surface or in the dense gas phase present above the surface during the laser pulse.     

Passively Q-switched laser performance of a diode-pump mixed Nd:Lu<Subscript>0.15</Subscript>Y<Subscript>0.85</Subscript>VO<Subscript>4</Subscript> crystal

A diode-pumped passively Q-switched Nd:Lu_0.15Y_0.85VO₄ laser with a GaAs output coupler is demonstrated. By using a mixed crystal Nd:Lu_0.15Y_0.85VO₄ as laser medium, the passively Q-switched laser can generate shorter pulse width with higher peak power in comparison with the passively Q-switched Nd:LuVO₄ or Nd:YVO₄ lasers under the same laser cavity. At the incident pump power 11.9 W, the minimum pulse width of 3.23 ns and the maximum peak power 1.67 kW can be obtained. The average output power and the pulse repetition rate of the laser are also measured. The experimental results show that the mixed crystal is a promising laser medium for shorter Q-switched pulse with higher peak power.     

Behavioral studies of gain and saturation energy density in a N2 laser with corona preionization

By the use of an oscillator-amplifier (OSC-AMP) TE N₂ laser system, both operating with corona preionizers, the laser parameters (small-signal gain g ₀ and saturation energy density E _s) have been measured at different N₂ gas pressure and for different states of the AMP preionizer. The details of our measurements are presented. In addition, the effect of He buffer gas on the laser parameters has also been investigated; it was found that both laser parameters remain almost constant up to 150 Torr of He gas pressure, indicating that He mainly affects the discharge uniformity. Finally, with the variation of the N₂ laser gain values in the literature, we found that the g ₀-N₂-laser parameter depends strongly on the length of the laser channel. Based on the most recent measurements, a graph showing this dependency is introduced.     

An X-ray preionised self sustained discharge HF/DF laser

We report the design and characterisation of a flash X-ray preionised, transversely excited HF/DF laser with energy outputs at the joule level. The laser used a H₂/D₂: SF₆ mixture at a pressure of around 120 Torr. X-ray photon fluxes and ionisation rates in the laser gas are presented and the laser dependence on these examined. It is shown that X-ray preionisation can be effective and it is estimated that the laser should operate satisfactorily with as little as 5% of the total stored electrical energy in the preionisation circuit. The laser performance is comparable to that of a UV preionised device with similar operating parameters.     

Gas contaminant effect in a discharge-excited ArF excimer laser

4 , O₂ and N₂ in a discharge-excited ArF-excimer laser. Measured characteristics include laser pulse energy, small-signal gain, and laser spectrum. Measurement results indicate that laser pulse energy degradation for such impurities (<100 ppm) is mainly due to optical absorption. It has also been found that for O₂ contaminants laser pulse energy degradation is strongly dependent on operational repetition rates; at higher repetition rates, an increased concentration of O₂ impurities results in a reduced small-signal gain and a consequent decline in laser pulse energy. Received: 12 June 1997/Revised version: 3 December 1997     

Laser (a pulsed Nd:YAG) cladding of AZ91D magnesium alloy with Al and Al2O3 powders

The laser surface cladding of an AZ91D magnesium alloy with Al and Al₂O₃ powders was investigated using a pulsed Nd:YAG laser. The optimum ratio of Al to Al₂O₃ and the suitable range of laser processing parameters were identified. The resulting microstructure in the modified surface layer was examined and the wear resistance property was evaluated. The results show that the wear resistance of the laser treated samples was much superior to that of the untreated samples.     

On the effects of using CO2 and F2 lasers to modify the wettability of a polymeric biomaterial

Enhancement of the surface properties of a material by means of laser radiation has been amply demonstrated previously. In this work a comparative study for the surface modification of nylon 6,6 has been conducted in order to vary the wettability characteristics using CO₂ and excimer lasers. This was done by producing 50 μm spaced (with depths between 1 and 10 μm) trench-like patterns using various laser parameters such as varying the laser power for the CO₂ laser and number of pulses for the excimer laser. Topographical changes were analysed using optical microscopy and white light interferometry which indicated that both laser systems can be implemented for modifying the topography of nylon 6,6. Variations in the surface chemistry were evaluated using energy-dispersive X-ray spectroscopy and X-ray photoelectron spectroscopy analysis which showed that the O₂ increased by up to 1.5 at% and decreased by up to 1.6 at% for the CO₂ and F₂ laser patterned samples, respectively. Modification of the wettability characteristics was quantified by measuring the advancing contact angle, which was found to increase in all instances for both laser systems. Emery paper roughened samples were also analysed in the same manner to determine that the topographical pattern played a major role in the wettability characteristics of nylon 6,6. From this, it is proposed that the increase in contact angle for the laser processed samples is due to a mixed intermediate state wetting regime owed to the periodic surface roughness brought about by the laser-induced trench-like topographical patterns.     

Comparison of eye-safe KTA OPOs pumped by Nd:YVO4 and Nd:YLF lasers

An eye-safe KTA OPO pumped by a Nd:YLF laser is demonstrated and a comparison with that pumped by a Nd:YVO₄ laser is performed. Although the slope efficiency of the continuous-wave free-running Nd:YLF laser is lower than that of the Nd:YVO₄ laser, the performance of KTA OPOs pumped by the Q-switched Nd:YLF laser is better, especially at lower repetition rates. The slope efficiency of KTA OPO pumped by a Nd:YLF laser is 14.6% at 30 kHz and 11.04% at 10 kHz. The better energy storage ability of Nd:YLF makes it an excellent laser medium in IOPOs.