Gyromagnetic ratios of excited states in 123, 125Te

The results of integral precession measurements are reported for $\text{3}\text{2}{}^{\mathrm{+}}$ and $\text{5}\text{2}{}^{\mathrm{+}}$ excited states in ^123,125Te. The measurements were made using the ion implantation perturbed angular correlation technique by recoiling the excited nuclei into polarized iron. The measured mean lifetimes and g-factors are: ${}^{123}\text{Te (440 keV,}\text{3}\text{2}{}^{\mathrm{+}}\text{) τ = 39±4 ps, g = 0.34 ± 0.06}$; $\text{(505 keV,}\text{5}\text{2}{}^{\mathrm{+}}\text{) τ = 26±3 ps, g = 0.04±0.025}$; and ${}^{125}\text{Te(443 keV,}\text{3}\text{2}{}^{\mathrm{+}}\text{) ρ = 27±3.3 ps, g = 0.39±0.06}$; $\text{(464 keV,}\text{5}\text{2}{}^{\mathrm{+}}\text{) g = 0.12±0.04}$. The results are compared with theoretical predictions.     

Gyromagnetic ratios of excited states in186W

The gyromagnetic ratios of the 4 ₁ ⁺ , 6 ₁ ⁺ , and 2 ₂ ⁺ states in¹⁸⁶W were measured relative to that of the 2 ₁ ⁺ level by means of the transient field implantation perturbedγ-ray angular distribution technique. The nuclei in the states of interest were Coulomb excited using a beam of 220-MeV⁶³Cu projectiles and recoiled swiftly through a thin, polarized Fe foil. The present measurements yielded ratiosg(4 ₁ ⁺ )/g(2 ₁ ⁺ )=1.04±0.07,g(6 ₁ ⁺ )/g(2 ₁ ⁺ )=1.03 ±0.20 andg(2 ₂ ⁺ )/g(2 ₁ ⁺ )=0.63±0.13. The sizable disparity between the measuredg-factors of the ground- and excited-band is examined within the context of the interacting boson approximation model.     

High spin states in126Xe

High spin states of¹²⁶Xe have been populated by means of the¹¹⁶Cd(¹³C, 3n) reaction using the OSIRIS-12 detector system. A level scheme consisting of 13 bands has been established. More than 40 new levels were observed and several spin and parity assignments could be made. Experimental Routhians and alignments of selected bands are presented.     

Gyromagnetic ratios of the 4+ and 6+ rotational states of184W

The nuclear Larmor precession has been observed for the 2⁺, 4⁺ and 6⁺ rotational states of¹⁸⁴W in the hyperfine field of WFe by application of the TDPAC and the IPAC techniques. A carrier free radioactive source of^184m Re alloyed with high purity iron was used for all three measurements. From the Larmor precession observed in the 2⁺ state by TDPACω _L = 944(15) MHz and the knowng-factor the hyperfine fieldB _{300 K} ^hf (WFe)=?69.6(27)T was derived. The deviation from the result of a spin echo experiment with¹⁸³WFe extrapolated to room temperature may be caused by the Bohr-Weisskopf effect (hyperfine anomaly). IPAC measurements with the same sample polarized in an external magnetic field of 1.6T gave for the 4⁺ and 6⁺ rotational states: ω _L τ(4⁺)=0.0609(22) andω _L τ(6⁺)=0.00735(102). By use of experimentalB(E2)-values theg _R -factors were derived asg _R (4⁺)=+0.276(26) andg _R (6⁺)=+0.281(45). The directional correlation of the 537?384 keVγ-γ cascade has been analysed in terms of anE1/M2/E3 mixture for theK-forbidden 537keV transition. We obtained the mixing ratiosδ(M2/E1)=±0.086(16),δ(E3/E1)=?0.028(5) with the sign convention of Krane and Steffen.     

Gyromagnetic ratios of 4+ and 6+ states in156Gd and158Gd

The followingg-factors have been derived from time integral measurements of γ-γ angular correlations in the static magnetic hyperfine field of magnetized gadolinium metal probes:¹⁵⁶Gd:g(4 ₁ ⁺ )=+0.310(19)g(6 ₁ ⁺ )=+0.25(21)g(4 ₃ ⁺ , 1511 keV)=+0.809(27)¹⁵⁸Gd:g(4 ₁ ⁺ )=+0.409(15). The 5.35d ¹⁵⁶Tb sources were produced by the reaction¹⁵⁶Gd(d, 2n)¹⁵⁶Tb in our cyclotron. A carrier-free 150y ¹⁵⁸Tb source was obtained from ISOLDE/CERN. In comparison with the precisely knowng-factors of the 2 ₁ ⁺ states,g(2 ₁ ^su+ ,¹⁵⁶Gd) =+0.386(4) andg(2 ₁ ⁺ ,¹⁵⁸Gd)=0.381(4), we observe a large reduction for the¹⁵⁶Gd 4 ₁ ⁺ state whereasg increases slightly for¹⁵⁸Gd. The half-life of the 4 ₁ ⁺ state of¹⁵⁸Gd was remeasured as¹⁵⁸Gd:T _1/2(4 ₁ ⁺ )=148(2) ps. A measurement of the rotation in the 4 ₃ ⁺ state of¹⁵⁶Gd in external magnetic fields of various strengths up toB _ext=9.5 T did not confirm the anomalous dependence of the magnetic hyperfine field in gadolinium metal on the external field, which has been reported by Persson et al. [29].     

Gyromagnetic ratios of collective states of166Er

The static hyperfine field ofB _hf ^4.2k (ErHo) = 739(18)T of a ferromagnetic holmium single crystal polarized in an external magnetic field of ± 0.48T at ～4.2K was used for integral perturbed γ-γ angular correlation (IPAQ measurements of the g-factors of collective states of¹⁶⁶Er. The 1,200y ^166m Ho activity was used which populates the ground state band and the γ vibrational band up to high spins. The results: $$\begin{gathered} g(4_g^ + ) = + 0.315(16) \hfill \\ g(6_g^ + ) = + 0.258(11) \hfill \\ g(8_g^ + ) = + 0.262(47)and \hfill \\ g(6_\gamma ^ + ) = + 0.254(32) \hfill \\ \end{gathered}$$ exhibit a significant reduction of the g-factors with increasing rotational angular momentum. The followingE2/M1 mixing ratios of interband transitions were derived from the angular correlation coefficients: $$\begin{gathered} 5_\gamma ^ + \Rightarrow 4_g^ + :\delta (810keV) = - (36_{ - 7}^{ + 11} ) \hfill \\ 7_\gamma ^ + \Rightarrow 6_g^ + :\delta (831keV) = - (18_{ - 2}^{ + 3} )and \hfill \\ 7_\gamma ^ + \Rightarrow 8_g^ + :\delta (465keV) = - (63_{ - 12}^{ + 19} ). \hfill \\ \end{gathered}$$ The results are discussed and compared with theoretical predictions.     

The g-factors of isomeric states in127, 128Xe

Excited states in^{127, 128}Xe were populated in the reaction⁹Be+¹²²Sn atE _lab=38 MeV. The de-excitation of the isomeric states 7/2⁺ in¹²⁷Xe and 8^? in¹²⁸Xe was studied using angular distribution and TDPAD methods on molten¹²²Sn targets. The results are $$\begin{gathered} T_{1/2} (7/2^ + ) = 37 \pm 1 ns, g(7/2^ + ) = + 0.241 \pm 0.009 \hfill \\ T_{1/2} (8^ - ) = 83 \pm 2 ns, g(8^ - ) = - 0.036 \pm 0.009. \hfill \\ \end{gathered}$$ The experimentalg-factors suggest the main configurationsvg _7/2 andvh _11/2 g _7/2 for the isomeric states. Detailed analysis of the combined information fromg-factors and transition rates set stringent limits on the admixtures of the wave functions. The quasirotational bands built on the two-quasiparticle 6^? and 10⁺ states are extended to higher spins, (14^?) and (16⁺), respectively, and their structures are analyzed within the framework of the Interacting Boson Model.     

Gyromagnetic ratios of low-lying rotational states in156, 158, 160Gd

Transient-field precessions were measured simultaneously for levels in the ground-state bands of^{156, 158, 160}Gd as ions of these nuclei traversed a thin polarized Fe foil. Relative g-factors of levels up to 6 ₁ ⁺ were deduced, those of the 4 ₁ ⁺ levels being determined with greatest precision. In contrast with the conclusions of the recent report by Alzner et al. [1], our results are consistent with g(4 ₁ ⁺ ) having the same value in all three isotopes and imply g(2 ₁ ⁺ )=g(4 ₁ ⁺ ) in¹⁵⁶Gd, consistent with nuclear structure models.     

Gyromagnetic ratios of excited states in 107, 109Ag

The gyromagnetic ratios of the lowest excited $\text{3}\text{2}{}^{\mathrm{?}}\text{and}\text{5}\text{2}{}^{\mathrm{?}}$ states in ^{107, 109}Ag were simultaneously measured relative to that of the 2₁⁺ level in ¹⁰⁸Pd. The thin-foil, perturbed γ-ray angular distribution technique was employed utilizing the transient hyperfine magnetic field present at the nuclei of these ions as they swiftly recoiled through a thin magnetized Co foil. The states of interest were Coulomb-excited using beams of 100 MeV ³²S ions. The present measurements yielded $\text{g(}\text{3}\text{2}{}^{\mathrm{?}}\text{;}{}^{107}\text{Ag}\text{) = +0.63 ± 0.09, g(}\text{5}\text{2}{}^{\mathrm{?}}\text{;}{}^{107}\text{Ag}\text{) = + 0.37±0.06, g(}\text{3}\text{2}{}^{\mathrm{?}}\text{;}{}^{109}\text{Ag}\text{) = +0.77 ± 0.10,}\text{and}\text{g(}\text{5}\text{2}{}^{\mathrm{?}}\text{;}{}^{109}\text{Ag}\text{) = +0.36 ± 0.05}$. These findings are compared with weak-coupling and other appropriate model calculations.     

Gyromagnetic ratios of excited states in 150Sm and 152Sm

The gyromagnetic ratios of the 2₁⁺, 4₁⁺, 6₁⁺, 2₂⁺, and 2₃⁺ states in ¹⁵⁰Sm and the 2₁⁺, 4₁⁺, 6₁⁺, 8₁⁺, 10₁⁺, 2₂⁺, and 2₃⁺ levels in ¹⁵²Sm have been measured using the transient field perturbed γ-ray angular correlation technique. States of interest were populated by multiple Coulomb excitation using 150- and 220-MeV ⁵⁸Ni beams. The present results display no significant deviation from constancy of the g-factors of all levels investigated in either isotope separately or of corresponding states in ^150,152Sm. These findings are compared with available prior measurements and assessed in terms of applicable theoretical model calculations.     

Sub-Coulomb transfer and fission in collisions of129Xe,132Xe and136Xe with238U

Integral cross sections for fission and for one- and two-neutron transfer reactions in the system¹³²Xe+²³⁸U were measured radiochemically in the energy range 0.7≦E/E _Coul≦1. The excitation functions for fission and transfer are found to be essentially parallel below 0.85×E _Coul. Even at the lowest energies the transfer cross sections exceed the fission cross section by more than one order of magnitude. With the other projectiles¹²⁹Xe and¹³⁶Xe different transfer cross sections illustrating their sensitivity for the ground stateQ-values,Q _gg , are observed while the fission cross sections are the same as in the¹³²Xe +²³⁸U reaction. The fission data are interpreted in terms of a continuous transition between Coulomb fission and several transfer-induced fission processes.     

Transition probabilities and the structure of some negative-parity states in126,130Xe and132Ba

The lifetimes of several negative-parity states in^126,130Xe and¹³²Ba have been determined by means of the generalized centroid-shift method. The reactions^124,128Te(α,2n) and¹²²Sn(¹³C, 3n) have been used. Following results were obtained:T _1/2(2758 keV)=1.3±0.2 ns in¹²⁶Xe,T _1/2(2060 keV)=0.20±0.10 ns,T _1/2(2104 keV)=0.50±0.10 ns,T _1/2(2376 keV)=0.30±0.10 ns andT _1/2(2973 keV)=4.6±0.4 ns in¹³⁰Xe as well asT _1/2(2120 keV)=0.40 _?0.10 ^+0.20 ns in¹³²Ba. A systematics of the B(E2; 7 _? ¹ ?5 ₁ ^? ) values in theN=76 nuclei is presented. Electric dipole and quadrupole transition rates are discussed in terms of octupole and quadrupole collectivity. The structure of the 5 ₁ ^? and 7 ₁ ^? states is considered. Nuclear reactions:^124,128Te(α, 2 _n ),E=26 MeV,¹²²Sn (¹³C, 3n),E=53 MeV; measuredE _γ I _γ , γ-r.f. DeducedT _1/2, B(σL) in^126,130Xe and¹³²Ba. Ge detectors. Generalized centroid-shift analysis.     

Transition probabilities and the structure of some negative-parity states in 126,130Xe and 132Ba

The lifetimes of several negative-parity states in ^126,130Xe and ¹³²Ba have been determined by means of the generalized centroid-shift method. The reactions ^124,128Te(α, 2n) and ¹²²Sn(¹³C, 3n) have been used. Following results were obtained: T_1/2(2758 keV) = 1.3 ± 0.2 ns in ¹²⁶Xe, T_1/2 (2060 keV) = 0.20 ± 0.10 ns, T_1/2 (2104 keV) = 0.50 ± 0.10 ns, T_1/2 (2376 keV) = 0.30 ± 0.10 ns and T_1/2 (2973 keV) = 4.6 ± 0.4 ns in ¹³⁰Xe as well as T _1/2(2120 keV) = 0.40 _?0.10 ^+0.20 ns in ¹³²Ba. A systematics of the B(E2; 7 ₁ ^? ? 5 ₁ ^? ) values in the N = 76 nuclei is presented. Electric dipole and quadrupole transition rates are discussed in terms of octupole and quadrupole collectivity. The structure of the 5 ₁ ^? and 7 ₁ ^? states is considered. Nuclear reactions: ^124,128Te(α, 2n), E = 26 MeV, ¹²²Sn (¹³C, 3n), E = 53 MeV; measured E_{gg}, I_{gg}, γ-r.f. Deduced T_1/2, B(σL) in ^126,130Xe and ¹³²Ba. Ge detectors. Generalized centroid-shift analysis.     

Nuclear deformation and the two-neutrino double- β decay in <Superscript>124, 126</Superscript>Xe , <Superscript>128, 130</Superscript>Te , <Superscript>130, 132</Superscript>Ba and <Superscript>150</Superscript>Nd isotopes

The two-neutrino double-beta decay of ^{124, 126}Xe , ^{128, 130}Te , ^{130, 132}Ba and ¹⁵⁰Nd isotopes is studied in the Projected Hartree-Fock-Bogoliubov (PHFB) model. Theoretical 2ν β^-β^- half-lives of ^{128, 130}Te , and ¹⁵⁰Nd isotopes, and 2ν β⁺β⁺ , 2ν β⁺ EC and 2ν ECEC for ^{124, 126}Xe and ^{130, 132}Ba nuclei are presented. Calculated quadrupolar transition probabilities B(E2 : 0⁺ → 2⁺) , static quadrupole moments and g -factors in the parent and daughter nuclei reproduce the experimental information, validating the reliability of the model wave functions. The anticorrelation between nuclear deformation and the nuclear transition matrix element M _2ν is confirmed.     

Search for a new reaction mechanism in the system132Xe+natFe

Thin targets of natural Fe have been irradiated with¹³²xe ions at beam energies of 5.00, 5.90, and 7.15 MeV/u. Mass yields for projectile-like and symmetric products were evaluated, and their ratio as a function of beam energy determined. The results are consistent with previously-determined thick-target radiochemical data, and are not consistent with published on-line counter data for the same system.     

Beta-decay of light rare-earth130, 132Pr and132, 134Pm nuclei

Gamma-ray spectra of neutron-deficient isotopes of^{130, 132}Ce and^{132, 134}Nd have been investigated from the β-decay of^130,132Pr and^132,134Pm new gamma-bands of states were identified and the systematic trends are presented.     

Evolution from quasielastic to deep-inelastic transfer in the system132Xe+natFe§

The pronounced isotope shift of⁸⁷Sr versus⁸⁷Sr observed recently in 5sns¹S₀ Rydberg states reflects the singlet-triplet mixing solely caused by magnetic hyperfine interaction. Using semiempirical estimates for the hyperfine coupling constant a_{5 s} and the singlet-triplet splitting ΔE_ST (n) excellent agreement between experimental and calculated values is obtained.     

Vibronic coupling in the first four electronic states of CH2F+2

Vibronic coupling in the energetically lowest first four electronic states of CH₂F⁺₂ is studied in this paper. A model 4×4 Hamiltonian is constructed in a diabatic electronic representation employing normal coordinates of vibrational modes and standard vibronic coupling theory. Extensive ab initio quantum chemistry calculations are carried out to determine the parameters of the Hamiltonian and energetic ordering of the electronic states. The topographical features of the latter are examined at length and several conical intersections are established. Nuclear dynamics calculations on coupled electronic states are carried out from first principles by propagating wave packet. Theoretically calculated broad band vibronic structure of the four states are found to be in good accord with the experimental results.