Nuclear orientation study of the excited states of 129I populated in the decay of 129gTe and 129mTe

From the angular distributions of γ-rays emitted by oriented ^129gTe and ^129mTe nuclei implanted in iron by isotope separator, unique spin assignments could be made for the excited states of ¹²⁹I at 487.4 keV $\text{(}\text{5}\text{2}{}^{\mathrm{+}}\text{)}$, 696.0 keV $\text{(}\text{11}\text{2}{}^{\mathrm{+}}\text{)}$, 729.6 keV $\text{(}\text{9}\text{2}{}^{\mathrm{+}}\text{)}$, 768.9 keV $\text{(}\text{7}\text{2}{}^{\mathrm{+}}\text{)}$, 1050.4 keV $\text{(}\text{7}\text{2}{}^{\mathrm{+}}\text{)}$ and 1111.8 keV $\text{(}\text{5}\text{2}{}^{\mathrm{+}}\text{)}$. In addition, E2/M1 amplitude ratios for the following ¹²⁹I γ-rays (energies are in keV) are derived: δ(459.6) = ?(0.076^+0.037_?0.148); δ(487.4) = 0.50^+0.17_?0.10 or δ^? = 0.35^+0.15_?0.09; δ(556.7) = 0.06±0.02 or δ^? = ?(0.10±0.02); δ(624.4) = 0.10±0.26 or δ^? > 0.4; the 696.0 keV γ-ray is pure E2; δ(729.6) = ?(0.34±0.06) or δ^?1 = 0.55±0.05; δ(741.1) = ?(0.27±0.10) or δ^?1 = ?(0.43±0.12); δ(817.2) = 0.46±0.04 or δ^?1 =0.20±0.03 if $\text{I}{}^{\mathrm{\pi }}\text{(845}\text{keV}\text{) =}\text{7}\text{2}{}^{\mathrm{+}}$; δ(1022.6) = ?(0.02 ±0.02) or δ^?1 = ?(0.23±0.02); $\text{δ(1084) = 0.56}{}^{\mathrm{+0.04}}{}_{\mathrm{?0.14}}$; δ(1111.8) = 0.06±0.05 or δ^?1 = ?(0.08±0.05). The anisotropy of the 531.8 keV γ-ray excludes $\text{1}\text{2}{}^{\mathrm{+}}$ as a possible spin assignment for the 559.6 keV level, so that no $\text{1}\text{2}{}^{\mathrm{+}}$ level is fed in the decay from ¹²⁹Te. Anisotropies for the 209, 250.7, 278.4 and 281.1 keV γ-rays are also measured. Comparison of the level scheme is made with theoretical predictions from both the pairing-plus-quadrupole model and the intermediate coupling unified model.     

Nanosecond lifetimes of the low-spin states in the nucleus 147Nd: A particle-rotor model interpretation of the results

Nanosecond lifetimes of several states in ¹⁴⁷Nd have been studied using the reaction ¹⁴⁶Nd(d, pγ)¹⁴⁷Nd with 10 MeV deuterons. The following lifetimes were observed: the $\text{7}\text{2}{}^{\mathrm{?}}$ level at 49.9 keV, 2.5±0.5 ns; the $\text{5}\text{2}{}^{\mathrm{?}}$ level at 127.9 keV, ≦ 0.8 ns; the $\text{9}\text{2}{}^{\mathrm{?}}$ level at 190.3 keV, 1.1±0.3 ns and the $\text{1}\text{2}{}^{\mathrm{?}}$ level at 214.6 keV, 5.8±0.8 ns. The wave functions of the states were constructed using an axial particle-plus-rotor model. The free parameters used are compared to the systematics observed in the neighbouring heavier N = 87 isotones as well as in the N = 89 and 91 isotones. Transition rates within the $\text{f}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}$ and $\text{h}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}$ based excitations, separately, are reasonably well reproduced, but the connecting transitions indicate too strong a mixing of the shells in the calculation.     

Negative-parity states in Pb isotopes: g-factor of the 480 ns,if Jπ = 9− isomer in 200Pb

The g-factor of the 480 ns, 9^? isomer at 2.237 MeV in ²⁰⁰Pb was measured by the time-differential perturbed angular distribution method. The result, g = ?0.0285±0.0011 confirms the rather pure $\text{(}\text{f}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}{}^{\mathrm{?1}}\text{i}{}_{\mathrm{<mtext>13</mtext><mtext>2</mtext>}}{}^{\mathrm{?1}}\text{)}$ quasiparticle structure of this state. Half-lives of 480±20 ns, 43±3 ns and 42±4 ns have been measured for the 2237 keV 9^?, 2154 keV 7^? states in ²⁰⁰Pb and the 2208 keV state in ²⁰²Pb, respectively; E2 transitions and g-factors of negative-parity states in even, neutron-deficient Pb isotopes are discussed.     

Remeasurement of the low-energy cross section for the 15N(p, α0)12C reaction

The cross section for the ${}^{15}\text{N(p}\text{, α}{}_0\text{)}{}^{12}\text{C}$ reaction has been measured at θ_lab = 135° over the proton energy range 93 ≦ E_p ≦ 418 keV. The results are in good agreement with the less precise but much earlier measurements of Schardt, Fowler and Lauritsen (1952). An analysis of the present data in terms of a two-level calculation including the 338 keV (1^?) and 1028 keV (1^?) resonances determines a zero-energy intercept for the astrophysical S-factor of S(0) = 78 ± 6 MeV · b.     

Lifetime and g-factor results for the 132− 1985 keV level in 91Nb and the 152− 2288 keV level in 91Zr

Lifetime and g-factor measurements have been made with pulsed beam-γ time-differential techniques using the ⁸⁹Y(α, 2n)⁹¹Nb and ⁸⁸Sr(α, n)⁹¹Zr reactions. A mean lifetime τ = 14.4 ± 0.5 nsec and a g-factor of 1.26 ± 0.04 were obtained for the $\text{13}\text{2}{}^{\mathrm{?}}$ 1985 keV level in ⁹¹Nb and τ = 41.9 ± 1.2 nsec and g = 0.70 ± 0.01 were obtained for the $\text{15}\text{2}{}^{\mathrm{?}}$ 2288 keV level in ⁹¹Zr. These results are compared to theoretical calculations for $\text{(π}\text{g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)}{}^2\text{(π}\text{p}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{)}$ and $\text{(π}\text{g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)(π}\text{p}\text{1}\text{2}\text{)(v}\text{d}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}\text{)}$ configurations in ⁹¹Nb and ⁹¹Zr, respectively.     

Coulomb excitation of 85Rb and 87Rb

Energy levels of ⁸⁵Rb and ⁸⁷Rb have been studied via de-excitation γ-rays following Coulomb excitation with ³⁵Cl ions. In addition to the known negative-parity states at 151.2 keV and 868.2 keV in ⁸⁵Rb, two states at 281.0 keV and 731.8 keV have been found with fourγ-ray transitions of 129.8, 281.0, 450.8 and 731.8 keV. Only one Coulomb excited state at 402.6 keV in ⁸⁷Rb has been observed. The B(E2↑) values (in units e² · b²) have been determined as 0.0035±0.0004 (151.2 keV), 0.0016±0.0002 (281.0 keV), 0.0101 ±0.0010 (731.8 keV), and 0.036±0.004 (868.2 keV) for the states in ⁸⁵Rb, and as 0.0054±0.0006 (402.6 keV) for the state in ⁸⁷Rb. The mean lifetimes of the 731.8 keV and 868.2 keV states have been measured by the Doppler shift attenuation method as 6.4±0.7 psec and 4.2±0.5 psec respectively. Angular distribution measurements allow unique spin and parity assignments of $\text{1}\text{2}{}^{\mathrm{?}}$ and $\text{3}\text{2}{}^{\mathrm{?}}$ to the 281.0 keV and 731.8 keV levels respectively. The spin and parity of the 868.2 keV level has been restricted to $\text{5}\text{2}{}^{\mathrm{?}}$ or $\text{7}\text{2}{}^{\mathrm{?}}$.     

Hydrogen burning of 20Ne and 22Ne in stars

The ²⁰Ne(p, γ)²¹Na capture reaction has been studied in the energy range E_p = 0.37–2.10 MeV. Direct-capture transitions to the $\text{332 (}\text{5}\text{2}{}^{\mathrm{+}}\text{)}\text{and}\text{2425}\text{keV}\text{(}\text{1}\text{2}{}^{\mathrm{+}}\text{)}$ states have been found with spectroscopic factors of C²S(1d) = 0.77±0.13 and C²S(2s) = 0.90±0.12, respectively. The high-energy tail of the 2425 keV state, bound by 7 keV against proton decay, has also been observed in the above energy range as a subthreshold resonance. The excitation function for this tail is consistent with a single-level Breit-Wigner shape for a γ-width of Γ_γ = 0.31±0.07 eV at E_x = 2425 keV. The extrapolation of these data to stellar energies gives an astrophysical S-factor of S(0) = 3500 keV · b. Two new resonances at E_p = 384±5 and 417± 5 keV have been observed with strengths of ωγ = 0.11±0.02 and 0.06±0.01 meV, corresponding to the known states at and 2829 keV (presumably $\text{9}\text{2}{}^{\mathrm{+}}$), respectively. For the known E_p = 1830 keV resonance, a strength of ωγ = 1.0± 0.3 eV and a total width of Γ = 180± 15 keV were found. Branching ratios as well as transition strengths have been obtained for these three states. The Q-value for the ²⁰Ne(p, γ)²¹Na reaction (Q = 2432.3 ± 0.5 keV) as well as excitation energies for many low-lying states in ²¹Na have been measured. No evidence was found for the existence of the state reported at E_x = 4308±4 keV.In the case of ²²Ne(p, γ)²³Na, direct-capture transitions to six final bound states have been observed revealing sizeable spectroscopic factors for these states. The astrophysical S-factor extrapolated from these data to stellar energies, is S(0) = 67 ± 12 keV · b.The astrophysical as well as the nuclear structure aspects of the present results are discussed.     

Band contour analysis of compounds with pure isotopes: The E fundamentals of HC35Cl3

The vibration-rotation transitions for v = 1 ← 0 of NO (${}^2\text{Π}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}$) have been studied by using the technique of laser magnetic resonance spectroscopy. Five magnetic resonance lines are observed with three CO laser lines in the range from 1859 to 1886 cm^?1. From these, three zero-field transition frequencies, v = 1 ← 0; $\text{R(}\text{3}\text{2}\text{)}$, $\text{P(}\text{7}\text{2}\text{)}$, and $\text{P(}\text{9}\text{2}\text{)}$ are obtained with an accuracy of ±0.0007 cm^?1. The molecular constants which have been determined by borrowing centrifugal constants from a previous infrared work are $\text{B}{}_{02}{}^1\text{= 1.72004 ± 0.00006}\text{cm}{}^{\mathrm{?1}}$, $\text{B}{}_{12}{}^1\text{= 1.70212 ± 0.00010}\text{cm}{}^{\mathrm{?1}}$, and $\text{G(v = 1) ? G(v = 0) (}\text{for}{}^2\text{Π}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{) = 1875.8470 ± 0.0007}\text{cm}{}^{\mathrm{?1}}$.     

Decay of the mirror nuclide 45V

The β⁺ decay of ⁴⁵V $\text{(J}{}^{\mathrm{\pi }}\text{, T=}\text{7}\text{2}{}^{\mathrm{?}}\text{,}\text{1}\text{2}\text{)}$ has been observed. The half-life was found to be 539 ± 18 ms; in addition to the superallowed transition to the mirror state (⁴⁵Ti ground state), it exhibits a (4.3 ± 1.5)% allowed branch to the $\text{5}\text{2}{}^{\mathrm{?}}$ state at 40.1 keV in ⁴⁵Ti. Decay data for the complete $\text{f}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}$ shell series of mirror nuclei are presented.     

Oscillator strengths in the Cameron system of carbon monoxide

Relative oscillator strengths in the Cameron system of CO(a³Π ← X¹Σ) have been observed in absorption for six bands (υ′ = 0–5, υ″ = 0) with the result, normalized to the absolute (0, 0) band measurement of Hasson and Nicholls, $\text{?}{}_{00}\text{= (1.62±0.07) × 10}{}^{\mathrm{?7}}$, $\text{?}{}_{10}\text{= (1.96±0.09) × 10}{}^{\mathrm{?7}}$, $\text{?}{}_{20}\text{= (1.41±0.04) × 10}{}^{\mathrm{?7}}$, $\text{?}{}_{\mathrm{3\; 0}}\text{= (0.72±0.03) × 10}{}^{\mathrm{?7}}$, $\text{?}{}_{40}\text{= (0.31±0.02) × 10}{}^{\mathrm{?7}}$, $\text{?}{}_{50}\text{= (0.14±0.01) × 10}{}^{\mathrm{?7}}$. The density of CO was modulated with a motor-driven vacuum valve and synchronous fluctuations (?1 per cent) in the transmitted intensity detected with a lock-in amplifier. Peak pressure in the 21 cm absorption cell was approximately 10 torr. A curve of growth analysis was used to correct saturation effects by less than 3 per cent.     

Nuclear matrix elements from L/K electron capture ratios in 59Ni decay

Using a recent theoretical method, the ratio of nuclear matrix elements $\text{R = (}{}^{\mathrm{v}}\text{F}{}^0{}_{220}\text{?√}\text{3}\text{2}{}^{\mathrm{A}}\text{F}{}^0{}_{221}\text{/}{}^{\mathrm{v}}\text{F}{}^0{}_{211}\text{)}$ was determined to be either 20.50^+0.35_?0.55 or 25.22^+0.28_?0.17 in the second-forbidden nonunique decay of 8 × 10⁴ y ⁵⁹Ni. These values of R were obtained from a value of L₃/K = 0.008 ± 0.002 found by subtracting the theoretical ratio $\text{(L}{}_1\text{+ L}{}_2\text{)}\text{K}$ = 0.113 (based on Q_PEC = 1070 ± 8 keV) from the total ratio L/K = 0.121 ± 0.002, which was measured with a reactor-produced, doubly-mass-separated ⁵⁹Ni source introduced as gaseous nickel-ocene, (C₅H₅)₂, into a wall-less, anticoincidence, multiwire proportional counter. The 854–1008 eV L and the 8.33 keV K peaks were measured simultaneously.     

Lifetimes of the low-lying 72− states in 113, 115Cd

The half-lives of the $\text{7}\text{2}{}^{\mathrm{?}}$ states at 522.6 and 393.9 keV in ¹¹³Cd and ¹¹⁵Cd have been determined to be 0.322±0.012 and 0.75± 0.03 ns, respectively. Values of the $\text{B(}\text{E}\text{2,}\text{7}\text{2}{}^{\mathrm{?}}\text{→}\text{11}\text{2}{}^{\mathrm{?}}$) and the energy difference in odd Cd (A = 113–119) are compared with those in neighbouring even Cd. The level properties are interpreted in the framework of the triaxial rotor model.     

Medium-spin levels and the character of the 20.4 ns 132+ isomer in 145Gd

Levels of the N = 81 nucleus ¹⁴⁵Gd have been investigated by in-beam γ-ray and conversion electron spectroscopy with the ¹⁴⁴Sm(³He, 2n) reaction. Fourteen new low- and medium-spin states between 1.0 and 2.4 MeV excitation, the known yrast levels up to spin $\text{21}\text{2}{}^{\mathrm{+}}$, five other high-spin non-yrast states and a new 20.4 ns $\text{13}\text{2}$ isomer at 2200.2 keV in ¹⁴⁵Gd have been observed. The isomer decays via a fast 927.3 keV E3 transition with B(E3) = 48 ± 7 W.u. Another weaker decay branch is a mixed, strongly hindered E1 + M2 + E3 transition to the $\text{v}\text{h}{}^{\mathrm{?1}}{}_{\mathrm{<mtext>11</mtext><mtext>2</mtext>}}$ state. We propose an octupole $\text{v}\text{f}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}\text{j}{}^{\mathrm{?2}}\text{× 3}{}^{\mathrm{?}}$ main configuration for the isomer, analogous to the 997 keV $\text{13}\text{2}{}^{\mathrm{+}}$ isomer in ¹⁴⁷Gd. The levels of ¹⁴⁵Gd are discussed on the basis of the spherical shell model.     

Lifetimes and g-factors of the 6− and 7− isomers in 66Ga and 68Ga

The 6^? and 7^? isomeric states in ⁶⁶Ga and ⁶⁸Ga at 1440.9 and 1229.6 keV, respectively, have been populated with the (¹³C, 2np) and (¹⁵N, n2p) reactions on natural Fe. The half-lives of these states have been measured to be $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{(6}{}^{\mathrm{?}}\text{,}{}^{66}\text{Ga}\text{) = 57.3 ± 1.2}\text{ns}$ and $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{(7}{}^{\mathrm{?}}\text{,}{}^{68}\text{Ga}\text{) = 64 ± 2}\text{ns}$. Using previous data on the hyperfine field of Ga in Fe, the g-factors of these states have been determined by means of the TDPAD method. The results are $\text{g(6}{}^{\mathrm{?}}\text{,}{}^{66}\text{Ga}\text{) = 0.129 ± 0.003}$ and $\text{g(7}{}^{\mathrm{?}}\text{,}{}^{68}\text{Ga}\text{) = 0.105 ± 0.003}$. These values are in very good agreement with the independent particle model if one assumes the and configurations and uses the empirical proton and neutron g-factors from odd-A neighboring nuclei instead of the Schmidt values. The large disagreements with experiment when Schmidt values are used show that core polarization effects are important in these nuclei.     

“Forbidden” rotational spectra of symmetric-top molecules: PH3 and PD3

A millimeter-wave spectrometer having a sensitivity of 4 × 10^?10 cm^?1 in the 2-mm region has been constructed for observation of extremely weak millimeter-wave spectra of gases. It has been used to measure J → J, K = 0 ← 3 transitions in PH₃ and J → J, K = 0 ← 3 as well as K = ±1 ← ±4 transitions in PD₃. The B₀ and C₀ spectral constants (in MHz) are: for PH₃, B₀ = 133 480.15 ± 0.12 and C₀ = 117 488.85 ± 0.16; for PD₃, B₀ = 69 471.10 ± 0.03 and C₀ = 58 974.37 ± 0.05. The effective ground-state values obtained for the bond angle and bond length are: for PH₃, $\text{r}{}_0\text{(}\text{A}\text{?}\text{) = 1.420}{}_0$ and $\text{α}{}_0\text{(}{}^{\mathrm{o}}\text{) = 93.34}{}_5$; for PD₃, $\text{r}{}_0\text{(}\text{A}\text{?}\text{) = 1.417}{}_6$ and $\text{α}{}_0\text{(}{}^{\mathrm{o}}\text{) = 93.35}{}_9$. The corresponding zero-point-average values were calculated to be: for PH₃, $\text{r}{}_{\mathrm{z}}\text{(}\text{A}\text{?}\text{) = 1.4269}{}_9\text{± 0.0002}$ and $\text{α}{}_{\mathrm{z}}\text{(}{}^{\mathrm{o}}\text{) = 93.228}{}_7$; for PD₃, $\text{r}{}_{\mathrm{z}}\text{(}\text{A}\text{?}\text{) = 1.4226}{}_5\text{± 0.0001}$ and $\text{α}{}_{\mathrm{z}}\text{(}{}^{\mathrm{o}}\text{) = 93.256}{}_7\text{± 0.004}$. For both species, the equilibrium values are $\text{r}{}_{\mathrm{e}}\text{(}\text{A}\text{?}\text{) = 1.4115}{}_9\text{± 0.0006}$ and $\text{α}{}_{\mathrm{e}}\text{(}{}^{\mathrm{o}}\text{) = 93.32}{}_8\text{± 0.02}$.     

Interference effects in 12C(p, γ)13N and direct capture to unbound states

Excitation functions of the capture reaction ¹²C(p, γ₀)¹³N have been obtained at θ_γ = 0° and 90° and E_p = 150–2500 keV. The results can be explained if a direct radiative capture process, E1(s and d → p), to the ground state in ¹³N is included in the analysis in addition to the two well-known resonances in this beam energy range $\text{[E}{}_{\mathrm{p}}\text{= 457(}\text{1}\text{2}{}^{\mathrm{+}}\text{)}$ and 1699 $\text{(}\text{3}\text{2}{}^{\mathrm{?}}\text{) keV]}$. The direct capture component is enhanced through interference effects with the two resonance amplitudes. From the observed direct capture cross section, a spectroscopic factor of C²S(l = 1) = 0.49 ± 0.15 has been deduced for the $\text{1}\text{2}{}^{\mathrm{?}}$ ground state in ¹³N. Excitation functions for the reaction ${}^{12}\text{C(p,γ}{}_1\text{p}{}^1\text{)}{}^{12}\text{C}$ have been obtained at θ_γ = 0° and 90° and E_p = 610–2700 keV. Away from the 1699 keV resonance the capture γ-ray yield is dominated by the direct capture process E1 (p → s) to the $\text{2366 (}\text{1}\text{2}{}^{\mathrm{+}}\text{) keV}$ unbound state. Above E_p = 1 MeV, the observed excitation functions are well reproduced by the direct capture theory to unbound states (bremsstrahlung theory). Below E_p = 1 MeV, i.e., E_p → 457 keV, the theory diverges in contrast to observation. This discrepancy is well known in bremsstrahlung theory as the “infrared problem”. From the observed direct capture cross sections at $\text{E}{}_{\mathrm{p}}\text{? 1 MeV}$, a spectroscopic factor of C²S(l = 0) = 1.02 ± 0.15 has been found for the $\text{2366 (}\text{1}\text{2}{}^{\mathrm{+}}\text{) keV}$ unbound state. A search for direct capture transitions to the $\text{3512 (}\text{3}\text{2}{}^{\mathrm{?}}\text{)}$and $\text{3547 (}\text{5}\text{2}{}^{\mathrm{+}}\text{) keV}$ unbound states resulted in upper limits of C²S(l = 1) ≦ 0.5 and C²S(l = 2) ? 1.0, respectively. The results are compared with available stripping data as well as shell-model calculations. The astrophysical aspect of the ¹²C(p, γ₀)¹³N reaction also is discussed.     

Observation of proton emission following thermal neutron capture in 34.5 d 84Rb

Using a target prepared by on-line isotope separation, thermal neutron capture in ⁸⁴Rb (I^π = 2^?) has been shown to induce proton emission to the ground state (0⁺) and first excited state (2⁺) of ⁸⁴Kr. The branching ratio was measured as $\text{Γ}{}_{\mathrm{<mtext>p</mtext>}}\text{(0}{}^{\mathrm{+}}\text{)}\text{Γ}{}_{\mathrm{<mtext>p</mtext>}}\text{(2}{}^{\mathrm{+}}\text{)}\text{= 4.7 ± 0.7}$, favouring a $\text{3}\text{2}{}^{\mathrm{?}}$ assignment of the capturing state without excluding $\text{5}\text{2}{}^{\mathrm{?}}$, and the (n_th, p) cross section as 12 ± 2 b. The energy available for the process was determined to be 3.45 ± 0.01 MeV, in agreement with other mass data in the region.     

Statistical analysis of high-resolution inelastic electron scattering spectra,level densities and missing magnetic quadrupole strength in 90Zr

A fluctuation analysis technique and the comparison of experimentally deduced strength distributions with a statistical one have been used to extract level densities as a function of excitation energy from high-resolution inelastic electron scattering spectra. Both methods yield for the J^π = 2^? states around $\text{E}{}_{\mathrm{<mtext>x</mtext>}}\text{= 9}\text{MeV}\text{in}{}^{90}\text{Zr}$ mean level spacings 〈D〉 = 6.5±1.6 keV and 〈D〉 = 5.5 ± 1.5 keV, respectively. Those level densities are then employed to estimate the magnetic quadrupole strength that is hidden in the background and escaped direct experimental detection.     

Nuclear orientation of negative parity states of 131Xe

The anisotropies of the 177, 326, and 503 keV γ-transitions between negative parity states of ¹³¹Xe have been remeasured in the decay of oriented ¹³¹I nuclei. In addition the linear polarization of the 503 keV radiation has been determined with a Compton polarimeter consisting of two Ge(Li) detectors. A combined analysis of the reported experiment and earlier internal conversion and angular distribution data yields the unique assignments $\text{9}\text{2}{}^{\mathrm{?}}\text{and}\text{7}\text{2}{}^{\mathrm{?}}$ for the levels at 341 and 667 keV. The $\text{E2}\text{M1}$ mixing ratios of the 177 and 326 keV transitions are δ(177) = ?4.5 ± 1.5 and δ(326) = ?4.4 ± 1.6. The intensity of the L = 2 component in the first forbidden β-decay to the 667 keV level is at most 60 %.     

Observed and calculated interactions between valence states of the NO molecule

No perturbation between two valence states of NO has ever been identified, although many valence-Rydberg and several Rydberg-Rydberg perturbations have been extensively studied. The first valence-valence crossing to be experimentally documented for NO is reported here and occurs between the ¹⁵N¹⁸O B²Π (v = 18) and B′²Δ (v = 1) levels. No level shifts larger than the detection limit of 0.1 cm^?1 are observed at the crossings near $\text{J = 6.5 [B}{}^2\text{Π}\text{(F}{}_1\text{) ～ B′}{}^2\text{Δ}\text{(F}{}_2\text{)]}$ and $\text{J = 12.5 [B}{}^2\text{Π}\text{(F}{}_1\text{) ～ B′}{}^2\text{Δ}\text{(F}{}_1\text{)]}$; two crossings involving higher rotational levels could not be examined. Semi-empirical calculations of spin-orbit and Coriolis perturbation matrix elements indicate that although the electronic part of the $\text{B}{}^2\text{Π}\text{～ B′}{}^2\text{Δ}$ interaction is large, a small vibrational factor renders the ¹⁵N¹⁸O B (v = 18) ? B′ (v = 1) perturbation unobservable. Semi-empirical estimates are given for all perturbation matrix elements of the operators $\text{Σ}{}_{\mathrm{i}}\text{a}\text{?}{}_{\mathrm{i}}\text{l}{}_{\mathrm{i}}\text{·s}{}_{\mathrm{i}}$ and $\text{B(L}{}_{\mathrm{\pm }}\text{S}{}_{\mathrm{?}}\text{? J}{}_{\mathrm{\pm }}\text{L}{}_{\mathrm{?}}\text{)}$ which connect states belonging to the configurations $\text{(σ2p)}{}^2\text{(π2p)}{}^4\text{(π}{}^1\text{2p)}$, $\text{(σ2p)(π2p)}{}^4\text{(π}{}^1\text{2p)}{}^2$, and $\text{(σ2p)}{}^2\text{(π2p)}{}^3\text{(π}{}^1\text{2p)}{}^2$.