Generation and detection of tunable ultrashort infrared and far-infrared radiation pulses of high intensity

We report on generation and detection of intense pulsed radiation with frequency tunability in the infrared and far-infrared spectral regions. Infrared radiation is generated with a transversally electrically excited high pressure CO₂ laser. A laser pulse of a total duration of about 300 ns consisted, due to self mode locking, of a series of single pulses, some with pulse durations of less than 450 ps and peak powers larger than 20 MW. Using these pulses for optical pumping of a Raman D₂O laser, trains of short far-infrared pulses with durations less than 400 ps were obtained. For detection a new ultrafast superconducting detector was used.     

The influence of pulse duration on the stress levels in ablation of ceramics: A finite element study

We present a finite element model to investigate the dynamic thermal and mechanical response of ceramic materials to pulsed infrared radiation. The model was applied to the specific problem of determining the influence of the pulse duration on the stress levels reached in human dental enamel irradiated by a CO₂ laser at 10.6 μm with pulse durations between 0.1 and 100 μs and sub-ablative fluence. Our results indicate that short pulses with durations much larger than the characteristic acoustic relaxation time of the material can still cause high stress transients at the irradiated site, and indicate that pulse durations of the order of 10 μs may be more adequate both for enamel surface modification and for ablation than pulse durations up to 1 μs. The model presented here can easily be modified to investigate the dynamic response of ceramic materials to mid-infrared radiation and help determine optimal pulse durations for specific procedures.     

Generation of frequency shifted picosecond pulses with low temporal jitter

Transient stimulated Raman scattering is used for the generation of a frequency shifted picosecond light pulse; part of this Raman shifted pulse is subsequently coherently scattered at a material excitation of a second Raman cell. Starting with the second harmonic pulse (t_p = 4 ps) of a mode-locked Nd : glass laser system, both the stimulated and the coherently produced pulses have durations of 2.3 ps at different wavelengths. By the appropriate choice of the Raman medium pulses between 13 000 and 21 000 cm^-1 can be generated. The coherent generation process minimizes the temporal jitter between the two pulses and allows to obtain a high time resolution of better than 0.3 ps in excite and probe experiments.     

Generator of picosecond laser pulses

The design of the generator of picosecond laser pulses and the results on semiconductor target (ZnSe, CdS, and others) excitation by electric field and electron beam pulses are presented. The maximum power of laser radiation reached 10 kW at pulse durations of 100–200 ps.     

A comparison of ns and ps steam laser cleaning of Si surfaces

We report a quantitative investigation on the efficiency of the steam laser cleaning process using ns and ps pulses. Well-characterized polymer particles with a diameter of 800 nm dispersed on commercial Si wafers were chosen as a modeling contaminant system. As a result of our investigation, we show for the first time the feasibility of performing efficient steam laser cleaning with ps laser pulses and compare the achieved efficiency with the one obtained for ns pulses. For ns pulses, we found a cleaning fluence threshold of 50 mJ/cm² that is independent of the pulse durations (2.5 ns and 8 ns) and the wavelengths (532 nm and 583 nm) used. The application of ps pulses (FWHM=30 ps, 5=583 nm) lowered this threshold to 20 mJ/cm². Both cleaning thresholds are far below the melting thresholds for these laser parameters. Cleaning efficiencies >90% were reached for both pulse durations.     

Experimental investigation of the impact of optical injection on vital parameters of a gain-switched pulse source

An analysis of optical injection on a gain-switched distributed feedback (DFB) laser and its impact on pulse parameters that influence the performance of the pulse source in high-speed optical communication systems is presented in this paper. A range of 10 GHz in detuning and 5 dB in injected power has been experimentally identified to attain pulses, from an optically injected gain-switched DFB laser, with durations below 10 ps and pedestal suppression higher than 35 dB. These pulse features are associated with a side mode suppression ratio of about 30 dB and a timing jitter of less than 1 ps. This demonstrates the feasibility of using optical injection in conjunction with appropriate pulse compression schemes for developing an optimized and cost-efficient pulse source, based on a gain-switched DFB laser, for high-speed photonic systems.     

Coupled-cavity passively Q-switched two-Stokes microchip laser

Experimental and theoretical studies of the coupled-cavity diode-pumped Nd:YAG/Cr:YAG microchip lasers with intracavity Raman conversion of laser pulses in a Ba(NO₃)₂ crystal into two Stokes pulses have been made. Two lasers with a different cavity length have been investigated. The minimal pulse durations at the 2nd Stokes wavelength were ??100 ps in the short-cavity laser at pulse energy of 5???J, and the pulse repetition rate reached 20?C24?kHz. The laser and Stokes pulse dynamics, as well as the spatial intensity distribution of the laser and the 1st Stokes beams at the output mirror have been recorded. A model describing such coupled-cavity microchip Raman lasers has been developed. The numerically simulated laser and Stokes pulse dynamics, and the calculated pulse energy, duration, and repetition rate are in good agreement with the experimental data.     

Effects of a prepulse on laser-induced EUV radiation conversion efficiency

The influence of prepulses on the conversion efficiency (CE) of laser radiation into 13 nm extreme ultraviolet (EUV) radiation, resulting from lithium-like oxygen ions from O20 μm water droplets, was investigated. The laser pulse durations in the experiment ranged from 200 fs to 120 ps. Applying prepulses preceding the main pulse at various delays of up to 11 ns, it was shown that the CE increases differently for each measured pulse duration. The strongest dependence on the introduction of a prepulse was observed for 2 ps laser pulses with a 20 mJ laser pulse energy. The EUV CE was improved by a factor of 15 by the introduction of a prepulse. Calculations on the atomic physics of oxygen ions and simulations of the laser–plasma interaction revealed the influence of the prepulse on the EUV yield. Received: 25 October 2002 / Published online: 22 January 2003 RID="*" ID="*"Corresponding author. Fax: +49-3641/947-202, E-mail: duesterer@ioq.uni-jena.de     

Sub-5-ps, multimegawatt peak-power pulses from a fiber-amplified and optically compressed passively Q-switched microchip laser

We report on high-energy picosecond pulse generation from a passively Q-switched and fiber-amplified microchip laser system. Initially, the utilized microchip lasers produce pulses with durations of around 100 ps at 1064 nm central wavelength. These pulses are amplified to energies exceeding 100 μJ, simultaneously chirped and spectrally broadened by self-phase modulation using a double stage amplifier based on single-mode LMA photonic crystal fibers at repetition rates of up to 1 MHz. Subsequently, the pulse duration of chirped pulses is reduced by means of nonlinear pulse compression to durations of 2.7 ps employing a conventional grating compressor and 4.7 ps using a compact compressor based on a chirped volume Bragg grating.     

A high-power subpicosecond distributed feedback dye laser system pumped by a mode-locked Nd: YAG laser

The design and operation characteristics of a distributed feedback dye laser (DFDL) system pumped by the second harmonic of a flashlamp pumped mode-locked Nd: YAG laser are described. The DFDL oscillator facilitates a large tuning range with nearly Fourier limited pulse durations of about 1.6 ps. The combined action of saturated absorption and amplification results in a pulse shortening to about 600 fs, with small fluctuations in the pulse duration. Output pulse energies of more than 400 J are achieved, corresponding to a peak power of more than 650 MW. Since the dye amplifiers are pumped by pulses of only 25 ps duration the amplified spontaneous emission (ASE) is very low, typically less than 10^–4.     

Collective stopping and ion heating in relativistic-electron-beam transport for fast ignition

The photoelectron spectra of C60 ionized using a 790 nm laser with pulse durations varying from 25 fs to 5 ps have been determined. For 25 fs pulses, in the absence of fragmentation, the ionization mechanism is direct multiphoton ionization with clear observation of above threshold ionization. As the pulse duration is increased, this becomes dominated by a statistical ionization due to equilibration among the electronic degrees of freedom. For pulse durations on the order of a ps coupling to the vibrational degrees of freedom occurs and the well-known phenomenon of delayed (&mgr;s) ionization is observed.     

100 ps far-infrared laser pulses from optically pumped D2O

In this paper we report the generation of ultrashort far-infrared laser pulses with durations less than 100 ps, powers exceeding 200 kW and intensities of more than 1.5 MW/cm². Far-infrared radiation was produced via stimulated resonance Raman scattering using a high-pressure CO₂-laser as pump source and the heavy water isotopes D₂¹⁶O and D₂¹⁸O as far-infrared laser media. Pulses achieved from this laser system were detected by a novel type of detector, sensitive over a broad spectral range from the far-infrared to the visible, basing on quasiparticle heating in a strip-line structured YBa₂Cu₃O_7−δ thin film.     

Passive compression of KrCl excimer laser pulses in naphthalene solutions

The width of KrCl laser pulses has been compressed from 5.2 ns to less than 800 ps using naphthalene as the saturable absorber dye. It was found that the width of the compressed laser pulse decreased with both the input laser intensity and the concentration of naphthalene in the solution. The pulse shortening mechanism is attributed to excited state S₂-S_n transitions in naphthalene.     

飞秒激光激发空气电离的阈值研究

报道在脉宽50fs—22ps,波长800nm脉冲激光作用下的空气电离阈值的研究结果.利用探测等离子体发光信号的方法,实验测量了激发空气电离所需的阈值激光强度.结果表明,当激光脉冲宽度从50fs增加到22ps时,阈值光强I_th从8.7×10¹⁴W/cm²下降到2.7×10¹³W/cm²;I_th经历了由迅速降低逐渐发展为缓慢降低的过程.在50fs—1p 关键词： 飞秒激光 阈值 多光子电离 碰撞电离     

300 Femtosecond pulses at 497 nanometer generated by an excimer laser pumped cascade of distributed feedback dye lasers

The setup is a cascade of 3 lasers: A competing cavity dye laser pumped by a XeCl excimer laser, followed by two distributed feedback dye lasers. The typical durations of the pulses from the lasers are 100 ps, 5 ps, and 300 fs, respectively. The output pulses at 497 nm are amplified up to 500 MW. The shortest pulse duration obtained was 198 fs.     

Characterization of laser-diode end-pumped intracavity frequency doubled, passively Q-switched and mode-locked Nd:YVO4 laser

Simultaneous Q-switching and mode-locking in a laser-diode end-pumped intracavity frequency doubled Nd:YVO₄/KTP green laser using Cr⁴⁺:YAG saturable absorber is experimentally demonstrated. The influence of the initial transmission (T₀) of the Cr⁴⁺:YAG crystal on the Q-switched mode-locked green pulses as well as on the average green power is characterized by using Cr⁴⁺:YAG crystal with various T₀. The effect of T₀ on the pulse build-up time in intracavity second harmonic configuration is theoretically investigated. It was found that the depth of modulation for the mode-locked pulses is greatly improved at the second harmonic wavelength as compared to that for the fundamental wavelength. The average pulse duration of the individual mode-locked pulse for the second harmonic beam measured to be less than 500 ps with a repetition rate of 400 MHz.     

飞秒激光激发空气电离的阈值研究

报道在脉宽50fs—22ps，波长800nm脉冲激光作用下的空气电离阈值的研究结果.利用探测等离子体发光信号的方法，实验测量了激发空气电离所需的阈值激光强度.结果表明，当激光脉冲宽度从50fs增加到22ps时，阈值光强I_th从8.7×10¹⁴W/cm²下降到2.7×10¹³W/cm²；I_th经历了由迅速降低逐渐发展为缓慢降低的过程.在50fs—1p     

Machining of submicron structures on metals and semiconductors by ultrashort UV-laser pulses

Ablation of submicron structures on copper and silicon by short ultraviolet laser pulses (0.5–50 ps, 248 nm) is presented. Features like periodic line structures with a line-spacing below 400 nm, and holes with characteristic sizes well below 1 µm are produced on the sample surface by single laser shot exposure. The structures are projection printed by a Schwarzschild-objective (N.A.=0.4) in air environment. The morphology of ablation sites made with different pulse durations (0.5 ps, 5 ps, 50 ps) is discussed in terms of thermal diffusion effects.     

Plasma-mediated ablation of brain tissue with picosecond laser pulses

Plasma-mediated ablations of brain tissue have been performed using picosecond laser pulses obtained from a Nd:YLF oscillator/regenerative amplifier system. The laser pulses had a pulse duration of 35 ps at a wavelength of 1.053 µm. The pulse energy varied from 90 µJ to 550 µJ at a repetition rate of 400 Hz. The energy density at the ablation threshold was measured to be 20 J/cm². Comparisons have been made to 19 ps laser pulses at 1.68 µm and 2.92 µm from an OPG/OPA system and to microsecond pulse trains at 2.94 µm from a free running Er:YAG laser. Light microscopy and scanning electron microscopy were performed to judge the depth and the quality of the ablated cavities. No thermal damage was induced by either of the picosecond laser systems. The Er:YAG laser, on the other hand, showed 20 µm wide lateral damage zones due to the longer pulse durations and the higher pulse energies.     

Tunable,sub-nanosecond KrF-Raman laser in the ultraviolet

A 0.5 cm^–1 bandwidth injection-locked KrF laser pumps a rare-gas Brillouin cell to produce a reflected pulse with a leading edge risetime of 1 ns, tunable from 248.1 to 248.7 nm. Consistent with Lamb theory of laser amplifiers, subsequent excimer amplification of this pulse produces an intense 500 ps spike on the pulse leading edge. Stimulated Raman scattering then separates the spike from the parent pulse, yielding a tunable short pulse at the first Stokes (S ₁) wavelength. Varying the Raman cell length results in a variable Raman threshold and an adjustable short pulse duration: 250 ps pulses at energies of 3–4 mJ at 268 nm with a 50 cm methane cell and 350 ps, 5 mJ pulses from a 100 cm cell are measured with a streak camera. First pass Raman conversion of the spike toS ₁ followed by second pass backward Raman amplification, where the parent 248 nm pulse serves as the pump beam for the reflectedS ₁ pulse, yields simultaneousS ₁ pulses of 20–25 mJ in the 800 ps range andS ₂ pulses of 550 ps at 5–6 mJ near 290 nm. This laser will avoid collision effects during laser excitation and enable quantitative, single pulse imaging of OH radicals in turbulent combustion because of its high pulse energy.