Study of elastic and inelastic scattering of protons from 74Ge at isobaric analogue resonances

Excitation functions of the elastic and the inelastic proton scattering leading to the ground state and to the 2⁺ (0.596 MeV) state in ⁷⁴Ge were measured at 90°, 125°, 140° and 165° at bombarding energies from 3.34 to 5.4 MeV. Ten isobaric analogue resonances in ⁷⁵As were identified. Five of these resonances decay to the 2⁺ excited state in ⁷⁴Ge. Angular distributions of the inelastically scattered protons were measured at bombarding energies corresponding to these resonances. The partial widths of the isobaric analogue states for decay to the ground state and to the 2⁺ excited state in ⁷⁴Ge were determined as well as the l-values of the captured protons and the spins of the resonances. The Coulomb displacement energy for the pair ⁷⁵As-⁷⁵Ge was found to be 10.01 MeV. A comparison is made with the parent analogue states in ⁷⁵Ge. The results indicate that several levels of ⁷⁵Ge may be described as having a large component of a single particle state coupled to the first 2⁺ excited state in ⁷⁴Ge, and that the 2⁺ state has a configuration with a large 2p-2h component.     

Electron scattering from 70Ge and 72Ge

Cross sections have been measured for the elastic and inelastic scattering of electrons from ⁷⁰Ge and ⁷²Ge for momentum transfers from 0.65 to 1.14 fm^?1. Values for the parameters of a Fermi type ground-state charge distribution were obtained from a phase shift analysis of the elastic cross sections. The rms charge radius corresponding to these parameters is 4.07±0.02 fm for ⁷⁰Ge and 4.05±0.03 fm for ⁷²Ge. Using DWBA analysis the reduced transition probabilities for the electroexcitation of the 2₁⁺ and 3₁^? states were found to be: B(E2, ω)↑ = 19.7±1.2, 26.8±2.0 W.u.; B(E3, ω)↑ = 36±5, 37±7 W.u. for ⁷⁰Ge and ⁷²Ge respectively. The J^π = 3^? assignments for the state at 2.562 MeV in ⁷⁰Ge and 2.515 MeV in ⁷²Ge are confirmed.     

E0 transitions in 70Ge and shape-coexistence interpretation of even-mass Ge isotopes

The branching ratios of E0 and E2 transitions depopulating the 0⁺₂ and 0⁺₃ states in ⁷⁰Ge have been studied using conversion-electron and γ-ray spectroscopy, as well as a new internal-pair measurement technique. A value of 3.7 (2) ns has been obtained in a remeasurement of the half-life of the 0⁺₂ state. Two new E0 transitions, 0⁺₃ → 0⁺₂ and 0⁺₃ → 0⁺₁, have been observed. A comparison of the measured X(E0/E2), ρ²(E0) and B(E2) values for the excited 0⁺ states in ⁷⁰Ge with the corresponding ¹⁵⁰Sm data supports a recent shape-coexistence interpretation of the even-mass Ge isotopes.     

Multiple Coulomb excitation of a 70Ge beam and the interpretation of the 02 + state as a deformed intruder

Electromagnetic properties of the low-lying states in a ⁷⁰Ge nucleus were studied through the multiple Coulomb excitation of a ⁷⁰Ge beam with a ^natPb target. Relative γ-ray intensities were measured as a function of emission angle relative to the scattered projectile. Sixteen E2 matrix elements, including diagonal ones, for 6 low-lying states have been determined using the least-squares search code GOSIA. The expectation values 〈Q ²〉 of 0₁ ⁺ and 0₂ ⁺ states in ⁷⁰Ge are compared with those in ^{72, 74, 76}Ge. Simple mixing calculations indicate that the 0₂ ⁺ states in ⁷⁰Ge and ⁷²Se can be treated as deformed intruder states. It is shown that the deformed intruder becomes the ground state in ⁷⁴Kr. These interpretations of the 0₂ ⁺ states in this region are compared with the potential-energy surface calculations by the Nilsson-Strutinsky model, which allow to interpret the experimental results in a qualitative way from the theoretical point of view. Received: 2 September 2002 / Accepted: 5 November 2002 / Published online: 25 February 2003 RID="a" ID="a"e-mail: sugawara@pf.it-chiba.ac.jp Communicated by D. Schwalm     

Influence of the entrance channel in the fusion reaction 318 MeV 74Ge+74Ge

Entrance channel effects in the fusion of heavy ions have been studied by using the ⁷⁴Ge+⁷⁴Ge reaction at 318 MeV. The population of the yrast superdeformed band in ¹⁴⁴Gd shows an increase when compared with the results obtained in the more asymmetric ⁴⁸Ti+¹⁰⁰Mo reaction at 215 MeV. The relative yields of the different evaporation residues produced in the ⁷⁴Ge+⁷⁴Ge and in the ⁴⁸Ti+¹⁰⁰Mo reactions are very similar, with the exception of the ^145,144Gd residual nuclei (3n and 4n decay channels) which are populated with a larger yield in the symmetric reaction. Statistical model calculations reproduce qualitatively such effect if a fission delay is explicitly taken into account. Effects related to fusion barrier fluctuations seem to be important in determining the spin distributions of the compound nucleus. The spectra of the high energy γ-rays emitted in the ⁷⁴Ge+⁷⁴Ge reaction have been measured as a function of the γ-ray multiplicity as well as in coincidence with selected evaporation residues. They are reproduced by standard statistical model calculations with GDR parameters taken from systematics, demonstrating that, in agreement with dynamical model prediction, the emission of γ-rays from the dinucleus formed in the earlier stage of the collision is unimportant.     

70Ge(α, γ)74Se cross section measurements at energies of astrophysical interest

The cross section of the reaction⁷⁰Ge(α, γ)⁷⁴Se has been measured over the bombarding energy range of 5.05 MeV <E _α < 7.80 MeV using single and coincidence gamma spectroscopy techniques. The experimental S-factor values are in agreement with theoretical statistical-model calculations. Reaction rates for the⁷⁰Ge(α, γ)⁷⁴Se and the inverse (γ, α) reactions have been determined for appropriate temperatures.     

High spin states in77Se populated by the74Ge(α,n γ) reaction

⁷⁷Se has been investigated by the reaction⁷⁴Ge(α,nγ) at 14 MeV. Gamma singles spectra, gamma angular distributions and gamma-gamma coincidences have been taken. A level scheme has been established, spins and parities have been assigned. States of a rotational band on the 1/2^? ground state, a rotational band on the 5/2^? 249.7 keV state and an anormal band have been identified. Nuclear Reaction ⁷⁴Ge(α,n γ)E _α=14 MeV; measuredE _γ ,I _γ ,γ-γ-Coin.,γ-ang. distr.⁷⁷Se deduced levels,J, π. Enriched target, Ge (Li).     

Coulomb excitation of 74Ge beam

⁷⁴Ge beam was Coulomb-excited on a ^natPb target. Ten E2 matrix elements including diagonal matrix elements for 5 low-lying states have been determined using the least-squares search code GOSIA. The expectation values of the rotational invariants 〈Q ²〉 and 〈cos3δ〉 show the small and triaxial deformation of the two lowest members of the ground-state band , while the 0₂ ⁺ and 2₂ ⁺ states are found to be almost spherical. Received: 31 August 2000 / Accepted: 4 December 2000     

Isobaric analogue resonances in71As through proton elastic scattering on70Ge

The analogues of the low-lying levels in⁷¹Ge have been observed as resonances in the compound nucleus⁷¹As through proton elastic scattering on⁷⁰Ge in the energy rangeE _p=3.5 to 5.3 MeV. The excitation functions cover the analogue resonances corresponding to states upto 2.3 MeV excitation in⁷¹Ge. The sub-structures in the 5.06 MeV resonance, first observed by Temmer and co-workers have been confirmed in the present experiment. The present investigation reveals similar sub-structures in the 4.13 MeV resonance lending further support to the existence of intermediate structure near an isobaric analogue resonance. The resonance parameters and the spectroscopic factors (for the corresponding parent states) have been extracted. The results are compared with the information available from the⁷⁰Ge(d, p)⁷¹Ge reaction.     

79Se investigated by the reaction76Ge(α, nγ)

⁷⁹Se has been investigated by the reaction⁷⁶Ge(α, nγ). Gamma excitation functions (E _{α=10?15 MeV)}, gamma angular distributions and gamma-gamma coincidences (both at (E _{α=12 MeV)}, have been taken. A level scheme has been established, spins and partities have been assigned. The results are compared with rotational bands in neighbouring odd Se isotopes. Nuclear reaction⁷⁶Ge(α, nγ)E _α =12 MeV; measuredE _γ,I _γ,γ-γ coincidences,γ-angular distribution,γ-excitation function.⁷⁹Se deduced levels,J, π. Enriched target, Ge(Li).     

Nuclear structure study of states in 72Ge and 74Ge with (p,t) reactions

^{74, 76}Ge(p, t) measurements at E_p = 35.4 MeV are reported. It is found that, except for a depression of the ⁷²Ge ground-state energy accompanying the occurrence of a low-lying 0⁺ excited state, the energy level structure of ⁷²Ge is nearly identical to that of ⁷⁴Ge. Dependence of angular distribution shapes at low angles on the transferred neutron configuration is observed, both experimentally and in the DWBA calculations.     

Recoil distance lifetime measurements in82Kr

The lifetimes τ=124±12, 6 _?2 ⁺⁴ and 380±100 ps of theE _x (I ^π )=3.46(8⁺), 2.92(6⁺) and 3.04(6^?) MeV states, respectively, populated by the reaction⁷⁶Ge(¹²C,α2n) were measured with the recoil distance method. In addition upper lifetime limits were obtained for nine states. The measured lifetimes and energies indicate a band crossing at aboutI ^π =8⁺, probably arising from the alignment of twog _9/2 neutrons. For the 3.04 MeV 6^? state as a second member of a band built on the 2.65 MeV 4^? state the measured lifetime points to a two-quasiparticle configuration. The positive-parity states have been discussed in the frame of the interacting boson approximation, nuclear field theory and the cranked shell model.     

Levels excited in73Ge by (d,p) and (p,p′) reactions

Angular distributions from the reactions⁷²Ge(d, p)⁷³Ge and⁷³Ge(p, p′)⁷³Ge have been studied with 8.0 MeV deuterons and 12.0 MeV protons, respectively, using the Aldermaston Tandem Van de Graaff generator and multi-angle magnetic spectrograph. The ground stateQ-value of the (d, p) reaction was measured to be 4.571±0.004 MeV. The energies, values of the transferred orbital angular momenta, parities and transition strengths in both reactions were determined by use of distorted-wave Bornapproximation calculations, for levels up to 3 MeV excitation energy. The sums of the transition strengths are compared with shell model calculations as well as with values obtained in neighbouring nuclei. Discrepancies between parity and possible spin assignments of states observed in the two reactions are discussed.     

The level structure of69Ge

Theγ-ray decay of the states in⁶⁹Ge has been studied using the reaction⁶⁶Zn(α, nγ)⁶⁹Ge atE _α =13 and 19 MeV. The level scheme and spin assignments were established by means of coincidence measurements, angular distributions and excitation functions. 27 new levels could be found or confirmed. It is suggested that⁶⁹Ge is a further example for the weak coupling phenomenon in the medium mass nuclei. Nuclear Reactions: ⁶⁶Zn(α, nγ)⁶⁹Ge,E _α =13–22 MeV, measuredE _γ ,I _γ ,I _γ (θ),E _γ =f(E _α ),γ-γ coincidences,⁶⁹Ge deduced levels,J, enriched target.     

A study of the 70, 72, 74, 76Ge(d,p)71, 73, 75, 77Ge reactions using polarized deuterons

Differential cross sections and vector analyzing powers were measured at an incident deuteron energy of 12.0 MeV for the ^{70, 72, 74, 76}Ge(d, p)^{71, 73, 75, 77}Ge reactions. The data were analyzed with the distorted-wave Bom approximation. Spin and parity assignments were made to 13 states in ⁷¹Ge, 19 states in ⁷³Ge, 13 states in ⁷⁵Ge and 11 states in ⁷⁷Ge. Spectroscopic factors were extracted and a simple sum rule analysis was applied to the data.     

Shape coexistence close to N=50 in the neutron-rich isotope ~(80)Ge investigated by IBM-2

The properties of the low-lying states,especially the relevant shape coexistence in~(80)Ge,close to one of most neutron-rich doubly magic nuclei at N=50 and Z=28,have been investigated within the framework of the proton-neutron interacting model(IBM-2).Based on the fact that the relative energy of the d neutron boson is different from that of the proton boson,the calculated energy levels of low-lying states and E2 transition strengths can reproduce the experimental data very well.Particularly,the first excited state 0_2~+,which is intimately related to the shape coexistence phenomenon,is reproduced quite nicely.Theρ~2(E0,0_2~+→0_1~+)transition strength is also predicted.The experimental data and theoretical results indicate that both collective spherical andγ-soft vibration structures coexist in~(80)Ge.     

Effect of chemical surface treatments on interfacial and electrical characteristics of atomic-layer-deposited Al2O3 films on Ge substrates

The Ge surfaces were cleaned and passivated by two kinds of chemical pretreatments: conventional combination of HF + (NH₄)₂S, and new one of HBr + (NH₄)₂S. The chemical states and stability at passivated Ge surfaces were carefully characterized. The influence of chemical surface treatments on the interface and electrical properties of Al₂O₃ gate dielectric films on Ge grown by atomic layer deposition (ALD) has been investigated deeply. It is found that the combination of HBr and (NH₄)₂S can remove more Ge-O bonds on the Ge surface compared to that of conventional HF and (NH₄)₂S with excellent stability. X-ray photoelectron spectroscopy (XPS) reveals that HBr and (NH₄)₂S treated Ge surface has a mixture states of GeO_x (9.25%) and GeS (7.40%) while HF and (NH₄)₂S treated Ge surface has a mixture states of GeO_x (16.45%) and GeS (3.37%). And the Ge-S peak from the surface of Ge substrates decreases a little after the HBr and (NH₄)₂S treated Ge surface was exposed in the ambient for 300 min, which suggests the Ge surface is stable to oxidants. The Al₂O₃ films on HBr and (NH₄)₂S treated Ge substrates exhibits better electrical properties such as large capacitance, decreased leakage current density by ∼two orders of magnitude, and less C-V hysteresis. This indicates that a reduction in charge traps possibly at the interface and more interface traps are terminated by sulfur. The surface treatment of HBr and (NH₄)₂S seems to be very promising in improving the quality of high-k gate stack on Ge substrates.     

Spectroscopy of neutron deficient 65Ge

Excited states of ⁶⁵Ge were populated via the ¹²C + ⁵⁸Ni (261 MeV) reaction using the NORDBALL detector array equipped with charged-particle and neutron detector systems for reaction channel separation. On the basis of γγ-coincidence relations and angular distribution ratios a significantly extended level scheme was constructed up to E _x = 9 MeV and J ^π = (33/2^?). The low-energy states of the nucleus are discussed in the framework of the interacting boson-fermion model.     

Gamma-spectroscopic investigations on 67Ge

By γ-γ coincidence measurements following the ⁵⁷Fe(¹²C, 2nγ) reaction at E_12C = 40 MeV several new states above 1.5 MeV excitation energy in ⁶⁷Ge have been established. Spin and parity assignments on the basis of the angular distribution, linear polarization and γ-ray yield function indicate very similar structures in ^{67, 69}Ge. The positive-parity states can be followed up to the $\text{17}\text{2}{}^{\mathrm{+}}$ state at E_x = 3.07 MeV followed by a sequence of negative-parity high-spin states at nearly the same excitation energy relative to the $\text{9}\text{2}{}^{\mathrm{+}}$ single-particle state as in the neighbouring nucleus ⁶⁹Ge where these states were found to have strong single-particle admixtures. A reinvestigation of the spin of the E_x = 2.75 MeV level in ⁶⁹Ge resulting in a change of its spin from $\text{15}\text{2}{}^{\mathrm{+}}\text{to}\text{17}\text{2}{}^{\mathrm{+}}$ and for all spins above, removed the discrepancy concerning the spin assignments of corresponding levels in ^{67, 69}Ge. The excitation pattern of the Ge isotopes with 34 ≦ N ≦ 39 clearly indicate same structures probably due to the strong competition between collective and single-particle excitations along the whole chain similar to the results for the Zn isotopes.     

Excited states of154Nd studied through the decay of154Pr

Excited states in the neutron-rich doubly-odd nucleus⁷⁸As have been identified for the first time by proton-γ and γ-γ coincidence measurements via the⁷⁶Ge(α, pn) reaction at 32, 36, and 40 MeV beam energy. Four levels have been found to decay with lifetimes in the nanosecond region. The 5⁽⁺⁾ to (10⁺) states are ascribed to the (πg _9/2?νg _9/2) intruder two-quasiparticle configuration with some collective components in the 9⁽⁺⁾ and (10⁺) states.