共查询到18条相似文献,搜索用时 62 毫秒
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在U型管声致发光装置的基础上建立了一套新型的声致发光装置—直管圆锥泡声致发光装置,详细地介绍了此装置的结构和实验操作步骤,利用此装置得到了超强的发光脉冲。测量得到了乙二醇溶液中圆锥泡声致发光的发光脉冲,结果显示脉冲半宽度大约为80 μs左右,远远高于其他声致发光形式所产生的脉冲宽度,这主要是由于圆锥泡可以获得远远高于超声声致发光中气泡所能得到的能量。发光光谱为一从紫外光至可见光波长范围的连续谱,上面叠加C2有d3Πg→d3Πu的跃迁形成的五个序列谱带,分别对应于Δν=-2,Δν=-1,Δν=0,Δν=1和Δν=2;同时叠加有CN的B2Σ+→X 2Σ+跃迁形成的3个序列谱带和CH的A2Δ→X 2Π 跃迁谱带。特别是实验中测量得到了斯旺带光谱序列谱带清晰的振动结构。最后,通过与理论模拟得到的斯旺带光谱相对强度的比较,估算得到了C2分子的振动温度大约为(4 200±200) K。 相似文献
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丙三醇溶液声致发光中的黑体辐射谱 总被引:1,自引:0,他引:1
利用U型管圆锥泡声致发光装置,测量到了丙三醇溶液中圆锥泡声致发光的光谱和光脉冲。结果表明,测量得到的发光光谱为光滑的连续谱,且与理论模拟得到的黑体辐射谱相吻合,拟合温度分布于2 600~3 500 K范围内。文章从空间和时间两方面分析了圆锥泡空化发光中存在黑体辐射的原因:较大的气泡体积(气泡塌缩半径为1.4 cm)与较长的发光时间(几十微秒)。另外,实验研究表明随着发光波长的增长,光脉冲宽度变宽,从而进一步证明了圆锥泡声致发光中的黑体辐射机制。最后,利用测量得到的发光光谱和脉冲计算得到了发光光强为0.18 J,远远高于其他方式得到的声致发光光强。 相似文献
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介绍两种使用流体动力学实现声致发光的方法:刹管法和U管圆锥泡法.这两种方法的设备简单,操作方便,容易在普通物理实验中进行,所得结果和传统单泡声致发光有所不同.U管圆锥泡法创造了发光功率和单脉冲能量的新记录,并首次用条纹相机得到了时间分辨发射光谱. 相似文献
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在溶有稀有气体的稀土盐氯化铽水溶液中进行了单泡声致发光光谱的研究. 在固定驱动超声频率、不同驱动声压下, 观察到了一系列OH自由基从第一激发态A2∑+到基态X2Π 各振动能级跃迁所产生的谱线, 包括波长307 nm处的(0, 0)跃迁谱线, 335 nm处的(0, 1)跃迁谱线以及276 nm处的(1, 0) 跃迁谱线等. 实验结果表明较高的驱动声压有利于 276 nm处谱线的产生, 而较低的驱动声压则有利于 307 与 335 nm 处谱线的产生. 通过定义线状光谱与连续谱的光强比, 定量地表征了线状光谱在总光谱中的相对强度, 并给出了驱动声压对各跃迁谱线光强比的影响.
关键词:
单泡声致发光
驱动声压
线状光谱
光强比 相似文献
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Cavitation luminescence is light emission from gases that are compressed to high temperature and high pressure inside a bubble or group of bubbles. The numerical simulation in this study indicates that if the temperature and pressure inside a bubble are not high enough, then dim and spectral line emission dominates. However, if the temperature and pressure inside the bubble are very high, then the light is bright and a continuum spectrum will be generated. Calculations of the spectrum using modified equations of bubble motion can simulate the spectral profile well. However, pulse width calculations using these equations only partly agree with the experimental results. 相似文献
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Numerical solutions of the differential equation for a bubble performing finite-amplitude vibration are given in detail for a variety of situations. The results demonstrate that in lower acoustic pressure (maximum Mach number very low) its vibration has bounce. When acoustic pressure is in excess of 1.18atm and the instantaneous radius of the bubble approaches its equivalent Van der Waals radius, the maximum velocity and acceleration on the surface of a bubble have a huge increase in a very short period, which seems to favour the sonoluminescence. In vacuum environment (0.1atm), an intensive sonoluminescence could be generated. 相似文献
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A modified U-tube conical bubble sonoluminescence device is used to
study the conical bubble photoluminescence. The spectra of conical
bubble sonoluminescence at different concentrations of rhodamine 6G
(Rh6G) solution in 1,2-propanediol have been measured. Results show
that the sonoluminescence from the conical bubbles can directly
excite Rh6G, which in turn can fluoresce. The light emission of this
kind is referred to as conical bubble photoluminescence. The maximum
of fluorescence spectral line intensity in the conical bubble
photoluminescence has a red shift in relative to that of the
standard photo-excited fluorescence, which is due to the higher
self-absorption of Rh6G, and the spectral line of conical bubble
photoluminescence is broadened in width compared with that of
photo-excited fluorescence. 相似文献
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Using the equations of fluid mechanics with proper boundary conditions and taking account of the gas properties, we can numerically simulate the process of single bubble sonoluminescence, in which electron-neutral atom bremsstrahlung, electron-ion bremsstrahlung and recombination radiation, and the radiative attachment of electrons to atoms and molecules contribute to the light emission. The calculation can quantitatively or qualitatively interpret the experimental results. We find that the accumulated heat energy inside the compressed gas bubble is mostly consumed by the chemical reaction, therefore, the maximum degree of ionization inside Xe bubble in water is much lower than that in sulfuric acid, of which the vapour pressure is very low. In addition, in sulfuric acid much larger pa and R0 are allowed which makes the bubbles in it much brighter than that in water. 相似文献
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In our previous paper, we derived a new single bubble model including the effect of bulk viscosity. To confront it to experiments, single bubble dynamics was measured here in 30% (v/v) glycerol-water mixture under different acoustic amplitudes and compared to models including or not the effect of bulk viscosity. The results showed that calculated bubble dynamics were not significantly affected by the bulk viscosity within the experimental conditions used in this study. However, there was a noticeable delay for the first rebound when bulk viscosity was considered. The corresponding sonoluminescence intensities were collected and compared with theoretical predictions. The results did not allow to discriminate between the two models (one includes the effect of bulk viscosity, the other does not), confirming the negligible effect of bulk viscosity in this condition (30% (v/v) glycerol-water mixture). Due to the instability of a single bubble in higher viscosity solutions, we could not implement experiments that can discriminate between the two models. 相似文献
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Rasoul Sadighi-Bonabi Mona Mirheydari Homa Ebrahimi Nastaran Rezaee Lida Nikzad 《中国物理 B》2011,20(7):74302-074302
Based on a quasi-adiabatic model,the parameters of the bubble interior for a moving single bubble sonoluminescence (m-SBSL) in water are calculated.By using a complete form of the hydrodynamic force,a unique circular path for the m-SBSL in water is obtained.The effect of the ambient pressure variation on the bubble trajectory is also investigated.It is concluded that as the ambient pressure increases,the bubble moves along a circular path with a larger radius and all bubble parameters,such as gas pressure,interior temperature and light intensity,increase.A comparison is made between the parameters of the moving bubble in water and those in N-methylformamide.With fluid viscosity increasing,the circular path changes into an elliptic form and the light intensity increases. 相似文献