用SHG-FROG方法测量超短光脉冲的振幅和相位

介绍了二次谐波振荡频率分辨光学快门(SHGFROG)测量超短脉冲的实验系统和二维相位恢复算法,这种方法可以实现对超短脉冲振幅和相位的完全测量.利用矩阵方法数值模拟了几种常见超短脉冲的SHGFROG迹线,并用主元素广义投影算法(PCGPA)从这些无噪音的SHGFROG迹线中恢复了脉冲的振幅和相位,误差接近收敛的标准.研究结果表明,这种测量方法结构简单,算法可靠,是测量超短脉冲的理想方法之一.     

Design of phase-modulated broadband refocusing pulses

Broadband linear-phase refocusing pulses were designed with the Shinnar-Le Roux (SLR) transformation and verified experimentally. The design works in several steps: initially, a linear-phase B polynomial is created with the Parks-McClellan/Remez exchange algorithm. The complementary A polynomial required for the SLR transformation is generated with the Hilbert transformation, yielding the minimum-phase response. The phase response of the A polynomial is altered by zero-flipping, which changes the overall pulse shape while retaining its refocusing profile. Optimal pulses in terms of minimal B(1max) and hence broadest bandwidth were found with non-linear optimisation of the zero-flipping pattern. These pulses are generally phase modulated with a time-symmetric amplitude and anti-symmetric phase modulation. In this work, a whole range of pulses were designed to demonstrate the underlying relationships. Five exemplary pulses were implemented into a PRESS sequence and validated by acquiring images of a water-oil phantom and lactate spectra at TE = 144 ms.     

The Measurement of Ultrashort Light Pulses—Simple Devices,Complex Pulses

We review the state of the art of ultrashort-light-pulse measurement using frequency-resolved-optical-gating (FROG). Recent developments have extended the state of the art considerably. FROG devices for measuring the intensity and phase of ultrashort laser pulses have become so simple that almost no alignment is required. In addition, such devices not only operate single shot, but they also yield the two most important spatio-temporal distortions, spatial chirp and pulse-front tilt. With other FROG variations, it is now possible to measure more general ultrashort light pulses (i.e., pulses much more complex than common laser pulses), with time-bandwidth products as large as several thousand and as weak as a few hundred photons, and despite other difficulties such as random absolute phase and poor spatial coherence.     

Inhibiting three-body recombination in atomic Bose-Einstein condensates

We discuss the possibility of inhibiting three-body recombination in atomic Bose-Einstein condensates via the application of resonant 2pi laser pulses. These pulses result in the periodic change in the phase of the molecular state by pi, which leads to destructive interference between the decay amplitudes following successive pulses. We show that the decay rate can be reduced by several orders of magnitude under realistic conditions.     

Femtosecond pulse shaping by dynamic holograms in photorefractive multiple quantum wells

Femtosecond pulses can be shaped in the time domain by diffraction from dynamic holograms in a photorefractive multiple quantum well placed inside a Fourier pulse shaper. We present several examples of shaped pulses obtained by controlling the amplitude or the phase of the hologram writing beams, which modifies the complex spectrum of the femtosecond output.     

Femtosecond diode laser MOPA system at 920 nm based on asymmetric colliding pulse mode-locking

We report on the generation of 267 fs long pulses with a peak power of 661 W emitted by an InGaAs diode laser master-oscillator power-amplifier (MOPA) system with an external grating compressor. The oscillator emits strongly chirped picosecond pulses with several nanometer of bandwidth, which can be amplified without significant phase modulation and are compressed to femtosecond pulses after leaving the amplifier. We used a diode laser module for asymmetric colliding pulse mode-locking and optimized the collision point and the relative intensity of the counter-propagation pulses.     

高次谐波产生阿秒极紫外和X光脉冲研究新进展

 近年来在可见光谱范围内已经把激光脉冲压缩到接近一个光学周期(2～3 fs)的物理极限,几fs的时间分辨精度可以描述分子化学反应过程,但是要探测远小于可见光周期的电子跃迁过程则需要阿秒(as)量级的光脉冲。利用脉冲间具有相同载波包络相位的阿秒脉冲序列能把可见光波段的光学频率梳向极紫外波段扩展;利用电子和离子碰撞复合过程短于一个光周期这个时间窗,通过测量激光场椭圆极化率对电子轨迹的微扰实现了as精度的分辨率;通过测量碰撞复合过程中的高能电子的辐射谱可以重构阿秒X光脉冲以及探测强场下束缚态和连续态电子动力学。     

光学参变啁啾脉冲放大相位失配啁啾脉冲频谱整形新方法

相位匹配是实现高效光学参变啁啾脉冲放大(OPCPA)能量转换的关键之一,通过对几种常用非线性晶体的光学参变啁啾脉冲放大过程进行数值模拟研究,结果表明一定程度的相位失配不但能增加光学参变啁啾脉冲放大增益带宽,而且会使啁啾脉冲光谱强度分布中间凹陷。提出利用光学参变啁啾脉冲放大相位失配放大作为啁啾脉冲频谱整形的新方法,通过理论分析和模拟计算,找到了光学参变啁啾脉冲放大相位失配啁啾脉冲频谱整形效果的控制量;并对几种常用非线性晶体在简并、近简并、非简并等条件下的光学参变啁啾脉冲放大相位失配放大特性进行了比较。     

Linear phase slope in pulse design: application to coherence transfer

Using optimal control methods, robust broadband excitation pulses can be designed with a defined linear phase dispersion. Applications include increased bandwidth for a given pulse length compared to equivalent pulses requiring no phase correction, selective pulses, and pulses that mitigate the effects of relaxation. This also makes it possible to create pulses that are equivalent to ideal hard pulses followed by an effective evolution period. For example, in applications, where the excitation pulse is followed by a constant delay, e.g. for the evolution of heteronuclear couplings, part of the pulse duration can be absorbed in existing delays, significantly reducing the time overhead of long, highly robust pulses. We refer to the class of such excitation pulses with a defined linear phase dispersion as ICEBERG pulses (Inherent Coherence Evolution optimized Broadband Excitation Resulting in constant phase Gradients). A systematic study of the dependence of the excitation efficiency on the phase dispersion of the excitation pulses is presented, which reveals surprising opportunities for improved pulse sequence performance.     

Generation of Extremely Short Pulses upon Excitation of a Resonant Medium by a Superluminal Light Spot

The possibility of generation of quasi-unipolar extremely short pulses (with a duration of several periods of field oscillations) is theoretically analyzed for the excitation of a circular, nonlinear, and resonant medium with a light spot. The light spot rotates along a circle with a velocity that exceeds the speed of light in vacuum, while particles of the medium are distributed uniformly along the circle. It is shown that, by introducing a delay in the form of a phase plate into the system, one can control the shape, the duration, and the amplitude of generated pulses.     

腔内相位调制全光纤脉冲激光器Ⅰ: 实验

报道了在低频直接相位调制下,掺铒光纤激光器的脉冲现象。在光纤激光器谐振腔中插入带尾纤的LiNbO3相位调制器,利用低频周期性信号进行相位调制,能够得到重复频率为几十千赫到几百千赫左右的均匀、稳定的脉冲光输出,且发现激光光谱变化等现象。分析表明,这种脉冲现象难以用调Q、锁模等传统的脉冲光理论进行有效地解释。简要讨论了脉冲光产生的物理机制,通过对相位调制与“驰豫振荡”关系的研究,唯象地认为相位调制和“驰豫振荡”是脉冲光产生的原因。     

Phase evolution of the reemitted field in the semiconductor quantum wells under the femtosecond pulse train intersubband excitation

Property of the phase of the reemitted field in the semiconductor quantum wells (QWs) excited by femtosecond pulse train is investigated. It is shown that the phase evolution of the reemitted field is controlled by the relative phase between the successive pulses of the incident train. For all the odd pulses excitation,the reemitted field is from out-of-phase to in-phase, then again to out-of-phase with the incident pulses,whereas for all the even pulses excitation, the situation is the opposite, i.e., it is from in-phase to out-of-phase, then again to in-phase with the incident pulses.     

A rotational approach to localized SPAMM 1-1 tagging

Magnetic resonance tagging usually relies on controlling the phase dispersion of the transverse magnetization component. Phase dispersion is, however, affected by the inherent phase of selective excitation pulses, thus limiting their combination with tagging sequences to the application of refocusable pulses, as in the localized spatial modulation of magnetization (L-SPAMM) technique. In this study, we examine the effect of selective excitation pulses on a L-SPAMM 1-1 sequence, showing that in the case of two identical pulses the phase component is canceled out, and thus preemphasis and refocus gradients are not needed, allowing us to take advantage of a constant gradient throughout the tagging sequence, and also that one might choose nonrefocusable maximum and minimum phase pulses.     

Effects of the carrier-envelope phase of chirped laser pulses in the multiphoton ionization regime

By solving the time-dependent Schr?dinger equation for the Cs atom, we find that, as long as the spectral bandwidth is sufficiently broad, the asymmetry of photoelectron ejection is strongly phase dependent and persists even when the chirped pulse duration becomes more than several cycles. The asymmetry survives even after the angle integration over the hemisphere, implying that the detection efficiency can be significantly improved. This counterintuitive and robust finding provides a simple way to measure the phase for both transform-limited and chirped pulses.     

Pressure-induced amorphization in silicon caused by the impact of electrosprayed nanodroplets

This Letter describes the shock-induced amorphization of single-crystal Si bombarded by nanodroplets. At impact velocities of several kilometers per second, the projectiles trigger strong compression pulses lasting tens of picoseconds. The phase transition, confirmed via transmission electron microscopy and electron backscatter diffraction, takes place when the projectile's stagnation pressure is approximately 15?GPa. We speculate that the amorphization results either from the decompression of the β-Sn phase or during the compression of the diamond phase.     

Passive mode-locking of a ruby laser using low-frequency stimulated brillouin scattering in birefingent crystals

A new technique of mode-locking Q-switched lasers using a birefringent crystal as an intracavity element is reported. Intense elastic waves are generated inside a birefringent crystal through the low-frequency, stimulated Brillouin scattering process and these in turn modulate the refractive index of the crystal and thus provide the necessary phase synchronization for mode-locking. Strong coupling between several neighboring modes of the laser is evidenced by the observation of high pulse repetition rates (several pulses circulating simultaneously within the cavity).     

Active mode locking of a phase-conjugating SBS-laser oscillator

We present a flashlamp-pumped Nd:YAG laser simultaneously emitting pulse structures on microsecond, nanosecond and picosecond time scales. Within a microsecond flashlamp pump pulse a nonlinear reflector based on stimulated Brillouin scattering (SBS) generates several Q-switch pulses. The phase-conjugating effect of the SBS reflector provides a compensation of phase distortions generated inside the laser rod, resulting in transverse fundamental mode operation. Additional acousto-optic loss modulation inside the resonator leads to mode locking. As a result, each Q-switch pulse is subdivided into several picosecond pulses. Energies of up to 2 mJ for the mode-locked pulses with durations between 220 and 800 ps are demonstrated. The wide variability of the lasers temporal output parameters as well as its high beam quality make it a splendid tool for fundamental research in laser materials processing. PACS 42.60.Fc; 42.60.Gd; 42.65.Es     

Nonlinear optics with phase-controlled pulses in the sub-two-cycle regime.

Nonlinear optical effects due to the phase between carrier and envelope are observed with 5 fs pulses from a Kerr-lens mode-locked Ti:sapphire laser. These sub-two-cycle pulses with octave spanning spectra are the shortest pulses ever generated directly from a laser oscillator. Detection of the carrier-envelope phase slip is made possible by simply focusing the short pulses directly from the oscillator into a BBO crystal. As a further example of nonlinear optics with such short pulses, the interference between second- and third-harmonic components is also demonstrated.     

Electro-optic modulation of single photons

We use the Stokes photon of a biphoton pair to set the time origin for electro-optic modulation of the wave function of the anti-Stokes photon thereby allowing arbitrary phase and amplitude modulation. We demonstrate conditional single-photon wave functions composed of several pulses, or instead, having Gaussian or exponential shapes.     

二次发射微波电子枪的模拟计算及其特性分析

 采用URMEL-T程序进行了二次发射微波电子枪的腔内电磁计算和特性分析。同时利用URMEL-T得出的腔内轴向电场及自编程序,模拟电子在该高频场作用下的运动。计算表明二次发射微波电子枪确实具有相位选择性,进而探讨了腔形尺寸、射频电场强度对相位选择性和产生二次倍增的有关条件的影响,以及输出电子的能量稳定性。模拟结果表明,这类电子枪（MPG）可得到高电流密度（5303A/cm²）及短脉冲（3.15~10ps）的电子束。