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1.
We present a numerical result of photoionization rate for the one-dimensional molecular hydrogen ion model exposed to intense light of 1 × 10^16-2×10^16 W/cm^2, 55-as pulse duration, and 800nm wavelength. In contrast to the previous calculation result of charge-resonance-enhanced ionization for lower intensity and much longer pulse, our result exhibits an ionization saturation. The numerical results are interpreted in the field-dressed potential picture as over-the-barrier liberation of electrons. This extremely short pulsewidth and relatively high field phenomenon requests experimental demonstration.  相似文献   

2.
On the platform of the 3D H2^+ system, we perform a numerical simulation of its photoionization rate under excitation of weak to intense laser intensities with varying pulse durations and wavelengths. A novel method is proposed for calculating the photoionization rate: a double exponential decay of ionization probability is best suited for fitting this rate. Confirmation of the well-documented charge-resonance-enhanced ionization (CREI) effect at medium laser intensity and finding of ionization saturation at high light intensity corroborate the robustness of the suggested double-exponential decay process. Surveying the spatial and temporal variations of electron wavefunctions uncovers a mechanism for the double-exponentially decayed photoionization probability as onset of electron ionization along extra degree of freedom. Henceforth, the new method makes clear the origins of peak features in photoionization rate versus internuclear separation. It is believed that this multi-exponentially decayed ionization mechanism is applicable to systems with more degrees of motion.  相似文献   

3.
By means of the numerical solution of time-dependent Schr6dinger equation, we verify a scaling law of photoionization in ultrashort pulses. We find that for a given carrier-envelope phase and duration of the pulse, identical photoionizations are obtained provided that when the central frequency of the pulse is enlarged by k times, the atomic binding potential is enlarged by k times, and the laser intensity is enlarged by ka times. The scaling law allows us to reach a significant control over direction of photoemission and offers exciting prospects of reaching similar physical processes in different interacting systems which constitutes a novel kind of coherent control.  相似文献   

4.
We present an alternative approach for determining the photoionization rate of hydrogen molecules under the interaction of intense light, by calculating the spatial overlap integral between the potential function and the time-dependent wavefunction. The suggested method was applied to varying excitation pulse shapes: square envelope and chirped hyperbolic secant envelope. The computed results confirmed that our method was robust and could be extended to general molecular dynamics calculations.  相似文献   

5.
Using a nonperturbative scattering theory, We study the photoelectron angular distributions (PADs) of Kr atoms irradiated by an infinite sequence of intense single-cycle pulses of circular polarization. We demonstrate the inversion asymmetry of PADs and the dependence of PADs on the carrier-envelop phase of the single-cycle pulses. The inversion asymmetry is caused by the interference between transition channels where the different channels are characterized by different combinations of absorbed-photon numbers in the ionization process. Our results provide a possible method to determine the value of carrier-envelop phase by the detected PADs.  相似文献   

6.
The essential goal of that paper (Chin. Phys. Lett. 26(2009) 124211) was to obtain a 2μm Tm:YAG laser with short pulse output. A Q-switched technique is used to realize the short pulse output in our laser system. The idea presented by Dr. Nieolaie Pavel is right. In our work, the directly Q-switched 2μm Tm:YAG pulse laser is not realized. As a matter of fact, the Q switch is used to directly switch the 1μm Nd:YAG laser.  相似文献   

7.
A flashlamp-pumped Cr:LiSAF laser system with a voltage controlled Q-switch structure in the cavity is designed. A dual-wavelength and dual-pulse tunable laser output is gained. The relation of laser output behavior with input energy is studied experimentally. The output is dual-pulsed with the energy of the 32m J/pulse producing the total output energy of 64mJ and the pulse width is about 27ns at 850nm. Then, we use one LBO crystal as the frequency doubling crystal to obtain a dual wavelength (448.1 nm and 449.15nm) and dual pulse laser. The output for one wavelength is about 10.3mJ and the line width is less than 0.02nm.  相似文献   

8.
A tightly focused femtosecond Ti:sapphire laser pulse is used to initiate micro-explosions on the surface and internal to an Fe:LiNb03 crystal. The resulting structure is morphologically different from that induced in an isotropic sample such as fused silica. The regular pyramid and irregular pyramid craters on the surface of the sample are produced at different positions of focal points. The craters suggest vaporization of materials in the process of micro-explosion due to the expansion of high temperature plasma. The embossment pyramids on the surface present the dynamical process of large volume material displacements under high temperature and pressure, and recrystallization of anisotropy crystal materials.  相似文献   

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