Rotational power loss of magnetic steel sheets in a circular rotational magnetic field in CCW/CW directions

This paper presents rotational power loss properties of magnetic steel sheets under high flux density conditions using two-dimensional vector magnetic properties measurement. Recently it was reported by some research groups that the magnetic power loss measured in a counter clockwise (CCW) rotating field differed from that in a clockwise (CW) rotating field. This phenomenon was only observed in case of higher magnetic flux density excitation condition. We call this the CCW/CW problem. To clarify the reasons why the disagreement exists in the CCW/CW direction, we have examined angle errors of H- and B-coils by using geometrical, optical and magnetic methods. Then we compensated the measured vector components including different signals due to the angle errors. In the components of irremovable small angle error, we have also used the measured field strength waveforms in CCW/CW conditions. We have applied the compensation method to measurement of a grain-oriented electrical steel sheet.     

Effect of sample shape on nonlinear magnetization dynamics under an external magnetic field

Effect of sample shape on the nonlinear collective dynamics of magnetic moments in the presence of oscillating and constant external magnetic fields is studied using the Landau–Lifshitz–Gilbert (LLG) approach. The uniformly magnetized sample is considered to be an ellipsoidal axially symmetric particle described by demagnetization factors and uniaxial crystallographic anisotropy formed some angle with an applied field direction. It is investigated as to how the change in particle shape affects its nonlinear magnetization dynamics. To produce a regular study, all results are presented in the form of bifurcation diagrams for all sufficient dynamics regimes of the considered system. In this paper, we show that the sample's (particle's) shape and its orientation with respect to the external field (system configuration) determine the character of magnetization dynamics: deterministic behavior and appearance of chaotic states. A simple change in the system's configuration or in the shapes of its parts can transfer it from chaotic to periodic or even static regime and back. Moreover, the effect of magnetization precession stall and magnetic moments alignment parallel or antiparallel to the external oscillating field is revealed and the way of control of such “polarized” states is found. Our results suggest that varying the particle's shape and fields’ geometry may provide a useful way of magnetization dynamics control in complex magnetic systems.     

Electronic structure and magnetic properties of Gd3Co11B4 compound

The electronic structure of hexagonal Gd₃Co₁₁B₄ compound has been studied by X-ray photoemission spectroscopy (XPS) and ab initio self-consistent tight binding linear muffin tin orbital (TB LMTO) method. We have found a good agreement between the experimental XPS valence band spectra and theoretical LMTO calculations. Results showed that the Gd₃Co₁₁B₄ compound is ferrimagnetic with the calculated total magnetic moment M=14.29 μ_B/f.u. The values of the magnetic moments on Co atoms strongly depend on the local environment. We have also compared the electronic structure and magnetic properties of Gd₃Co₁₁B₄ compound with those of Nd₃Co₁₁B₄ compound.     

The use of symmetry in the search for canted ferromagnetism, its application to the molecular magnets Mn[N(CN)2]2 and Fe[N(CN)2]2

Canted ferromagnets present a important class of molecular magnets. In these materials the uncompensated magnetisation, created by the DzyaloshinskyMoriya interaction, has the particular property of being compatible with the symmetry of the underlying antiferromagnetic Hamiltonian. If the ordering transition is continuous, Landau theory and simple symmetry arguments about the crystal structure can be used to determine whether such parasitic ferromagnetism is possible, and therefore to aid the systematic search for new molecular ferromagnets.     

Theory of spin transfer phenomena in magnetic metals and semiconductors

We propose a general theory of the spin-transfer effects that occur when current flows through inhomogeneous magnetic systems. Our theory does not rest on an appeal to conservation of total spin, can assess whether or not current-induced magnetization precession and switching in a particular geometry will occur coherently, and can estimate the efficacy of spin-transfer when spin-orbit interactions are present. We illustrate our theory by applying it to a toy-model twodimensional-electron-gas ferromagnet with Rashba spin-orbit interactions.     

Theory of carrier mediated ferromagnetism in dilute magnetic oxides

We analyze the origin of ferromagnetism as a result of carrier mediation in diluted magnetic oxide semiconductors in the light of the experimental evidence reported in the literature. We propose that a combination of percolation of magnetic polarons at lower temperature and Ruderman-Kittel-Kasuya-Yosida ferromagnetism at higher temperature may be the reason for the very high critical temperatures measured (up to ∼700 K).     

Dependence of magnetic anisotropy of the La0.67Ca0.33MnO3 films on substrate and film thickness

Strain in the La_0.67Ca_0.33MnO₃ films has been tuned by varying substrate and film thickness, and its effects on magnetic anisotropy are studied based on the measurements of isothermal magnetization. Measuring the strain in the films by the out-of-plane lattice parameter (c), we found a strong dependence of the magnetic anisotropy constant (Ku) on strain. Ku decreases linearly from ∼−1.1×10⁶ erg/cm³ for c=0.763 nm to 1.2×10⁶ erg/cm³ for c=0.776 nm, corresponding to a change from tensile strain to compressive strain. Positive Ku signifies a uniaxial anisotropy with the easy axis perpendicular to the film plane, while negative Ku demonstrates an anisotropy of the easy plane character. Smaller or larger c leads a decrease or increase in Ku, which indicates the presence of other effects in addition to those associated with strain. Three distinctive processes for the magnetization are observed along the hard magnetic axis of the films on (001)SrTiO₃, suggesting a possibility of strain relaxation even in ultra-thin films.     

The magnetic orderings and phase transitions of rare-earth rhodium borides

Perturbation theory and mean-field approach have been employed in the present work to estimate the Heisenberg coupling constants 's for the ferromagnet DyRh₄B₄ and the antiferromagnet TmRh₄B₄ from their magnetic transition temperatures T_M's in comparison with GdRh₄B₄. We found that the 's of these substances are different from each other, which may be attributed to their different electronic structures and also the anisotropic nature of the Heisenberg exchange coupling.     

Out-of-plane exchange bias and magnetic anisotropy in MnPd/Co multilayers

Magnetic and structural properties in [MnPd/Co]₁₀ multilayers deposited onto Si(1 1 1) substrates have been investigated. The dependences of anisotropy and exchange bias on the thicknesses of both MnPd and Co layers have been studied. In most of the samples, the out-of-plane magnetic anisotropy and both large out-of-plane and in-plane exchange biases have been observed at cryogenic temperature below the blocking temperature T_B≈240 K. With appropriate MnPd and Co thicknesses, we have obtained samples with a large out-of-plane exchange bias along with a large out-of-plane magnetic anisotropy. The origin of the out-of-plane magnetic anisotropy in the samples has been suggested to be due to the formation of CoPd interfacial alloys which have tensile in-plane strains, while the spin structure of the antiferromagnetic layer at the interface which is believed to be responsible for exchange bias may be the same as that of the bulk material. Also, the present study shows that the interplay between the out-of-plane magnetic anisotropy and exchange bias is evident in our multilayers and plays an important role in the out-of-plane exchange-bias mechanism.     

An evaluation method of cross-type H-coil angle for accurate two-dimensional vector magnetic measurement

Recently, two-dimensional vector magnetic measurement has become popular and many researchers concerned with this field have attracted to develop more accurate measuring systems and standard measurement systems. Because the two-dimensional vector magnetic property is the relationship between the magnetic flux density vector B and the magnetic field strength vector H, the most important parameter is those components. For the accurate measurement of the field strength vector, we have developed an evaluation apparatus, which consists of a standard solenoid coil and a high-precision turntable. Angle errors of a double H-coil (a cross-type H-coil), which is wound one after the other around a former, can be evaluated with this apparatus. The magnetic field strength is compensated with the measured angle error.     

Phase diagram of Fe1−xCox ultrathin film

Concentration-driven reorientation phase transitions in ultrathin magnetic films of FeCo alloy have been studied. It is established that, in addition to the easy-axis and easy-plane phases, a spatially inhomogeneous phase (domain structure), a canted phase, and also an “in-plane easy-axis” phase can exist in the system. The realization of the last phase is associated with the competition between the single-ion anisotropy and the magnetoelastic interaction. The critical values of Co concentration corresponding to the phase transitions are evaluated, the types of phase transitions are determined, and the phase diagrams are constructed.     

Spin-wave resonance and magnetic anisotropy in FePt thin films

Ferromagnetic Resonance (FMR) measurements at room temperature and X-band microwave frequency were performed on polycrystalline FePt thin films with face-centered cubic structure. With the external field perpendicular to the film plane, the absorption fields H_n of the odd and even spin-wave resonance modes n detected for the Fe_0.44Pt_0.56(45 nm)/Si(1 0 0) and Fe_0.51Pt_0.49(105 nm)/Pt(55 nm)/MgO(1 0 0) films, were found to obey the well-known H_n×n² ratio, giving for these films the exchange stiffness constant values of 3.9×10⁻⁸ and 4.4×10^–7 erg/cm, respectively. The study of the out-of-plane angular dependence of the absorption field of the uniform FMR mode allowed the measurement of the effective magnetic anisotropy constants of 5.3×10⁶ , 6.4×10⁶ , and 6.7×10⁶ erg/cm³, related, respectively, to the [1 1 1], [1 0 0], and [1 1 0] textures present in the films.     

Effect of Co-Substitution on Magnetic Properties in Spinels GeNi2O4 Systems

The magnetic properties of spinel GeNi_2-2xCo_2xO₄ systems in the range 0≤x≤1 are studied by mean field theory and high-temperature series expansions. The nearest neighbouring and the next-neighbouring super-exchange interactions J₁ (x) and J₂(x) are evaluated for these systems in the range 0≤x≤1, by using the first theory. The intra-planar and the inter-planar interactions and the exchange energy are deduced. The second theory is applied in the spinel GeNi_2-2xCo_2xO₄ systems, combined with the Padé approximants method, to determine the magnetic phase diagrams (T_N versus dilution x) in the range 0≤x≤1. The obtained theoretical results are in agreement with experimental data obtained by magnetic measurements. The critical exponents associated with the magnetic susceptibility γ and the correlation lengths ν are deduced.     

Soft X-ray magnetic circular dichroism of Heusler-type alloy Co2MnGe

Co and Mn 2p core absorption (XAS) and X-ray magnetic circular dichroism (XMCD) spectra have been measured for the ferromagnetic ternary alloy Co₂MnGe. The observed Co 2p XAS spectrum can be understood on the basis of the unoccupied Co 3d partial density of states, whereas the overall features of the Mn 2p XAS and XMCD spectra have been partly reproduced by the Mn 2p⁵3d⁶ final state multiplets. We have found that the orbital polarization of the Co 3d and even the Mn 3d states are recognizable, which suggests that a spin-orbit coupling should be taken into account in the energy band structure in order to reproduce the half metallic nature of this alloy.     

Spin dynamics and spin correlations in the spinS=1 two-dimensional square-lattice Heisenberg antiferromagnet La2NiO4

The static and dynamic spin fluctuations in the spinS=1, two-dimensional (2D) square-lattice antiferromagnet La₂NiO₄ have been studied over a wide temperature range using neutron scattering techniques. The spin correlations in La₂NiO₄ exhibit a crossover from two- to three-dimensional (3D) behavior as the Néel temperature is approached from above. Critical slowing down of the low-energy spin fluctuations is also observed just aboveT _N . The correlation length, (T), and the static structure factor,S(0), have been measured and are compared with recent theoretical calculations for the quantum 2D Heisenberg antiferromagnet using microscopic parameters determined from previous spin-wave measurements. Good agreement for (T) is found with the exact low-temperature result of Hasenfratz and Niedermeyer provided that 2 p _s is renormalized by 20% from the spin-wave value.     

Zn Doping Effect on Magnetic Properties of Znx Cdl-xCr2S4 Systems by High-Temperature Series Expansions

The effect of Zn doping on the magnetic properties of CdCr2S4 systems is studied by mean field theory and high-temperature series expansion （HTSE）. The nearest neighbouring and the next-neighbouring super-exchange interactions Jl（x） and J2（x） are evaluated for the spinel system Zn, Cd1-xCr2S4 in the range 0 〈 x 〈 1. The intra-planar and the inter-planar interactions are deduced. The HTSE combined with the Padd approximant method （PA） is applied to the spinel system ZnxCdl-,Cr2S4. The magnetic phase diagram, i.e. Tc versus dilution x, is obtained. The critical exponents associated with the magnetic susceptibility 7 and the correlation length u are deduced. The obtained theoretical results are in agreement with the experimental data obtained by magnetic measurements.     

The study of relatively low density stellar matter in presence of strong quantizing magnetic field

The effect of strong quantizing magnetic field on the equation of state of matter at the outer crust region of magnetars is studied. The density of such matter is low enough compared to the matter density at the inner crust or outer core region. Based on the relativistic version of semi-classical Thomas-Fermi-Dirac model in presence of strong quantizing magnetic field a formalism is developed to investigate this specific problem. The equation of state of such low density crustal matter is obtained by replacing the compressed atoms/ions by Wigner-Seitz cells with nonuniform electron density. The results are compared with other possible scenarios. The appearance of Thomas-Fermi induced electric charge within each Wigner-Seitz cell is also discussed.     

Two-dimensional electron gas in a periodic magnetic field

We study the energy spectrum and electronic properties of a two-dimensional (2D) spinless electron gas in a periodic magnetic field which has the symmetry of a triangular lattice. We show that the energy bands depend strongly on the value of the magnetic field. For large field the low-energy electrons are localized on closed rings where the magnetic field vanishes. This results in the appearance of persistent currents around these rings. We also calculate the intrinsic Hall conductivity, which is quantized when the Fermi level is in a gap.     

Magnetic properties of the compounds ThCO2Ge2 and ThCo2Si2

Rather old preparation of the compounds ThCo₂Ge₂ and ThCo₂Si₂ and their magnetic study in the temperature range 100–570 K, published by Omejec and Ban [Z. Anorg. Allg. Chem. 380 (1971) 111], indicated that both compounds ordered ferrromagnetically below 100 K. In order to verify the old data, polycrystalline samples of ThCo₂Ge₂ and ThCo₂Si₂ have been prepared by arc melting and subsequent annealing, and studied by X-ray diffraction at room temperature (RT), by superconducting quantum interference device (SQUID)-magnetization and AC-susceptibility measurements at 2–320 K, and by dc-magnetization measurements in variable magnetic fields up to 120 kOe at 5, 80, and 283 K. The magnetic measurements confirm the ferromagnetic ordering in both compounds, but with totally different Curie temperatures: ≈120(20) K for ThCo₂Ge₂ and above 320 K for ThCo₂Si₂. The paramagnetic values of ThCo₂Ge₂ and the ordering of both compounds are discussed and compared with the old results of Omejec and Ban.