Cluster fermionic Ising spin glass model with a transverse field

The fermionic Ising spin glass (SG) model in the presence of a transverse magnetic field Γ is studied within a cluster mean field theory. The model considers an infinite-range interaction among magnetic moments of clusters with a short-range ferromagnetic intracluster coupling J₀. The spin operators are written as a bilinear combination of fermionic operators. In this quantum SG model, the intercluster disorder is treated by using a framework of one-step replica symmetry breaking (RSB) within the static approximation. The effective intracluster interaction is then computed by means of an exact diagonalization method. Results for several values of cluster size n_s, Γ and J₀ are presented. For instance, the specific heat can show a broad maximum at a temperature T^∗ above the freezing temperature T_f, which is characterized by the intercluster RSB. The difference between T^∗ and T_f is enhanced by Γ, which suggests that the quantum effects can increase the ratio T^∗/T_f. Phase diagrams (T versus Γ) show that the critical temperature T_f(Γ) decreases for any values of n_s and J₀ when Γ increases until it reaches a quantum critical point at some value of Γ_c.     

Inverse freezing in the Hopfield fermionic Ising spin glass with a transverse magnetic field

The Hopfield fermionic Ising spin glass (HFISG) model in the presence of a magnetic transverse field Γ is used to study the inverse freezing transition. The mean field solution of this model allows introducing a parameter a that controls the frustration level. Particularly, in the present fermionic formalism, the chemical potential μ and the Γ provide a magnetic dilution and quantum spin flip mechanism, respectively. Within the one step replica symmetry solution and the static approximation, the results show that the reentrant transition between the spin glass and the paramagnetic phases, which is related to the inverse freezing for a certain range of μ, is gradually suppressed when the level of frustration a is decreased. Nevertheless, the quantum fluctuations caused by Γ can destroy this inverse freezing for any value of a.     

Replica symmetry breaking in a fermionic cluster spin glass model in a transverse field

We analyze a fermionic Ising spin glass model in the presence of a transverse magnetic field Γ within a cluster mean field theory. The model considers a Sherrington-Kirkpatrick type interaction between magnetic moments of clusters with a ferromagnetic intra-cluster coupling J₀. The spin site operators are written as a bilinear combination of fermionic operators. In these quantum spin glass model, the inter-cluster disorder is treated by using a framework of one-step replica symmetry breaking within the static approximation. The effective intra-cluster interaction is then computed by means of an exact diagonalization method. Results for several cluster size n_s, values of Γ and J₀ are presented. For instance, the specific heat shows a broad maximum (for n_s>1) at a temperature above the freezing temperature T_f, which is characterized by the inter-cluster replica symmetry breaking. Phase diagrams T versus Γ show that the critical temperature T_f(Γ) decreases for any value of n_s when Γ increases until it reaches a quantum critical point at some value of Γ_c.     

Stability conditions for fermionic Ising spin-glass models in the presence of a transverse field

The stability of a spin-glass (SG) phase is analyzed in detail for a fermionic Ising SG (FISG) model in the presence of a magnetic transverse field Γ. The fermionic path integral formalism, replica method and static approach have been used to obtain the thermodynamic potential within one step replica symmetry breaking ansatz. The replica symmetry (RS) results show that the SG phase is always unstable against the replicon. Moreover, the two other eigenvalues λ_± of the Hessian matrix (related to the diagonal elements of the replica matrix) can indicate an additional instability to the SG phase, which enhances when Γ is increased. Therefore, this result suggests that the study of the replicon cannot be enough to guarantee the RS stability in the present quantum FISG model, especially near the quantum critical point. In particular, the FISG model allows changing the occupation number of sites, so one can get a first order transition when the chemical potential exceeds a certain value. In this region, the replicon and the λ_± indicate instability problems for the SG solution close to all ranges of a first order boundary.     

Antiferromagnetic Ising spin glass competing with BCS pairing interaction in a transverse field

The competition among spin glass (SG), antiferromagnetism (AF) and local pairing superconductivity (PAIR) is studied in a two-sublattice fermionic Ising spin glass model with a local BCS pairing interaction in the presence of an applied magnetic transverse field Γ. In the present approach, spins in different sublattices interact with a Gaussian random coupling with an antiferromagnetic mean J₀ and standard deviation J. The problem is formulated in the path integral formalism in which spin operators are represented by bilinear combinations of Grassmann variables. The saddle-point Grand Canonical potential is obtained within the static approximation and the replica symmetric ansatz. The results are analysed in phase diagrams in which the AF and the SG phases can occur for small g (g is the strength of the local superconductor coupling written in units of J), while the PAIR phase appears as unique solution for large g. However, there is a complex line transition separating the PAIR phase from the others. It is second order at high temperature that ends in a tricritical point. The quantum fluctuations affect deeply the transition lines and the tricritical point due to the presence of Γ.     

Incommensurate phases in ferromagnetic spin-chains with weak antiferromagnetic interchain interaction

We study planar ferromagnetic spin-chain systems with weak antiferromagnetic inter-chain interaction and dipole-dipole interaction. The ground state depends sensitively on the relative strengths of antiferromagnetic exchange and dipole energies κ = J′a ² c/(g _L μ _B )². For increasing values of κ, the ground state changes from a ferromagnetic via a collinear antiferromagnetic and an incommensurate phase to a 120° structure for very large antiferromagnetic energy. Investigation of the magnetic phase diagram of the collinear phase, as realized in CsNiF₃, shows that the structure of the spin order depends sensitivly on the direction of the magnetic field in the hexagonal plane. For certain angular domains of the field incommensurate phases appear which are seperated by commensurate phases. When rotating the field, the wave vector characterizing the structure changes continously in the incommensurate phase, whereas in the commensurate phase the wave vector is locked to a fixed value describing a two-sublattice structure. This is a result of the competition between the exchange and the dipole-dipole interaction.     

Random magnetic interactions and spin glass order competing with superconductivity: Interference of the quantum Parisi phase

We analyse the competition between spin glass (SG) order and local pairing superconductivity (SC) in the fermionic Ising spin glass with frustrated fermionic spin interaction and nonrandom attractive interaction. The phase diagram is presented for all temperatures T and chemical potentials μ. SC-SG transitions are derived for the relevant ratios between attractive and frustrated-magnetic interaction. Characteristic features of pairbreaking caused by random magnetic interaction and/or by spin glass proximity are found. The existence of low-energy excitations, arising from replica permutation symmetry breaking (RPSB) in the Quantum Parisi Phase, is shown to be relevant for the SC-SG phase boundary. Complete 1-step RPSB-calculations for the SG-phase are presented together with a few results for -step breaking. Suppression of reentrant SG-SC-SG transitions due to RPSB is found and discussed in context of ferromagnet-SG boundaries. The relative positioning of the SC and SG phases presents a theoretical landmark for comparison with experiments in heavy fermion systems and high superconductors. We find a crossover line traversing the SG-phase with as its quantum critical (end)point in complete RPSB, and scaling is proposed for its vicinity. We argue that this line indicates a random field instability and suggest Dotsenko-Mézard vector replica symmetry breaking to occur at low temperatures beyond. Received 26 November 1998 and Received in final form 25 January 1999     

Magnetic phase diagram for HO-50%tb from anomalies in ultrasonic propagation

Measurements of the elastic constant c₃₃ for Tb-50% Ho, as a function of temperature and magnetic field, have been used to determine the magnetic phase diagram of the alloy. Evidence for the four phases:paramagnetic, spiral spin antiferromagnetic, fan and ferromagnetic are presented. The true ferromagnetic phase is only found below 100 K even in fields of up to 7 Tesla.     

Low-temperature spectrum and damping of elementary excitations in biquadratic exchange systems (S = 1)

The diagrammatic technique for the standard basis operators and the expansion in powers of 1/z (where z is the number of spins interacting with any given spin) are used to calculate the energies of magnons (in the ferromagnetic and quadrupolar phases) and quadrons (in the ferromagnetic phase) and the bipolar and quadrupolar order parameters (in both phases) in the (1/z)¹ approximation and at low temperatures. it is shown that magnons are damped with the exception of the (ferromagnetic and quadrupolar) case of the Schrödinger exchange model and quadrupolar phase; the quadrons are undamped only in a special case of the ferromagnetic phase, i.e. in the ferrogmatic case of the Schrödinger exchange model. In the limit K → 0, i.e. the biquadratic exchange interaction tends to zero, the spectrum of magnons and their damping are identical with the results by Balakhonov et al. The spin waves and quadrupolar order parameter are discussed in more detail in the following cases of the quadrupolar phase: ferromagnetic-quadrupolar limit, isotropic purely quadrupolar interactions, and quadrupolar-antiferromagnetic limit.     

Frequency (field) dependent NMR relaxation rate in the interrupted metallic strand model

We calculate the nuclear magnetic resonance rate T^?1₁ arising from the electron-nuclear hyperfine contact interaction, within the interrupted metallic strand model. The electron levels are assumed to have an energy half width Γ and a mean spacing Δ₀ and it is assumed that all segments have the same nuclear spin temperature. In the limit Γ ? Δ₀, T^?1₁ has nearly the same behaviour for kT ? Δ₀ and kT?Δ₀. It is proportional to temperature but has a Lorentzian magnetic field dependence with halfwidth H= Γ/μ_B. At low fields it is enhanced over the value for a normal metal by the factor Δ₀/Γ.This anomalous behaviour arises from the suppression of electron spin flip processes by a magnetic field and should always occur when electronic states are localised, that is when there is a locally discrete electron energy spectrum. Therefore it may be relevant not only to certain linear chain conductors but to other cases of electron localisation.The present model provides an additional possible source of frequency dependence of T₁ in linear chain materials. In certain materials especially those containing defects, it may be more appropriate than the currently accepted mechanism which involves electron spin diffusion in one dimension.     

Fermionic Ising glasses with BCS pairing interaction. Tricritical behaviour

We have examined the role of the BCS pairing mechanism in the formation of the magnetic moment and henceforth a spin glass (SG) phase by studying a fermionic Sherrington-Kirkpatrick model with a local BCS coupling between the fermions. This model is obtained by using perturbation theory to trace out the conduction electrons degrees of freedom in conventional superconducting alloys. The model is formulated in the path integral formalism where the spin operators are represented by bilinear combinations of Grassmann fields and it reduces to a single site problem that can be solved within the static approximation with a replica symmetric ansatz. We argue that this is a valid procedure for values of temperature above the de Almeida-Thouless instability line. The phase diagram in the T-g plane, where g is the strength of the pairing interaction, for fixed variance J ² /N of the random couplings J_ij, exhibits three regions: a normal paramagnetic (NP) phase, a spin glass (SG) phase and a pairing (PAIR) phase where there is formation of local pairs.The NP and PAIR phases are separated by a second order transition line g=g _c (T) that ends at a tricritical point T ₃ =0.9807J, g ₃ =5,8843J, from where it becomes a first order transition line that meets the line of second order transitions at T _c =0.9570J that separates the NP and the SG phases. For T<T _c the SG phase is separated from the PAIR phase by a line of first order transitions. These results agree qualitatively with experimental data in . Received 14 May 1998     

Magnetic properties and magnetic interactions in chromium-rich Cr-Fe alloys

The results of magnetization measurements on several disordered b.c.c. Cr-Fe alloys with 1, 1.5, 2.4, 5.3, 12 and 14.2 at % of Fe are reported. The measurements were done in pulsed magnetic fields up to 330 kOe and for the two last alloys also in static magnetic fields up to 44 kOe as in function of temperature. The data support the recently proposed model of magnetic interactions in these alloys by Friedel and Hedman. For the alloys with iron concentration equal to and greater than 2.4 at % we observe, at low temperature, the occurence of a ferromagnetic component in the magnetization curves saturating at an external field of about 140 kOe arising from ferromagnetic iron-rich cluster. At liquid helium temperature the localized iron moments within such iron clusters increase from 1.4μ_B to 1.8μ_b when the iron concentration changes from 2.4 at % to 14.2 at %. At higher iron concentrations we observe a spin glass like transition connected with a freezing of ferromagnetic clusters at very low temperature. Both phase boundaries connected with supermagnetic-paramagnetic and superamagnetis-spin glass like transitions are given.     

Phase transition in antiferromagnets with anisotropic exchange interactions and uniaxial anisotropy

Abstract

Following the Bogoliubov variational principle, the equilibrium and stability equations of the free energy for the two sublattice antiferromagnetic system with inter- and intrasublattice exchange interactions and with an external magnetic field are investigated. For the Ising spin system with uniaxial anisotropy, the phase diagrams have been calculated for various values of anisotropy constant d and the ratio of intra- to intersublattice interaction constants γ. It is shown that first-order, as well as second-order transitions, occur for γ > 0, whereas only a second-order transition occurs for γ ≦ 0, irrespective of the sign of d. Furthermore, similar calculations are extended for the anisotropic Heisenberg spin system and quite interesting phase diagrams have been obtained. Next, the effects of the anisotropic exchange interactions on the magnetic ordered states and the magnetizations of the singlet ground state system of spin one and with a uniaxial anisotropy term are investigated in the vicinity of the level crossing field H ? D/gμ _B . A field-induced ordered state without the transverse component of magnetization is shown to appear in a certain range of magnetic field as the spin dimensionality decreases. It has also turned out that the phase transition between this ordered state and the canted antiferromagnetic state ordinarily found for the isotropic singlet ground state system is of first order. Lastly, the stable spin configurations at a temperature of absolute zero for a two-sublattice uniaxial antiferromagnet under an external magnetic field of arbitrary direction are studied. In particular, the effects of a single ionic anisotropy D-term and anisotropy in the exchange interactions on the magnetic phases are investigated. The antiferromagnetic state has turned out to appear only for the external magnetic field along the easy axis of sublattice magnetization, and makes a first-order phase transition to the canted-spin state or the ferromagnetic state. For other field directions, no antiferromagnetic state appears and only a second-order phase transition between the canted-spin and the ferromagnetic states occurs. The critical field as a function of external field direction has been calculated for several D-values.     

Magnetocaloric effect in the ferromagnetic Kondo lattice model

The Kondo lattice model describes a lattice of localized spins S_i interacting with the conduction electrons via a local exchange coupling J. Assuming a ferromagnetic Hund's rule coupling J>0, the model can be used to describe some itinerant magnetocaloric materials such as Gd(Si_xGe_1-x)₄, La(Fe_1-xSi_x)₁₃, and LaCa_1-xMn_xO₃, which are important for magnetic refrigeration near room temperature. The localized magnetic moments are described in the model Hamiltonian by spin operators, and the conduction electrons by fermionic operators. To study the magnetocaloric effect, a uniform external magnetic field is added through a Zeeman term. By averaging the fermionic degrees of freedom, one obtains an indirect exchange coupling between spins at sites i and j, which corresponds to the RKKY interaction. The self-consistent mean value is evaluated in the effective Heisenberg Hamiltonian within the random phase approximation (RPA). The conduction electron magnetization for a given value of is obtained from the corresponding Green's functions through the equation of motion method. The pressure and doping dependence of the Curie temperature are taken into account in the evaluation of . The magnetocaloric effect is characterized by the isothermal entropy change ΔS and the adiabatic temperature change ΔT_ad upon magnetic field variations in the neighborhood of the ferromagnetic phase transition. The results are obtained for and compared to measurements with Gd compounds.     

Critical nuclear relaxation in cobalt metal

Nuclear magnetic resonance of cobalt metal was investigated in the paramagnetic and ferromagnetic states and in the critical region below T_c. The Knight shift and spin lattice relaxation times were measured in the paramagnetic phase in the solid and liquid states from 1578 K to 1825 K. The resonant frequency, spin-lattice and spin-spin relaxation times were measured in the ferromagnetic phase from room temperature to 1385 K. The main part of (T₁T)^-1 results from fluctuating orbital moments in both phases except near T_c where this process forms the background for critical spin relaxation. The critical exponents for T^-1₁ and for the magnetization in the ferromagnetic state were found to be n' = 0.96 ± 0.07 and β = 0.308 ± 0.012, respectively.     

A testable prediction of the no-signalling condition using a variant of the EPR-Bohm example

Predictive power of the no-signalling condition (NSC) is demonstrated in a testable situation involving a non-ideal Stern–Gerlach (SG) device in one of the two wings of the EPR-Bohm entangled pairs. In this wing, for two types of measurement in the other wing, we consider the spin state of a selected set of particles that are confined to a particular half of the plane while emerging from the SG magnetic field region. Due to non-idealness of the SG setup, this spin state will have superposing components involving a relative phase for which a testable quantitative constraint is obtained by invoking NSC, thereby providing a means for precision testing of this fundamentally significant principle.     

Generation of an external magnetic field with the spin orientation effect in a single layer Ising nanographene

In this work, the magnetic properties of the single layer Ising nanogaphene (SLING) are investigated by using Kaneyoshi approach (KA) within the effective field theory for different spin orientations of its magnetic atoms. We find that the magnetizations of the SLING has no phase transition, certain Curie temperature and distinct peak of susceptibility at T_c for the some spin orientations at the zero external magnetic field (H=0.0). Because these behaviors occur at H≠0.0, we suggest that the SLING generates an external magnetic field and behaves as an external magnetic field generator for these spin orientations. However, the SLING exhibits ferromagnetic behaviors for only one spin orientations. But, it exhibits antiferromagnetic behaviors for the others. For the AFM cases, diamagnetic susceptibility behaviors and type II superconductivity hysteresis behaviors are obtained. We hope that these results can open a door to obtain new class of single layer graphene and graphene-based magnetic field generator devices with the spin orientation effect.     

Quantum Phase Diagram of an Exactly Solved Mixed Spin Ladder

We investigate the quantum phase diagram of the exactly solved mixed spin-(1/2,1) ladder via the thermodynamic Bethe ansatz (TBA). In the absence of a magnetic field the model exhibits three quantum phases associated with su(2), su(4), and su(6) symmetries. In the presence of a strong magnetic field, there is a third and full saturation magnetization plateaux within the strong antiferromagnetic rung coupling regime. Gapless and gapped phases appear in turn as the magnetic field increases. For weak rung coupling, the fractional magnetization plateau vanishs and the model undergoes new quantum phase transitions. However, in the ferromagnetic coupling regime, the system does not have a third saturation magnetization plateau. The critical behaviour in the vicinity of the critical points is also derived systematically using the TBA.     

Exchange bias in structure-phase separated K0.8Fe2−xNixSe2 (x=0.015) single crystal: Interface evidence

Exchange bias behavior is observed in Ni slightly doped K_0.8Fe_2−xNi_xSe₂ (x=0.015) single crystal. Two distinguished phases with epitaxial growth were observed in X-ray diffraction experiments, indicating the structure phase separation in our samples. The magnetic hysteresis loop shifts in both horizontal and vertical directions when the sample was cooled down to 3 K in a magnetic field. The nature of this magnetic anisotropy could be understood as a result of the freezing properties of the local spin disorders in cluster like spin-glass system. Our results suggest that the sample contains short range weak ferromagnetic clusters (phase 2) embedding in the antiferromagnetic backgrounds (phase 1), in which the random distribution of Ni on Fe or Fe-vacancy sites quenched the superconductivity and induced spin disorders.     

Transition order and dynamics of a model with competing exchange and dipolar interactions

We performed Monte Carlo simulation of phase transitions from isotropic stripe phase with short-range order to long-range stripe phase in a model with competing ferromagnetic exchange and antiferromagnetic dipolar interactions on triangular lattice. We calculated phase diagram for different values of exchange and dipolar interaction constants ratio, η. We also determined the order of the transitions to stripe phases AFh of different stripe widths h: first-order phase transition was found to transitions into AF1 and AF2 phases, while transitions to AF3 and AF4 phases were of the second order. In the phase diagram the tricritical point was determined at the AF2 and AF3 phase boundary. We observed the peak of nematic phase at the transition region to the AF1 phase, but found it metastable at low values of η. We have also found that in AF1 phase spin relaxation corresponds to the Ising model dynamics. In phases AF3 and AF4 the dynamics slows down, and stripe domain growth with time is proportional to logt.