Effect of Radial Density Profile on Resonance Absorption in Laser‐Cluster Interaction

The spatial non‐uniformities in the hydrodynamic parameters of an expanding plasma in laser‐cluster interaction plays an important role in determining the region of resonance absorption. It is shown that, in the case of uniform density, the surface resonance at three times the critical density is responsible for laser absorption. However, it is volume resonance at critical density responsible for the laser absorption, if the non‐uniform nature of plasma density inside the hydrodynamically expanding cluster is taken into account (© 2009 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)     

Generation of THz Radiation by Laser Plasma Interaction

This paper presents the three wave parametric decay process to generate the Terahertz (THz) radiations in magnetized plasma. The pump wave (Laser beam) is considered in the extraordinary mode (x‐mode), propagating perpendicular to the background magnetic field. This pump wave decays into an upper hybrid wave and a THz wave which is in magnetosonic mode. The appropriate expressions for the coupling coefficients of the threewave interaction and THz wave amplitude have been derived. Subsequently, the growth rate of this decay instability is also calculated. Various laser and plasma parameters were optimized and we report efficiency of the order of ～1.4 × 10^–2 for current scheme. (© 2013 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)     

THz Radiation Generation via the Interaction of Ultra‐short Laser Pulses with the Molecular Hydrogen Plasma

In this paper, a two dimensional Particle In Cell‐Monte Carlo Collision simulation scheme is used to examine the THz generation via the interaction of high intensity ultra‐short laser pulses with an underdense molecular hydrogen plasma slab. The influences of plasma density, laser pulse duration and its intensity on the induced plasma current density and the subsequent effects on the generated THz signal characteristics are studied. It is observed that the induced current density in the plasma medium and THz spectral intensity are increased at the higher laser pulse intensities, laser pulse durations and plasma densities. Moreover, the generated THz electric field amplitude is reduced at the higher laser pulse durations. A wider frequency range for the generated THz signal is shown at the lower laser pulse durations and higher plasma densities. Additionally, it is found that the induced current density in hydrogen plasma medium is the dominant factor influencing the generation of THz pulse radiation. (© 2016 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)     

Lβ2 satellites in the X‐ray emission spectra of elements 72Hf, 73Ta, 74W, 81Tl, 83Bi and 92U

The satellite spectra arising due to the L₃M_x–M_xN_4,5 (x = 1–5) transition array in the X‐ray emission spectra of ₇₂Hf, ₇₃Ta, ₇₄W, ₈₁Tl, ₈₃Bi and ₉₂U have been calculated using available HFS data on K–LM and L–MN Auger transition energies. The agreement between the calculated and measured energies, that between calculated and measured separations in energies and the consideration of the relative probabilities of all the L₃M_x–M_xN_4,5 transitions have been used as the basis for deciding the origin of the satellites. It has been established that two satellites observed in the Lβ₂ region of the X‐ray spectra of various elements, named β₂^I and β₂^II in the order of increasing energy, are mainly emitted by the L₃M_4,5–M_4,5N_4,5 transitions. It is observed that satellite β₂^I in the spectra of elements with ₇₂Hf to ₇₄W has been assigned to the superposition of the ³F₄–³G₅ and ³F₄–³D₃ transitions and must be the most intense one among all these satellites. The same transition has been proved to be the main origin of satellite β₂^II, reported in the element with ₈₁Tl, ₈₃Bi and ₉₂U. Further, satellite β₂^I, reported in the spectra of elements with ₈₁Tl and ₉₂U, has been associated with the transitions ³D₃–³F₄ and ¹D₂–¹F₃. Finally, line β₂^II, reported in the spectra of elements with Z = 72–74, has been assigned to the ¹F₃–¹G₄ and ³P₀–³D₁ transitions. The possible contributions of other transitions of the L₃M_x–M_xN_4,5 (x = 1–5) array having intensities comparable with those of the above transitions, as well as the corresponding lines that have not yet been observed, have also been discussed. Copyright © 2011 John Wiley & Sons, Ltd.     

Generalised ABCD matrix treatment for laser resonators and beam propagation

A generalised ABCD matrix treatment for laser resonators and beam propagation is developed for computer programming. In this treatment, imaginary parts are introduced into the matrixes for all optical elements, and the beam quality factor M² and the index of the medium are also taken into account. When the imaginary parts of the complex matrix are zero and the beam quality factor M² and medium index are unity, the stated method is transformed back into the more classic ABCD matrix format in which the fundamental-mode Gaussian beam transmits through real elements in the vacuum. Based on this method, laser resonator software is realised by the VB programme language. The software can be used to analyse and design stable/unstable standing/travelling cavities, phase-conjugate cavities and beam transformations.     

Evaporation of a thin film coated on a substrate induced by a pulsed laser

The two-dimensional Laplace integral transform technique has been applied to get the spatial and temporal temperature distributions in both the molten layer thickness of a thin film coated on a substrate, the still solid part of the thin film of the target and the temperature distribution in the substrate. Also a formula for the time dependence of the evaporated part of the thin film of the target as well as the molten layer thickness of the thin film were obtained. Calculations of the obtained relations were carried out during the irradiation with a pulsed laser. The derivation has taken into account the temperature-dependent absorption coefficient of the irradiated surface and the chemical reaction in the vapor of the thin film. As an illustrative example, computations were carried out on an aluminum thin film coated on a glass substrate.     

The temperature profile in the molten layer of a semi-infinite target induced by irradiation using a pulsed laser

The two-dimensional Laplace integral transform technique has been used to compute the temperature profile of the molten layer on the surface of a semi-infinite target when irradiated by a pulsed laser. Mathematical expressions for the temperature distribution in the molten layer thickness and the solid part of the target, taking cooling and the temperature-dependent absorption coefficient of the irradiated surface into account, were obtained. As an illustrative example computations were carried out on a semi-infinite aluminum (Al) target.     

Laser Spectra and Efficiencies of Pyrazolo Derivatives of Coumarins

Abstract

Of the new laser dyes of coumarin series reported earlier, pyrazolo derivatives have been further studied. The paper reports their laser spectra and efficiencies in various solvents compared to a standard coumarin laser dye C₅₁₅. One of the derivatives shows comparable output under optimum concentration conditions as compared to the standard.     

Non‐paraxial polarization spatio‐temporal coupling in ultrafast laser material processing

Two hundred years after Malus' discovery of optical anisotropy, the study of polarization‐driven optical effects is as active as ever, generating interest in new phenomena and potential applications. However, in ultrafast optics, the influence of polarization is frequently overlooked being considered as either detrimental or negligible. Here we demonstrate that spatio‐temporal couplings, which are inherent for ultrafast laser systems with chirped‐pulse amplification, accumulate in multi‐pulse irradiation and lead to a strongly anisotropic light‐matter interaction. Our results identify angular dispersion in the focus as the origin for the polarization dependence in modification, yielding an increase in modification strength. With tight focusing (NA ≥ ∼0.4), this non‐paraxial effect leads to a manifestation of spatio‐temporal couplings in photo‐induced modification. We devise a practical way to control the polarization dependence and exploit it as a new degree of freedom in tailoring laser‐induced modification in transparent material. A near‐focus, non‐paraxial field structure analysis of an optical beam provides insight on the origin of the polarization dependent modification. However, single pulse non‐paraxial corrected calculations are not sufficient to explain the phenomena confirming the experimental observations and exemplifying the need for multi‐pulse analysis.

     

Electron‐Ion Relaxation,Phase Transitions,and Surface Nano‐Structuring Produced by Ultrashort Laser Pulses in Metals

Fundamental physical phenomena in metals irradiated by ultrashort laser pulses with absorbed fluences higher than few tens of mJ/cm² are investigated. For those fluences, laser‐produced electron distribution function relaxes to equilibrium Fermi distribution with electron temperature T_e within a short time of 10‐100 fs. Because the electron subsystem has T_e highly exceeding much the ion subsystem temperature T_i the well‐known twotemperature hydrodynamic model (2T‐HD) is used to evaluate heat propagation associated with hot conductive electron diffusion and electron‐ion energy exchange. The model coefficients of electron heat conductivity κ (?, T_e, T_i) and electron‐ion coupling parameter α (?, T_e) together with 2T equation of state E (?, T_e, T_i) and P (?, T_e, T_i) are calculated. Modeling with 2T‐HD code shows transition of electron heat wave from supersonic to subsonic regime of prop‐agation. At the moment of transition the heat wave emits a compression wave moving into the bulk of met al. Nonlinear evolution of the compression wave after its separation from the subsonic heat wave till spallation of rear‐side layer of a film is traced in both 2T‐HD modeling and molecular dynamics (MD) simulation. For fluences above some threshold the nucleation of voids in frontal surface layer is initiated by strong tensile wave following the compression wave. If the absorbed fluence is ～30 % above the ablation threshold than void nucleation develops quickly to heavily foam the molten met al. Long‐term evolution of the metal foam including foam breaking and freezing is simulated. It is shown that surface nano‐structures observed in experiments are produced by very fast cooling of surface molten layer followed by recrystallization of supercooled liquid in disintegrating foam having complex geometry. Characteristic lengths of such surface nanostructures, including frozen pikes and bubbles, are of the order of thickness of molten layer formed right after laser irradiation. (© 2013 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)     

不同脉冲激光波形在打孔实验上的比较与分析

为了获得高质量小孔,克服单脉冲激光打孔的不足,设计了一种能够产生多脉冲激光波形的激光器电源.并在1mm厚的薄钢片上得到直径小于1mm的小孔.多脉冲打孔理论分析表明,多脉冲激光打孔不但减少了熔融物和等离子体的产生,而且降低了激光打孔对高能量的要求,获得的小孔质量优于单脉冲激光打孔.另外脉冲宽度和脉冲间距的选择对激光小孔加工质量起决定性作用,在加工高质量孔的时候,应该选用较短的激光脉冲宽度.实验表明,利用三脉冲激光输出波形打孔所获得的小孔质量要优于单脉冲激光打孔效果,有效脉冲平均能量为350mJ,宽度为100μs,脉冲间距为100μs.     

激光科学和生命科学

激光科学与生命科学相互渗透,正在形成一门新兴边缘学科──“激光生命科学”.本文就激光生命科学下述几个重要领域的研究进展进行概述：1)激光生物学与激光诱变育种;2)激光遗传工程及激光微束在遗传操作中的应用;3)激光在分子生物学中的应用;4)用于生命科学研究的激光光谱技术;5)激光医学;6)激光生物物理技术。