Conductivity of ionic crystals when they are irradiated by picosecond electron beams

This paper discusses the pulsed electron conductivity σ of KCl, KBr, and NaCl crystals when they are excited by an electron beam (0.2 MeV, 50 ps) with current densities in the interval j=(30–10⁴) A/cm². It is shown that the lifetime of the electrons in the conduction band is τ≪100 ps. To explain the experimental σ(j) dependences, a model is proposed that includes electron capture by structural defects and stable radiation defects at low excitation densities and electron capture predominantly by unstable radiation defects generated by the excitation pulse at high excitation densities. Fiz. Tverd. Tela (St. Petersburg) 41, 1200–1203 (July 1999)     

Temperature dependence of light scattering by the one-magnon excitation in NiF2 crystals

We have studied the one-magnon excitation in NiF₂ crystals by the method of right-angle light scattering from 1 to 73°K. The temperature dependence of frequency and line width agrees very well with previous far infrared absorption data. The temperature dependence of the integrated intensity follows the theoretical prediction but deviates from the previous far infrared data.     

The temperature dependence of the resistive response of superconducting Pb films upon picosecond optical excitation

We report a study of the temperature dependence of the transient resistivity of superconducting Pb thin films excited by short duration (70 ps) laser pulses of varying irradiances. The results are analyzed in terms of a model proposed by Elesin which features the existence of a nonstationary, inhomogeneous, intermediate state.     

Calculation of intraband electronic and interband hole luminescence spectra of various alkali halide crystals under pulsed excitation by intense electron and laser beams in the nanosecond and picosecond regimes

We perform a theoretical analysis of the spectra of two rather new kinds of fundamental luminescence in dielectrics: intraband electronic and interband hole emissions. The primary photon emitters are radiative transition of ionization-passive conduction-band electrons and valence-band holes. These types of luminescence have been observed and studied experimentally by the use of two powerful nanosecond and picosecond radiation sources: strong electronic accelerators and lasers with ultraviolet harmonic generators. Good agreement is obtained between the calculated spectra and the ones measured experimentally. Comparison of the results with the experimental data makes it possible to determine certain important parameters of the electron spectrum, in particular the upper boundary of the passive region for ionization of the conduction band in crystalline CsI. Institute for Ultraprecise Electronics, Siberian Division, Russian Academy of Sciences. Polytekhnic University, Tomsk. Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 12, pp. 103–115, December, 1995.     

Temperature dependence of the time-resolved emissions of CsI:Tl

Abstract

Time-resolved emissions of Csl:T1 are investigated. The system is laser-excited in the A-band at 308 nm and the emissions are observed in the range 370–650 nm, from 30 K to 300 K. Their analysis by means of a deconvolution permits the valuation of decay-times down to 1 ns. At every temperature many bands are observed and some of them show slow and fast components. The decay-times of the fast components are in the range 1–10 ns while the slow ones are even longer than 1 μs. In many cases intermediate decay-times of the order of 100 ns exist. The competition among the bands interests the application of this system as active material for tunable solid-state laser.     

Observation of picosecond modulated electron beams from the plasma focus

The electron beam emitted from the plasma focus was investigated by means of a ?erenkov detector streak camera equipment. The electron beam is measured to be strongly modulated with periods of about 25 ps.     

Temperature dependence of ZnCdS: Ag cathodoluminescence efficiency under electron beam excitation

The temperature dependence of the efficiency of ZnCdS: Ag phosphor excited by a constant electron beam was investigated. Three well expressed maxima were observed at temperatures of about 60, 160, and 230 K.     

Nonequilibrium phonons in SiGe quantum-well nanostructures upon excitation by picosecond laser pulses

The phonon pulses initiated by photoexcitation of structures containing Si_0.8Ge_0.2 double quantum wells under picosecond radiation of a MIRA 900P titanium-sapphire laser (λ = 760 nm) are studied. The propagation of nonequilibrium acoustic phonons is detected with a superconducting bolometer. The recorded bolometer response is found to differ substantially from that observed in photoexcitation of the same structure by nanosecond pulses of a nitrogen laser (λ = 337 nm). The generation of coherent acoustic phonons is suggested as an explanation.     

Simulation of the formation of an electron ring by picosecond electron beams in a cusp-type magnetic system

The possibility of using picosecond high-current relativistic electron beams for the formation of tubular rotating relativistic electron rings is investigated. Longitudinal compression of a tubular beam in a cusp is simulated numerically disregarding the space charge effects. The behavior of the characteristics of a compressed beam, which determines the tolerances in the initial parameters and magnetic system parameters, is investigated.     

Relaxation of the conductivity of CsI-Tl after excitation by subnanosecond electron pulses

The pulsed conductivity is investigated for a CsI-Tl crystal having a Tl⁺ concentration N=8×10¹⁷cm⁻³ and excited by an electron beam (0.2 MeV, 50 ps, 10²–10⁴ A/cm ²). It is shown that the amplitude of the conduction current pulse is almost an order of magnitude lower than for “pure” CsI crystals irradiated under like conditions. The conduction current relaxation time is preserved up to τ=100 ps in this case. Under the experimental conditions, therefore, the lifetime of electrons in the conduction band is controlled by trapping at Tl⁺ centers. The electron capture cross section at a Tl⁺ center is determined: σ=7×10⁻¹⁶ cm², which agrees in order of magnitude with estimates of the capture cross section for a neutral trapping center. Fiz. Tverd. Tela (St. Petersburg) 40, 66–67 (January 1998)     

Parametric excitation of X-waves by downconversion of Bessel beams in nonlinear crystals

We predict that in traveling-wave degenerate parametric downconversion the Bessel beam pump stimulates the appearance of a nondiffracting X-wave from quantum noise amplification. Numerical simulation results of downconversion in ADP crystal are presented, along with preliminary experimental data.     

Time-resolved optical spectroscopy of CsI(Tl) crystals by pulsed electron beam irradiation

Properties of the color and emission centers induced with an electron pulse beam at temperature within 80-300 K have been studied in CsI(Tl) crystals. It has been established by optical spectrometry with time resolution that initial color centers in this crystal are only Tl⁰ and V_k centers, which spontaneously recombine emitting visible light at 2.25 and 2.55 eV. It has been shown that the emission decay kinetics at 80 K include two fast exponential components with decay constants 3 and 14 μs as well as slow hyperbolic component with the power index depending on the wavelength of the emitting light. The temperature effect on the emission kinetics has been studied and it has been directly proved that the emission rise stage at the temperature above 170 K is caused by the recombination of electrons, which are thermally released from single Tl⁰ centers, with V_kA centers. The origin of scintillations in CsI(Tl) crystal is discussed in terms of the tunnel electron transitions from ground state of Tl⁰ centers to ground state of V_k centers at different distances from each other.     

Temperature dependence of hole mobility in n-type InSb upon electron bombardment

The mobility of the minority carriers, in n-InSb was investigated from the photomagnetoelectric effect as a function of temperature in the range of 12–80 K prior to and after bombardment with 1 MeV average energy beta particles. The hole mobility shows a minimum near 40 K which can be due to the h-e scattering becoming predominant in the region where other scattering mechanisms are relatively weak. After bombardment the curves have the same form but higher mobilities. This is due to a decrease of h-e scattering resulting from the decrease of the electron concentration, as determined from independent measurements.     

Transient absorption spectra of tetraazaporphine and its reduced derivatives upon picosecond excitation

Transient absorption spectra of tetraazaporphine and substituted derivatives of tetraazachlorin and tetraazabacteriochlorin were obtained upon picosecond excitation with various probe pulse delay times in order to resolve the open question about the reasons for fluorescence quenching in tetraazaporphine hydrogenated derivatives. The quantum yield of triplet state T ₁ formation has been estimated. It has been shown that in all investigated cases radiationless de-excitation of the fluorescent level S ₁ occurs by two channels: S ₁ ⤳ T ₁ and S ₁ ⤳ S ₀, the latter being predominant. As the S ₁ level becomes lower, the transition rate for this channel increases. For tetraazaporphine and its derivatives, a quasi-photochemical mechanism is proposed that accounts for the anomalous efficiency of the S ₁ ⤳ S ₀ channel in the dissipation of the electronic excitation energy.     

Luminescence of complex organic molecules upon electron excitation

Pesults of investigation of the luminescence of complex organic compounds upon excitation with electrons of various energies are reported. Data on spectra of energy losses of electrons, fluorescence excitation cross sections and functions, fluorescence emission spectra, fluorescence kinetics, polarization, and energy yield, effects of impurity gases, and theoretical analysis of the processes taking place in the system are presented. Results of investigation of the luminescence of complex molecules in electric discharges (dc, pulsed, high-frequency, non-self-maintained, and plasma-beam) and in a condensed state (solutions, molecular crystals, and thin solid films) are discussed. Institute of Molecular and Atomic Physics, National Academy of Sciences of Belarus, 70, F. Skorina Ave., Minsk 220072, Belarus. Transtated from Zhurnal Prikladnoi Spektroskopii, Vol. 65, No. 5, pp. 694–708, September–October, 1998.