Broadband four-wave optical parametric amplification in bulk isotropic media in the ultraviolet

We report on four-wave optical parametric amplification of the ultrashort ultraviolet light pulses in bulk fused silica and CaF₂. Exact phase-matching in these isotropic media is achieved by means of non-collinear interaction with cylindrical beam focusing. Four-wave optical parametric amplifier efficiently operates in the UV spectral range with 1-ps laser pulses, delivering amplified signal energy exceeding 50 μJ using millijoule pump pulses in the visible (527 nm). Results of scanning of the parametric gain profile suggest that broad amplification bandwidth as wide as ∼20 nm (at FWHM) under these experimental settings is achieved, which might support amplification of sub-10-fs ultraviolet pulses with central wavelength around 330 nm. It is also shown experimentally and verified theoretically that the parametric gain profile exposes a distinct inhomogeneity and its bandwidth notably broadens due to effects of self- and cross-phase modulation imposed by the intense pump beam.     

Sum and difference frequency generation of white light continuum with the ps pulses of Nd:YAG laser in a thick BBO crystal

The white light continuum (WLC) generated in water/D₂O mixture by pumping with the fundamental of ps Nd⁺³:YAG laser has been used as a variable frequency source for the sum frequency generation as well as for its amplification. 35 ps long pulses with 8 mJ energy at 1064 nm were mixed collinearly with the WLC generated by the same laser beam in a 20 mm thick BBO crystal. The obtained tunable output has been identified as the sum frequency between the fundamental and a portion of the WLC with the required phase matching. Theoretical simulations are also given along with a few initial experiments to use this combination for the difference frequency generation (optical parametric amplification) under non-collinear geometry.     

High-peak power multi-wavelength picosecond pulses generated from a BaWO4 Raman-seeded optical parametric amplifier

We report the generation of high-peak power multi-wavelength picosecond laser pulses using optical parametric amplification (OPA) in BBO seeded with pulses generated in a 5-mm length BaWO₄ crystal by stimulated Raman scattering of 18-ps laser pulses at 532 nm. The maximum output energy of the amplified first-Stokes component at 559.7 nm was about 1.76 mJ. The corresponding maximum peak power, pulse duration and spectral line width were measured to be 117.3 MW, 15 ps and 18.0 cm⁻¹, respectively. The multi-wavelength picosecond laser pulses were in the visible and near infrared ranges. Using this Raman-seeded OPA technique, the beam quality of the stimulated Raman scattering pulses can be improved.     

High efficiency and high energy parametric wavelength conversion using a large aperture periodically poled MgO:LiNbO3

We have demonstrated an efficient high energy 2 μm laser generation with a 36 mm long large aperture 5 mol% MgO-doped periodically poled LiNbO₃ (PPMgLN) nonlinear optical crystal. A high power Q-switched Nd:YAG laser (1.064 μm) was used to pump the quasi-phase matched (QPM) optical parametric oscillator (OPO). A total output energy of 186 mJ with 58% slope efficiency was obtained in two separate beams at 2 μm.     

Efficient multi-frequency generation of ultrashort light pulses using stimulated Raman scattering and optical parametric amplification

Optical parametric amplification of multi-frequency seed pulses generated in a mixture of compressed hydrogen and methane by stimulated Raman scattering of 1 ps, 1 kHz laser pulses at 395.8 nm has been studied. Efficient generation of spectrally narrow ultrashort pulses with a spatial distribution close to the Gaussian profile of the pump beam was obtained in the visible and near infrared ranges.     

High energy and short pulses generation by Nd:yttrium aluminum garnet laser mode-locked using frequency-doubling nonlinear mirror

The generation of laser pulses with energies of >40 mJ at 25 Hz and durations variable from 15 ps to 45 ps using an Nd:yttrium aluminum garnet laser mode-locked with a Stankov nonlinear mirror is demonstrated. This laser is used to pump an optical parametric generator-amplifier, which is tunable in the visible spectral range.     

Amplification of kW peak power femtosecond pulses in single quantum well InGaAs tapered amplifiers

The amplification of ps and fs pulses with peak powers of up to 4.5 kW has been investigated in a single quantum well InGaAs tapered amplifier. The pulses with durations of 100 fs or 2 ps were generated by a modelocked titanium-sapphire laser. The amplified pulses indicate strong gain saturation and carrier generation due to photon absorption in the laser active region which causes a temporal broadening of the amplified pulses as well as modifications of the optical spectrum. The gain recovery time was measured by a pump-probe experiment. The experimental results are analyzed with respect to the sub-ps gain dynamics which is described by a relaxation time approximation.     

Optimization of optical parametric chirped pulse amplification with different pump wavelengths

Optical parametric chirped pulse amplification with different pump wavelengths was investigated using LBO crystal, at signal central wavelength of 800 nm. According to our theoretical simulation, when pump wavelength is 492.5 nm, there is a maximal gain bandwidth of 190 nm centered at 805 nm in optimal noncollinear angle using LBO. Presently, pump wavelength of 492.5 nm can be obtained from second harmonic generation of a Yb:Sr₅(PO₄)₃F laser. The broad gain bandwidth can completely support ∼6 fs with a spectral centre of seed pulse at 800 nm. The deviation from optimal noncollinear angle can be compensated by accurately tuning crystal angle for phase matching. The gain spectrum with pump wavelength of 492.5 nm is much better than those with pump wavelengths of 400, 526.5 and 532 nm, at signal centre of 800 nm.     

Widely tunable optical parametric oscillator driven by a pulsed diode-pumped nonlinear-mirror mode-locked Nd:YAG laser

We report on the development of a pulsed diode end-pumped Nd:YAG laser mode-locked by a nonlinear mirror and stabilized by an acousto-optical modulator. With the introduction of appropriate intracavity loss, the laser is able to generate 22.8 ps pulses with the energy of 4.5 μJ. After amplification and frequency doubling stages, the second harmonic radiation is used to non-collinearly synchronously pump a β-barium borate optical parametric oscillator in a walk-off compensated scheme. The system demonstrates a wide-tuning range from 635 nm to 2.55 μm for the signal output, with maximum average conversion efficiency as high as 42%.     

Prospects for increasing average power of optical parametric chirped pulse amplifiers via multi-beam pumping

We demonstrate optical parametric amplification of broadband chirped pulses in BBO crystal pumped by several intersecting beams extracted from independent laser amplifiers. The energy of amplified signal ranged from 0.23 to 0.72 mJ depending on a number of pump beams used as well as pumping configuration employed. The conversion efficiency dependence on intersection angles of pump beams is revealed and modeling of interplay of interacting waves is presented.     

Detection of scattered light pulses at femto-Joule level by using a picosecond BBO optical parametric amplifier

We report a technique for detecting weak scattered light pulses based on a 532 nm pumped picosecond β-barium-borate collinear optical parametric amplifier. The measured maximum slope gain factor of the amplifier was found to be around 10⁷, and the energy detection limit was of the order of fJ/pulse for the signal of 730 nm and the idler of 1.5 μm at a pumping intensity of 2.83 GW/cm². The linearity of the gain for this amplifier was found to be excellent for a seeding level of lower than 420 fJ per pulse. The maximum gains and the energy detection limits for the scattered light pulses from various scattering targets were found to be poorer than that from the reflective mirror, owing to the degraded beam quality and the depolarization of the scattered light. A reduction of the maximum gain for the scattered light with the increase of the angle of incidence, which causes pulse broadening and reduces the photon flux of the signal, was investigated. The feasibility of detecting weak scattered light in the infrared by using idler-to-signal frequency up-conversion was also demonstrated, in which the infrared seeder located in the idler branch of the amplifier was injected as the seeding beam and was then parametrically up-converted into the visible signal branch, with an even higher gain.     

Diode-pumped, chirped-pulse Yb:S-FAP regenerative amplifier for laser-Compton X-ray generation

We present a diode-pumped, chirped-pulse Yb:S-FAP regenerative amplifier. This regenerative amplifier was developed as a first amplifier in an all-solid-state Yb:S-FAP laser system for laser-Compton X-ray generation. The amplifier delivers pulse energies above 24 mJ at a repetition rate of 50 Hz. Pulse compression reduces pulse widths to approximately 2.0 ps.     

Characterization of ultra-weak fluorescence using picosecond non-collinear optical parametric amplifier

We report a technique for characterization of ultra-weak fluorescence based on a 355-nm pumped picosecond non-collinear optical parametric amplifier (OPA). In the experiment, we effectively reduced the strong super-fluorescence background by using a series of methods. With the picosecond OPA as the pre-amplifier and the gating pulse, the decay of the fluorescence of Rhodamine 6G dye in ethanol was measured and the fluorescence lifetime was found to be about 941 ps. The gain factor of this parametric fluorescence amplifier was measured to be ∼4.2 × 10⁶, while the energy detection limit was ∼160 aJ per pulse within a 15-ps gating pulse.     

Development of a nearly transform-limited, low-repetition-rate, picosecond optical parametric generator

A low-repetition-rate (10-Hz), picosecond (ps) optical parametric generator (OPG) seeded at the idler wavelength with a high-power diode laser is demonstrated. The output of the OPG at ∼566 nm is amplified in dye cells, resulting in signal enhancement by more than three orders of magnitude. The nearly transform-limited beam at ∼566 nm has a pulsewidth of ∼170 ps, with an overall output of ∼2.3 mJ/pulse. The laser is tuned either by tuning the nonlinear crystal or the seed-laser current. The applications of such a simple, compact, high-performance, tunable ps laser system for linear and nonlinear spectroscopies are outlined.     

Directivity influence of signals propagation through EDFA gain medium of Brillouin-erbium fiber laser

We experimentally demonstrate a multiwavelength Brillouin-erbium fiber laser in two configurations; uni-directional and bi-directional propagation of Brillouin pump and Brillouin Stokes signals through an Erbium-doped fiber gain. The influence of these configurations on the performance of the output parameters in terms of lasing threshold, output channel generation and tuning range of the generated output channels are investigated. We discovered that there is a trade-off between these two fiber laser configurations. The uni-directional amplifier configuration provides greater tuning range of 46.8 nm against 23 nm at maximum Brillouin pump power of 2 mW and 1480-nm pump power of 130 mW. On the other hand, the bi-directional amplifier configuration provides 13 output channels against 6 output channels obtained from the uni-directional amplifier configuration at the same pumping powers. Nevertheless, the bi-directional amplifier configuration requires much lower pump power to initiate lasing.     

SOA-based actively mode-locked fiber ring laser by forward injecting an external pulse train

An actively mode-locked fiber ring laser based on cross-gain modulation (XGM) in a semiconductor optical amplifier (SOA) is demonstrated to operate stably with a simple configuration. By forward injecting an easily-generated external pulse train, the mode-locked fiber laser can generate an optical-pulse sequence with pulsewidth about 6 ps and average output power about 7.9 mW. The output pulses show an ultra-low RMS jitter about 70.7 fs measured by a RF spectrum analyzer. The use of the proposed forward-injection configuration can realize the repetition-rate tunability from 1 to 15 GHz for the generated optical-pulse sequences. By employing a wavelength-tunable optical band-pass filter in the laser cavity, the operation wavelength of the designed SOA-based actively mode-locked fiber laser can be tuned continuously in a wide span between 1528 and 1565 nm. The parameters of external-injection optical pulses are studied experimentally to optimize the mode-locked fiber laser.     

Generation and amplification of dual-color femtosecond pulses by a noncollinear optical parametric up-conversion process

Noncollinear optical parametric up-conversion generation and amplification are realized in a thick β-barium borate (BBO) crystal, and a couple of visible femtosecond up-conversion laser pulses can be achieved by a femtosecond pulse at 800 nm as the pump sources. The theoretical and experimental results indicate that there exist phase-matching conditions for dual-color noncollinear parametric up-conversion generation and amplification, and their wavelengths can be tuned by rotating the BBO crystal. This parametric up-conversion generation and amplification can be attributed to three and five-wave mixing in a thick BBO crystal, and it shows the potential application on optical parametric chirped pulse amplification (OPCPA) to generate multi-color ultraviolet or visible femtosecond laser pulses pumped directly by femtosecond fundamental laser pulses without frequency-doubling or tripling.     

Tunable, high-power, narrow-band picosecond IR radiation by optical parametric amplification in KTP

We report on an optical parametric amplifier (OPA) based on two potassium titanyl phosphate (KTP) crystals in a walk-off compensating geometry. An Nd:YLF regenerative amplifier at a 1-kHz repetition rate serves as the pump source. The seed beam is delivered by a synchronously pumped frequency-stabilized optical parametric oscillator (OPO) based on periodically poled lithium niobate (PPLN). At pump intensities of about 7 GW/cm² large amplification factors of more than 10⁴ were achieved, resulting in pulse energies of more than 450 μJ and 350 μJ for the signal and idler pulses, respectively, at a 1-kHz repetition rate. In the saturation regime the time–bandwidth product increases from two to three times the Fourier limit, with a pulse duration of 105 ps and a bandwidth of 12.7 GHz at the highest intensities employed. Received: 2 November 2001 / Published online: 14 March 2002     

Generation of high-contrast and high-intensity laser pulses using an OPCPA preamplifier in a double CPA, Ti:sapphire laser system

We demonstrate a high-contrast, high-intensity double chirped-pulse amplification (CPA) Ti:sapphire laser system using an optical parametric chirped-pulse (OPCPA) pre- amplifier. By injecting cleaned microjoule seed pulses into the OPCPA, a temporal contrast greater than 10¹⁰ within picosecond times before the main femtosecond pulse is demonstrated with an output pulse energy of 1.7 J and a pulse duration of 30 fs, corresponding to a peak power of 60 TW at a 10 Hz repetition rate. This system uses a cryogenically-cooled Ti:sapphire final amplifier and generates focused peak intensities in excess of 10²⁰ W/cm².     

Femtosecond hybrid mode-locked semiconductor laser and amplifier dynamics

We describe the generation of femtosecond high power optical pulses using hybrid passive-active mode-locking techniques. Angle stripe geometry GaAs/AlGaAs semiconductor laser amplifiers are employed in an external cavity including prisms and a stagger-tuned quantum-well saturable absorber. An identical amplifier also serves as an optical power amplifier in a stretched pulse amplification and recompression sequence. After amplification and pulse compression this laser system produces 200 fs, 160 W peak power pulses. We discuss and extend our theory, and supporting phenomenological models, of picosecond and subpicosecond optical pulse amplification in semiconductor laser amplifiers which has been successful in calculating measured spectra and time-resolved dynamics in our amplifiers. We have refined the theory to include a phenomenological model of spectral hole-burning for finite intraband thermalization time. Our calculations are consistent with an intra-band time of approximately 60 fs. This theory of large signal subpicosecond pulse amplification will be an essential tool for understanding the mode-locking dynamics of semiconductor lasers and for analysis of high speed multiple wave-length optical signal processing and transmission devices and systems based on semiconductor laser amplifiers.