Large index of refraction without absorption via decay-induced coherence in a three-level V system

We study the effects of quantum interference from spontaneous emission on the dispersion-absorption properties in a three-level V-type atomic system with two near-degenerate excited levels. We found that due to the quantum interference between two spontaneous decay channels, large index of refraction without absorption always can be obtained just by choosing proper values of the relative phase between the two applied fields.Received: 27 February 2004, Published online: 26 May 2004PACS: 42.50.Gy Effects of atomic coherence on propagation, absorption, and amplification of light; electromagnetically induced transparency and absorption - 42.50.Hz Strong-field excitation of optical transitions in quantum systems; multiphoton processes; dynamic Stark shift     

The coherent time evolution of two coupled quantum dots in a two-mode cavity

For two coupled identical quantum dots in a two-mode cavity, we determine the conditions of two-photon and single-photon resonance. It is shown that the exciton-phonon interaction reduces the Rabi frequencies of each model and the Förster interaction between double quantum dots even at absolute zero temperature. The exciton-phonon interaction also makes a contribution to the static exciton-exciton dipole interaction energy. Furthermore, the additional interactions can modify the conditions of photon resonance significantly. A more realistic case of two nonidentical quantum dots is also considered. The influence of parameter misfits on the quantum system is discussed.Received: 8 July 2004, Published online: 3 November 2004PACS: 73.21.La Quantum dots - 71.35.-y Excitons and related phenomena - 42.50.Pq Cavity quantum electrodynamics; micromasers     

Effect of exciton-phonon coupling in the calculated optical absorption of carbon nanotubes

We find that the optical properties of carbon nanotubes reflect remarkably strong effects of exciton-phonon coupling. Tight-binding calculations show that a significant fraction of the spectral weight of the absorption peak is transferred to a distinct exciton+phonon sideband, which is peaked at around 200 meV above the main absorption peak. This sideband provides a distinctive signature of the excitonic character of the optical transition. The exciton-phonon coupling is reflected in a dynamical structural distortion, which contributes a binding energy of up to 100 meV. The distortion is surprisingly long ranged, and is strongly dependent on chirality.     

On the possibility of the exciton-phonon bound states in GaSe

The experimental results of the optical absorption and the photoconductivity of GaSe layered crystals in the exciton region are presented. On the basis of the results obtained, we conclude the existence of the exciton-phonon quasibound states.     

强耦合激子-声子系统中的三阶非线性光学系数的理论计算

应用Dyson-Maleev变换,对强耦合激子—声子系统中非线性光学性质进行了理论研究.结果表明,当信号光场频率与激子频率的失谐量等于光学声子的频率时,系统的非线性光学吸收和克尔（Kerr）系数显著增大,从而证明了激子-声子的强相互作用对介质的非线性光学性质的影响相当大,并且当考虑激子偏离玻色子模型时,这种影响将进一步增大.     

Doppler-free spectroscopy in driven three-level systems

We demonstrate two techniques for studying the features of three-level systems driven by two lasers (called control and probe), when the transitions are Doppler broadened as in room-temperature vapor. For -type systems, the probe laser is split to produce a counter-propagating pump beam that saturates the transition for the zero-velocity atoms. Probe transmission then shows Doppler-free peaks which can even have sub-natural linewidth. For V-type systems, the transmission of the control beam is detected as the probe laser is scanned. The signal shows Doppler-free peaks when the probe laser is resonant with transitions for the zero-velocity group. Both techniques greatly simplify the study of three-level systems since theoretical predictions can be directly compared without complications from Doppler broadening and the presence of multiple hyperfine levels in the spectrum.Received: 10 September 2003, Published online: 6 January 2004PACS: 42.50.Gy Effects of atomic coherence on propagation, absorption, and amplification of light; electromagnetically induced transparency and absorption - 42.50.-p Quantum optics     

激子-声子相互作用对三阶非线性光学性质的影响

在对激子不作任何近似的条件下,对强耦合激子声子系统中非线性光学性质在理论上进行了研究,结果表明当信号光场频率与激子频率的失谐量等于光学声子的频率时,系统的非线性光学吸收和克尔系数显著增大,从而证明了激子声子的强相互作用对介质的非线性光学性质的影响相当大。并且,与对激子作代松马利夫(Dyson-Maleev)变换近似和玻色近似的结果进行仔细的比较,发现对激子不作近似时,这种影响将进一步增大。     

Direct experimental evidence of exciton-phonon bound states in carbon nanotubes

We present direct experimental observation of exciton-phonon bound states in the photoluminescence excitation spectra of isolated single-walled carbon nanotubes (SWNT) in aqueous suspension. The photoluminescence excitation spectra from several distinct SWNTs show the presence of at least one sideband related to the tangential modes, lying 0.2 eV above the main absorption or emission peak. Both the energy position and line shapes of the sidebands are in excellent agreement with recent calculations [Phys. Rev. Lett. 94, 027402 (2005)] that predict the existence of exciton-phonon bound states, a sizable spectral weight transfer to these exciton-phonon complexes, and that the amount of this transfer depends on the specific nanotube structure and diameter.     

Collective effects in the dynamics of driven atoms in a high-Q resonator

We study the quantum dynamics of N coherently driven two-level atoms coupled to an optical resonator. In the strong coupling regime the cavity field generated by atomic scattering interferes destructively with the pump on the atoms. This suppresses atomic excitation and even for strong driving fields prevents atomic saturation, while the stationary intracavity field amplitude is almost independent of the atom number. The magnitude of the interference effect depends on the detuning between laser and cavity field and on the relative atomic positions and is strongest for a wavelength spaced lattice of atoms placed at the antinodes of the cavity mode. In this case three dimensional intensity minima are created in the vicinity of each atom. In this regime spontaneous emission is suppressed and the dominant loss channel is cavity decay. Even for a cavity linewidth larger than the atomic natural width, one regains strong interference through the cooperative action of a sufficiently large number of atoms. These results give a new key to understand recent experiments on collective cavity cooling and may allow to implement fast tailored atom-atom interactions as well as nonperturbative particle detection with very small energy transfer.Received: 18 May 2004, Published online: 19 October 2004PACS: 32.80.Pj Optical cooling of atoms; trapping - 42.50.Pq Cavity quantum electrodynamics; micromasers - 42.50.Fx Cooperative phenomena in quantum optical systems     

Compositional behaviour of Urbach absorption edge and exciton-phonon interaction parameters in Cu6PS5I1−xBrx superionic mixed crystals

Temperature behaviour of optical absorption edge in Cu₆PS₅I_1−xBr_x mixed crystals is studied in the interval 77-325 K. It is shown that the absorption edge has Urbach shape in the 215-325 K temperature interval. The influence of temperature and compositional disorder on the Urbach absorption edge parameters is presented. The mechanism of the Urbach bundle formation and the effect of I→Br anionic substitution on the exciton-phonon interaction parameters is elucidated.     

声子辅助的电磁感应透明和超慢光效应的研究

在对激子不作任何近似的条件下，对强耦合激子-声子系统中光的线性极化率进行了理论计算，证明了当信号光场频率与激子频率的失谐量等于光学声子的频率时，会出现电磁感应透明现象和超慢光效应.并且与对激子作Dyson-Maleev变换近似和玻色近似的结果进行比较，发现对激子无论是否作近似对产生电磁感应透明现象和超慢光效应都没有实质的影响. 关键词： 量子光学 电磁感应透明 激子 声子     

Quantum memory based on $\mathsf{\Lambda}$-atoms ensemble with two-photon resonance EIT

We study the -atoms ensemble based quantum memory for the quantum information carried by a probe light field. Two atomic Rabi transitions of the ensemble are coupled to the quantum probe field and classical control field respectively with a same detuning. Our analysis shows that the dark states and dark-state polaritons can still exist for the present case of two-photon resonance EIT. Starting from these dark states we can construct a complete class of eigen-states of the total system. A explicit form of the adiabatic condition is also given in order to achieve the memory and retrieve of quantum information.Received: 8 June 2004, Published online: 10 August 2004PACS: 03.67.-a Quantum information - 42.50.Gy Effects of atomic coherence on propagation, absorption, and amplification of light; electromagnetically induced transparency and absorption - 03.65.Fd Algebraic methods     

Polaron effect on the optical absorption and refractive index of an exciton in quantum dots

We have studied the optical absorption of an exciton and its refractive index in a disc-like quantum dot, taking into account of the confined longitudinal optical (LO) phonons. Calculations are performed in the framework of the effective-mass approximation using the compact density-matrix approach. With typical semiconducting GaAs materials, the linear, third-order nonlinear, total optical absorption coefficients and refractive index changes with and without considering the exciton-phonon interaction have been examined. By comparing the polaron effect of the two-electron quantum dot, it is found that the corrections due to the LO phonons on the optical absorption and refractive index are very important and cannot be ignored.     

On the problem of exciton-phonon interaction

The main part of the exciton-phonon interaction is considered to be a consequence of a local deformation of the electromagnetic field due to the molecular vibrations.     

Evolution of photoelectron angular distributions in a train of identical,circularly polarized few-cycle laser pulses

Photoelectron angular distribution (PAD) of atoms irradiated by a train of identical, circularly polarized few-cycle laser pulses is studied in the frame of a nonperturbative scattering theory. Our study shows that the PADs vary with the kinetic energy of photoelectron, the carrier-envelope phase, and the pulse duration. We find that along with increasing of the kinetic energy of photoelectron or with decreasing of the pulse duration or the both, the original one maximum of PAD splits into two maxima; the newly produced two maxima evolve to the opposite pole of the symmetric axis, and finally incorporate as a new maximum located in the symmetric axis.Received: 26 February 2004, Published online: 10 August 2004PACS: 32.80.Rm Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states) - 42.50.Hz Strong-field excitation of optical transitions in quantum systems; multiphoton processes; dynamic Stark shift - 42.65.Re Ultrafast processes; optical pulse generation and pulse compression     

Ground-state energy of the exciton-phonon system in a magnetic field

Upper bounds for the ground-state energy of the exciton-phonon system in a magnetic field are calculated variationally using a wavefunction whose symmetry is suited both to low and high magnetic fields. The displacement amplitudes for the exciton-phonon interaction are those known from the free field case. The results compare satisfactorily with experimental data for TlCl and TlBr.     

Calculation of Linear and Nonlinear Intersubband Optical Absorptions in Electric-Field-Biased Semiparabolic Quantum Wells

By using the compact density matrix approach and iterative procedure, a detailed procedure for the calculation of the linear and nonlinear intersubband optical absorption coefficients is given in the electric-field-biased semi-parabolic quantum wells (QWs). The simple analytical formulas for the linear and nonlinear optical absorption coefficients in the systems are also deduced. Numerical result on typical GaAs materials shows that, the linear and nonlinear optical absorption coefficients sensitively depend on the applied electric field and the confined potential frequency of the semiparabolic QW systems as well as the incident optics beam intensity.