光学参量啁啾脉冲放大中时间抖动对飞秒脉冲对比度的影响

 基于宽带脉冲的计算模型,采用4阶龙格-库塔法研究了光学参量放大所满足的三光波耦合方程。数值结果表明:时间不同步导致大量本底能量不能被压缩,使本底形成,导致飞秒脉冲展宽,如抖动从0变化到150 ps,则其预脉冲宽度由0.2 ps展宽到0.7 ps,降低了输出飞秒激光对比度,并导致输出能量稳定性降低。采用长而平滑泵浦光脉冲、选择适当长度的非线性晶体、并使系统工作于增益饱和区,能实现高对比度和高稳定的飞秒激光输出。     

光学参量啁啾脉冲放大中时间抖动对飞秒脉冲对比度的影响

基于宽带脉冲的计算模型,采用4阶龙格-库塔法研究了光学参量放大所满足的三光波耦合方程。数值结果表明:时间不同步导致大量本底能量不能被压缩,使本底形成,导致飞秒脉冲展宽,如抖动从0变化到150 ps,则其预脉冲宽度由0.2 ps展宽到0.7 ps,降低了输出飞秒激光对比度,并导致输出能量稳定性降低。采用长而平滑泵浦光脉冲、选择适当长度的非线性晶体、并使系统工作于增益饱和区,能实现高对比度和高稳定的飞秒激光输出。     

双轴晶体光学参量放大的研究

介绍了新近提出的光学啁啾脉冲参量放大技术,并以高增益、宽谱带的双轴非线性晶体LBO为例,研究了抽运光和信号光的相位匹配的关系、增益、增益带宽、匹配角的选择,以及增益随晶体长度变化的趋势和双曲正割和高斯脉冲输入非线性晶体前后变化的情况。     

超连续谱注入飞秒光参量放大实验研究

提出了一种很有特色的基于超连续谱注入的飞秒光参量放大技术,该种技术方法不仅克服了常规1 053 nm脉冲在前端小能量放大时的增益窄化现象,而且可实现800 nm激光和1 053 nm激光的零时间同步。通过系统的实验研究,获得了大于4 mJ的1 053 nm宽带信号光能量     

超连续谱注入飞秒光参量放大实验研究

 提出了一种很有特色的基于超连续谱注入的飞秒光参量放大技术,该种技术方法不仅克服了常规1 053 nm脉冲在前端小能量放大时的增益窄化现象,而且可实现800 nm激光和1 053 nm激光的零时间同步。通过系统的实验研究,获得了大于4 mJ的1 053 nm宽带信号光能量     

空气中飞秒激光等离子体荧光辐射光谱研究

系统地研究了不同聚焦条件下飞秒激光空气等离子体的荧光辐射特性以及空间演化情况.在紧聚焦情况下,由于焦点附近比较高的激光强度以及比较高的电子密度,辐射光谱表现为连续谱和线状原子光谱的叠加.在弱聚焦情况下,辐射光谱主要由很多分子线谱组成,而没有观测到连续谱的产生.还研究了光谱谱线强度随激光传输距离的演化情况,结果显示,光谱谱线的强度变化在一定程度上间接反映了等离子体细丝的演化情况.     

基于荧光非共线光参量放大光谱技术的溶剂化动力学研究中的光谱矫正

利用荧光非共线光参量放大光谱技术测量了DCM染料乙醇溶液的溶剂化动力学过程. 实验结果表明,瞬态荧光光谱经过光谱矫正后,可以产生准确的溶剂化相关函数以及溶剂化过程中瞬态光谱峰值频率移动. 本文的工作表明荧光非共线光参量放大光谱技术有益同时关注荧光强度动力学以及光谱谱型演化的研究领域.     

飞秒光学参量振荡器中谐振腔的最佳聚焦设计

本文运用ABCD定律对光学参量振荡器共线谐振腔的聚焦参数及其匹配进行了计算分析。数值计算给出了当OPO腔增益最高时,泵浦光聚焦透镜焦距及聚焦束腰尺寸随振荡光聚焦镜曲率半径的变化及相应的拟合曲线,并对结果进行了讨论。在考虑非线性晶体的接收角的情况下,讨论了光束聚焦镜容许的最短曲率半径。计算同时指出,非临界相位匹配结构比临界相位匹配结构具有更大的接收角.     

飞秒光参量放大中三波群速失配的补偿

为了消除群速失配对参量放大的不利影响，描述了利用脉冲波面倾斜与非共线相位匹配相结 合，完全补偿飞秒光参量放大（OPA）中三波群速失配的新方法.计算了在BBOⅠ类、Ⅱ类相 位匹配条件下， 三波实现群速匹配时，相位匹配角、脉冲波面倾斜角以及非共线角随信号 光波长的变化.并分析了三波群速匹配对空间走离长度、参量增益和参量带宽的影响.结果表 明，在BBOⅠ类、Ⅱ类相位匹配条件下，利用该方法均能实现飞秒OPA连续调谐时三波的群速 匹配，从而大大增加了三波的有效互作用长度，为能够获得高增益，窄脉宽的参量光脉冲提 供了理论依据和指导. 关键词： 群速匹配 脉冲波面倾斜 非共线相位匹配 飞秒光参量放大     

超连续谱注入光参量放大的宽带1053nm飞秒脉冲产生技术

光参量放大技术在理论上既可以支持窄脉宽、也可以支持大能量输出，并且可以获得非常好的光束质量和非常高的信噪比，峰值功率可以大于10PW，是非常理想的强场物理和天体物理的实验研究平台，但由于其在时间同步、能量转换效率、增益稳定性方面的限制，它的实际输出功率非常有限。文中在100Tw钛宝石激光装置研究的基础上，结合快质子实验平台的研制要求和对光参量放大及产生技术、光参量放大增益稳定性技术已有的研究，有特色的提出了以800nm的飞秒脉冲作为泵浦光，利用光参量产生和光参量放大技术直接获得大能量的l053nm种子光。     

Lasing dynamics study by femtosecond time-resolved fluorescence non-collinear optical parametric amplification spectroscopy

Femtosecond time-resolved fluorescence non-collinear optical parametric amplification spectroscopy(FNOPAS) is a versatile technique with advantages of high sensitivity, broad detection bandwidth, and intrinsic spectrum correction function. These advantages should benefit the study of coherent emission, such as measurement of lasing dynamics. In this letter,the FNOPAS was used to trace the lasing process in Rhodamine 6G(R6G) solution and organic semiconductor nano-wires.High-quality transient emission spectra and lasing dynamic traces were acquired, which demonstrates the applicability of FNOPAS in the study of lasing dynamics. Our work extends the application scope of the FNOPAS technique.     

Acquiring 1053 nm femtosecond laser emission by optical parametric amplification based on supercontinuum white-light injection

We report a terawatt-Ti:sapphire-laser-pumped high-energy femtosecond optical parametric amplifier (OPA) with supercontinuum white-light injection. Signal pulses with a duration less than 100 fs and energy up to 4 mJ are obtained with large-aperture LiNbO3 crystals. This megajoule-class femtosecond OPA at 1053 nm presents a feasible alternative to optical parametric chirped-pulse amplification and is ready to be applied to petawatt lasers.     

35 J broadband femtosecond optical parametric chirped pulse amplification system

We report on what is believed to be the first large-aperture and high-energy optical parametric chirped pulse amplification system. The system, based on a three-stage amplifier, shows 25% pump-to-signal conversion efficiency and amplification of the full 70 nm width of the seed spectrum. Pulse compression to 84 fs achieved after amplification indicates a potential of 300 TW pulse power for 35 J amplified pulse energy.     

飞秒BBO光参量放大中闲频光二次谐波的产生

由于相位匹配条件和非线性晶体透光范围的限制，400nm蓝光抽运的飞秒β-BaB₂O₄（BBO）光参量放大（OPA）输出的参量光调谐范围有限，很难得到波长小于460nm的蓝光和近紫外光.实验采用1kHz钛宝石九通啁啾脉冲放大器的倍频蓝光作抽运光，超连续白光 作种子光，在Ⅰ类非共线相位匹配条件下，利用宽带的飞秒BBO OPA，在一定的实验参数下 获得了530—810nm放大的信号光，以及810nm—17μm波段范围的闲频光.与此同时 ，还获得了410—700nm连续可调的闲频光的二次谐波，其与闲频光层叠分布，单脉冲能量 为26μJ，转换效率大于5%.仅利用单块晶体的飞秒BBO OPA就可以获得410—810nm连 续可调的飞秒脉冲输出，从而为更多研究和应用的需要提供了重要的光源.对飞秒光参量放 大中闲频光二次谐波产生的条件也进行了理论分析. 关键词： 二次谐波 闲频光 非共线相位匹配 飞秒光参量放大     

Generation and amplification of dual-color femtosecond pulses by a noncollinear optical parametric up-conversion process

Noncollinear optical parametric up-conversion generation and amplification are realized in a thick β-barium borate (BBO) crystal, and a couple of visible femtosecond up-conversion laser pulses can be achieved by a femtosecond pulse at 800 nm as the pump sources. The theoretical and experimental results indicate that there exist phase-matching conditions for dual-color noncollinear parametric up-conversion generation and amplification, and their wavelengths can be tuned by rotating the BBO crystal. This parametric up-conversion generation and amplification can be attributed to three and five-wave mixing in a thick BBO crystal, and it shows the potential application on optical parametric chirped pulse amplification (OPCPA) to generate multi-color ultraviolet or visible femtosecond laser pulses pumped directly by femtosecond fundamental laser pulses without frequency-doubling or tripling.     

Laser-diode-seeded single and double stage femtosecond optical parametric amplification in the mid-infrared

Tunable mid-infrared pulses are generated with a MgO:LiNbO₃-based traveling-wave optical parametric amplifier in single and double stage operation regime pumped by a 1-kHz Ti:sapphire regenerative amplifier system. For the first time to our knowledge a pulsed laser diode is successfully used in the femtosecond regime as a compact seed source at the signal wavelength where the tunability of the generated idler pulses can be realized by tuning the seed wavelength. Almost transform limited mid-infrared pulses as short as 130 and 160 fs with pulse energies as high as 5 and 15 J are produced near 3.5 m by the single and double stage scheme, respectively. The pulse to pulse fluctuations in both cases do not exceed 2% which corresponds to the stability of the pump source.     

100-TW femtosecond laser based on parametric amplification

In experiments on the parametrical amplification of femtosecond pulses in wide-aperture DKDP crystals, a power of more than 100 TW has been reached, which is much higher than the record level achieved in such lasers. The energy efficiency obtained for the parametric amplifier is equal to 27%. The energy of a 72-fs pulse is equal to 10 J.     

Amplification of fluorescence using collinear picosecond optical parametric amplification at degeneracy

We demonstrate the output characteristic of broadband parametric amplification of incoherent light pulses in a 355-nm pumped degenerate picosecond optical parametric amplification with either saturated or unsaturated amplification.The optical parametric amplifier is seeded by the fluorescence generated in a solution of pyridine-1 dye in ethanol.With the saturated amplification,we can obtain high energy incoherent light pulses,whose full width at half maximum bandwidth varies from 16 nm to 53 nm for the different phase matching angles near degeneracy.Moreover,the unsaturated bandwidth of the amplified pulses fits well to the calculated result at degeneracy.Selecting s-polarized fluorescence with a Glan-Taylor prism,the maximum bandwidth of the amplified fluorescence is found to be 59 nm for a purely s-polarized seed.The maximum output energy is 0.67 mJ for the optical parametric amplifier.By using an optical filter and compressor,the generated high energy incoherent light has great potential as the incoherent pump,signal or idler wave of a parametric down-conversion process,so that a wave with a high degree of coherence can be generated from an incoherent pump light.     

Efficient femtosecond traveling-wave optical parametric amplification in periodically poled KTiOPO(4)

We report, for the first time to our knowledge, high-power femtosecond traveling-wave optical parametric amplification by use of periodically poled KTiOPO(4) . With a single pass through a 4-mm-long sample of 1.23-mm thickness we achieved 40% internal conversion efficiency and 5microJ of single-pulse idler energy near 3.8microm , using only 75microJ of energy from the output of a conventional 1-kHz Ti:sapphire regenerative amplifier. The 210-fs-long idler pulses were almost transform limited. We discuss the specific problems encountered in high-power parametric conversion, such as unwanted quasi-phase-matched upconversion processes for polarization configurations that utilize the largest (d(33)) nonlinear coefficient and the related formation of color centers (gray tracking) in KTiOPO(4) .