The modular group and super-KMS functionals

Every normal, faithful, self-adjoint functional on a von Neumann algebraA canonically determines a one-parameter-weakly continuous *-automorphism group (the analog of the modular group) and a canonical ₂ grading onA, commuting with . We show that the functional satisfies the weak super-KMS property with respect to and Furthermore, we prove that and are the unique pair of a-weakly continuous one-parameter *-automorphism group and a grading of the algebra, commuting with each other, with respect to which is weakly super-KMS. The above results thus provide a complete extension of the theory of Tomita and Takesaki to the nonpositive case.Supported in part by the National Science Foundation under Grant DMS-8922002.     

Averaged electron Green function and CDW pinning in one-dimensional random potential

The averaged retarded electron Green functionG ⁺(,k) in 1d disordered metal is calculated using the Berezinsky diagram technique. Using the Gorkov's theory it is shown, that the substitution of inG ⁺ (,k) by the square of the external frequency atk=0 gives the dependence of Fröhlich conductivity _F(). This dependence describes the impurity pinning of CDW in 1d disordered metals. The good agreement of this dependence with experimental data Zeller et al. about _F() in quasi-1d conductor KCP is found     

Spectral superbroadening of self-focused picosecond laser pulses in D2O

Intense picosecond light pulses of a mode-locked Nd: glass laser at _L =1054 nm (fundamental wavelength) and _SH =527 nm (second harmonic wavelength) are passed through a sample of D₂O under self-focusing conditions. Spectrally structured superbroadened, spatially bell-shaped emission in the forward direction is obtained. Primary generation processes are pump-pulse-degenerate stimulated parametric four-photon interaction (₁ + _{1 3} + ₄) and stimulated Raman scattering (_{1 R} + ), which occur concurrently (₁= _L or _SH angular pump frequency, #x03C9; _R first Stokes frequency, #x03C9; signal frequency, #x03C9;₃ signal frequency, #x03C9;₄ idler frequency). The parametric four-photon interaction occurs under collinear non-phase-matched conditions and under longitudinally phase-matched, transversally non-phase-matched (erenkov-like) conditions. Subsequent interaction processes are pump-pulse-nondegenerate four-photon interaction of the type ₁ + _{R 3} + ₄, coherent antiStokes Raman scattering (CARS, ₁ + ₁ – _{4 3}), inverse Raman scattering ( _A + ₁ + ), and cascading light up-conversion of the type ₁ + _(i) – _{R (i+1)}.     

Derivation and solution of a low-friction Fokker-Planck equation for a bound Brownian particle

The low-friction region of an anharmonically bound Brownian particle is examined using systematic elimination procedures. We obtain an asymptotic expression for the spectrum of the Fokker-Planck operator. Asymptotic means both small anharmonicities and small friction constants compared to the oscillatory frequency . We conclude that Kramers' low-friction equation is generally valid only for 0<0.01 and has to be modified for 0.01 by including phase-dependent terms. From these the nonlinear part of the force field in connection with a finite temperature is shown to shorten the correlation time of the equilibrium velocity autocorrelation function and to renormalize the frequency of the corresponding spectral density.     

Excited-state absorption and third-order optical nonlinearities in symmetric π-electron organic molecules

Excited-State Absorption (ESA), Two-Photon Absorption (TPA) and the third-order polarizability (;,, – ) have been investigated for a model dichloride derivative of a symmetrically substituted benzylidene analine (SBAC), using a multielectron configuration-interaction procedure. The calculations indicate that SBAC exhibits ESA across the visible region of the spectrum, but that it is not as extensive as for molecules such as the phthalocyanines. The magnitude of the third-order polarizability is dominated by resonance enhancement from a very strongA _g B _u one-photon absorption. The calculated off-resonance value for (;,, – ) suggests that SBAC is a potential candidate for ultrafast switching applications.     

Periodic Motion of Atoms Near a Charged Wire

We study the classical motion of an atom in the vicinity of an infinite straight wire which carries an oscillating uniform charge. This system has been proposed as a mechanism for trapping cold neutral atoms. The parameters of the problem are the magnitude Q and frequency of oscillation of the charge, the mass M and polarizability of the atom, and the angular momentum L of the atom about the wire. For 0 and 2MQ ² greater than, but close to, L ², we prove that the atom's radial motion is periodic (with period 2/), and that the atom moves in a helical path around the wire. For 2MQ ² L ² we prove that the atom must either collide with the wire or else escape to infinity in the radial direction.     

The third-order electric susceptibilities of NaCl and KCl monocrystals

The dispersion of the third-order electric susceptibilities(; , , –) and(; , 0, 0) of NaCl and KCl monocrystals has been calculated by means of experimental data on the electro-optic Kerr effect. The result has been obtained by using semi-classical models of anharmonic oscillators. An ionic contribution to the electro-optic coefficients has been presented. From the result obtained it follows that the third-order electric susceptibilities are of the order of 10^–22 m² V^–2.     

Lifshitz tails for periodic plus random potentials

We prove that the integrated density of states () for a potentialW =V _per +V has Lifshitz tails where V_per is a periodic potential with reflection symmetry andV is a random potential, e.g., of the formV =q _i ()f(x–i).research partially supported by DFG.research partially supported by USNSF under grant No. MCS-81-20833.     

Calculation of the dispersion of the third-order optical nonlinearity in C60 films

Using wave functions determined from ground-state local-density calculations, we have calculated the wave-dispersed free response of the optical nonlinear polarizability ⁽³⁾(–3;,,), for the C₆₀ molecule and ⁽³⁾(–3;,,) i.e. Third-Harmonic Generation (THG) for films using a sum-over-states approach. The influence of screening was determined by applying an external static electric field in separate selfconsistent calculations to evaluate induced dipole moments which was used to determine the static linear and nonlinear polarizabilities. The polarizabilities calculated in the static limit were used to determine an effective screening parameter which was, in turn, used together with an RPA approach to calculate screened wave-dispersed, third-order nonlinear optical properties such as ⁽³⁾(–3;,,) and ⁽³⁾(–3;,,). Comparing evaluated polarizabilities with experimental values we found that the non-resonant free polarizability compares well in absolute magnitude with experimental results. Inclusion of screening results in a polarizability about two orders of magnitude below the experimental values.Paper presented at the 129th WE-Heraeus-Seminar on Surface Studies by Nonlinear Laser Spectroscopies, Kassel, Germany, May 30 to June 1, 1994     

Ultrasound in spin glasses

The change of the sound velocity v(,T) and the damping of sound waves (,T) in spin glasses are calculated in the frame-work of an Ising model with a random distribution of exchange interactions. The calculation is based on linearized equations of motion for the spins and on an improved mean field approximation which includes the Onsager reaction field. Near to the freezing temperatureT _f and at high temperatures v(,T) and (,T) turn out to be approximately proportional to the real and the imaginary parts of the dynamical susceptibility. For the special case of infinite range interactions atT=T _f one has v(, T_f) ( )^1/2 and (, T_f) (/)^1/2 where is the relaxation time of independent spins. However, already slightly aboveT _f the frequency dependence of both quantities becomes rather small for RKKY spin glasses. At high temperatures both, v(,T) and (,T) vary asT ^–1.SFB 125 Aachen-Jülich-Köln     

Harmonic mixing by weakly pinned charge density waves

Third order harmonic mixing voltageE ₀ in case of frequency matching, =₂–₁=0, and third order pseudo harmonic mixing currentj() in the detuned case, 0, are evaluated for the one-dimensional Fukuyama-Lee-Rice model for weakly pinned charge density waves in the region of sub-threshold bias electric fields. After a perturbation expansion of the phase response to the ac driving fields the impurity averaging is performed diagrammatically. Specific statistical properties of the charge density wave phase in the weak pinning limit and a non-trivial result for the pinning of the static phase are utilized to expressE ₀ andj() in terms of the dielectric function (). A recent evaluation of () within the self-consistent Born approximation is used to present the results explicitly in a number of diagrams. In comparison to the overdamped anharmonic oscillator the following differences are found: Randomness leads to interference contributions which increase the amplitudes and decrease the phase shifts. The more realistic form for () at lower frequencies lead to a downward shift in the maximum ofj() when ₁ is decreased below the cross-over frequency _c . The present theory retains inertia in the dynamical equations and remains valid for frequencies near and above the pinning frequency. It fails, however, for small frequencies _{1 c} due to the neglect of metastable states and screening.     

Low frequency limits of third-order harmonic coefficients for atomic hydrogen in any level of discrete energy spectrum

In this paper the analytical expression is derived for the third-order optical harmonic coefficients x _abcd ^v (,,) of the atomic hydrogen at very low frequencies 0 in many level of the discrete energy spectrum.The author expresses his thank to Prof. Nguyen Van Hieu for suggesting the problem and fruitful discussions.     

Some results on electronic two- and one photon raman scattering in CdS

Two photon Raman scattering (TPRS) via virtually excited biexcitons is observed in CdS over a rather large spectral region in a scattering configuration which favours stimulated emission. We observe either a pure longitudinal exciton or-for the first time—a bound exciton (I ₂) as final state particles. Furthermore, the anomaly in the relation between _exc and _R at _exc= E_blex is observed for the first time in a II–VI compound, indicating an energy of the ₁ biexciton level of 5.098 eV in agreement with two photon absorption measurements. With an applied magnetic fieldB, the corresponding shift of the exciton eigenenergies can be observed. For the longitudinal exciton, the diamagnetic shift is 0.35 meV atB=10T forBc in agreement with theoretical predictions. In this configuration also a stimulated one photon spin flip Raman scattering is observed, yielding the well known electronicg-value of 1.78.     

Stochastic linear maps and transition probability

Some aspects of the transition probability P(, ) between states , on unital ^*-algebras are discussed. It is shown that P increases under the action of any stochastic linear map T, i.e., P(T, T)P(, ). Some properties of P are derived in starting from a recently-proved characterization of the quantity in question.     

Ferromagnetic resonance in media with an inhomogeneous saturation magnetization

The method of transition probabilities is used to calculate the line width of ferromagnetic resonance in a medium with an inhomogeneous saturation magnetization. It is shown that in addition to linear (with respect to the Fourier components of the function describing inhomogeneities) terms, the perturbation Hamiltonian must include also quadratic terms. The frequency dependence of the contribution of the porosity to H is fundamentally different from the frequency dependence of the magnetic anisotropy contribution. This anisotropy contribution H_a() decreases on increase in the frequency and has a maximum at = (2/3)_M, whereas the porosity contribution H_p increases on increase in the frequency and vanishes at = (2/3)_M.deceasedTranslated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 12, pp.48–52, December, 1980.     

Total dynamic structure factor of icosahedral and As-quenched and relaxed glassy Pd58.8Si20.6U20.6 measured at 296 K

The total dynamic structure factorsS(Q, ) of icosahedral, glassy Pd_58.8Si_20.6U_20.6, and the crystallized sample have been determined at room temperature using inelastic scattering of cold neutrons (IN6 of ILL). In contrast to the static structure factorS(Q), where the long range bond orientational order (BOO) leads to pronounced diffraction peaks with finite half width, the dynamic structure factor shows little or no influence of the long range BOO on the atomic dynamics of icosahedral PdSiU in the range of frequencies (0.525 meV) and momentum transfers Q(5Q30 nm^–1 for inelastic scattering) investigated here. The wavelength-dependence of the atomic dynamics of icosahedral PdSiU is very similar to that of the metallic glass and is different from that of the crystallized sample. As for glassy PdSiU no well defined vibrational collective excitations are found as peaks in the inelastic part ofS(Q, ) of the icosahedral sample,-quite in contrast to theoretical expectations and to the dispersions of pronounced excitations determined under identical experimental conditions fromS(Q, ) of the crystallized sample. On structural relaxation of the metallic glass Pd_58.8Si_20.6U_20.6 the largest amount of low energy modes is annealed out at lowest energy.Dedicated to Professor Harry Thomas on the occasion of his 60th birthday     

Scaling characteristics of ac conductivity and dielectric function in fractal regime of the metal-insulator transition

An analysis of the ac conductivity _ac(), and the ac dielectric constant, (), of the metal-insulator percolation systems is presented in the critical regime near the transition threshold. It is argued that the polarization and relaxation of the finite fractal metallic clusters play dominant roles in controlling the dynamic response of the system on both sides of the threshold. The relaxation time constant of a fractal cluster is shown to scale with its size as withd _t = 4 – 2d +d _c + /, whered is tge Euclidean dimension, andd _c , , and are the scaling indices for the charging, the dc conductivity, and the correlation length respectively. The average time dependent response of the system is shown to scale with a new time scale , where is the correlation length and ₀ is a microscopic time constant. It is shown that at frequencies and with /d_t 1, in close agreement with experiments. The effects of the anomalous transport along the infinite cluster and the medium polarizability are also discussed.     

Experimental survey of the sticking problem in muon catalyzed dt fusion

The sticking process dt + n, which constitutes the most severe limit to the number of fusions which a muon can catalyze, is reviewed. Many attempts were made to determine by calculations and measurements the probability for initial sticking _s ⁰ (immediately after dt fusion) and for final sticking _s (after the came to rest). Previous results based on neutron disappearance rates and on the observation of -X-rays were controversial and also in some disagreement with theory. New data are reported from PSI on direct observation of final sticking, using a setup with the St. Petersburg ionization chamber. These data mark a significant improvement in reliability and may clarify questions concerning previous discrepancies. The new results is _s(0.56±0.04)%, lower than the theory prediction _s=(0.65±0.03)%, at medium density.     

Some exact models for nonspherical collapse. III

The gravitational nonradiative collapse of dust configurations in the presence of electromagnetic field is analyzed in terms of exact dynamical solutions for a wide range of spacetime symmetries: cylindrical, pseudoplanar, toroidal, and also spherical, planar, and pseudospherical [when the anisotropy factor of the (x ²,x ³) surfaces,(R, T), is replaced by a massless scalar field]. The condition that the collapse is nonradiative leaves three possibilities for the coordinate dependence of(R,T) (i)=(a),a (R, T) being the scale factor of the (x ²,x ³) surfaces, (ii)=(T), and (iii)=(R). Almost all (in the meaning indicated in the text) solutions for charged dust with=(a) and for dust in the external electromagnetic field with=(T) and=(R) have been obtained and discussed. A wideranging discussion concerning the topics of papers I–III is given. Special attention is paid to the question of horizon existence and formation and also the perspective of extension of the techniques developed onto the more realistic case of axial symmetry.     

QCD sum rule analysis of the coupling constant g ωσγ

We employ QCD sum rules to calculate the coupling constant g by studying the three point -correlation function. Our result complements the analysis of this coupling constant utilizing the experimental value of the ⁰⁰ decay rate studied within the framework of chiral perturbation theory including vector meson and meson intermediate states.