Self-pumped phase conjugation in a ring cavity at 1.06 μm in cw and nanosecond regimes using photorefractive BaTiO3:Rh

We present self-pumped phase conjugation experiments in a ring cavity at 1.06 μm in a BaTiO₃:Rh crystal both in the cw and in the nanosecond regime. The measured reflectivities are respectively 50% and 66%. At 4 W cm⁻² of cw illumination, it only takes 90 s to reach the steady state. A preliminary experiment of correction of the focusing effect of a lens is reported.     

Two-wave mixing in photorefractive BaTiO(3):Rh at 1.06 mum in the nanosecond regime

We present two-beam coupling experiments in the nanosecond regime at 1.06 mum , using photorefractive BaTiO(3):Rh. The maximum observed exponential gain coefficient is 14.2 cm(-1) . No intensity-dependent electron-hole competition and no strong saturation of the photoionized charge carriers are observed for intensities of less than 20MW cm(-2) . The energy required for recording the photorefractive grating is not significantly different in the nanosecond and the cw regimes.     

Double phase conjugation with orthogonally polarized beams in a BaTiO(3) crystal

We have demonstrated experimentally the simultaneous self-conjugation of extraordinarily and ordinarily polarized light waves (lambda=514 nm), with the polarization state preserved, in a Ce:BaTiO(3) crystal. Conjugate o waves originate from coupling between o and e waves by means of a circular photogalvanic effect. The conjugator also takes advantage of the Ce:BaTiO(3) crystal, for which it is easy to generate an extraordinary conjugate beam by photorefractive backscattering. This beam of light is necessary for double phase conjugation.     

Thermal and acoustic effects in optical phase conjugation in Rhodamine 6G solutions with nanosecond pulses

Thermally induced phase conjugation by degenerate four-wave mixing in solutions of Rhodamine 6G in ethanol in the weak absorption region, low-reflectivity regime, and nonosecond time domain is reported. Evidence of oscillatory acoustic modes in the nonlinear medium is presented and existing theories are shown to explain satisfactorily the experimental results.     

用He—Ne激光在KNSBN晶体中实现高反射率自泵浦相位共轭

本文报道了用He-Ne激光在(K_(O.5)Na_(0.5)_2y(Sr_(0.61)B_(0.39)))_(1-y)Nb_2O_6(KNSBN)光折变晶体中实现高反射率自泵浦相位共轭,其共轭光的反射率高达40%.研究了共轭光反射率随入射角度变化的关系以及响应时间与入射光功率密度的关系.     

Nd:YAG master-oscillator power amplifier with a rhodium-doped BaTiO(3) self-pumped phase-conjugate mirror

We investigate Nd:YAG master-oscillator power amplifier arrangements with an infrared-sensitive rhodium-doped BaTiO(3) photorefractive phase-conjugate mirror. In these setups the phase-conjugate mirror is simple to implement, compact, passive, and completely self-contained. We demonstrate a reasonable extraction efficiency (~50%), response times in the range of several minutes with our experimental conditions and an excellent ability of the phase-conjugate mirror to compensate for severe phase aberrations.     

Self-pumped phase conjugation in a liquid crystal light valve with a tilted feedback mirror

We report self-pumped phase conjugation in a photorefractive liquid crystal light valve with a tilted feedback mirror. This is a new scheme for the self-generation of a phase-conjugate replica and can in general be applied to thin nonlinear layers, opening the way to distortion-correction applications of thin media.     

Self-pumped phase conjugation in Bi12TiO20 crystal without external cavity

We present an experimental study of the self-pumped phase-conjugate-mirror (SPPCM) recording in a Bi₁₂TiO₂₀ sample due to the partial internal reflection of the pump beam from the rear face. SPPCM has been recorded under an external alternating electric field of a square-wave form with response time equal to 170 s at the pump beam intensity of 520 mW/cm². The mechanism of the SPPCM formation is similar to that of photorefractive double-phase-conjugate mirrors. The most effective SPPCM is recorded at the much larger pump-beam-incident angle than it could be supposed from the typical angular dependence of the two-wave-mixing gain factor. Strong dependence of the gain distribution on the pump-beam-propagation angle is observed. It is found that the response time strongly depends on the preliminary history of the sample. Received: 11 August 1998 / Revised version: 14 January 1999 / Published online: 28 April 1999     

Photorefractive properties and self-pumped phase conjugation in a series of BaTiO3 crystals

This paper presents the experimental results of two-wave mixing and self-pumped phase conjugation (SPPC) in barium titanate (BaTiO₃) crystals doped with Rh or Ce. It has been shown that the main parameters of SPPC depend very strongly on the concentrations of dopants, the incident angles and the crystal cut used. High gain in two-wave mixing corresponds to low phase-conjugate reflectivity in all samples. It is impossible to maintain the highest reflectivity and gain simultaneously, because the gain will definitely be limited when we try to get the highest reflectivity, and vice versa. Some qualitative explanation of the experimental results is also given. Received: 5 January 2001 / Final version: 25 May 2001 / Published online: 19 September 2001     

High photorefractive sensitivity at 860 nm in reduced rhodium-doped KNbO(3)

We show that high-temperature reduction in a CO-CO(2) atmosphere increases the photorefractive sensitivity of KNbO(3):Rh at 860nm by 4 orders of magnitude compared with that of the as-grown crystal. The effective trap density is increased by a factor of 3, and the photoconductivity by a factor of 30, and the photorefractive response at a grating spacing of 0.15 mu;m is accelerated by a factor of 400. The grating buildup time at a grating spacing of 0.7 microm and an intensity of 1Wcm(-2) is 0.5 s, a value comparable with that of as-grown KNbO(3):Fe at visible wavelengths. The optical and photorefractive parameters of Rh-doped KNbO(3) subjected to reduction treatment are characterized for wavelengths of 0.48-1.064 microm .     

Structural and phase transformations of sulfide mineral surfaces irradiated by nanosecond electromagnetic pulses

The effect of high-voltage nanosecond electromagnetic pulses on the phase composition of chalcopyrite and sphalerite surfaces is investigated by IR-Fourier spectroscopy, XPS, and UVS. Electromagnetic pulse treatment results in the formation and accumulation of copper and/or iron sulphates Me _x (SO₄) _y in superficial chalcopyrite layers, zinc sulphate ZnSO₃, and carbonate ZnCO₃ on sphalerite surfaces, changing their electrochemical and physicochemical properties; i.e., a rise in electrode potentials creates favorable conditions for anionic collector sorption and promotes sulfide flotation activity.     

Interdiffusion studies in Bi-based layered systems with nanosecond laser pulses

Interdiffusion processes are induced by nanosecond laser pulses from an excimer laser. The Bi-based systems studied are formed by a Bi layer and a Sb or Ge layer. Configurations with Bi at the surface layer or at the innermost layer are both studied. Real-time reflectivity measurements are performed during the irradiation to determine the process kinetics and times and Rutherford backscattering spectrometry is used to obtain the concentration depth profiles. It will be shown that there is an interfacially initiated diffusion process in the Bi-Sb system and that the diffusion coefficients of this system within the liquid phase are in the 10^–5–10^–6 cm²/s range. The Bi-Ge system shows instead little mixing, the diffusion coefficients of the system within the liquid phase being at least two orders of magnitude lower. The differences observed when Bi is the surface layer or the innermost one are related to the different thermal responses of the system.     

Changes in the surface phase composition of sulfide minerals upon irradiation by high-power nanosecond pulses

The effect of high-power (high-voltage) nanosecond pulses on the phase composition and chemical state of atoms of surface layers of sulfide minerals with different semiconductor properties (galenite, molybdenite, and sphalerite) is investigated by means of XPES. Common patterns and characteristic features of the structural phase transformations of sulfide surfaces under the pulsed energetic effect are the formation and growth of a surface layer by the nonstoichiometric sulfur-enriched sulfide phase and Zn and Mo oxides and hydroxides; the staged character of the transformation of sulfur atoms in the composition of galenite and sphalerite surface layers; and the stability of the chemical state of sulfur in the molybdenite composition and lead atoms in the galenite composition.     

Laser ablation of silicon in water with nanosecond and femtosecond pulses

We describe laser ablation of Si under water by 5 ns, 355 nm and 100 fs, 800 nm pulses. Compared to that in air, an approximately twofold improvement in the ablation rate is found in water for femtosecond and nanosecond pulses. For higher laser irradiances, the plasma that forms at the water-air interface hampers further improvement of the ablation rate. We investigated the enhanced ablation process in water and found that the cavity-confinement geometry that increases the laser energy coupling to the target and allows more energy to be transferred to the cavity sidewalls plays an important role in the escalated material removal process. In addition, we show that the water layer that effectively reduces the oxidation and redeposition of the ablated debris is also responsible for improvements in the ablation process.     

Ferroelectric phase transitions in ultrathin films of BaTiO3

We present molecular dynamics simulations of a realistic model of an ultrathin film of BaTiO3 sandwiched between short-circuited electrodes to determine and understand effects of film thickness, epitaxial strain, and the nature of electrodes on its ferroelectric phase transitions as a function of temperature. We determine a full epitaxial strain-temperature phase diagram in the presence of perfect electrodes. Even with the vanishing depolarization field, we find that ferroelectric phase transitions to states with in-plane and out-of-plane components of polarization exhibit dependence on thickness; it arises from the interactions of local dipoles with their electrostatic images in the presence of electrodes. Secondly, in the presence of relatively bad metal electrodes which only partly compensate the surface charges and depolarization field, a qualitatively different phase with stripelike domains is stabilized at low temperature.