Absorption spectroscopy of mid and neighboring Z plasmas: Iron, nickel,copper and germanium

Opacities of four medium Z element plasmas (iron, nickel, copper and germanium) have been measured at the LULI-2000 facility in similar conditions: temperatures between 15 and 25 eV and densities between 2 and 10 mg/cm³, in a wavelength range (8–18 Å) including the strong 2p–3d structures.Two laser beams from the LULI facility were used in the nanosecond-picosecond configuration. The NANO-2000 beam (at λ = 0.53 μm) heated a gold hohlraum with an energy between 30 and 150 J with a duration of 0.6 ns. Samples covering half a hohlraum hole were thus radiatively heated. The picosecond pulse PICO-2000 beam (at λ = 1.053 μm) has been used to produce a short (about 10 ps) X-ray backlighter in order to reduce time variations of temperatures and densities during the measurement. A crystal high-resolution spectrometer was used as the main diagnostic to record at the same time the non-absorbed and the absorbed backlighter spectra. Radiation temperatures were measured using a broadband spectrometer. 1D and 2D simulations have been performed in order to estimate hydrodynamic plasmas parameters.The measured spectra have been compared with theoretical ones obtained using either the superconfiguration code SCO or the detailed term accounting code HULLAC. These comparisons allow us to check the modeling of the statistical broadening and of the spin-orbit splitting of the 2p–3d transitions and related effects such as the interaction between relativistic subconfigurations belonging to the same non-relativistic configuration.     

K-shell spectroscopy of plasmas created by intense laser irradiation of micron-scale pyramid and sphere targets

K-shell spectra of targets with microstructured features irradiated by an intense femtosecond laser have been studied. Examination of K_α emission from laser irradiated Si targets coated with micron-scale polystyrene spheres indicates that the emission is enhanced by a factor of 3 over emission from planar solids. Sphere-coated targets also emit K-shell He-like Si radiation indicating the presence of a hot dense plasma beneath the microspheres. Furthermore, K_α from Ti foils coupled to micro-tipped reentrant pyramid and wedge shaped targets has been studied, however, no significant enhancement of the K_α yield is observed for these kinds of targets. These studies illustrate that, with correct tailoring of the target surface, field enhancements can be used to increase X-ray emission from intensely irradiated targets.     

Plasma jets produced by low energy laser pulse interaction with planar and cratered targets

Laser experiments of the plasma jet formation using nanosecond laser pulses with low energy, i.e., <20 J, are presented. Planar and cratered gadolinium and aluminum targets are irradiated with laser intensities of several 10¹⁴ W/cm². Spatially-resolved time-integrated X-ray spectra were recorded in the spectral range from 7 to 10 Å. A jet-like structure is obtained from aluminum targets with a preformed crater, which is not seen in planar target irradiation. For gadolinium, a jet is observed from both planar and preformed cratered targets, suggesting that the collimation is dominated by radiative cooling. A radiation-hydrodynamics code coupled to a non-LTE ionization code was used to model the plasma. The calculated plasma emission was found to be consistent with the experimental results.     

WENO schemes applied to the quasi-relativistic Vlasov–Maxwell model for laser–plasma interaction

In this paper we focus on WENO-based methods for the simulation of the 1D Quasi-Relativistic Vlasov–Maxwell (QRVM) model used to describe how a laser wave interacts with and heats a plasma by penetrating into it. We propose several non-oscillatory methods based on either Runge–Kutta (explicit) or Time-Splitting (implicit) time discretizations. We then show preliminary numerical experiments.     

Environmental conditions in near-wall plasmas generated by impact of energetic particle fluxes

Directional flows of energetic ions produced by laser-exploded foils were used to investigate transient phenomena accompanying the plasma interaction with surfaces of solid targets (walls). In experiments carried out on the iodine laser system PALS, the formation of energetic plasma jets from burn-through foils of Al and Ta was optimized using the three-frame interferometry and applied to a design of alternate experimental configurations. The interaction of the directional plasma flows with secondary targets was studied via X-ray imaging, optical and high-resolution X-ray spectroscopy. The environmental conditions in near-wall plasmas created at surfaces of plasma-exposed solids, in particular the velocity distribution of impinging and back-scattered ions, were determined via analysis of the observed spatially-resolved spectra of Al Lyα and Heα groups. The validity of the ion velocity gradients derived from the Doppler effect induced shifts and splitting of the spectral lines was supported by theoretical modeling based on a combination of hydrodynamic, atomic and collisional-radiative codes.     

Simultaneous imaging of K-α radiation and coherent transition radiation from relativistic-intensity laser-irradiated solid target plasmas

Laser acceleration of hot electrons and their transport through 12-32 μm thick Ti foils was explored experimentally using two complementary diagnostics, a bent crystal imaging the Ti K_α emission and optical imaging of the coherent transition radiation (CTR) produced by the exit of the hot electrons from the foil. The spatial extent of the hot electron production measured by these two diagnostics is dramatically different. Electrons producing CTR emerge in a spot of less than 7 μm and appear to maintain a high degree of collimation during transport through the foil while electrons that produce K_α emission appear to diverge to sizes of 50-100 μm as viewed from the back surface of the foil. These results indicate that there is a large difference in the transport of the highest energy electrons contributing to CTR signal as compared with the bulk of the hot electron population generating K_α signal.     

Measurement and simulations of hollow atom X-ray spectra of solid-density relativistic plasma created by high-contrast PW optical laser pulses

K-shell spectra of solid Al excited by petawatt picosecond laser pulses have been investigated at the Vulcan PW facility. Laser pulses of ultrahigh contrast with an energy of 160 J on the target allow studies of interactions between the laser field and solid state matter at 10²⁰ W/cm². Intense X-ray emission of KK hollow atoms (atoms without n = 1 electrons) from thin aluminum foils is observed from optical laser plasma for the first time. Specifically for 1.5 μm thin foil targets the hollow atom yield dominates the resonance line emission. It is suggested that the hollow atoms are predominantly excited by the impact of X-ray photons generated by radiation friction to fast electron currents in solid-density plasma due to Thomson scattering and bremsstrahlung in the transverse plasma fields. Numerical simulations of Al hollow atom spectra using the ATOMIC code confirm that the impact of keV photons dominates the atom ionization. Our estimates demonstrate that solid-density plasma generated by relativistic optical laser pulses provide the source of a polychromatic keV range X-ray field of 10¹⁸ W/cm² intensity, and allows the study of excited matter in the radiation-dominated regime. High-resolution X-ray spectroscopy of hollow atom radiation is found to be a powerful tool to study the properties of high-energy density plasma created by intense X-ray radiation.     

Relativistic electron transport and confinement within charge-insulated, mass-limited targets

We present experimental results on the interaction of short-pulse ultra-high-intensity laser beams with small size (“mass-limited”) targets. Several diagnostics (X-ray spectroscopy, K_α and optical imaging of target rear side) have been simultaneously used in order to characterize the laser-generated fast electron transport and energy deposition into the target material. Our results show that fast electrons are effectively confined inside the target by the induced space charge. This electrostatic confinement opens new opportunities to create “Warm Dense Matter” states characterized by solid-state density and temperatures of the order of a few tens of eV.     

Atomic modeling of the plasma EUV sources

We present the development of population kinetics models for tin plasmas that can be employed to design an EUV source for microlithography. The atomic kinetic code is constrained for the requirement that the model must be able to calculate spectral emissivity and opacity that can be used in radiation hydrodynamic simulations. Methods to develop compact and reliable atomic model with an appropriate set of atomic states are discussed. Specifically, after investigation of model dependencies and comparison experiment, we improve the effect of configuration interaction and the treatment of satellite lines. Using the present atomic model we discuss the temperature and density dependencies of the emissivity, as well as conditions necessary to obtain high efficiency EUV power at λ = 13.5 nm.     

Collimated quasi-monoenergetic electron beam generation from intense laser solid interaction

A quasi-monoenergetic electron beam with divergence of 3° and energy peak of 1 MeV is observed along the target surface from interaction of a bulk Cu target and an intense relativistic laser pulse of 1 TW and 70 fs at a grazing incident angle. A preplasma formed by high-contrast picosecond prepulse plays a crucial role. Particle-in-cell simulations broadly reproduce the result and show that a preplasma with the proper density and a large angle of incidence is required. The preplasma sets up a static electric field along the surface can accelerate electrons. The static electric field is formed just after the passage of the laser. This approach can be extended to higher intensities to generate higher energy beams.     

Characterization of gold/PMMA hybrid nanomaterials synthesized by hard X-ray synchrotron radiation

In this study,new types of hybrid gold poly(methyl methacrylate) (PMMA) nanomaterials are synthesized.Both PMMA spheres coated with gold nanoparticles and gold nanoparticles coated with PMMA can be synthesized using different ratios of HAuCl4 and MMA precursors,by exposing the mixtures to hard X-ray synchrotron radiation without the use of a reducing agent.According to the photochemical mechanism,gold nanoparticles will precipitate from a solution of HAuCl4 on exposure to synchrotron radiation,followed by the synthesis of PMMA by the polymerization of MMA monomers.These reactions can result in the formation of two different types of new hybrid nanomaterials.When a 1:1 volume ratio of HAuCl4 to MMA is used,we obtain PMMA spheres coated with gold nanoparticles.When a 10:1 ratio of HAuCl4 and MMA is used,we obtain gold nanoparticles coated with PMMA.The hybrid gold/PMMA nanostructures are characterized by transmission electron microscopy,elemental analysis,dynamic-light scattering analysis,gel permeation chromatography and Raman spectroscopy.The hybrid nanomateriais have potential application in the fields of biosensors and drug delivery.     

Investigations involving shock waves generation and shock pressure measurement in direct ablation regime and confined ablation regime

Recent investigations involving shock waves generation and shock pressure measurement in direct ablation regime and confined ablation regime for aluminium, copper, titanium and steel (40C130) materials are reported. Experimental measurements demonstrated that in direct ablation regime the peak pressures typically are less than 10 Pa when the incident laser intensity is about 10 W/cm and the time duration of the applied pressure is roughly equal to the laser pulse duration. It is shown that confinement of the surface with a transparent overlayer provided an effective method of enhancing laser-induced shock waves pressure in the target material with an order of magnitude for same laser intensity. Also, in this second regime, the pressure is applied over a period much longer than the laser-pulse duration. As an application measurements of the hardness of target surface before and after laser irradiation in direct ablation regime and confined ablation regime are given, and it is shown that the maximum value of surface hardness is obtained in confined ablation regime. Received 10 March 2001 / Accepted 13 April 2001     

导弹水下点火推力峰值问题的数值研究

通过对燃烧室内燃气采用常微分控制方程,对喷管-燃气泡流场采用准一维模型,数值研究了导弹水下点火初期推力峰值与燃气泡初始体积、喷管尾盖打开压强、发射深度等参数的关系.对水流场采用势流理论并通过边界元方法求解,水流场和燃气泡流场由交界面上的压力连续和速度连续条件相互耦合;利用准一维气流场模型计算得到的结果表明导弹在水下点火后瞬间所受推力将急剧增大,与利用球形气泡模型得到的结果一致.计算结果还表明推力峰值随着燃气泡初始体积的增加迅速降低,随着喷管尾盖打开压强的增加而增大,随尾盖质量的增加而增大;在一定范围内发射深度的变化对推力峰值影响较小,计算结果可为工程设计部门提供参考.     

Modeling of the oscillating field effects on the Heβ line emission in short pulse laser-produced plasmas

Strong oscillating fields may induce strong modifications of the emission spectra of ions. We discuss here the possibility of observing such effects in actual laser experiments where space- and time-integration effects can easily mask their existence. Focusing on the Al He_β transition, we first discuss the calculation of its spectral broadening in the presence of a strong laser field. Then, starting from 1D hydro-simulations of short, intense, laser pulse-produced plasmas that provide the density, temperature and laser intensity profiles as a function of time, full integrated collisional-radiative calculations of the laser field-dependent emissivity of the Al He_β line, are presented.