Properties of N=84, even-even nuclei populated in the spontaneous fission of 248Cm

Excited states in the neutron-rich, N=84 nuclei ¹³⁴Sn, ¹³⁶Te and ¹³⁸Xe, populated in the spontaneous fission of ²⁴⁸Cm, were studied to medium spins using the EUROGAM2 array. OXBASH code calculations support the experimental identification of maximum aligned configurations in these isotopes. Empirical shell model calculations agree with the proposed excitation energy of the neutron h_9/2 excitation in the ¹³²Sn region. A discrepancy between the observed and calculated excitation energy of the I^π= 12⁺ level in ¹³⁶Te indicates possible admixtures of collective excitations in this nucleus. Clear signs of collective excitations are observed in ¹³⁸Xe. Received: 10 November 1999 / Revised version: 22 December 1999     

Spectroscopy of neutron deficient 108Te

The neutron deficient nucleus ¹⁰⁸Te was studied in the ⁵⁴Fe(⁵⁸Ni,2p2n) reaction. A detector system consisting of 4 Euroball cluster detectors, a charged-particle detector ball and a 16 element neutron multiplicity filter was used to detect the emitted particles and γ rays. A new, significantly extended level scheme was constructed on the basis of γγ-coincidence relations. Spin values for the states were determined from angular distribution ratios. The experimental results are discussed in terms of the shell model. Received: 7 September 1998     

Three-valence-particle fission product 51 135Sb84

By analysis of fission product γ-ray data measured at Eurogam II using a ₂₄₈Cm source, yrast levels up to about 2 MeV in the N=84 three-particle nucleus ₁₃₅Sb have been identified. These levels are interpreted as π g^7/2ν f^7/2 ₂ and π g^7/2ν f^7/2h^9/2 states with the help of shell model calculations using empirical nucleon-nucleon interactions. Received: 30 July 1998     

Observation of superdeformed states in 88Mo

High-spin states in ⁸⁸Mo were studied using the Gammasphere germanium detector array in conjunction with the Microball CsI(Tl) charged-particle detector system. Three γ-ray cascades with dynamic moments of inertia showing similar characteristics to superdeformed rotational bands observed in the neighbouring A= 80 region have been identified and assigned to the nucleus ⁸⁸Mo. The quadrupole moment of the strongest band, deduced by the Residual Doppler Shift Method, corresponds to a quadrupole deformation of β₂≈ 0.6. This confirms the superdeformed nature of this band. The experimental data are interpreted in the framework of total routhian surface calculations. All three bands are assigned to two-quasi-particle proton configurations at superdeformed shape. Received: 20 May 1999 / Revised version: 25 August 1999     

Level structure of 99Rh at high spins

High spins states in ⁹⁹Rh were populated via the ⁶⁶Zn(³⁷Cl, 2p2n)⁹⁹Rh reaction at an incident beam energy of 130 MeV. Seventeen new transitions have been observed in the present study and the level scheme has now been extended up to a spin of J∼ 25ħ and an excitation energy of about E _x∼ 10 MeV. The observation of a positive parity E2 cascade based on the 9/2⁺ isomeric level is suggestive of collective behaviour in this nucleus up to high spins. Spherical shell model (within restricted model space) and Cranked shell model calculations were performed to obtain an insight into the observed level structure. The new collective band observed up to a spin of J∼ 25ħ is suggested to be based on (πg _9/2 ³) ⊗ (νg _7/2 ²) quasi-particle excitations. Received: 12 July 1999 / Revised version: 14 September 1999     

Quadrupole moment measurement of the highly deformed πg 9/2⊗νh 11/2 band in 130Pr

The quadrupole moment for the πg _9/2⊗νh _11/2 band in the ^130>Pr nucleus has been measured using the Doppler-shift attenuation method. A centroid shift analysis was carried out and a value of Q₀=6.1±0.4 eb, corresponding to an axial prolate deformation of β₂=0.35(3), has been determined. This is the first direct experimental confirmation of the deformation-driving character of the πg _9/2 orbital in an odd-odd nucleus in the A≃135 superdeformed region. Received: 23 April 1998     

The A = 51 mirror nuclei 51Fe and 51Mn

Eighteen previously unknown γ-ray transitions were identified in the T _z = - 1/2 nucleus ⁵¹Fe following the fusion-evaporation reaction ³²S(²⁸Si,2α1n)⁵¹Fe. The level scheme reaches the fully aligned I ^π = 27/2^- terminating state of the five holes in the f _7/2 shell. The 17/2^- state was found to be isomeric, and the lifetime was measured to be 2.87 ns. The mirror symmetry of ⁵¹Fe and ⁵¹Mn is discussed, and the level scheme of ⁵¹Fe is compared to shell-model calculations. Received: 20 July 2000 / Accepted: 1 August 2000     

Lifetimes in the ground-state band and the structure of 118Te

Lifetimes of excited states in ¹¹⁸Te have been measured using the Doppler Shift Attenuation (DSA) and Recoil Distance (RD) methods in the ¹⁰⁹Ag(¹³C, p3n) reaction at a beam energy of 54 MeV. Lifetime values of the ground-state band levels with spins I ^π = 2⁺-16⁺ have been obtained. The excitation energies and B(E2) values are interpreted in the framework of a version of IBFM ( IBM + 2qp) with the maximum boson number exceeding its standard value. A satisfactory agreement with experimental level scheme and B(E2) values for the ground-state band is achieved. Received: 7 June 2001 / Accepted: 7 February 2002     

Evidence for a proton halo in 27P through measurements of reaction cross-sections at intermediate energies

Measurements of reaction cross-sections ( σ_R's) for some proton-rich nuclei ( N = 11–15 isotones) on carbon target at intermediate energies have been performed on RIBLL of HIRFL. A larger enhancement of the σ_R for ²⁷P has been observed than for its neighboring nuclei. A large difference between the proton and neutron density distributions (proton halo) is necessary to explain the enhanced cross-section for ²⁷P within the framework of the Glauber model. Density distributions with HO-type core plus Yukawa-square tail and rms radii for ²⁷P have been deduced from the measured σ_R data for the first time, which conform the long tail in its densities as predicted by RMF calculations. Received: 23 May 2001 / Accepted: 7 November 2001     

Super-allowed α decay above doubly-magic <Superscript>100</Superscript>Sn and properties of <Superscript>104</Superscript>Te = <Superscript>100</Superscript>Sn ⊗ α

α-decay half-lives for ^{104, 105, 106}Te and ^{108, 109, 110}Xe close above the doubly-magic ¹⁰⁰Sn are calculated from systematic double-folding potentials. The derived α preformation factors are compared to results for ^{212, 213, 214}Po and ^{216, 217, 218}Rn above the doubly-magic ²⁰⁸Pb. α-decay energies of Q _α = 5.42±0.07MeV and 4.65±0.15MeV are predicted for ¹⁰⁴Te and ¹⁰⁸Xe; the corresponding half-lives are T _1/2 ≈ 5ns for ¹⁰⁴Te and of the order of 60μs for ¹⁰⁸Xe. Additionally, the properties of rotational bands in ¹⁰⁴Te are analyzed, and the first excited 2⁺ state in ¹⁰⁴Te is predicted at E _x = 650±40keV; it decays preferentially by γ emission with a reduced transition strength of 10 Weisskopf units to the ground state of ¹⁰⁴Te and with a minor branch by α emission to the ground state of ¹⁰⁰Sn.     

High-spin shell-model states near 56Ni

High-spin states of nuclei near doubly magic ⁵⁶Ni were studied with the reaction ²⁸Si(³⁶Ar,xpynzα) at 136 MeV beam energy. The Gammasphere array in conjunction with the 4π charged-particle detector array Microball and neutron detectors were used to detect γ rays in coincidence with evaporated light particles. The resulting extensive decay schemes of ⁵⁴Fe, ^54,55Co, ^56,57Ni, and ⁵⁸Cu are compared to shell model calculations in the fp shell. Received: 19 September 1998 / Revised version: 27 November 1998     

Gamma-spectroscopy of the 199At nucleus with the Recoil Filter Detector

The neutron deficient ¹⁹⁹At nucleus has been studied in the ¹⁷⁵Lu+²⁸Si reaction at E_b= 141 MeV. In order to select events of interest in the presence of the very strong background caused by fission, γ-rays have been detected in coincidence with recoiling evaporation residues. The excited states of ¹⁹⁹At observed for the first time may indicate that this nucleus is deformed. Received: 17 September 1998 / Revised version: 14 October 1998     

Is the 4.742 MeV state in 88Sr the 1− two-phonon state?

A nuclear resonance fluorescence experiment on ⁸⁸Sr has been performed with bremsstrahlung of 6.7 MeV endpoint energy. The γ-ray linear polarisation has been measured with a EUROBALL CLUSTER detector used as a Compton polarimeter. The results indicate positive parity for the J= 1 state at 4.742 MeV in ⁸⁸Sr, in contrast to the previous interpretation as a 1⁻ two-phonon (2⁺ ₁⊗ 3⁻ ₁) state and in conflict with the predictions of the quasiparticle-phonon model. On the basis of such calculations the 1⁺ state at 3.486 MeV may be considered as the 1⁺ ₁ one-phonon state and the very strong 1⁺ ₁→ 0⁺ ₁ deexcitation as proton spin-flip 2p_1/2→ 2p_3/2 transition. Received: 3 November 1999     

New insight in the level structure of <Superscript>153</Superscript>Er

The high-spin level structure of the ¹⁵³Er nucleus has been reinvestigated by in-beam γ-ray and electron spectroscopy with (¹⁴N,pxn) reaction. Excitation energies, spin and parity assignments are unambiguously established for the two lowest isomers T _1/2≃ 380 ns and T_1/2\simeq 10 ns. The characteristics of the third one (T _1/2≃ 250 ns) at 5.2 MeV are still questionable but its main decay modes are better known. An extension of the level scheme is proposed up to 8.4 MeV.Experimental results have been discussed in terms of shell model multiplets and compared with the other structures observed in N=85 neighbouring nuclei. Received: 8 November 1999 / Revised version: 13 December 1999     

On the nature of the 17 μs isomer of the <Superscript>133</Superscript>Sb valence nucleus

The decay of the 17 μs isomer of ¹³³Sb was re-investigated experimentally. It was produced by thermal neutron induced fission of ²⁴¹Pu. Its detection is based on time correlation between fission fragments selected by the LOHENGRIN spectrometer at ILL (Grenoble), and the γ-rays, and conversion electrons from the isomer. The interpretation of the level scheme is based on shell model calculations, where empirical two-body matrix elements were employed. The good agreement between theory and experiment suggests that the isomer is the 21/2⁺ member of the 2p-1h πg _7/2ν(f _7/2 h _11/2 ⁻¹) configuration. Received: 20 January 2000 / Revised version: 28 February 2000     

Configuration assignments and decay of 126La high-spin bands

High spin states of ¹²⁶La have been populated using the reaction ¹¹⁶Sn+¹⁴N at 68 MeV. γ-rays and conversion electrons were detected with the GAREL array. Multipolarities of the lowest-lying in-band dipole transitions have been determined from the deduced internal conversion coefficients. Experimental B(M1)/B(E2) ratios have been derived for the bands and compared with calculated values using the D?nau-Frauendorf geometrical model. Configurations are proposed for the bands comparing them with cranked shell model calculations and on the basis of the measured B(M1)/B(E2) ratios. The β-decay of ¹²⁶La has also been revisited. The population of the ¹²⁶Ba levels gives a probable spin value of five for the decaying high-spin ¹²⁶La state with T _1/2≈ 64 s which may indicate a signature inversion in the πh_11/2νh_11/2 band. Received: 12 October 1999     

Terminating high-spin bands in 101Rh

High spin states of ¹⁰¹Rh have been populated using the reaction ⁷⁰Zn+³⁶S at 130 MeV. γ-rays were detected with the EUROGAM2 array. New high-spin bands have been observed in this nucleus up to 45/2⁻, 57/2⁻ and 65/2⁺ states. They have been interpreted using the Nilsson-Strutinsky cranking formalism as terminating configurations. Two of the bands were observed up to the predicted terminating states which are built up from g_9/2 protons as well as d_5/2, g_7/2 and h_11/2 neutrons relative to a ⁹⁰Zr core. Received: 30 October 1998     

Identification of a high-K isomer in neutron-rich 185Ta

A t _1/2 > 1 ms, high-K isomeric state feeding a strongly coupled rotational band has been identified following the deep inelastic reaction ²³⁸ ₉₂U +¹⁸⁶ ₇₄W at 1600 MeV. Examination of γ-ray and X-ray data combined with a g-factor analysis derived from in-band branching ratios suggests the assignment of the new states to the neutron-rich nucleus ¹⁸⁵ ₇₃Ta. Received: 11 May 1999     

Lifetimes and configuration mixing in 110Cd

Lifetimes of excited states in ¹¹⁰Cd have been measured by the Doppler shift attenuation method in the reaction (α,2nγ) at E _α= 25 MeV. Lifetime values for 8 states and lifetime limits for 3 states were obtained. The band structures of ¹¹⁰Cd have been interpreted in terms of a modified version of the interacting boson model (IBM + 2 q.p.). The calculations explain well the excitation energies and electromagnetic transition probabilities up to J ^π= 16⁺, except for the 10⁺ ₁ state. The structural features are discussed in terms of collective and two quasiparticle excitations. Received: 20 March 1999 / Revised version: 28 May 1999     

New high-spin microsecond isomers in 131Sb

In this work we have identified and studied the decay of two new microsecond isomers 19/2^- and 23/2⁺ in ¹³¹Sb. This neutron-rich nucleus was produced by thermal neutron-induced fission of ²⁴¹Pu. The detection is based on time correlation between fission fragments selected by the LOHENGRIN spectrometer at ILL (Grenoble) and the γ-rays or conversion electrons from isomers. These new data on high-spin states complete the level scheme previously obtained from β-decay. A large fraction of the members of the πg _7/2ν(h _11/2 ^-1 d _3/2 ^-1) and πg _7/2νh _11/2 ^-2 multiplets are now known and were compared with a multi-particle shell model calculation. Received: 7 June 2000 / Accepted: 19 September 2000