Automatically tunable continuous-wave optical parametric oscillator for high-resolution spectroscopy and sensitive trace-gas detection

We present a high-power (2.75 W), broadly tunable (2.75–3.83 μm) continuous-wave optical parametric oscillator based on MgO-doped periodically poled lithium niobate. Automated tuning of the pump laser, etalon and crystal temperature results in a continuous wavelength coverage up to 450 cm^-1 per poling period at <5×10^-4 cm^-1 resolution. The versatility of the optical parametric oscillator as a coherent light source in trace-gas detection is demonstrated with photoacoustic and cavity ring-down spectroscopy. A 17-cm^-1-wide CO₂ spectrum at 2.8 μm and multi-component gas mixtures of methane, ethane and water in human breath were measured using photoacoustics. Methane (at 3.2 μm) and ethane (at 3.3 μm) were detected using cavity ring-down spectroscopy with detection limits of 0.16 and 0.07 parts per billion by volume, respectively. A recording of ¹²CH₄ and ¹³CH₄ isotopes of methane shows the ability to detect both species simultaneously at similar sensitivities. PACS 42.65.Yj; 42.72.Ai; 42.62.Fi     

Stable, continuously tunable operation of a diode-pumped doubly resonant optical parametric oscillator

We demonstrate, for what is the first time to our knowledge, long-term stable, continuously tunable operation of a doubly resonant optical parametric oscillator (OPO) pumped by a single-stripe diode laser without the use of an external semiconductor amplifier. The OPO is based on periodically poled lithium niobate and is pumped by a 150-mW distributed Bragg grating diode laser. 18-mW total output power is generated at 1.3- and 2.3-mum wavelengths. A cavity-length servo system allows continuous signal tuning of 17 GHz and idler tuning of 10 GHz, limited only by the range of a piezoelectric cavity mirror mount. OPO tuning is demonstrated from 1.1 to 1.4 mum and from 2.2 to 3.7 mum.     

A continuously tunable long-wavelength cw IR source for high-resolution spectroscopy and trace-gas detection

A new widely tunable source in the infrared for use in high-resolution spectroscopy and trace-gas detection is described. This spectroscopic source is based on Difference Frequency Generation (DFG) in gallium selenide (GaSe) and is continuously tunable in the 8.8–15.0 m wavelength region. Such a DFG source operates at room temperature which makes it a useful alternative to a lead-salt diode-laser- based detection system that requires cryogenic temperatures and numerous individual diode lasers.Prof. F. P. Schäfer on the occasion of his 65th birthday.     

Ultra-sensitive mid-infrared cavity leak-out spectroscopy using a cw optical parametric oscillator

We report a portable, all-solid-state, mid-infrared spectrometer for trace-gas analysis. The light source is a continuous-wave optical parametric oscillator based on PPLN and pumped by a Nd:YAG laser at 1064 nm. The generated single-frequency idler output covers the wavelength region between 2.35 and 3.75 μm. With its narrow line width, this light source is suitable for precise trace-gas analysis with very high sensitivity. Using cavity leak-out spectroscopy we achieved a minimum detectable absorption coefficient of 1.2×10^-9 /cm (integration time: 16 s), corresponding, for example, to a detection limit of 300 parts per trillion ethane. This sensitivity and the compact design make this trace-gas analyzer a promising tool for various in situ environmental and medical applications. Received: 19 September 2002 / Published online: 15 November 2002 RID="*" ID="*"Corresponding author. Fax: +49-228/733-474, E-mail: frank.kuehnemann@iap.uni-bonn.de     

A narrow-linewidth optical parametric oscillator for mid-infrared high-resolution spectroscopy

We present a narrow-linewidth, singly-resonant cw optical parametric oscillator, emitting more than 1 W in the 2.7–4.2?µm range. The OPO is pumped by a narrow linewidth (40?kHz) fibre-laser system and the signal frequency is locked to a high-finesse Fabry–Pérot cavity in order to increase the spectral resolution, thus obtaining a residual linewidth of 70?kHz for the signal. We tested the spectral performance of our OPO on several transitions in the ν₁ rovibrational band of CH₃I, measuring line intensities and showing sub-Doppler dip detection.     

Characteristics of a cw monolithic optical parametric oscillator

4 as a nonlinear crystal and obtained a pump threshold of 7 mW and an output power of 6 mW for a pump power of 40 mW. The OPO operated in a single longitudinal mode pair of a signal and an idler, over 1 h without mode hopping in the free-running condition. The signal and the idler wavelengths were tunable by 1 nm by changing the crystal temperature by 20 °C. The continuous tuning of the beat frequency between the signal and the idler was achieved by temperature tuning (slow control, 80 MHz/K) and E-field tuning (fast control, 0.75 MHz/V). We demonstrated the feasibility of frequency control by phase locking the beat frequency. The beat frequency could be successfully phase locked to a signal generated by a synthesizer through the electrooptic effect of the crystal. The phase locking could be maintained over 1 h. Received: 27 January 1998/Revised version: 9 March 1998     

High-repetition-rate ultrashort-pulse optical parametric oscillator continuously tunable from 2.8 to 6.8 mum

We describe a synchronously pumped femtosecond optical parametric oscillator based on periodically poled LiNbO(3) that is broadly tunable in the mid infrared. A transmission window of periodically poled lithium niobate beyond the conventionally accepted infrared absorption edge of 5.4 mum has been exploited to produce idler pulses that are tunable across a wavelength range of 4 mum , with milliwatt-level output powers at wavelengths as long as 6.8 mum . We also present experimental tuning results that are in good agreement with the theoretical phase matching predicted from published infrared-corrected Sellmeier equations for LiNbO(3) .     

Development of injection-seeded, pulsed optical parametric generator/oscillator systems for high-resolution spectroscopy

We report the development and application of pulsed optical parametric generator (OPG) and optical parametric oscillator (OPO) systems that are injection seeded with near-infrared distributed feedback diode lasers. The OPG is injection seeded at the idler wavelength without the use of a resonant cavity. Two counter-rotating, beta-barium-borate (β-BBO) crystals are used in the OPG. These crystals are pumped by the third harmonic, 355-nm output of an injection-seeded Nd:YAG laser. An OPO version of the system has also been developed by placing two flat mirrors around the two β-BBO crystals to form a feedback cavity at the signal wavelength. The OPO cavity length is not actively controlled. The output signal beam from the OPG or OPO is amplified using an optical parametric amplifier (OPA) stage with four β-BBO crystals. The frequency bandwidths of the signal and idler laser radiation from OPG/OPA and OPO/OPA systems have been determined to be slightly greater than 200 MHz. The temporal pulses from each system are smooth and near-Gaussian. High-resolution optical absorption measurements of acetylene (C₂H₂) were performed as another check of the frequency spectrum of the idler beam. The frequency-doubled signal output of the OPO/OPA system was used to perform high-resolution, single-photon, laser-induced fluorescence (LIF) spectroscopic studies of the (0,0) vibrational band of the A ²Σ⁺−X ²Π electronic transition of nitric oxide (NO) at low pressure. Excellent agreement was obtained between the theory and the experiment. The signal output of the OPG/OPA system was also used for sub-Doppler, two-photon LIF spectroscopic studies of the same vibration–rotation manifold of NO.This revised version was published online in August 2005 with a corrected cover date.     

Pulsed injection-seeded optical parametric oscillator with low frequency chirp for high-resolution spectroscopy

An injection-seeded optical parametric oscillator (OPO), based on periodically poled KTiOPO4 and pumped by a frequency-doubled, nanosecond-pulsed Nd:YAG laser, generates continuously tunable, single-longitudinal-mode, pulsed output at approximately 842 nm for high-resolution spectroscopy. Optical-heterodyne measurements show that the OPO frequency chirp increases linearly with detuning from the free-running (unseeded) OPO frequency and can be maintained as low as 10 MHz. Other factors affecting chirp are identified.     

Stabilized diode laser pumped, idler-resonant cw optical parametric oscillator

We present a diode laser pumped continuous wave, pump-enhanced singly-resonant optical parametric oscillator (OPO). The cavity is stabilized by a Pound?CDrever?CHall scheme using direct modulation of the diode laser. The system provides stable signal powers of up to 220?mW. The wavelength can be tuned between 1.40?C1.60???m for a ring or a linear cavity design by changing the crystal temperature. The relative fluctuations of the stabilized OPO??s wavelength are less than 10^?7 for more than one hour. Using a self-heterodyne technique, we measure a linewidth of the signal wave of 3.5?MHz.     

Mid-infrared high-resolution absorption spectroscopy by use of a semimonolithic entangled-cavity optical parametric oscillator

By recording low-pressure absorption lines of N2O around 3.9 microm, we fully qualify a pulsed entangled-cavity doubly resonant optical parametric oscillator as a power tool for high-resolution spectroscopy. This compact source runs at a high repetition rate (>10 kHz) with a low threshold of oscillation (<8 microJ), is mode-hop-free tunable over 5 cm(-1), and displays single-frequency Fourier-transformed-limited operation (linewidth <0.005 cm(-1)). A high potential for nonlinear spectroscopy is also expected given the high peak power (70 W) and the good quality (M2 < 2) of the output beam.     

Tuning characteristics of a cw dual-cavity KTP optical parametric oscillator

Received: 21 April 1997/Revised version: 15 June 1997     

Widely tunable single-frequency pulsed optical parametric oscillator

The spectral output of a nanosecond dual-cavity doubly resonant optical parametric oscillator has been investigated versus the relative length of the signal and idler cavities. Regions of stable single-frequency operation are determined by use of a type II phase-matched KTP crystal and compared with the predictions of a mode-overlap model. A wide mode-hop-free tuning range is obtained over 40 GHz, limited only by piezoelectric biases. Furthermore, discrete tuning is investigated over the full parametric gain curve. For demonstration purposes, experiments are performed in the domain that is most inclined to multifrequency emission, i.e., near degeneracy.     

Widely tunable femtosecond fiber optical parametric oscillator

The phase-matching condition in a fiber is discussed. A balance among the different orders of fiber dispersion can be found to achieve a widely tuning modulation instability gain for pumping around the normal dispersion regime. Three coupled nonlinear wave equations are used to simulate the femtosecond fiber optical parametric oscillator. The numerical results show that, through appropriate choice of dispersion, femtosecond pulses with a 180-nm tunable range can be generated when pump wavelength near a fiber’s zero-dispersion wavelength is tuned only 7 nm. Further tuning is limited by the walk-off between the pump and the signal pulses.     

Stable operation of a cw optical parametric oscillator near the signal-idler degeneracy

The frequency stability of a cw optical parametric oscillator (cw OPO) near the signal-idler degeneracy has been studied. The strong tendency of a near-degenerate OPO to mode hop has been suppressed by using a bulk Bragg grating as a spectral filter in the OPO cavity. An experimental demonstration of stable parametric oscillation in a single longitudinal mode of the OPO cavity is reported, together with the capability of tuning the signal-idler difference frequency from 1 to 4 THz. The OPO has potential use in cw terahertz generation.     

Wavelength-swept optical parametric oscillator for broadband mid-infrared spectroscopy

In this work we describe a wavelength-swept continuous-wave optical parametric oscillator (OPO) for the rapid acquisition of mid-infrared spectra spanning over hundreds of wavenumbers. Rapid tuning of a ytterbium-doped fibre pump laser resulted in the OPO idler tuning over 900 cm^?1 in 3.36 ms at a resolution of 4.5 cm^?1, within a total accessible range of 2.67 to 4.34 μm (2304–3752 cm^?1). Predictable tuning characteristics allowed simple online calibration of recorded spectra for absolute mid-infrared frequency. The system thus offers a viable approach to broadband spectral acquisition in applications requiring high-radiance illumination.     

Widely and continuously tunable optical parametric oscillator based on a cylindrical periodically poled KTiOPO(4) crystal

We report on what is to our knowledge the first realization of a quasi-phase-matched optical parametric oscillator (OPO) based on a crystal with a cylindrical shape. The main reason for interest in this device is its broad, continuous tuning. In experiments with a 1064-nm pump, the signal tuning range was equal to 525 nm (1515-2040 nm), and the corresponding idler was continuously tuned over 1340 nm (2220-3560 nm). The angular tuning was 26 degrees , with only a minor variation of the OPO threshold over the entire tuning range.     

Widely and continuously tunable optical parametric generator infrared laser

The experimental results of a high efficiency infrared laser are demonstrated on a quasi phase matched optical parametric generator in PPMgLN (5% MgO doping) pumped by a 1064 nm Nd:YAG laser. A broad continuous signal spectrum 1.56?C1.67 ??m are obtained by tuning the crystal temperature from 20°C to 200°C. When the average pump power is 1.82 W with about 70 ns pulse duration operating at a repetition rate of 10 kHz, the maximum total output power of the PPMgLN OPG is about 323.58 mW consisting of 210 mW of 1.639 ??m signal radiation and 113.58 mW of 3.02 ??m idler radiation.     

可调谐PPLN中红外光参量振荡器失调特性

 通过对晶体进行周期调谐,实现了中红外参量光输出,在此基础上研究了晶体移动、腔镜偏转等对失调特性的影响。结果表明：由于PPLN通道的小尺寸波导特性和参量振荡特性,其失调特性不同于常规激光器。PPLN晶体沿不同轴移动的功率变化曲线有不同的特点,沿x轴移动的失调容限大于沿y轴移动的失调容限;腔镜的失调容限与腔镜偏转方向有关,腔镜横向偏转的失调容限大于纵向偏转的失调容限;PPLN晶体温度和通道对失调容限几乎没有影响。     

可调谐PPLN中红外光参量振荡器失调特性

通过对晶体进行周期调谐,实现了中红外参量光输出,在此基础上研究了晶体移动、腔镜偏转等对失调特性的影响。结果表明：由于PPLN通道的小尺寸波导特性和参量振荡特性,其失调特性不同于常规激光器。PPLN晶体沿不同轴移动的功率变化曲线有不同的特点,沿x轴移动的失调容限大于沿y轴移动的失调容限;腔镜的失调容限与腔镜偏转方向有关,腔镜横向偏转的失调容限大于纵向偏转的失调容限;PPLN晶体温度和通道对失调容限几乎没有影响。