Spin correlations in nonlinear optical response: light-induced Kondo effect

We study the role of spin correlations in nonlinear absorption due to transitions from a deep impurity level to states above a Fermi sea. We demonstrate that the Hubbard repulsion between two electrons at the impurity leads to a logarithmic divergence in chi(3) at the absorption threshold. This divergence is a manifestation of the Kondo physics in the nonlinear optical response of Fermi sea systems. We also show that, for off-resonant pump excitation, the pump-probe spectrum exhibits a narrow peak below the linear absorption onset. Remarkably, the light-induced Kondo temperature, which governs the shape of the Kondo-absorption spectrum, can be tuned by varying the intensity and frequency of the pump.     

HMO in nonlinear optics

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Experimental reconstruction of nonlocal response of thermal nonlinear optical media

We study experimentally and theoretically the nonlocal response of a medium with thermal nonlinearity and show that despite its inherently infinite range it can be accurately characterized by a well-defined nonlocal response function. We retrieve the shape of this function and analyze its transformation with the change of boundaries.     

Filamentation nonlinear optics

A filamenting femtosecond laser pulse self-stabilizes the intensity fluctuation inside the filament core due to intensity clamping and generates an excellent spatial beam quality inside the core due to self-spatial filtering. The high quality of the core can be sampled by nonlinear processes. A few experimental examples are shown: self-phase modulation, four-wave mixing, third-harmonic generation and waveguide writing in glass. PACS 42.65.Jx; 52.35.Mw     

Computational chaos in nonlinear optics

A few models of nonlinear optical systems, known experimentally to possess both stable and unstable dynamical modes, are approximated by different dynamical models and integrated by different numerical methods. It is shown that the onset of instabilities and chaotic behavior in the same physical system may be dependent on the model used and on the numerical method applied. Finite order difference schemes should be applied with caution to infinite dimensional dynamical systems displaying irregular behavior.     

Phase measurements in nonlinear optics

Measurement of the phase, and not only the intensity, of the nonlinear optical response of a system is important in many applications which are reviewed here. We demonstrate and compare several techniques for direct measurement of the phase of the nonlinear susceptibilities through nonlinear interferometry. Different ways of imparting a controllable phase shift are discussed. Unless the coherence length is impractically large, the preferred method is to use a variable-pressure gas cell to control the phase difference between the input laser pulse and the nonlinear optical signal.Prof. F. P. Schäfer on the occasion of his 65th birthday.     

Oscillating solitons in nonlinear optics

Oscillating solitons are obtained in nonlinear optics. Analytical study of the variable-coefficient nonlinear Schrödinger equation, which is used to describe the soliton propagation in those systems, is carried out using the Hirota’s bilinear method. The bilinear forms and analytic soliton solutions are derived, and the relevant properties and features of oscillating solitons are illustrated. Oscillating solitons are controlled by the reciprocal of the group velocity and Kerr nonlinearity. Results of this paper will be valuable to the study of dispersion-managed optical communication system and mode-locked fibre lasers.     

Quantum fluctuations in nonlinear optics

We consider nonlinear optical devices which are excited by coherent light from a laser and in which several other waves are generated by nonlinear processes. We develop a general theory to treat the noise properties of the generated waves. In particular a probability distribution function is found which in principle can be measured experimentally. This formulation allows a thermodynamic study of phase transitions.     

基于统计光学的正负热光非定域成像

本文, 基于经典统计光学, 建立符合热光特性的统计模型, 通过数值模拟证明了吴令安和Meyers提出的图像重构算法, 并进行了定性的理论分析. 在关联成像获得的数据样本中, 根据桶探测器的光强涨落进行分组, 分别以某个阈值作为下限和上限, 再将分组后的独立样本和相应的面探测器信号进行强度关联, 则可以得到物体的正像或负像. 然而, 不经过关联运算, 直接对分组后的面探测器信号进行算数平均也可以得到物体的正像或负像, 同时成像的对比度得到较大提高. 这种分组对应的非定域成像进一步说明强度涨落在热光成像中的重要性. 最后以字符掩膜版作为成像物体, 分别运用关联成像和分组对应正负成像算法重构物体的图像, 实验结果证明这种新的正负算法可以提高非定域成像的对比度. 关键词： 统计光学 热光 关联成像 正负非定域成像     

能谷与非线性光学

能谷自由度是近年来随着新型二维量子材料的研究而兴起的新焦点,而非线性光学则是现代光学学科中的重要分支。这两个看似没有任何交集的领域由于都对物质材料的中心反演对称破缺极度敏感而密切关联。文章将以过渡金属二硫属化物的单层和少层为代表,介绍能谷自由度与非线性光学中最基本的二次谐波过程之间的关系。由此得出,非线性光学可以成为研究能谷物理的重要技术和手段。同时,过渡金属二硫属化物等能谷材料也大大丰富了非线性光学的研究对象,预期二维材料和器件可以成为非线性光学研究的新机遇和新热点。     

Anderson localization in nonlocal nonlinear media

We theoretically and numerically investigate the effect of focusing and defocusing nonlinearities on Anderson localization in highly nonlocal media. A perturbative approach is developed to solve the nonlocal nonlinear Schr?dinger equation in the presence of a random potential, showing that nonlocality stabilizes Anderson states.     

Two-dimensional stationary nonlinear surface solitons in nonlocal nonlinear media

We address two-dimensional surface solitons occurring at the interface between a semi-infinite linear medium and a semi-infinite nonlocal nonlinear medium. We find that there exist stable single and dipole surface solitons. The properties of the surface solitons can be affected by the degree of nonlocality. Interestingly, only when the degree of nonlocality is greater than a critical value, the surface solitons can exist.     

Tracking azimuthons in nonlocal nonlinear media

We study the formation of azimuthons, i.e., rotating spatial solitons, in media with nonlocal focusing nonlinearity. We show that whole families of these solutions can be found by considering internal modes of classical non-rotating stationary solutions, namely vortex solitons. This offers an exhaustive method to identify azimuthons in a given nonlocal medium. We demonstrate formation of azimuthons of different vorticities and explain their properties by considering the strongly nonlocal limit of accessible solitons.     

Periodic solitons in nonlocal nonlinear media

We identify periodic solitons in nonlocal nonlinear media: multi-hump soliton solutions propagating in a fully periodic fashion. We also demonstrate recurrences and breathers whose evolution is statistically periodic and discuss why some systems support periodic solitons while others do not.     

Polarization nonlinear optics of quadratically nonlinear azopolymers

The polarization properties of second harmonic and sum-frequency signals generated by femtosecond laser pulses in films of polymers containing covalent groups of an azobenzothiazole chromophore polarized by an external electric field are investigated. It is shown that the methods of polarization nonlinear optics make it possible to determine the structure of oriented molecular dipoles and reveal important properties of the motion of collectivized π electrons in organic molecules with strong optical nonlinearities. The polarization measurements show that the tensor of quadratic nonlinear optical susceptibility of chromophore fragments oriented by an external field in macromolecules of the noted azopolymers has a degenerate form. This is indicative of a predominantly one-dimensional character of motion of collectivized π electrons along an extended group of atoms in such molecules.     

Extreme midinfrared nonlinear optics in semiconductors

We have observed extreme nonlinear optical phenomena produced by intense midinfrared (MIR) pulses in semiconductors. These phenomena include multiple off-resonance optical sidebands (up to +/-3 MIR photons interacting with a near-infrared photon), multiple MIR harmonics (up to the seventh harmonic), and significant broadening and modification of MIR harmonic spectra. The generation of these extreme MIR nonlinear optical phenomena is primarily aided by cross-phase modulation.