声子角动量与手性声子

在经典的物理学理论中,声子广泛地被认为是线极化的、不具有角动量的.最近的理论研究发现,在具有自旋声子相互作用的磁性体系(时间反演对称性破缺)中,声子可以携带非零的角动量,在零温时声子除了具有零点能以外还带有零点角动量;非零的声子角动量将会修正通过爱因斯坦-德哈斯效应测量的回磁比.在非磁性材料中,总的声子角动量为零,但是在空间反演对称性破缺的六角晶格体系中,其倒格子空间的高对称点上声子具有角动量,并具有确定的手性;三重旋转对称操作给予声子量子化的赝角动量,赝角动量的守恒将决定电子谷间散射的选择定则;此外还理论预测了谷声子霍尔效应.     

Optical Force Sensing with Cylindrical Microcontainers

Quantitative force sensing reveals essential information for the study of biological systems. Forces on molecules, cells, and tissues uncover functioning conditions and pathways. To analyze such forces, spherical particles are trapped and controlled inside an optical tweezers (OT) trap. Although these spherical particles are well‐established sensors in biophysics, elongated probes are envisioned for remote force sensing reducing heat damage caused by OT. There is thus a growing demand for force metrology with OT using complexly shaped objects, e.g., sac‐like organelles or rod‐like bacteria. Here, the employment of Zeolite‐L crystals as cylindrical force sensing probes inside a single optical trap is investigated. It is shown that cylindrical objects can be used as force probes since existing calibration assays can be performed with suitable corrections. Forces of active driving assays are compared with passive calibration methods. Finally, the investigations are extended to direct force measurements based on momentum calibration, in which the influence of rotation due to torque in a single optical trap is unveiled. Simulations reveal the relation between torque and the position of equilibrium in the trap. The results highlight the functionality of Zeolite‐L crystals as probes for force sensing, while opening perspectives for enhanced, accurate force metrology in biophotonics.     

Dynamic optical manipulation with a higher-order fractional bessel beam generated from a spatial light modulator

Higher-order Bessel beams have been demonstrated to have the ability to trap and rotate low- and high-index particles simultaneously [Phys. Rev. A 66, 063402 (2002)]. The rotation and trapping is caused by the presence of orbital angular momentum arising from its azimuthal phase variation (that changes at integer multiples of 2pi) and the concentric rings of the Bessel mode. We demonstrate for the first time to our knowledge a branch from the family of higher-order Bessel beams that has fractional azimuthal variation at its beam axis. This new family of laser beams has the ability to perform dynamic optical manipulation with dynamic control of a spatial light modulator. Furthermore, we take the opportunity to explore the propagation characteristics of higher-order Bessel beams for which the azimuthal phase changes at noninteger multiples of 2pi.     

平板式螺旋相位板的设计与应用

传统的螺旋相位板是一种利用沿方位角方向介质材料高度递增实现对光束相位调控产生涡旋光束的光学器件,由于这种特殊的几何结构特征使其不能通过相位板的叠加而调控出射光束所携带的角量子数.本文基于坐标变换方法将介质材料沿方位角方向折射率不变而高度递增的传统螺旋相位板变换为一种介质材料沿方位角方向高度不变而折射率递增的平板式螺旋相位板.通过理论分析与数值模拟,发现本文所设计的平板式螺旋相位板不仅与传统螺旋相位板一样能够产生高质量的涡旋光束,而且平板式螺旋相位板的高度和涡旋光束携带的角量子数可以根据介质材料的折射率选取而任意调节.为了实际应用的需要,可以通过叠加多层平板式螺旋相位板以获得不同角量子数的涡旋光束.这种平板式螺旋相位板在光传输、光通信等领域具有广阔的潜在应用价值.     

碳酸钙微粒光致旋转的实验和理论研究

理论分析了由于光束轨道角动量和自旋角动量传递以及微粒的特殊形状导致微粒旋转的机理.实验建立了单光束激光光镊装置,不仅可以捕获并移动直径为微米量级的微小粒子,而且利用圆偏振光与微粒之间角动量的传递,实现了对具有双折射特性的碳酸钙微粒的光致旋转.实验中发现微粒的旋转不仅取决于光束的偏振态,还与微粒本身的形状有关,解释了实验中观察到的几种旋转现象.碳酸钙微粒旋转的最高转速达到12转/秒,转速与激光功率成正比.     

Mechanical equivalence of spin and orbital angular momentum of light: an optical spanner

We use a Laguerre-Gaussian laser mode within an optical tweezers arrangement to demonstrate the transfer of the orbital angular momentum of a laser mode to a trapped particle. The particle is optically confined in three dimensions and can be made to rotate; thus the apparatus is an optical spanner. We show that the spin angular momentum of +/-?per photon associated with circularly polarized light can add to, or subtract from, the orbital angular momentum to give a total angular momentum. The observed cancellation of the spin and orbital angular momentum shows that, as predicted, a Laguerre-Gaussian mode with an azimuthal mode index l=1 has a well-defined orbital angular momentum corresponding to ? per photon.     

Axial radiation force exerted by general non-diffracting beams

The axial radiation force exerted by a general non-diffracting beam on an object of arbitrary shape in lossless medium is analyzed. The object may be on or off the beam's axis. The analysis is based on the plane-wave representation of the beam using an azimuthal function and conical angle. The analytical expression relates the force to axial projections of the extracted and scattered momentum. Using an extended optical theorem, the extinction is related to the scattering at the forward direction of the beam's plane wave components. The axial force is expressed using the scattering amplitude and known angular functions.     

Calculation and optical measurement of laser trapping forces on non-spherical particles

Optical trapping, where microscopic particles are trapped and manipulated by light is a powerful and widespread technique, with the single-beam gradient trap (also known as optical tweezers) in use for a large number of biological and other applications. The forces and torques acting on a trapped particle result from the transfer of momentum and angular momentum from the trapping beam to the particle. Despite the apparent simplicity of a laser trap, with a single particle in a single beam, exact calculation of the optical forces and torques acting on particles is difficult. Calculations can be performed using approximate methods, but are only applicable within their ranges of validity, such as for particles much larger than, or much smaller than, the trapping wavelength, and for spherical isotropic particles. This leaves unfortunate gaps, since wavelength-scale particles are of great practical interest because they are readily and strongly trapped and are used to probe interesting microscopic and macroscopic phenomena, and non-spherical or anisotropic particles, biological, crystalline, or other, due to their frequent occurance in nature, and the possibility of rotating such objects or controlling or sensing their orientation. The systematic application of electromagnetic scattering theory can provide a general theory of laser trapping, and render results missing from existing theory. We present here calculations of force and torque on a trapped particle obtained from this theory and discuss the possible applications, including the optical measurement of the force and torque.     

Probing Dual Asymmetric Transverse Spin Angular Momentum in Tightly Focused Vector Beams in Optical Tweezers

The spin-orbit interaction (SOI) of light generated by tight focusing in optical tweezers is regularly employed in generating angular momentum - both spin and orbital - the effects being extensively observed in trapped mesoscopic particles. Specifically, the transverse spin angular momentum (TSAM), which arises due to the longitudinal component of the electromagnetic field generated by tight focusing is of special interest, both in terms of fundamental studies and associated applications. This study provides an effective and optimal strategy for generating TSAM in optical tweezers by tightly focusing first-order radially and azimuthally polarized vector beams with no intrinsic angular momentum (AM) into a refractive index stratified medium. The choice of such input fields ensures that the longitudinal spin angular momentum (LSAM) arising from the electric (magnetic) field for the radial (azimuthal) polarization is zero. As a result, the effects of the electric and magnetic TSAM are exclusively observed separately in the case of input first-order radially and azimuthally polarized vector beams on single optically trapped birefringent particles. This research opens up new and simple avenues for exotic and complex particle manipulation in optical tweezers.     

激光捕获技术及其发展

激光捕获技术是利用光辐射力来捕捉、移动和操纵微粒的先进技术。光镊即单光束梯度力光阱是通过在高度会聚的激光束束腰附近所产生的极高的场强梯度来形成皮牛顿量级的力,可以三维地捕获和操纵微小粒子。阐述了激光捕获技术的模型和原理以及系统的基本结构;追踪了激光捕获技术的最新研究进展;介绍了非高斯型光阱、光纤光阱和全息光镊等几种特殊形式,并分析了每种形式的特点。展望了激光捕获技术的发展前景。     

Spin force and torque in non-relativistic Dirac oscillator on a sphere

The spin force operator on a non-relativistic Dirac oscillator (in the non-relativistic limit the Dirac oscillator is a spin one-half 3D harmonic oscillator with strong spin–orbit interaction) is derived using the Heisenberg equations of motion and is seen to be formally similar to the force by the electromagnetic field on a moving charged particle. When confined to a sphere of radius R, it is shown that the Hamiltonian of this non-relativistic oscillator can be expressed as a mere kinetic energy operator with an anomalous part. As a result, the power by the spin force and torque operators in this case are seen to vanish. The spin force operator on the sphere is calculated explicitly and its torque is shown to be equal to the rate of change of the kinetic orbital angular momentum operator, again with an anomalous part. This, along with the conservation of the total angular momentum, suggests that the spin force exerts a spin-dependent torque on the kinetic orbital angular momentum operator in order to conserve total angular momentum. The presence of an anomalous spin part in the kinetic orbital angular momentum operator gives rise to an oscillatory behavior similar to the Zitterbewegung. It is suggested that the underlying physics that gives rise to the spin force and the Zitterbewegung is one and the same in NRDO and in systems that manifest spin Hall effect.     

非线性晶体产生的空心光束中大尺寸粒子囚禁与导引

提出了一种基于非线性ZnSe晶体产生的空心光束与光泳力的大尺寸粒子二维囚禁与一维导引、三维囚禁方案.理论上分析并计算了单个非线性ZnSe晶体产生的空心光束内粒子受到的横向与纵向光泳力,纵向光泳力的大小同粒子尺寸与光束尺寸比例的四次方成正比,与空心光束功率成正比,方向与光束传播方向一致.粒子尺寸与空心光束尺寸越接近时,横向光泳力的大小越大.结果表明该光泳力可以实现对大尺寸粒子的二维囚禁,同时可对粒子进行长距离(米量级)一维定向导引;理论上分析并计算了基于双非线性ZnSe晶体产生的局域空心光束内粒子所受横向与纵向光泳力情况,光泳力与系统参数的依赖关系与单个非线性晶体产生的空心光束中的粒子受力情况类似,不同的是该条件下纵向光泳力指向光束中心.结果表明该局域空心光束可以实现大尺寸粒子的三维有效囚禁.基于非线性ZnSe晶体产生的空心光束或者局域空心光束可以作为大尺寸粒子非接触式有效操控的工具,在现代光学以及生物医学中有潜在的应用.     

Higher-order Poincaré sphere, stokes parameters, and the angular momentum of light

A higher-order Poincaré sphere and Stokes parameter representation of the higher-order states of polarization of vector vortex beams that includes radial and azimuthal polarized cylindrical vector beams is presented. The higher-order Poincaré sphere is constructed by naturally extending the Jones vector basis of plane wave polarization in terms of optical spin angular momentum to the total optical angular momentum that includes higher dimensional orbital angular momentum. The salient properties of this representation are illustrated by its ability to describe the higher-order modes of optical fiber waveguides, more exotic vector beams, and a higher-order Pancharatnam-Berry geometric phase.     

Asymmetry in photoelectron emission from chiral molecules induced by circularly polarized light

In photoionization of free, unoriented chiral molecules with circularly polarized radiation, a significant circular dichroism, i.e., an asymmetry in the forward-backward electron emission, has been observed in the photoelectron angular distribution. This leads also to an asymmetry in the momentum transfer to the photoions. The spectra for the left- and right-handed enantiomers of bromocamphor exhibit asymmetries up to several percent which vary as a function of orbital binding energy. This enantioselective effect can similarly occur for biomolecules with handedness, like amino acids, and may thus be a contributing factor related to the origin of the terrestrial biomolecular homochirality.     

Superchiral fields generated by nanostructures and their applications for chiral sensing

Chirality is ubiquitous in natural world. Although with similar physical and chemical properties, chiral enantiomers could play different roles in biochemical processes. Discrimination of chiral enantiomers is extremely important in biochemical, analytical chemistry, and pharmaceutical industries. Conventional chiroptical spectroscopic methods are disadvantageous at a limited detection sensitivity because of the weak signals of natural chiral molecules. Recently, superchiral fields were proposed to effectively enhance the interaction between light and molecules, allowing for ultrasensitive chiral detection. Intensive theoretical and experimental works have been devoted to generation of superchiral fields based on artificial nanostructures and their application in ultrasensitive chiral sensing. In this review, we present a survey on these works. We begin with the introduction of chiral properties of electromagnetic fields. Then, the optical chirality enhancement and ultrasensitive chiral detection based on chiral and achiral nanostructures are discussed respectively. Finally, we give a short summary and a perspective for the future ultrasensitive chiral sensing.     

飞秒激光光镊横向光学力的理论分析

旨在将飞秒激光脉冲序列视为对连续光的周期抽样结果,分析飞秒激光脉冲序列作为光镊光源捕获电介质微粒时产生的横向光学力,并给出受光微粒所受横向光学势阱力的理论模型及计算公式.数值计算结果表明,飞秒激光脉冲所产生的横向光学力能抵消由于布朗运动引起的微粒中心偏移的影响,实现对微粒的稳定束缚.     

Gradient force evolution of Gaussian beam induced by a phase plate

The evolution of gradient force pattern induced by an annular phase distribution plate is numerically investigated in this paper. The phase plate, which may alter the wavefront phase of incident Gaussian beam with tunable topological charge, consists of two concentric portions, one center circle portion and one annular portion. Numerical simulations show that the proposed plate can induce the tunable gradient force on the particles in the focal region. By adjusting the geometrical parameters or changing the topological charge of the phase-shifting plate, some novel trap patterns may occur, such as triangle shape trap, quadrangle shape trap, pentagon shape trap, hexagon shape trap, and the shapes of optical traps change very considerably. Therefore, the phase plate may be very advantageous for constructing tunable optical traps. The method is more versatile in that it allows precise control of the parameters and has the possibility of generating specific patterns of optical vortices. The gradient force pattern focal of intensity distribution depends on both the annular width and the topological charge.     

Observation of lasing mediated by collective atomic recoil

We observe the buildup of a frequency-shifted reverse light field in a unidirectionally pumped high-Q optical ring cavity serving as a dipole trap for cold atoms. This effect is enhanced and a steady state is reached, if via an optical molasses an additional friction force is applied to the atoms. We observe the displacement of the atoms accelerated by momentum transfer in the backscattering process and interpret our observations in terms of the collective atomic recoil laser. Numerical simulations are in good agreement with the experimental results.     

Perturbative chiral nucleon-nucleon potential for the 3P0 partial wave

We study perturbativeness of chiral nuclear forces in the ³P₀ channel. In previous works, the focus has been on the one-pion exchange, and the applicable window of perturbative pion exchanges has been shown to span from the threshold to center-of-mass momentum k≃180 MeV. We will examine, instead, whether the cancellation of short- and long-range parts can sufficiently soften the ³P₀ chiral force to make it more amenable to perturbation theory. The result is encouraging, as the combined ³P₀ force is shown to be perturbative up to k≃280 MeV, covering many nuclear-structure calculations.     

Reverse orbiting of microparticles in optical vortices

We report the observation of particles trapped at an air-water surface orbiting in a reverse direction with respect to the orbital angular momentum of the light field. The effect is explained by a combination of asymmetric particle shape and confinement of the particle on the 2D air-water interface. The experiment highlights the strong influence of the particle shape on the momentum transfer, an effect that is often not considered in optical trapping experiments.