铁电体中极化长程涨落的光子关联谱实验研究

从极化团簇的随机涨落出发, 利用维纳过程模型, 推导了铁电体中极化长程涨落的弛豫规律以及光强自相关函数所可能的表现形式. 阐述了微观极化团簇的弛豫过程与宏观测量弛豫规律之间的联系. 通过对原有氦氖激光光子关联谱实验装置进行改进, 观测了BaTiO₃和0.71Pb(Mg_1/3Nb_2/3)O₃-0.29PbTiO₃单晶中极化团簇长程涨落在居里点和立方到四方相变点附近的弛豫过程. 在BaTiO₃中发现极化团簇长程涨落在居里点之上4 K存在双弛豫现象, 此现象与其有序无序相变机理相联系. 在Pb(Mg_1/3Nb_2/3)O₃-0.29PbTiO₃中发现极化团簇长程涨落在相变点两侧都存在双弛豫现象. 利用推导的理论结果很好地拟合了实验结果并提取了极化团簇长程涨落的弛豫时间. 两种样品中极化团簇长程涨落的弛豫时间都在相变点出现突变, 并呈现临界慢化现象.     

准晶

一、什么是准晶及准晶的发现过去人们一直把固态物质划分为晶体(crystal)和无序体(amorphous)。晶体在短程和长程上都是有序的,突出的特点是组成晶体的原子或离子在空间排列的点阵具有周期性,即长程平移序。无序体具有短程有序,但在长程上无序,即它的点阵在空间长程范     

半导体电子态理论简介(Ⅲ)

四、非晶态半导体 非晶态半导体属于无序系统的物质.无序系统包括固溶体、非晶体、准晶体等,它们都不存在晶体的平移对称性.固溶体的特点是结构有序、组分无序.非晶体的特点是短程有序,长程(结构)无序.准晶体的特点是短程有序,长程部分有序,有点群对称性但无平移对称性、无序的分布都是随机的.与有序系统相比,无序系统有一些新的特点,例如局域化. 关于局域化问题,常用紧束缚方法来讨论,哈密顿量其中　　是原子态　的能量,V是原子间的相互作用能量.对于晶体,　　是常数.如果晶体是三维简单立方,则它的能带(取　　=0)为态密度如图 11(a)所示,…     

混合交通流时间序列的去趋势波动分析

应用去趋势波动分析法研究交通流时间序列的复杂性,探讨了混合交通流时间序列演变行为的标度指数.根据标度指数的变化特征,进而揭示交通流时间序列所具有的长程相关性和短程相关性.通过分析发现,存在一密度ρ,当ρ₁<ρ<ρ₂时,交通流时间序列具有长程相关性;而当ρ<ρ₁或ρ>ρ₂时,交通流时间序列具有短程相关性,即密度的变化影响着标度指数的变化.另外分析了在不同慢车比率条件下时间序列的标度指数,发现慢车比率的变化 关键词： 混合交通流 去趋势波动分析 时间序列 长程相关     

高熵合金短程有序现象的预测及其对结构的电子、磁性、力学性质的影响

如何有效预测高熵合金的稳态结构,是开展研究其物理及化学等性能的基础.以FeCuCrMnMo合金为例,在有限晶胞尺寸内,采用蒙特卡洛结合密度泛函理论杂化计算方法(Monte Carlo/density functional theory,MC/DFT)预测高熵合金的平衡态结构.与准随机近似方法(special quasirandom structures,SQS)不同,该方法不再追求高熵合金结构的理想随机状态,而是充分考虑合金中原子尺寸、混合焓、原子间相互作用等物理因素.通过第一性原理计算体系能量来实现,使得蒙特卡洛(Monte Carlo,MC)方法保证结构在原子交换过程中体系能量逐渐收敛于平衡态.最终预测得到的平衡态结构出现Cu原子的短程有序现象(short range order,SRO)与实验上合金中的Cu偏析现象相一致.相较于由SQS方法获得的随机状态,该SRO结构在能量上更加稳定.同时本文对稳态结构通过序参数及径向分布函数进行表征,并对SRO现象的出现进行物理解释,进一步揭示了SRO的出现对高熵合金结构性质的影响.     

钴镍铁基金属玻璃结构弛豫的X射线研究

本工作在测定了Co_50.7Ni_19.5Fe_7.8Si₆B₁₆和Co_42.9Ni_27.3Fe_7.8Si₈B₁₄两种金属玻璃结构的基础上,进一步研究了不同保温时间的等温退火和不同温度下的等时退火对它们结构的影响,并测定了各退火态样品的小角度X射线散射强度,对其变化作了比较,分析了它们的结构弛豫现象。实验结果表明:结构弛豫可分为两种不同的类型,即拓扑短程序(TSRO)和化学短程序(CSRO)弛豫过程。本工作特别对后一种过程提供了直接的证据。最后还对这两种弛豫的原子过程作了初步的分析,强调了它们的并存和相关性。 关键词：     

弛豫铁电体队Pb(Mg,Nb)O_3系统中有序畴的生长模型

本文基于有序-无序相变模型,从热力学上给出在的Pb(Mg,Nb)O_3系统中的有序态,同时得到了长程序参量与B位离子组份的关系曲线,并在此基础上,利用电荷平衡条件,在二维平面上和三维空间里分别提出了有序畴的生长模型。计算结果与实验结果基本符合。     

极端事件再现时间长程相关性与群发性研究

利用百分位阈值方法定义极端事件,从极端事件再现时间的角度,研究了极端事件发生时间间隔的长程相关性.发现若原时间序列具有长程相关性,则它的极端事件再现时间序列也具有长程相关性,计算表明两者的标度指数α相当接近,这一特性与随机产生的再现时间序列有着本质的差别,再现时间序列的长程相关性是由原序列的长程相关性决定的.具有长程相关性的时间序列再现时间的概率分布明显不同于随机序列,其小值再现时间的概率较大,反映出极端事件的群发现象.本文根据这一特征定义了再现时间的群发性指数,发现时间序列的长程相关性是导     

弛豫铁电体队Pb(Mg,Nb)O3系统中有序畴的生长模型

本文基于有序-无序相变模型,从热力学上给出在的Pb(Mg,Nb)O₃系统中的有序态,同时得到了长程序参量与B位离子组份的关系曲线,并在此基础上,利用电荷平衡条件,在二维平面上和三维空间里分别提出了有序畴的生长模型。计算结果与实验结果基本符合。 关键词：     

面心立方(001)方向AB合金薄膜表面层的有序无序相变

采用平均场近似方法对两组元面心立方合金薄膜的有序无序相转变过程进行模拟计算,结果表明,合金薄膜的有序无序相变受薄膜层数奇偶性的影响.薄膜层数奇偶性不同,会导致薄膜具有不同的相结构和热力学性质.在弱表面偏析作用下,对于偶数层薄膜,由于薄膜边界对称性破缺,对应体组分x=0.5的化学势区间,偶数层薄膜有序无序相变过程中出现了中间温度相和浸润现象.而奇数层薄膜的有序无序相变类似体材料的相变.在强表面偏析作用下,由于受表面偏析作用和有限尺寸效应影响,对应体组分x=0.5的化学势区间,奇数层薄膜中出现AB(AB)nA相,它不存在严格热力学意义上的有序无序相变.     

计算机网络的长程相关特性

针对一种计算机网络模型，利用节点排队长度累计量的均方涨落函数，研究了网络节点在时间上的长程相关特性.结果表明，随着负载的增加，网络节点数据包排队长度在时间上由自由流状态的不相关或短程相关逐渐演变为临界和拥塞时的长程相关，关联范围逐渐增大，长程关联特性开始显现.在自由流状态时，节点的不相关或短程相关，并且有一致的数值为0.5的幂指数这一典型特征.而在临界状态时，节点数据包排队长度长程相关，有大于0.5的幂指数为特征.并且随网络规模的增大，节点间的群体作用逐渐显著，幂指数呈下降趋势. 关键词： 计算机网络 相变 长程相关 幂律     

Geometry effect on the magnetic ordering of geometrically frustrated rectangular and triangular magnets

We investigate the effect of geometry on the ground-state ordering of artificially frustrated magnetic rectangular and triangular lattices by Monte Carlo method. By varying the vertical lattice spacing while keeping the horizontal one fixed, we show that when the ratio of vertical to horizontal lattice spacing, labeled by η, is less than 1.82, the ground state of the rectangular lattice presents long-range antiferromagnetic order and for η?1.82 the ground state changes to long-range mixed ferromagnetic and antiferromagnetic order. For the frustrated triangular lattice, the short-range ordered state as well as two long-range ordered ground states occurs transiently at η=0.87 and 2, where the energies of the two ground states with long-range order are approximately equal. In addition, the level of frustration of both frustrated lattices is found to be largely relevant to the ratio η.     

Equilibrium properties of classical systems with long-range forces. BBGKY equation,neutrality, screening,and sum rules

We introduce a generalization of the BBGKY equation to define the equilibrium states for systems with long-range forces and study the properties of such states. We show that there are properties typical of short-range forces (shape independence, normal fluctuations, asymptotic behavior of correlation functions) and others which are typical of long-range forces (possible shape dependence, neutrality, sum rules and screening, abnormal fluctuations, boundedness of the internal electric field). If the force decreases at infinity faster than the Coulomb force, the properties will be those typical of short-range forces; on the other hand, if the force decreases at infinity as the Coulomb force or slower, the properties will be those typical of long-range forces.     

Photoinduced melting of antiferromagnetic order in La(0.5)Sr(1.5)MnO4 measured using ultrafast resonant soft x-ray diffraction

We used ultrafast resonant soft x-ray diffraction to probe the picosecond dynamics of spin and orbital order in La(0.5)Sr(1.5)MnO(4) after photoexcitation with a femtosecond pulse of 1.5 eV radiation. Complete melting of antiferromagnetic spin order is evidenced by the disappearance of a (1/4,1/4,1/2) diffraction peak. On the other hand, the (1/4,1/4,0) diffraction peak, reflecting orbital order, is only partially reduced. We interpret the results as evidence of destabilization in the short-range exchange pattern with no significant relaxation of the long-range Jahn-Teller distortions. Cluster calculations are used to analyze different possible magnetically ordered states in the long-lived metastable phase. Nonthermal coupling between light and magnetism emerges as a primary aspect of photoinduced phase transitions in manganites.     

Spin waves and phase transition on a magnetically frustrated square lattice with long-range interactions

We investigate the effects of long-range interactions on the spin wave spectra and the competition between magnetic phases on a frustrated square lattice with large spin S. Applying the spin wave theory and assisted with symmetry analysis, we obtain analytical expressions for spin wave spectra of competing Neel and (π, 0) stripe states of systems containing any-order long-range interactions. In the specific case of long-range interactions with power-law decay, we find surprisingly that the staggered long-range interaction suppresses quantum fluctuation and enlarges the ordered moment, especially in the Neel state, and thus extends its phase boundary to the stripe state. Our findings illustrate the rich possibilities of the roles of long-range interactions, and advocate future investigations in other magnetic systems with different structures of interactions.     

RHIC和LHC能区两粒子关联函数研究

应用多源热模型研究了相对论性重离子对撞机（RHIC）上PHENIX合作组测得的每核子对质心能量√sNN=200 GeV的氘-金（d+Au）碰撞中快度长程方位角关联,和大型强子对撞机（LHC）上CMS合作组测得的质心能量√s=0.9,2.36,7 TeV的质子质子（p+p）碰撞中高多重数短程赝快度关联,在误差范围内模型结果很好地重现了实验数据。用4个参数分析了长程方位角关联,结果表明,参数可以清楚地显示出脊结构的变化趋势,说明脊结构与集体效应、流体力学流效应、粒子对的横动量及信号等有关。用3个参数分析了小系统高多重数短程赝快度关联,结果表明,参数σ和c₃与能量相关,能量越大,两粒子越靠近,关联越强。The multi-source thermal model is used in this paper to analyze the long-range azimuth correlation in deutron-gold (d+Au) collisions at center-of-mass energy per nucleon pair √sNN=200 GeV measured by the PHENIX Collaboration at the relativistic heavy ion collider (RHIC), and the short-range pseudorapidity correlation in high multiplicity event in proton-proton (p+p) collisions at center-of-mass energy √s=0.9, 2.36, 7 TeV measured by the CMS Collaboration at the large hadron collider (LHC). The modeling results are in approximately agreement with the experimental data in error ranges. Four parameters are used in the analysis of long-range azimuth correlation, which show that the parameters describe the change trend of ridge structure. The ridge structure is related to the collective effect, hydrodynamic flow effect, transverse momentum and signal of particle pair, and so forth. Three parameters are used in the analysis of the short-range pseudorapidity correlation in high multiplicity event in small system, which show that the parameters σ and c3 are related to collision energy. Large collision energy results in strong correlation due to close distance between particles.     

Orientational correlations and order in A3C60

A tight-binding method which has been previously applied to study the effect of uncorrelated orientational disorder on conduction-band properties is extended here to the case of systems with long-range order and/or short-range correlations. The density of states and conductivity are not highly sensitive to the specific short-range correlations, so long as the system is not too close to being fully ordered. Hence the strong effects of disorder found previously appear to be robust and should play an important role in the interpretation of normal-state properties of A₃C₆₀.     

CO和K在Fe(110)面共吸附的高分辨电子能量损失谱研究

本工作用高分辨电子能量损失谱(HREELS)对Fe(110)面CO和K的共吸附进行了研究,发现存在三种CO吸附状态,表现为不同的C—O振动频率,当θ_k=0.03时,存在与K近程、中程和远程三种不同相互作用的CO,当θ_k=0.06时,与K远程作用的CO吸附状态消失,近程作用的CO占据主要地位,所有CO的C—O振动频率均随CO暴露量的增加向高波数方向移动,随着表面K的增多,CO—Fe振动损失峰消失。 关键词：