Appraisal of radioactivity and associated radiation hazards in sand samples of four rivers of Punjab province,Pakistan

Natural and anthropogenic radioactivity of sand and water samples collected from the four big rivers of Punjab province, Pakistan, was measured using a high-purity germanium detector coupled with a high resolution multichannel analyser. The average concentration of the naturally occurring radionuclides ²²⁶Ra, ²³²Th and ⁴⁰K in all the sand samples from the rivers Jhelum, Chenab, Ravi and Indus was found to be 22±0.6, 36±1 and 287±10 Bq?kg ^?1, respectively, while the concentration of the anthropogenic radionuclide ¹³⁷Cs was found to be below the minimum detectable activity, i.e. ～ 1.2 Bq?kg ^?1. All the sand samples have Ra_eq concentrations lower than the limit of 370 Bq?kg ^?1. Indoor (H _in) and outdoor (H _out) radiation hazard indices were calculated for the samples to assess the radiation hazards arising due to the use of this sand in construction, and were found to be less than unity in the study area. Calculated values of the absorbed dose rate were less than the typical world average value of 59 nGy?h ^?1, and the annual effective dose rate was also less than the typical world value of 70 μSv, except in the Indus river, in which it is slightly higher then the world average. Results show that the measured values are comparable with other global radioactivity measurements. None of the studied riverbeds was considered a radiological hazard, and their sand can be safely used in construction.     

Estimation of cosmic radiation doses in Punjab,Pakistan

Cosmic radiation is one of the most important sources of human exposure to natural radiation. Data regarding the level of cosmic radiation in different areas of Pakistan are lacking. The aim of the present study was therefore to estimate the annual outdoor effective doses from cosmic radiation in the Punjab province of Pakistan. The Punjab province is located between geodetic latitudes 28° and 34° N, and longitudes 69° and 75° E. The mean value of the outdoor annual effective dose was found to be 333 μ Sv, which generates a radiation dose of 0.33 mSv y^?1 per caput. This is 87% of radiation dose received by the population in the region from terrestrial sources reported elsewhere. The results of this study will contribute to regional as well as world data regarding the exposure of the population to cosmic radiation.     

Natural radioactivity and associated radiation hazards in building materials used in Peloponnese,Greece

Five different kinds of building materials (Pozzolanic and Portland cements, limestone, white cement, marble powder and sand) commonly used in building construction in Peloponnese, Greece, and Portland cement's raw materials were analyzed for their natural radioactivity content, using $\gamma$-ray spectrometry. Pozzolanic and Portland cement (Cem II) samples were found to contain the highest average ²²⁶Ra, ²³²Th and ⁴⁰K activity concentrations compared with the other examined building material samples. This could be attributed to their containing fly ash, which was found to contain high natural radionuclide concentrations, especially that of ²²⁶Ra $(1041\mathrm{Bq}{\mathrm{kg}}^{-1})$. Results obtained were compared with the results reported by other Greek researchers and the worldwide values for building materials and soil. The calculated activity concentration index $(I)$ values for all the examined building material samples were lower than the recommended exception limits for exposure to external $\gamma$-radiation.     

Natural radioactivity and radiation hazards assessment of soil samples from the area of Tuzla and Lukavac,Bosnia and Herzegovina

The results of activity concentration measurements of natural occurring radioactive nuclides ²³⁸U, ²³⁵U, ²³²Th, ²²⁶Ra, and ⁴⁰K in surface soil samples collected in the area of cities Tuzla and Lukavac, northeast region of Bosnia and Herzegovina were presented. Soil sampling was conducted at the localities that are situated in the vicinity of industrial zones of these cities. The measured activity was in the range from (8?±?4) to (95?±?28) Bq kg^–1 for ²³⁸U, from (0.41?±?0.06) to (4.6?±?0.7) Bq kg^–1 for ²³⁵U, from (7?±?1) to (66?±?7) Bq kg^–1 for ²³²Th, from (6?±?1) to (55?±?6) Bq kg^–1 for ²²⁶Ra, and from (83?±?12) to (546?±?55) Bq kg^–1 for ⁴⁰K. In order to evaluate the radiological hazard of the natural radioactivity for people living near industrial zones, the absorbed dose rate, the annual effective dose and the radium equivalent activity have been calculated and compared with the internationally approved values.     

Measurement of natural radioactivity in Jordanian sand

Sand samples were collected from Adasiah (near Amman), Jerash and Ghor As-Safi (near Karak). ²²⁶Ra, ²³²Th and ⁴⁰K activities, present in these samples, were measured using a gamma ray spectroscopy technique. The average values of the radium equivalent activities were calculated and were found to be 41.06 Bq kg⁻¹, 54.7 Bq kg⁻¹ and 85.53 Bq kg⁻¹ in samples collected from Adasiah, Jerash and Ghor As-Safi, respectively. These values are within the limit (i.e. less than 370 Bq kg⁻¹) recommended for the safe use of construction materials for dwellingsby OECD.     

Natural radioactivity levels and associated health hazards from the terrestrial ecosystem in Rosetta branch of the River Nile,Egypt

Twenty soil and 25 sediment samples were collected from the banks and bottom of the River Nile in the surroundings of biggest cities located close to it. Natural radioactivity concentrations of ²²⁶Ra, ²³²Th and ⁴⁰K have been evaluated for all samples by means of γ spectrometric analysis. The radioactivity levels of soil and sediment samples fall within the internationally recommended values. Nevertheless, high natural background radiation zones are detected in the Kafr El-Zayat region due to the presence of a fertilizer factory, and in the Rosetta region due to the presence of black sand deposits. The absorbed dose rate, the γ index and excess life time cancer risk are calculated. High values for some of the radiation health parameters are detected in the Kafr El-Zayat and Rosetta regions representing a serious problem to public health because the soil and sediment are used as constructing material for buildings. Furthermore, the isotope analysis of uranium for representative collected sediment samples via α spectrometry showed average specific activities of 18.7?±?3.6, 0.087?±?0.0038 and 18.6?±?3.8 Bq kg^–1 for ²³⁴U, ²³⁵U and ²³⁸U, respectively. In general, these values confirm the balance in the isotopic abundance of U isotopes.     

Transfer of radioactivity from soil to vegetation in Rechna Doab,Pakistan

In Rechna Doab, samples of the most common vegetation, perennial grass Desmostachya bipinnata (dab), were collected along with soil samples from 29 sites. Natural radioactivity of ²²⁶Ra, ²³²Th/²²⁸Ac and ⁴⁰K was measured by using high purity germanium-based gamma ray spectrometer. Activity concentration levels of ²²⁶Ra, ²³²Th/²²⁸Ac and ⁴⁰K in soil were found to be 46.8±6.2 (36.0–57.6), 61.4±5.9 (48.2–73.2) and 644.8±73.9 (537.7–868.4) Bq kg^?1 (dry mass), respectively, and those in vegetation were 2.74±1.70 (1.00–6.39), 2.24±0.59 (1.56–2.61) and 172.72±113.37 (53.14–469.24) Bq kg^?1 (dry mass), respectively. The measured values of the activity concentration in vegetation are comparable with some other international data. Calculated soil to vegetation transfer factors of ²²⁶Ra, ²²⁸Ac and ⁴⁰K were 0.06±0.03 (0.02–0.14), 0.04±0.01 (0.03–0.04) and 0.26±0.16 (0.09–0.69). The mean outdoor absorbed dose rate in air for the area under study was determined as 8.22 nGy h^?1 and the mean indoor absorbed dose rate in air was 11.52 nGy h^?1. The total annual effective dose to the general public from the vegetation was found to be (0.02–0.16) mSv, which is below the recommended limit value of 1 mSv y^?1 for the general public. The dab vegetation under study was found to be radiologically safe for the population and environment.     

Transfer of radioactivity from soil to vegetation in Rechna Doab, Pakistan

In Rechna Doab, samples of the most common vegetation, perennial grass Desmostachya bipinnata (dab), were collected along with soil samples from 29 sites. Natural radioactivity of 22?Ra, 232Th/22?Ac and ??K was measured by using high purity germanium-based gamma ray spectrometer. Activity concentration levels of 22?Ra, 232Th/22?Ac and ??K in soil were found to be 46.8 ± 6.2 (36.0-57.6), 61.4 ± 5.9 (48.2-73.2) and 644.8 ± 73.9 (537.7-868.4) Bq kg?1 (dry mass), respectively, and those in vegetation were 2.74 ± 1.70 (1.00-6.39), 2.24 ± 0.59 (1.56-2.61) and 172.72±113.37 (53.14-469.24) Bq kg?1 (dry mass), respectively. The measured values of the activity concentration in vegetation are comparable with some other international data. Calculated soil to vegetation transfer factors of 22?Ra, 22?Ac and ??K were 0.06 ± 0.03 (0.02-0.14), 0.04 ± 0.01 (0.03-0.04) and 0.26 ± 0.16 (0.09-0.69). The mean outdoor absorbed dose rate in air for the area under study was determined as 8.22 nGy h?1 and the mean indoor absorbed dose rate in air was 11.52 nGy h?1. The total annual effective dose to the general public from the vegetation was found to be (0.02-0.16) mSv, which is below the recommended limit value of 1 mSv y?1 for the general public. The dab vegetation under study was found to be radiologically safe for the population and environment.     

The determination of concentrations of radioisotopes in some granite samples in Turkey and their radiation hazards

The primordial radionuclides activity concentrations (²²⁶Ra, ⁴⁰K and ²³²Th) are measured in some granite samples in this study. The collected granite materials are analyzed with NaI(Tl) gamma-ray spectrometry. The specific activity of ²²⁶Ra, ²³²Th and ⁴⁰K values are in range 2.60?±?0.10 to 178.9?±?0.6?Bq?kg^?1, 1.46?±?0.10 to 162.50?±?0.75?Bq?kg^?1 and 19.8?±?0.3 to 579.7?±?2.8?Bq?kg^?1 respectively. The radium’s equivalent activity, annual effective dose, absorbed dose rate, hazard index, radioactivity level index, activity utilization’s index and exposure rate are calculated for determination of radiological risk. The concentration of ²²⁶Ra (in the 71.4% of samples), ²³²Th (in the 71.4% of samples) and ⁴⁰K (in the 14.3% of samples) in the granite samples are higher than average radioactivity concentrations of this radio-isotopes defined by ICRP (35.0, 30.0 and 400.0?Bq?kg^?1, respectively).     

Essay review - Nuclear radiation,radioactivity and safety

Review of Practical Applications of Radioactivity and Nuclear Radiations . By G.C. LOWENTHAL and P.L. AIREY. (Cambridge University Press, 2001). Pp. xvii+337. £65.00, US $95.00 (hbk). ISBN 0 521 55305 9. Scope: textbook. Level: specialist and non-specialist.     

238U and total radioactivity in drinking waters in Van province,Turkey

As part of the national survey to evaluate natural radioactivity in the environment, concentration levels of total radioactivity and natural uranium have been analysed in drinking water samples. A survey to study natural radioactivity in drinking waters was carried out in the Van province, East Turkey. Twenty-three samples of drinking water were collected in the Van province and analysed for total α, total β and ²³⁸U activity. The total α and total β activities were counted by using the α/β counter of the multi-detector low background system (PIC MPC-9604), and the ²³⁸U concentrations were determined by inductively coupled plasma-mass spectrometry (Thermo Scientific Element 2). The samples were categorised according to origin: tap, spring or mineral supply. The activity concentrations for total α were found to range from 0.002 to 0.030 Bq L^?1 and for total β from 0.023 to 1.351 Bq L^?1. Uranium concentrations ranging from 0.562 to 14.710 μg L^?1 were observed in drinking waters. Following the World Health Organisation rules, all investigated waters can be used as drinking water.     

Uranium analysis in some food samples collected from Bathinda area of Punjab, India

To strengthen the radiation protection infrastructure in Bathinda, the uranium concentration in daily diet of the residents has been measured and its associated radiation risks were estimated for the adult population. Food samples were collected from major cancer prone areas of the district, from which daily diets were prepared. These diet samples were analyzed using fission track technique. The measured values of the uranium content were found to vary from 0.38 mBq/g in mustard seeds to 4.60 mBq/g in wheat. In case of milk the uranium content is found to vary from 28.57–213.36 mBq/ℓ with mean concentration of 61.35 mBq/ℓ. This leads to a daily dietary intake of 0.90 Bq/day. The measured value of 0.90 Bq d⁻¹, contributes to 1.12 mSv to the cumulative effective dose to the population. This dose is much large than the International Commission for Radiological Protection (ICRP) annual effective dose limit of 1 mSv for the general public [1]. Therefore, it would pose significant health hazard.      

Health and ecological hazards due to natural radioactivity in soil from mining areas of Nasarawa State,Nigeria

Nasarawa State is located in north central Nigeria and it is known as Nigeria's home of solid minerals. It is endowed with barite, copper, zinc, tantalite and granite. Continuous releases of mining waste and tailings into the biosphere may result in a build-up of radionuclides in air, water and soil. This work therefore aims to measure the activity concentration levels of primordial radionuclides in the soil/sediment samples collected from selected mines of the mining areas of Nasarawa State. The paper also assesses the radiological and radio ecological impacts of mining activities on the residents of mining areas and their environment. The activity concentrations of primordial radionuclides (²²⁶Ra, ²³²Th and ⁴⁰K) in the surface soils/sediment samples were determined using sodium iodide-thallium gamma spectroscopy. Seven major mines were considered with 21 samples taken from each of the mines for radiochemistry analysis. The human health hazard assessment was conducted using regulatory methodologies set by the United Nations Scientific Committee on the Effects of Atomic Radiation, while the radio ecological impact assessment was conducted using the ERICA tool v. 1.2. The result shows that the activity concentrations of ⁴⁰K in the water ways of the Akiri copper and the Azara barite mines are 60 and 67?% higher than the world average value for ⁴⁰K, respectively. In all mines, the annual effective dose rates (mSv y^?1) were less than unity, and a maximum annual gonadal dose of 0.58 mSv y^?1 is received at the Akiri copper mine, which is almost twice the world average value for gonadal dose. The external hazard indices for all the mines were less than unity. Our results also show that mollusc-gastropod, insect larvae, mollusc-bivalve and zooplankton are the freshwater biotas with the highest dose rates ranging from 5 to 7 µGy h^?1. These higher dose rates could be associated with zinc and copper mining at Abuni and Akiri, respectively. The most exposed terrestrial reference organisms are lichen and bryophytes. In all cases, the radio ecological risks are not likely to be discernible. This paper presents a pioneer data for ecological risk from ionizing contaminants due to mining activity in Nasarawa State, Nigeria. Its methodology could be adopted for future work on radioecology of mining.     

Radon exhalation rate in Chhatrapur beach sand samples of high background radiation area and estimation of its radiological implications

Chhatrapur beach placer deposit, situated in a part of the eastern coast of Orissa, is a newly discovered high natural background radiation area (HBRA) in India. The sand samples containing heavy minerals, were collected from Chhatrapur region by the grab sampling method at an interval of ∼1 Km. Radon exhalation rates were measured by “Sealed Can Technique” using LR-115 type type II in the sand samples containing heavy minerals collected from the beach. Radon activity is found to vary from 1177.1 to 4551.4 Bq m-3 whereas the radon exhalation rate varies from 423.2 to 1636.3 mBq m⁻²h⁻¹ with an average value of 763.9 mBq m⁻²h⁻¹. Effective dose equivalent in sand samples estimated from exhalation rate varies from 49.9 to 193.0 μSv y⁻¹ with an average value of 90.1 μSv y⁻¹. From the activity concentration of ²³⁸U, ²³²Th and ⁴⁰K computed radium equivalent is found to vary from 864.0 to 11471.5 Bq kg⁻¹ with an average value of 3729.0 Bq kg⁻¹. External hazard index, H_ex range from 2.3 to 31.0 with a mean value of 10.1, which is quite high. This value supports the conclusion based on high mean absorbed gamma dose rate in air due to the naturally occurring radionuclides as 1627.5 nGy h⁻¹. A positive correlation has been found between U concentration and radon exhalation rate in the sand samples. The use of sand as construction material may pose a radiation risk to ambient environment.      

Measurement of radionuclides and absorbed dose rates in soil samples of Peshawar, Pakistan, using gamma ray spectrometry

The analysis of gamma-emitting radionuclides in nature, i.e. (226)Ra, (232)Th, (40)K and (137)Cs, has been carried out in soil samples collected from Peshawar University Campus and surrounding areas using a high purity germanium detector coupled with a computer-based high-resolution multichannel analyser. The activity concentrations in soil ranged from 30.20±0.65 to 61.90±0.95, 50.10±0.54 to 102.80±1.04, 373.60±4.56 to 1082±11.38 and 9.50±0.11 to 46.60±0.42?Bq?kg(-1) for (226)Ra, (232)Th, (40)K and (137)Cs, with a mean value of 45±7.70, 67±12.50, 878±180 and 19±9.20?Bq?kg(-1), respectively. The radium equivalent activity, internal and external hazard indices have mean values of 203.40±29.40?Bq?kg(-1), 0.56 and 0.68, respectively. The mean values of outdoor and indoor absorbed dose rates in air and the annual effective dose equivalents were found to be 106.50 and 128?nGy?h(-1) and 0.19 and 0.54?mSv?y(-1), respectively. In the present study, (40)K was the major radionuclide present in soil samples. The presence of (137)Cs indicates that this area also received some fallout from the nuclear accident of the Chernobyl power plant in 1986. The activity concentrations of radionuclides found in soil samples during the current investigation were nominal. Therefore, they are not associated with any potential source of health hazard to the public.     

Measurement of radionuclides and absorbed dose rates in soil samples of Peshawar,Pakistan, using gamma ray spectrometry

The analysis of gamma-emitting radionuclides in nature, i.e. ²²⁶Ra, ²³²Th, ⁴⁰K and ¹³⁷Cs, has been carried out in soil samples collected from Peshawar University Campus and surrounding areas using a high purity germanium detector coupled with a computer-based high-resolution multichannel analyser. The activity concentrations in soil ranged from 30.20±0.65 to 61.90±0.95, 50.10±0.54 to 102.80±1.04, 373.60±4.56 to 1082±11.38 and 9.50±0.11 to 46.60±0.42 Bq kg^?1 for ²²⁶Ra, ²³²Th, ⁴⁰K and ¹³⁷Cs, with a mean value of 45±7.70, 67±12.50, 878±180 and 19±9.20 Bq kg^?1, respectively. The radium equivalent activity, internal and external hazard indices have mean values of 203.40±29.40 Bq kg^?1, 0.56 and 0.68, respectively. The mean values of outdoor and indoor absorbed dose rates in air and the annual effective dose equivalents were found to be 106.50 and 128 nGy h^?1 and 0.19 and 0.54 mSv y^?1, respectively. In the present study, ⁴⁰K was the major radionuclide present in soil samples. The presence of ¹³⁷Cs indicates that this area also received some fallout from the nuclear accident of the Chernobyl power plant in 1986. The activity concentrations of radionuclides found in soil samples during the current investigation were nominal. Therefore, they are not associated with any potential source of health hazard to the public.     

Soil radioactivity levels and radiation hazard assessment in the highlands of northern Jordan

Determination of the natural radioactivity has been carried out, by means of gamma-ray spectrometry system, in surface soil samples collected from various geological formations in urban areas of the northern highlands of Jordan. These highlands, extending from Yarmouk River in the north to Wadi Wala in the south, form the agriculturally important regions of Jordan. Soils of the study region, at which about 70% of the total population of the country are living, mainly originated from limestones that are locally used in construction materials, making the evaluation of environmental radioactivity and estimating the current radiation hazards to the population an interesting issue. The total average concentrations of radionuclides ²²⁶Ra, ²³⁸U, ²³²Th, and ⁴⁰K were 42.5, 49.9, 26.7, and 291.1 Bq kg⁻¹, respectively. Correlations made among these radionuclides prove the existence of secular equilibrium in the investigated soils. The total average absorbed dose rate in the study areas is found to be 51.5 nGy h⁻¹, whereas the annual effective dose equivalent has an average value of 63.2 μSv y⁻¹. The external and internal hazard indices, the radium equivalent activity, and the annual gonadal dose equivalent associated with the investigated soils do not exceed the permissible limits except for soils originated from phosphate rocks. Moreover, the radio-elemental concentrations of uranium, thorium and potassium, evaluated for the various geological features in the study areas were calculated to indicate whether relative depletion/enrichment of radioisotopes had occurred. The results of the present study were discussed and compared with internationally recommended values.