Dimer state in the two-dimensional anisotropic alternated-exchange Heisenberg model

An analysis is made of the two-dimensional Heisenberg model with S=1/2, anisotropic exchange interaction between nearest neighbors, and alternating exchange in two directions, [100] and [010] (corresponding to condensation of the (π, π) mode) and in one direction [100] (corresponding to condensation of the (π, 0) mode). The quantum Monte Carlo method is used to calculate the thermodynamic characteristics and the spin correlation functions which are used as the basis to determine the boundary of stability of an anisotropic antiferromagnetic with respect to alternation of exchange δ=(1−J ^x,y /J ^z )^0.4 in the (π,π) model and δ=(1−J ^x,y /J ^z )^0.31 in the (π,0) model. In the (π,0) model a disordered quantum state exists in the range (1−J ^x,y /J ^z )^0.31<δ<(0.3–0.35). The energy (E−0.68)=0.36δ ^1.80(6) and 0.21 δ ^2.0(5), the energy gap between the ground and excited states H _c (δ)=1.96δ ^2.(1), 1.8(1) (δ−0.35(3))^0.67(2) were determined as a function of the alternation of exchange in the (π,π)-and (π,0) models, respectively. Fiz. Tverd. Tela (St. Petersburg) 40, 1080–1085 (June 1998)     

Quantum Monte Carlo investigation of the 2D Heisenberg model with S=1/2

The two-dimensional (2D) Heisenberg model with anisotropic exchange (Δ = 1−J _x /J _z ) and S=1/2 is investigated by the quantum Monte Carlo method. The energy, susceptibility, specific heat, spin-spin correlation functions, and correlation radius are calculated. The sublattice magnetization (σ) and the Néel temperature of the anisotropic antiferromagnet are logarithmic functions of the exchange anisotropy: 1/σ+1+0.13(1)ln(1/Δ). Crossover of the static magnetic structural factor as a function of temperature from power-law to exponential occurs for T _c /J≈0.4. The correlation radius can be approximated by 1/ξ=2.05T ^1.0(6)/exp(1.0(4)/T). For La₂CuO₄ the sublattice magnetization is calculated as σ=0.45, the exchange is J=(1125–1305) K; for Er₂CuO₄ J∼625 K and the exchange anisotropy Δ∼0.003. The temperature dependence of the static structural magnetic factor and the correlation radius above the Néel temperature in these compounds can be explained by the formation of topological excitations (spinons). Fiz. Tverd. Tela (St. Petersburg) 41, 116–121 (January 1999)     

Magnetism,exchange and crystal field parameters in the orbitally unquenched Ising antiferromagnet FePS3

FePS₃ is a layered antiferromagnet (T _N=123 K) with a marked Ising anisotropy in magnetic properties. The anisotropy arises from the combined effect of the trigonal distortion from octahedral symmetry and spin-orbit coupling on the orbitally degenerate⁵ T _2g ground state of the Fe²⁺ ion. The anisotropic paramagnetic susceptibilities are interpreted in terms of the zero field Hamiltonian, ℋ=Σ_i [δ(L _iz ² −2)+|λ|L _i .S _i ]−Σ _ij J _ij S _i .S _j . The crystal field trigonal distortion parameter Δ, the spin-orbit coupling λ and the isotropic Heisenberg exchange,J _ij, were evaluated from an analysis of the high temperature paramagnetic susceptibility data using the Correlated Effective Field (CEF) theory for many-body magnetism developed by Lines. Good agreement with experiment were obtained for Δ/k=215.5 K; λ/k=166.5 K;J _nn k=27.7 K; andJ _nnn k=−2.3 K. Using these values of the crystal field and exchange parameters the CEF predicts aT _N=122 K for FePS₃, which is remarkably close to the observed value of theT _N. The accuracy of the CEF approximation was also ascertained by comparing the calculated susceptibilities in the CEF with the experimental susceptibility for the isotropic Heisenberg layered antiferromagnet MnPS₃, for which the high temperature series expansion susceptibility is available.     

How accurate is the cancelation of the first even zonal harmonic of the geopotential in the present and future LAGEOS-based Lense-Thirring tests?

The strategy followed so far in the performed or proposed tests of the general relativistic Lense-Thirring effect in the gravitational field of the Earth with laser-ranged satellites of LAGEOS type relies upon the cancelation of the disturbing huge precessions induced by the first even zonal harmonic coefficient J ₂ of the multipolar expansion of the Newtonian part of the terrestrial gravitational potential by means of suitably designed linear combinations of the nodes Ω of more than one spacecraft. Actually, such a removal does depend on the accuracy with which the coefficients of the combinations adopted can be realistically known. Uncertainties of the order of 2 cm in the semimajor axes a and 0.5 milliarcseconds in the inclinations I of LAGEOS and LAGEOS II, entering the expression of the coefficient c ₁ of the combination of their nodes used so far, yield an uncertainty δc ₁ = 1.30 × 10⁻⁸. It gives an imperfectly canceled J ₂ signal of 10.8 milliarcseconds per year corresponding to 23% of the Lense-Thirring signature. Uncertainties of the order of 10–30 microarcseconds in the inclinations yield δc ₁ = 7.9 × 10⁻⁹ which corresponds to an uncanceled J ₂ signature of 6.5 milliarcseconds per year, i.e. 14% of the Lense-Thirring signal. Concerning a future LAGEOS-LAGEOS II-LARES combination with coefficients k ₁ and k ₂, the same uncertainties in a and the less accurate uncertainties in I as before yield δk ₁ = 1.1 × 10⁻⁸, δk ₂ = 2 × 10⁻⁹; they imply a residual J ₂ combined precession of 14.7 milliarcseconds per year corresponding to 29% of the Lense-Thirring trend. Uncertainties in the inclinations at ≈ 10 microarcseconds level give δk ₁ = 5 × 10⁻⁹, δk ₂ = 2 × 10⁻⁹; the uncanceled J ₂ effect is 7.9 milliarcseconds per year, i.e. 16% of the relativistic effect.     

Mott-insulator-superfluid-liquid transition in a one-dimensional bosonic Hubbard model: Quantum Monte Carlo method

The values of the insulator gap Δ in one-dimensional systems of interacting bosons described by the Hubbard Hamiltonian are calculated at low temperatures by the quantum world-line Monte Carlo algorithm. The dependence of Δ on the size of the system, the temperature, and the parameters of the model is investigated. It is shown that a chain with N _a=50 sites is already sufficient to estimate the thermodynamic value of the critical quantity (t/U)_c for which a transition from the insulator into the superfluid state occurs in a commensurate system. To within the computational error, this value, (t/U)_c=0.300±0.005, agrees with the value (t/U)_c=0.304±0.002 obtained previously by the combined “exact diagonalization + renormalization-group analysis” method. The characteristic Kosterlitz-Thouless behavior of the insulator gap is demonstrated near the critical region: Δ∼exp[−b(1−t/t _c)^−1/2]. Pis’ma Zh. éksp. Teor. Fiz. 64, No. 2, 92–96 (25 July 1996)     

Effect of γ irradiation on the hysteresis phenomena at the incommensurate-commensurate phase transition in Rb2ZnBr4

The effect of γ irradiation on the temperature hysteresis in dielectric permittivity ɛ and loss tangent tan δ of crystalline Rb₂ZnBr₄ has been studied in the vicinity of the incommensurate-commensurate phase transition. The ɛ(T) and tan δ(T) curves were found to exhibit anomalies in the form of maxima. Hysteresis was observed in the measured properties, including the transition temperature T _c (ΔT=T _c ^h −T _c ^c ), in both unirradiated and irradiated samples. It is shown that, as the radiation dose increases the extent of the hysteresis ΔT increases, the values of ɛ _max and tan δ _max at the transition point decrease, and the anomalies wash out. Fiz. Tverd. Tela (St. Petersburg) 40, 1911–1914 (October 1998)     

Spectroscopy of quasiparticle excitations of superconducting bismuth cuprate at high pressures

We study the energy spectrum of Bi2223 (Bi_1.6Pb_0.4Sr_1.8Ca_2.2Cu₃O_x) at high hydrostatic pressures by Andreev-and tunneling-spectroscopy methods. We determine the gap anisotropy in the basal ab plane and find the following values for the parameters Δ(ϕ): Δ_max=42 mV, and Δ_min=19.5 mV (T _c =110 K and dT _c /dP=0.16 K/kbar). We detect an increase in the ratio R=2Δ_max/kT _c with pressure P; for Bi2223 cuprate, dR/dP≈0.017 kbar⁻¹. In the phonon-frequency region we detect a “softening,” due to pressure, of the high-frequency part of the phonon spectrum corresponding to “breathing” modes of oxygen, as well as other optical modes of Cu-O. The characteristic frequencies of the spectrum for ℏΩ>60 mV are found to decrease, with increasing pressure, at a rate d ln(ℏΩ)/dP≈−6.5±0.5×10⁻³ kbar⁻¹. This result explains the observed increase in the ratio 2Δ/kT _c (P) in the model of strong electron-phonon interaction. Zh. éksp. Teor. Fiz. 113, 1397–1410 (April 1998)     

Dispersion of the Voigt effect in the magnetic semiconductors Cd1−x MnxTe

Spectral measurements of the Voigt birefringence Δn were performed for the cubic magnetic semiconductor Cd_1−x Mn _x Te (0≤x≤0.52) in order to investigate how the exchange interaction of Mn²⁺ ions with itinerant electrons depends on the electron wave vector. It was determined that Δn/x ² is independent of x and the magnetic field direction, i.e., the effect is due to the Mn²⁺ ions and is isotropic. Below the band gap edge the dispersion of the birefringence Δn can be described well in all samples by the unusual dependence Δn∼(E _g −ℏω) ^−3.5. This can be explained by a decrease of the exchange interaction of Mn²⁺ ions with itinerant electrons with increasing distance from the center of the Brillouin zone. Pis’ma Zh. éksp. Teor. Fiz. 67, No. 8, 569–573 (25 April 1998)     

Josephson and single-particle currents between partially dielectricized superconductors with charge-density waves

The amplitudes of the nonstationary Josephson current I ¹, the interference current I ², and the quasiparticle current J through symmetric and asymmetric tunnel junctions, including superconductors with charge density waves, are calculated. In the symmetric (s) case the dependence of the Josephson current I _s ¹ on the voltage V on the junction has a logarithmic singularity at |eV|=2Δ, Δ+D, and 2D, where , Δ and Σ are the superconducting and dielectric order parameters, and e is the unit charge. At temperatures T≠0 jumps appear in the current-voltage characteristics I _s ¹ (V) at |eV|=D−Δ. Jumps and singularities are observed in the currents I _s ² and J _s at the same voltages at which singularities and jumps appear in I _s ¹ , respectively. In the nonsymmetric (ns) junctions which include an ordinary superconductor, singularities and jumps occur at |eV|=D+Δ_BCS, Δ+Δ_BCS, and (for T≠0) |D−Δ_BCS| and |Δ−Δ_BCS|, where Δ_BCS is the order parameter of an ordinary superconductor. The quasiparticle current J _ns is an asymmetric function of the voltage V and does not depend on the sign of Σ. The results are compared with experiment. Fiz. Tverd. Tela (St. Petersburg) 39, 991–999 (June 1997)     

Influence of quantum fluctuations on the Néel temperature of a dilute two-dimensional anisotropic antiferromagnet

A quantum Monte Carlo procedure is used to calculate the energy, sublattice magnetization, Néel temperature, and the slopes of the S=[1/T _N(x=0)]dT _N(x)/dx curves as functions of the hole concentration and the exchange anisotropy Δ=1−J _x,y/J _z in the Heisenberg model with anisotropic negative interactions between nearest neighbors in a square lattice with dilution among the lattice sites. The slope diverges in the limit Δ→0: S∼ln(6.5/Δ). Fiz. Tverd. Tela (St. Petersburg) 39, 898–900 (May 1997)     

d-symmetry superconductivity due to valence bond correlations

It is shown that d-symmetry superconductivity due to valence bond correlations is possible. Valence bond correlations are compatible with antiferromagnetic spin order. In order to explictly construct a homogeneous state with the valence bond structure in the two-dimensional Hubbard model for an arbitrary doping, we have used the variational method based on unitary local transformation. Attraction between holes in the d-channel is due to modulation of hopping by the site population in course of the valence bond formation, and corresponding parameters have been calculated variationally. An important factor for the gap width is the increase in the density of states on the Fermi level due to antiferromagnetic splitting of the band. The gap width and its ratio to the T _c are 2Δ≃0.1t and 2Δ/kT _c≃4.5−4 for U/t≃8. The correspondence between the theoretical phase diagram and experimental data is discussed. The dependence of T _c on the doping δ=|n−1| and the Fermi surface shape are highly sensitive to the weak interaction t′ leading to diagonal hoppings. In the case of t′>0 and p-doping, the peak on the curve of T _c(δ) occurs at the doping δ _opt, when the energy of the flattest part of the lower Hubbard subband crosses the Fermi level at k∼(π,0). In underdoped samples with δ<δ _opt, the anisotropic pseudogap in the normal state corresponds to the energy difference |E(π,0)−μ| between this part of the spectrum and the Fermi level. Zh. éksp. Teor. Fiz. 114, 985–1005 (September 1998)     

ESR study of exchange coupled pairs in copper diethyldithiocarbamate

ESR investigations on exchange coupled pairs of Cu ions in single crystals of Cu(dtc)₂, isomorphously diluted with the corresponding diamagnetic zinc salt, are reported. The spin Hamiltonian parameters for the coupled species (S=1) are:g _‖=2.1025,g ₊=2.031,A=75.1×10⁻⁴ cm⁻¹,B=14.8×10⁻⁴,D=276.0×10⁻⁴ cm⁻¹ andE=46.7×10⁻⁴ cm⁻¹. While theg andA tensors show tetragonal symmetry, the zeor-field splitting tensor is rhombic and has principal axes different from those of theg andA tensors. Intensity measurements made down to 4.2 K indicate that the exchange is ferromagnetic with |FFF| ∼ 10 cm⁻¹. Direct dipole-dipole interaction appears to be the major contribution to the zero-field splitting. A calculation on the distributed point dipole model shows that dipolar interaction is considerably modified by the high covalency of the Cu-S bond and accounts for the rhombic nature of the tensor. The possible exchange mechanisms in Cu(dtc)₂—direct exchange and superexchange through the bridging sulphurs—are discussed.     

Spontaneous photorefractive effect in Sr1−x CaxTiO3 (x=0.014)

The temperature dependence of the principal values of the refractive index in Sr_1−x Ca_xTiO₃ (x=0.014) has been measured in the 17–275 K range under various conditions of sample illumination with 1.96 eV photons. The spontaneous photorefractive contribution δn ^ph to the temperature-induced variation of the refractive index of Sr_1−x Ca_xTiO₃, which appears after illumination of the sample in the ferrophase (transition temperature T _c=32 K) and persists in the paraphase under heating up to 150 K, has been separated. The photoinduced polarization has been estimated. Fiz. Tverd. Tela (St. Petersburg) 39, 711–713 (April 1997)     

Weak exchange interactions in the heteronuclear crystal CuPr2(CCl3COO)8·6H2O

The new heteronuclear crystal CuPr₂(CCl₃COO)₈·6H₂O, constructed of chains containing copper and praseodymium atoms, has been synthesized and investigated by EPR at 9.3 GHz at temperatures ranging from room temperature down to 10 K. At temperatures T∼300–130 K, EPR spectra are observed which are characteristic of isolated polyhedra of copper ions with g _z=2.330±0.005, g _x,y =2.053±0.005, A _z=139×10⁻⁴ cm⁻¹, and A _x,y <26×10⁻⁴ cm⁻¹. At temperatures T<130 K a complex spectrum is observed, associated with the appearance of weak exchange interactions between the copper ions in the chain (J _Cu-CuΣS _i·S _i+1), comparable in magnitude with the hyperfine interactions J _Cu-Cu=0.015 cm⁻¹ at T=10 K. The magnitude of the exchange interaction decreases smoothly as the temperature is raised. It is conjectured that orbitals of the praseodymium ions participate in the process of indirect exchange between the copper ions. Fiz. Tverd. Tela (St. Petersburg) 41, 2154–2157 (December 1999)     

Pseudogap and precursor superconductivity in underdoped cuprate high temperature superconductors: A far-infrared ellipsometry study

With the technique of infrared ellipsometry we performed a detailed study of the temperature- and doping dependence of the c-axis response of a series of YBa₂Cu₃O_7−δ single crystals. In particular, we explored the anomalous electronic properties at temperatures above the macroscopic superconducting transition temperature, T _c, whose conflicting explanations range from a precursor superconducting state to electronic correlations that compete with superconductivity. We show that the c-axis spectra provide evidence that both kinds of correlations are present and that their contributions can be disentangled based on an analysis with a so-called multilayer-model. We find that the onset temperature, T ^*, and the energy scale, Δ_PG, of the competing pseudogap increase rapidly towards the underdoped side whereas they vanish on the overdoped side. In addition, we provide evidence that in a strongly underdoped sample the precursor superconducting correlations develop below an onset temperature, T ^ons, that is considerably lower than T ^* but still much higher than T _c.     

Field dependence of spin-lattice relaxation of Nd3+ ions in Y3Al5O12 crystals

Our studies involve measuring spin-lattice relaxation times for Nd³⁺ ions in yttrium-aluminum garnets over the temperature range 4–50 K at 9.25 and 36.4 GHz for different orientations of the external magnetic field in relation to the crystallographic axes. The temperature dependence of the relaxation rate is described by T ₁ ⁻¹ =AT ⁿ+b exp(−Δ/kT), where n varies from sample to sample, with n=1 for “perfect” samples (i.e., with the longest relaxation times). Here Δ is approximately 130 cm⁻¹, which is the energy of the excited Kramers doublet of the neodymium ion closest to the ground state, and this makes it possible to interpret the second term in T ₁ ⁻¹ as the contribution of two-stage relaxation proceeding through the intermediate level Δ. A strong field dependence of these processes has been discovered: when the frequency was increased fourfold, the relaxation rate increased by a factor of 10. The effect is a specific manifestation of the degeneracy of the excited level, breaking of the symmetry of the crystalline field due to lattice defects, and the prevalence of deformations of a certain type in the spin-lattice interaction. Zh. éksp. Teor. Fiz. 111, 332–343 (January 1997)     

Intrinsic Josephson junctions in Bi2Sr2CaCu2O8+δ single crystals

We report on thec-axis superconducting energy gap parameter Δ _c (T) of intrinsic Josephson tunnel junctions inBi ₂ Sr ₂ CaCu ₂ O _8+δ (Bi2212) single crystals. Δ _c (4.2K)≈10−13 meV, which is approximately a factor of two smaller than reported in the majority of tunneling experiments. Δ _c (T) deviates strongly from the BCS temperature dependence. These observations may be explained by a multilayer model of Bi2212 which assumes that theBi−O layers are superconducting due to the proximity effects. The Josephson tunneling then takes place between adjacentBi−O layers while there is a strong proximity coupling betweenBi−O andCu−O layers. The work is supported by Swedish Supercon-ductivity Consortium and NUTEK, and, in part, by Russian Foundation for Basic Research, grant #95-02-04307     

Entanglement entropy fluctuations in quantum Ising chains

The behavior of Ising chains with the spin-spin interaction value λ in a transverse magnetic field of constant intensity (h = 1) is considered. For a chain of infinite length, exact analytical formulas are obtained for the second central moment (dispersion) of the entropy operator Ŝ = -lnρ with reduced density matrix ρ, which corresponds to a semi-infinite part of the model chain occurring in the ground state. In the vicinity of a critical point λ_c = 1, the entanglement entropy fluctuation ΔS (defined as the square root of dispersion) diverges as ΔS ∼ [ln(1/|1 − λ|)]^1/2. For the known behavior of the entanglement entropy S, this divergence results in that the relative fluctuation δS = ΔS/S vanishes at the critical point, that is, a state with almost nonfluctuating entanglement is attained.     

A Remark on Lp-Boundedness of Wave Operators¶for Two Dimensional Schrödinger Operators

Let H=−Δ+V be a two dimensional Schr?dinger operator with a real potential V(x) satisfying the decay condition , δ > 6. Let H ₀=−Δ. We show that the wave operators are bounded in L ^p (R ²) under the condition that H has no zero resonances or bound states. In this paper the condition , imposed in a previous paper (K. Yajima, Commun. Math. Phys. 208, 125–152 (1999)), is removed. Received: 13 September 2001 / Accepted: 15 October 2001     

Different types of vortex pinning contribution to critical current density in YBa2Cu3O7−δ /YSZ quasi-multilayer

The quasi-multilayer films of YBa₂Cu₃O_7−δ /YSZ (YSZ denotes Yttria Stabilized Zirconia) are prepared by means of pulsed laser deposition (PLD), and a systematic study of the magnetic-field and temperature dependence of the critical current density J _c(H,T) for the YBCO/YSZ quasi-multilayer film is presented. Angular-dependent J _c(H,T) measurements have demonstrated that the growth control strategy is very effective in preventing the vortex motion at high fields and high temperatures. The temperature dependence of isotropic and anisotropic contribution to J _c is investigated in order to evaluate the strength of the defects. It is suggested that at high applied fields (such as 7 T), the pinning contribution of the YBCO/YSZ quasi-multilayer is dominated by the anisotropic disorders, while at intermediate-low fields (such as 1 and 3 T) the pinning contribution is determined by both isotropic and anisotropic disorders.