Levels of 190Os populated in the decays of 3.3 h 190mRe and 12 d 190Ir and in the 189Os(d,p)190Os reaction

The level structure of ¹⁹⁰Os has been investigated by the techniques of radioactive decay and neutron transfer reaction spectroscopy. The existence of 3.3 h ^190mRe has been confirmed; it decays ≈ 49% by isomeric transitions and ≈ 51% by β^? decay to levels in ¹⁹⁰Os with spins $\text{\$}\text{?}\text{= 5}$. In a re-investigation of the 12 d ¹⁹⁰Ir decay, a virtually complete decay scheme has been established and discrepancies between the I^π values assigned to several ¹⁹⁰Os levels by earlier workers have been resolved. The reaction ¹⁸⁹Os(d, p)¹⁹⁰Os has been studied and information about the locations of two-quasiparticle states involving the $\text{3}\text{2}\text{[512]ν}$ orbital and about the microscopic compositions of collective excitations has been derived. Various aspects of the ¹⁹⁰Os level structure are discussed in the light of the combined radioactivity and transfer reaction results.     

Intrinsic states,high-spin rotational bands and rotation alignment in 177Os and 179Os

Low-lying intrinsic states and their associated rotational bands have been identified in ¹⁷⁷Os and ¹⁷⁹Os. They are the mixed i_{$\text{13}\text{2}$} neutron states and the $\text{1}\text{2}$^?[521] states in ¹⁷⁷Os and ¹⁷⁹Os, as well as the $\text{5}\text{2}$^?[512] state in ¹⁷⁷Os and the $\text{7}\text{2}$^?[514] state in ¹⁷⁹Os. The $\text{1}\text{2}$^? sta is assumed to be the ground state, the other intrinsic states giving rise to isomers. The in-band decay properties of the $\text{7}\text{2}$^?[514] band, and the i_{$\text{13}\text{2}$} bands show the effect of mixing. In the rotational bands in ¹⁷⁷Os a low frequency backbending anomaly is observed but no anomaly is observed in the i_{$\text{13}\text{2}$}. band. In ¹⁷⁹Os the i_{$\text{13}\text{2}$} band does backbend but at a higher frequency than in the yrast bands of the even neighbours. The systematics of the backbending frequencies, and the effects of blocking, are discussed. The rotation aligned angular momentum is deduced, and a comparison made between the i_{$\text{13}\text{2}$} bands and the s-bands in the even neighbours. The results broadly support the identification of the s-bands with the aligned (i_{$\text{13}\text{2}$})² configuration.     

The level structure of 184Os from 184Ir decay and 185Re(p, 2nγ) in-beam spectroscopy

Levels of ¹⁸⁴Os populated in the decay of 3.1 h ¹⁸⁴Ir and in the ¹⁸⁵Re(p, 2nγ) reaction have been investigated. The measurements included γ-ray singles, β⁺ ray endpoint, conversion coefficient, β⁺-γ coincidence and detailed γ-γ coincidence determinations. The results have established an extensive ¹⁸⁴Os level scheme, which includes well developed ground state, γ-vibrational and K = 3 octupole bands and which accommodates all the intense transitions observed in both the radioactivity and in-beam γ-ray measurements. Deviations of the level energies in the K^π = 0⁺and K^π = 2⁺ bands and of the interband reduced transition probabilities from the predictions of the strong-coupling model are discussed in terms of the rotationvibration interaction, and the systematics of the octupole vibrational excitations in even-mass W and Os nuclei are reviewed. It is concluded that the ¹⁸⁴Ir ground state configuration has a spin of 5, and that it contains large admixtures of K = 0 or K = 1 character.     

High-spin yrast and non-yrast bands in 176Os, 178Os and 180Os

High-spin yrast and non-yrast states have been identified in ¹⁷⁶Os, ¹⁷⁸Os and ¹⁸⁰Os using (¹⁶O, xn) reactions, and γ-ray techniques. Band crossing anomalies are observed in each of the positive-parity yrast bands. The magnitude of these anomalies decreases with decreasing neutron number, an effect attributed to the change in the moment of inertia of the ground state rotational bands. A 23 ns isomer, predominantly K^π = 7^?, is identified at 1930 keV in ¹⁸⁰Os. The configuration of this isomer is discussed on the basis of the properties of its rotational band. Negative parity, odd and even spin, sideband sequences are observed in each isotope. Their relationship to rotation-aligned octupole and 2-quasiparticle bands is discussed from their excitation energies, band spacings, and decay properties. Detailed calculations for Coriolis mixed bands are carried out for the likely 2-quasiproton and 2-quasineutron configurations. An anomaly observed at spin 17 in the odd-spin negative-parity sequence in ¹⁸⁰Os is attributed to a band crossing with a fourquasiparticle configuration.     

The level structure of 187Os

A study of the level structure of ¹⁸⁷Os has been performed by means of (d, p), (d, t) and (d, d$\text{)}\text{?}$ reactions. Based upon the data presented and information available from the 10.5 h decay of ¹⁸⁷Ir, a level scheme including several new states and level assignments is proposed. The low-lying rotational bands built on the $\text{1}\text{2}{}^{\mathrm{?}}$ [510] and the $\text{3}\text{2}{}^{\mathrm{?}}$ [512] single-particle states have been analysed by means of Coriolis-coupling calculations including attenuations of the coupling matrix elements. The calculations involve fits to energies, to neutron transfer cross sections and to ratios of B (E2) values.     

States in 163Dy and 169Er populated in the (t,p) reaction

Angular distributions of protons from the ¹⁶¹Dy(t, p)¹⁶³Dy and ¹⁶⁷Er(t, p)¹⁶⁹Er reactions were studied, using 15 MeV and 17 MeV tritons from the McMaster University tandem Van de Graaff accelerator. The reaction products were analyzed with a magnetic spectrograph and detected with nuclear emulsions. Since the ¹⁶¹Dy target ground state is the $\text{5}\text{2}$⁺[642] orbital, a strong L = 0 transition was observed to the $\text{5}\text{2}$⁺[642] bandhead in ¹⁶³Dy, which was previously assigned at 251 keV. Also transitions to the $\text{7}\text{2}$, $\text{9}\text{2}$ and $\text{11}\text{2}$ band members were observed. Similarly, a strong L = 0 transition was observed to the $\text{7}\text{2}$⁺[633] bandhead at 244 keV in ¹⁶⁹Er, with the other band members only weakly populated. The angular distributions to the various members of these two bands can be described when higher-order reaction processes are taken into account. In ¹⁶³Dy, surprisingly strong L = 0 transitions were observed to levels at 1831 keV, 1937 keV and 2053 keV, with strengths of 23%, 30% and 37% of that for the $\text{5}\text{2}$⁺[642] bandhead. In ¹⁶⁹Er, the 905 keV level was populated with an L = 0 transition that had 31% of the strength observed for the strong L = 0 transition to the 244 keV level. The nature of these states is at present not understood.     

The level structure of 189Os

The level structure of ¹⁸⁹Os has been studied by (d, p), (d, t) and (d, d') reaction spectroscopy at E_d = 12.1 MeV. Assignments of a number of levels at excitation energies below ≈ 1700 keV are given. The assignments are discussed in terms of a unified model based on the Nilsson model including pairing, rotational motion and attenuated Coriolis coupling. Deviations between predicted and experimental excitation energies and wave functions are generally found to be consistent with trends observed in ¹⁸⁷Os and in the odd W isotopes. Evidence for the existence of collective non-rotational states is found from the (d, d') reactions. Results of (³He, α) and high resolution γ-ray and conversion electron studies were also included at various stages of the investigation to supplement the data from the deuteron induced reactions. Comparisons between calculated and measured B(E2) values are found to indicate an intrinsic quadrupole moment of the ground-state band of ≈ 5.0 b, in agreement with values in adjacent even Os isotopes. Details of the Coriolis coupling calculations are given.     

Nuclear structure effect in internal conversion of the isomeric transition in 191Os

Measurements have been performed on relative conversion line intensities of the hindered 74.38 keV isomeric transition in ¹⁹¹Os with the $\text{1}\text{2}\text{π√13}$ iron-free β-ray spectrometer. Anomalies were observed for the L, M and N subshell intensity ratios and were explained with a nuclear structure parameter λ = 9.4 ± 0.5 and a mixing ratio $\text{¦δ(}\text{E4/M3}\text{)¦ = (3.0 ± 0.3) × 10}{}^{\mathrm{?3}}$.     

Oblate ground-state shapes of 11 h 189Pt and 2.8 d 191Pt

With nuclear orientation on $\text{11}\text{h}\text{3}\text{2}{}^{\mathrm{?189}}\text{Pt}\text{, 2.8}\text{d}\text{3}\text{2}{}^{\mathrm{?191}}\text{Pt}$ and $\text{4.0}\text{d}\text{13}\text{2}{}^{\mathrm{<mtext>+\; 195\; </mtext><mtext>m</mtext>}}\text{Pt}$ in Os and NMR on oriented ¹⁸⁹Pt and ¹⁹¹Pt in Fe electric and magnetic hyperfine splitting frequencies were measured. The nuclear moments are deduced to be: ¹⁸⁹Pt: |μ| = 0.434(9) μ_N, Q = ?0.65(26) b; ¹⁹¹Pt: |μ| = 0.500(10) μ_N, Q = ?0.64(26) b; ^195mPt: Q = +1.42(60)b. The negative spectroscopic ground-state quadrupole moments of ¹⁸⁹Pt and ¹⁹¹Pt must be due to oblate ground-state deformations, thus indicating that the prolate-oblate phase transition in Pt is located at A < 189.     

The microwave spectrum of 14NH3 in the v = 000011 state

The frequencies and assignments of 50 lines in the pure inversion spectrum of ¹⁴NH₃ in the 0001¹ vibrational state are reported in the microwave frequency region 18–53 GHz and in selected regions up to 58 GHz.The J = 0 inversion frequency, K-type doubling constant K, l = 2, ?1 and molecular dipole moment in this state are 32 904.7 ± 2.0 MHz, 1.958 ± 0.040 MHz and 1.459 ± 0.002 D, respectively, where model inadequacies are included in the uncertainties of the first two parameters. The dipole moment measurements for this and the ground state are in excellent agreement with Stark laser measurements. An expression containing the effective l-type doubling constant is obtained from the combination of frequencies $\text{[ν(1, 1, 1) ? ν(1, 1, ?1) ? ν(2, 1, 1) + ν(2, 1, ?1)]}\text{8}\text{= 10 361.894 ± 0.004}\text{MHz}$. A preliminary value for the l-type doubling constant is 10 655 ± 20 MHz.     

Multi-step processes in the interpretation of the 28Si(d, 3He)27Al reaction

Results from a CCBA analysis of the ²⁸Si(d, ³He)²⁷Al reaction are reported. The transfers are assumed to occur between dominant components of (λμ) symmetry (0, 12) and (2, 10) in the initial and final nuclear eigenstates respectively. The results show that cross sections to four of the six levels observed below 3 MeV can be fairly well reproduced within a pure K_(J) band framework. However, consistent with electromagnetic results, all six levels can be fit if the K_(J) band purity of the analysis, SU(3) model. $\text{5}\text{2}{}^{\mathrm{+}}\text{(}\text{ground and}\text{2.73}\text{MeV}\text{)}$ states and $\text{9}\text{2}{}^{\mathrm{+}}\text{(3.00}\text{MeV}\text{)}$ state is abandoned.     

Neutron correlations in the 41K ground state and T = 1 2p-2h states in 40K

Differential cross sections have been measured for ⁴¹(d, t)⁴⁰K and ⁴¹K(p, d)⁴⁰K at 15 MeV using a magnetic spectrograph with electronic detection by proportional-counter-scintillator telescopes or semiconductor detectors. Knowledge of the structure of the ⁴⁰K multiplets ($\text{ν}\text{f}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}\text{, π}\text{d}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}{}^{\mathrm{?1}}$) and ($\text{ν}\text{p}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}\text{, π}\text{d}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}{}^{\mathrm{?1}}$) permits the determination of amplitudes and relative phases for various configurations and neutron correlations in the ⁴¹K ground state. Spectroscopic factors for neutron pick-up to states in ⁴⁰K are strongly influenced by the interference of transition amplitudes. In the (d, t) reaction T= 1, 2p-2h states are also observed.     

Odd-even features in 3He + 3H scattering

The single-channel resonating-group method is used to study effects of the Pauli principle on ³He + ³H scattering. Comparison is made with previous similar calculations for d + ³He scattering, and it is found that the Pauli principle affects the s = 0 state of the ³He + ³H system rather similarly to the way it affects the s = 1 state, whereas the Pauli principle affects the $\text{s =}\text{3}\text{2}$ state of the d + ³He system quite differently from the way it affects the $\text{s =}\text{1}\text{2}$ state. Mention is made of the possibility of observing similar effects of the Pauli principle in other nuclear systems.     

Study of band crossings in 182Os

High-spin states in ¹⁸²Os have been populated by the (¹⁸O, 4n) reaction and studied using in-beam spectroscopy methods. Seven side bands have been established for the first time. Three of the side bands show a band crossing. The features of the bands have been interpreted in the framework of the cranking model considering the motion of independent particles in a rotating deformed potential. The band crossings of the yrast band and of these three side bands can be explained by the rotation-alignment of a pair of $\text{i}{}_{\mathrm{<mtext>13</mtext><mtext>2</mtext>}}$ quasineutrons.     

Proton states in the N = 88 nuclei 149Pm, 151Eu and 153Tb populated in the (τ, d) and (α, t) reactions

The (τ, d) and (α, t) reaction on targets of ¹⁴⁸Nd, ¹⁵⁰Sm and ¹⁵²Gd have been studied, using beams of 24 MeV ³He and 27 MeV ⁴He from the McMaster University FN tandem Van de Graaff accelerator. The reaction products were analyzed with a magnetic spectrograph and detected with photographic emulsions. The (α, t) spectra were measured at two angles for each target, and the (τ, d) reactions were studied at 8 or 9 angles. The l-values for a number of low-spin states were determined from the (τ, d) angular distributions, and ratios of the (α, t) and (τ, d) cross sections were used to obtain l-values for several other states. There are some striking similarities in the observed structures of the three final nuclei, ¹⁴⁹Pm, ¹⁵¹Eu and ¹⁵³Tb. In each case there are low-lying strongly populated $\text{11}\text{2}$^? states and a higher lying l = 5 level somewhat below 1 MeV of excitation energy. Several states (10 in ¹⁴⁹Pm, 17 in ¹⁵¹Eu and 8 in ¹⁵³Tb) appear to be populated via l = 2 transitions, and there are strongly excited $\text{1}\text{2}$⁺ levels at $\text{≧ 1}\text{MeV}$ of excitation energy in each case. Of particular interest is a $\text{7}\text{2}$^? state located ≦ 50 keV above the lowest $\text{11}\text{2}$^? state in each nuclide. The relatively strong populations of these $\text{7}\text{2}$^? levels in the present experiments are contrary to expectations based on the simple shell model as there are no f_{$\text{7}\text{2}$} states in the 50 < Z < 82 shell.     

The 48Ti(t,d)49Ti reaction: A comparison with magnetic electron scattering

The reaction ⁴⁸Ti(t, d)⁴⁹Ti leading to the ground and first excited states of ⁴⁹Ti has been studied at triton energies of 2.75 and 3.0 MeV. The cross section to the ground state of ⁴⁹Ti has been analysed using the DWBA with a previously determined bound-state well geometry to obtain a value for the (t, d) normalization factor of D² = (3.29 ± 0.40) × 10⁴ MeV² · fm³. This value is in agreement with that obtained from a comparison of the (d, t) reaction with heavy-ion single-neutron transfer reactions. Using this value of the normalization factor the rms radius of the $\text{2}\text{p}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}$ component in the $\text{3}\text{2}{}^{\mathrm{?}}$ first excited state of ⁴⁹Ti is found to be 4.42 ± 0.07 fm (point neutron), corresponding to the use of a local bound-state potential well.     

Nuclear reaction studies of 168Tm

The intrinsic structure of ¹⁶⁸Tm has been studied using the (³He, d) and (α, t) proton stripping reactions as well as the (d, t) and (³He, α) neutron pick-up reactions. The beams of 24 MeV ³He particles, 25 MeV α-particles and 12 MeV deuterons were obtained from the McMaster tandem Van de Graaff accelerator. The reaction products were analyzed with an Enge-type magnetic spectrograph and detected with photographic emulsions. The spectra have been interpreted in terms of the coupling of an odd proton and an odd neutron, each moving independently in a spheroidal potential, which gives rise to intrinsic two-quasiparticle states with $\text{K = ¦Ω}{}_1\text{±Ω}{}_2\text{¦}$. The identification of the intrinsic states was made by comparing the experimental cross-section patterns with those predicted with the aid of Coriolis coupling and distorted-wave Born approximation (DWBA) calculations. Rotational bands superimposed on the K^π = 3⁺ and $\text{K}{}^{\mathrm{\pi }}\text{= 4}{}^{\mathrm{+}}\text{, {}\text{7}\text{2}{}^{\mathrm{+}}\text{[633]}{}_{\mathrm{n}}\text{±}\text{1}\text{2}{}^{\mathrm{+}}\text{[411]}{}_{\mathrm{p}}\text{}}$ configurations, the first of which is the ground state, ha been observed in the spectra of all four reactions. New assignments have been made for configurations resulting from coupling the $\text{1}\text{2}$^? [541], $\text{7}\text{2}$⁺ [404], $\text{5}\text{4}$⁺ [402] and $\text{1}\text{2}$^? [530] p to the $\text{7}\text{2}$⁺ [633] neutron state. The neutron pick-up measurements confirmed the earlier assignments based on (d, t) reaction studies and suggested tentative assignments for the {$\text{1}\text{2}$⁺ [400]_n±$\text{1}\text{2}$⁺ [411]_p} and {$\text{3}\text{2}$⁺ [402]_n±$\text{1}\text{2}$⁺ [411]_p}     

An isomeric two-particle state in 236U

A new isomeric state with 125 ± 20 ns half-life has been found in a ²³⁵U(d, pγ)²³⁶U experiments. Of the 12 observed delayed λ-lines, 11 have been fitted into a tentative decay scheme. The isomeric level is deduced to be the K, J^π = 4,4^? two-quasineutron state at 1052 keV with configuration $\text{[743]}\text{7}\text{2}{}^{\mathrm{?}}$; $\text{[631]}\text{1}\text{2}{}^{\mathrm{+}}$ that is also seen in (d, p) experiments.     

Contrasting high-spin yrast bands in 172Os and 174Os and an unexpected low-frequency anomaly in 172Os

The yrast bands of the neutron deficient isotopes ¹⁷²Os and ¹⁷⁴Os have been identified to spins of about 24. The yrast band in ¹⁷⁴Os shows no bandcrossing anomalies, confirming the shell effect observed in other N = 98 nuclei. In contrast, a strong backbend observed at a frequency of about 0.26 MeV in ¹⁷²Os is attributed to the s-band crossing. A weaker band-crossing is also observed at a lower frequency, about 0.24 MeV, in ¹⁷²Os. This unexpected anomaly may be due to either a deformation effect, or to a change in the s-band structure.