Far infrared absorption in normal H2 from 77 to 298 K

The translational-rotational absorption spectrum of normal H₂ has been measured from 80 to 900 cm^?1 at seven temperatures from 77.4 to 298 K. These results have been accurately fitted by a three-parameter line-shape function, thereby providing a reliable way of predicting the absorption of H₂ anywhere in this frequency and temperature region.     

Optical absorption by atomically doped carbon nanotubes under strong atom–field coupling

We analyze optical absorption by atomically doped carbon nanotubes with a special focus on the frequency range close to the atomic transition frequency. We derive the optical absorption line-shape function and, having analyzed particular achiral nanotubes of different diameters, predict the effect of absorption line splitting due to strong atom–vacuum–field coupling in small-diameter nanotubes.     

水下材料声学性能宽频段测量方法

本文根据脉冲法和传递函数法的测试原理,建立水下声学材料吸声性能宽频段测量方法,在同一水声声管,相同状态下,对橡胶材料吸声性能进行测试分析。分析表明:常压及加压环境下,采用传递函数法和脉冲法测量材料的吸声性能,在重合频段(4 kHz～5.5 kHz)测试结果基本一致,测试偏差小于5%,从而验证了不同测量原理,测试材料水下声学性能的通用性。因此,采用传递函数法和脉冲法,可以实现水下材料声学性能宽频带测试。     

Cross section of supercooled238UF6 in multiphoton absorption induced by 16 micrometer Raman-laser radiation

Measurements of multiphoton absorption of 16 µm Raman-laser radiation in supercooled²³⁸UF₆ at 90 K were performed by using a pulsed Laval nozzle with an optical path length of 50 cm. The laser fluence was varied between 50 and 500 mJ/cm² for four frequencies in the range from 625 to 629 cm^–1. The energy absorbed by²³⁸UF₆ molecules was investigated as a function of laser frequency or fluence, and highly accurate results were obtained with the use of the nozzle whose optical path length is much greater than that of nozzles used before. The results indicated that the absorption cross section at the peak absorption frequency (627.8cm^–1) was proportional to the –1/3 power of the fluence.     

氧气A带吸收系数的温度依赖关系研究

氧气A带是理想的大气要素反演通道,吸收系数是重要的参数之一,它影响到反演结果的精度.结合HITRAN2012数据库和大气温度廓线图,分析氧气A带吸收系数的影响因素,推出各因素与温度的依赖关系,确定吸收系数随温度的变化.结果表明,氧气A带谱线半宽度受温度依赖系数影响较小,而受温度影响较大.线型因子随温度产生了两种变化,在谱线半宽度以外的谱线位置上,随温度的增大,函数值减小,而在中心频率到谱线半宽度的谱线位置上,随温度的升高而增大.谱线线强对温度具有强依赖关系.利用逐线积分算法计算氧气A带吸收系数,同时考虑了谱线半宽度的压力展宽效应和谱线线强及半宽度对温度的依赖关系,得出氧气A带吸收系数对温度的依赖关系主要来源于线强的温赖关系,尤其是中心频率处温度影响较大;而Lorentzian线型函数的温赖关系不明显.利用布鲁克光谱仪在1 cm-1下测量63 m处氧气A带的吸收光谱,与理论模型在同等条件下的透过率比较,误差小于0.83%,验证了温度校正模型的正确性.     

A model comparison of the absorption coefficient of a Microperforated Insertion Unit in the frequency and time domains

The absorption coefficient of acoustic materials can be measured either in the frequency or the time domain. At normal incidence, a sample of the material is fitted within an impedance tube and the absorption coefficient is calculated in the frequency domain from the measurement of the transfer function between two microphones [ISO 10534-2. Acoustics - determination of sound absorption coefficient and impedance in impedance tubes - Part 2: transfer function method. ISO, Geneva, Switzerland; 1996]. When the acoustic material must be characterized at oblique incidence or in situ (noise barriers, for instance) the absorption coefficient is calculated from measurements of the loudspeaker-microphone impulse response in the time domain, both in free field and in front of the sample [CEN/TS 1793-5. Road traffic noise reduction devices - test method for determining the acoustic performance - Part 5: intrinsic characteristics - in situ values of sound reflection and airborne sound insulation. CEN, Brussels, Belgium; 2003, ISO 13472-1. Acoustic measurement of sound absorption properties of road surfaces in situ - Part I: extended surface method. ISO, Geneva, Switzerland; 2002]. Since the absorption is an intrinsic property of the acoustic material, its measurement in either domain must provide the same result. However, this has not been formally demonstrated yet. The aim of this paper is to carry out a comparison between the absorption coefficient predicted by the impedance model of a Microperforated Insertion Unit and the absorption coefficient predicted from a simulated reflection trace taken into account the finite length of the time window.     

Frequency integration for radiative transfer problems involving homogeneous non-gray gases: The inverse transmission function

It is shown that narrow-band frequency integration for radiative-transfer problems, involving homogeneous non-gray gases, can be accomplished by an integration with respect to the absorption coefficient. The kernel of the absorption-coefficient integral is a property of the gas and can be obtained directly from the absorption coefficient for a simple dependence of the absorption coefficient on frequency. It is shown that the kernel (called the ‘inverse transmission function’) can also be obtained as the inverse Laplace transform of the transmission function, without explicit knowledge of the absorption coefficient. The kernel has been obtained using the inverse transmission-function method for two statistical band models: the Goody model and the Malkmus model. The kernel for the Malkmus model offers a simple, accurate, straightforward method for narrow-band frequency integration.     

On optimal design of half-wave resonators for acoustic damping in an enclosure

Acoustic design parameters of a half-wave resonator are studied experimentally for purely acoustic tuning of the resonator. According to the standard acoustic-test procedures, acoustic-pressure signals in the model enclosure with the resonators are measured. Based on the signals, quantitative acoustic properties of damping factor and sound absorption coefficient are evaluated and thereby, the acoustic-damping capacity of the resonator is characterized. Sound absorption coefficient has the advantages of the damping factor in various aspects. The coefficient indicates clearly the tuning frequency of the resonator, absorption effectiveness as a function of frequency, and overall damping capacity. The diameter and the number of a half-wave resonator, its distribution, and the blockage ratio at its inlet are selected as design parameters for optimal tuning of the resonator in the model enclosure. The resonators with larger diameter have the advantage of those with smaller one with respect to purely acoustic damping at the tuning frequency. The optimum number of resonators or the optimum open-area ratio decreases as boundary absorption decreases. When the open-area ratio exceeds the optimum value, over-damping appears, leading to a decrease in peak absorption coefficient and a broadening of absorption bandwidth. Blockage at the resonator inlet controls both peak absorption coefficient and its absorption bandwidth and it can be considered one of design factors for acoustic tuning.     

管束穿孔板的管腔耦合共振吸声机理研究

为了揭示管束穿孔板共振吸声结构的吸声机理,利用热黏性条件下基于有限元算法的管束穿孔板仿真模型,研究了平面声波正入射条件下,管束穿孔板内部声场分布特征,并利用阻抗管对吸声系数的理论仿真结果进行了试验验证.结果表明,管束穿孔板在低频主要靠腔体共振吸声,在高频主要靠管共振吸声,管束穿孔板整体呈现出较为明显的管腔耦合共振吸声特征。管束穿孔板共振时管中声强和质点法向振速较大,高频次吸声峰频点处管中和腔中均有驻波形成,频率越高驻波数量越多.管束穿孔板的耦合共振受到管长、腔深、穿孔率和管内径等参数变化的影响,管长对高频耦合共振的影响最大,管长增大使高频主吸声峰频点移向低频,并使相邻主吸声峰之间的间距减小.      

碳纳米管吸收电磁波特性

本文研究碳纳米管阵列的介电谱函数与吸收电磁波的特性。应用等离激元和无规相近似方法给出碳纳米管的介电谱函数,进而求出吸收系数和反射功率比。介电函数随电磁波的频率变化,在光子能量与系统电子的能谱差相匹配时产生共振吸收,吸收系数出现多个大的吸收峰。反射功率比随薄层厚度的增加而指数衰减,其衰减速率和饱和值与电磁场的频率和碳纳米管的结构有密切的联系。     

Temperature effect on the threshold frequency of absorption in a quantum pseudodot

The threshold frequency of absorption in a quantum pseudodot under the influence of temperature and applied magnetic field is calculated. The threshold frequency of absorption is computed as a function of temperature and applied magnetic field. The linear and nonlinear dependence of the absorption threshold frequency on magnetic field and temperature has been showed. According to the results obtained from the present work, we find that the linear and nonlinear dependence of the absorption threshold frequency depends on used range of the temperatures and magnetic fields.     

ZnSe－ZnS量子阱的光学非线性

半导体量子阱及超晶格材料具有室温激子效应以及强的光学非线性从而得到人们广泛的重视。利用半导体量子阱和超晶格可以制备出高速度、低闭值、小尺寸及室温工作的半导体激光器、光双稳器件等一系列光电子器件.     

Resonance phenomena in domain boundary movement in ferrites

The frequency dependence of magnetic losses in certain ferrites over the frequency range 20–110 MHz is studied. A series of absorption lines was observed in many ferrites. On the basis of an investigation of the change in absorption spectrum as a function of the magnetic history of the specimen, the size of the powder particles, and the external magnetic field, it was concluded that the resonance lines observed are produced by domain boundary resonance.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 7, pp. 41–45, July, 1973.     

High resolution emission spectra of laser-excited molecular iodine as the excitation frequency is tuned through and away from resonance

We have studied the ΔJ = 2 rotationally shifted emission lines in the region of the strong absorption of molecular iodine which occurs within the 5145 Å argon ion laser line. We used an etalon tuned, single frequency argon ion laser with a linewidth of 20 MHz to excite the iodine emission and recorded the spectra of the rotational lines with Fabry-Perot spectrometers having resolutions up to 70 MHz (0.0023 cm^-1). To overcome Doppler linewidth limitations we took spectra of the emission at small angles to the exciting beam and found the lines to have widths less than our instrumental resolution and frequencies which accurately tuned with the incident laser frequency. We recorded the emission lines for laser frequencies in the absorption line center and out into the absorption wing. Our spectra show that the intensity of the emission lines follows the absorption line profile while the frequency of the emission lines is determined by the laser frequency; the intensity is maximum at the absorption line center, falling by 10⁴ as the laser frequency is moved off the line center, while the line position maintains a constant frequency shift from the laser frequency.     

Separate reconstruction of the speed of sound,density of the medium,and coefficient of absorption in tomographic problems

A procedure is proposed for separating contributions to the scatterer function by inhomogeneities of the speed of sound, density of a medium, and coefficient of absorption. The scatterer function is reconstructed by solving the inverse problem. The power index of the absorption coefficient’s frequency dependence is determined simultaneously. The resistance to interference of this procedure is investigated by simulations in the multifrequency mode.     

Ultrasonic absorption in aqueous solutions of amino acids at neutral pH

Ultrasonic absorption coefficients in aqueous solutions of glycine, L-alanine, imidazole, L-phenylalanine, L-histidine and L-tryptophan at neutral pH were measured in the range from 0.8 to 220 MHz at 25 degrees C. A characteristic ultrasonic relaxation phenomenon was observed only in the solution of L-histidine with a relaxation frequency at around 2 MHz at neutral pH. It was proposed from the concentration independent relaxation frequency and the linear concentration dependence of the maximum absorption per wavelength that the relaxation mechanism was associated with a perturbation of the rotational isomeric equilibrium of the L-histidine molecule. The existence of two rotational isomeric forms of L-histidine in water was examined by semiempirical quantum chemical methods, in order to determine the free energy difference between the two states. The forward and backward rate constants were determined from the relaxation frequency and the energy change. Also, the standard volume change of the reaction was estimated from the concentration dependence of the maximum absorption per wavelength. It was speculated that L-histidine fulfills a specific function among amino acids because of the rotational motion in the molecule, in addition to its well-established acid-base properties.     

The shape of the statistical wing of an absorption line: Derivation by the Green’s function method

A formula is derived for the absorption coefficient in the statistical wing of an absorption line in the case in which both levels of a two-level system are involved in collisions. For this purpose, the kinetic equations for two-level particles in a strong field at an arbitrary detuning of the field frequency from the transition frequency are used, which were derived previously with the Green’s function method for nonequilibrium systems.     

Two-photon absorption in organic dyes — Relation with the symmetry of the levels

We studied two-photon absorption in a number of organic dyes and found that the two-photon cross-section does not follow Schäfer-Schmidt's rule. We found that the ratio δ_ω/σ_2ω is a function of the difference between the peak absorption frequency and twice the laser frequency, ω_max - 2ω_L. We pointed out the importance of the symmetry of the energy levels by studying three families of dyes.     

双光子吸收的Franz-Keldysh效应

从实验上证实Hg_0.695Cd_0.305Te 光电二极管空间电荷区中存在双光子吸收的Franz-Keldysh效应.利用一个皮秒Nd:YAG激光器抽运的光学参量产生器和差频产生器作为激发光源,测量了入射波长为λ₀=7.92μm的脉冲激光所激发的光响应随入射光强的变化关系.脉冲光响应峰值强度随入射光强的增大呈现二次幂函数增强趋势.采用等效RC电路模型将脉冲光伏信号峰值与入射光强相关联,得到空间电荷区中强电场下单光束 关键词： Franz-Keldysh效应 碲镉汞 双光子吸收 脉冲光伏信号     

The scattering of line radiation—I. A generalized redistribution function

The theory of the frequency redistribution of radiation during scattering is re-investigated with the aim of producing a generalized frequency redistribution function. The assumption, commonly made, that the atom performing the scattering of the radiation has a constant velocity for the duration of the scattering event is not made in the present investigation. As a result a formal theory is developed which does indeed lead to a generalized redistribution function. Two limiting cases are discussed: in one of the limits, we reconsider the case where the velocity of the atom is constant during the scattering event; the other limiting case describes the situation which occurs when the velocity at absorption, of the atom performing the scattering, is completely uncorrelated with its velocity at emission. This latter case is then more fully discussed with a view to overcoming one of the major difficulties encountered with the existing theories of frequency redistribution, i.e. that complete redistribution in the radiation scattered from an atmosphere being viewed by a distant observer can not be predicted.