Field-induced magnetic reorientation and effective anisotropy of a ferromagnetic monolayer within spin wave theory

The reorientation of the magnetization of a ferromagnetic monolayer is calculated with the help of many-body Green's function theory. This allows, in contrast to other spin wave theories, a satisfactory calculation of magnetic properties over the entire temperature range of interest since interactions between spin waves are taken into account. A Heisenberg Hamiltonian plus a second-order uniaxial single-ion anisotropy and an external magnetic field is treated by the Tyablikov (Random Phase Approximation: RPA) decoupling of the exchange interaction term and the Anderson-Callen decoupling of the anisotropy term. The orientation of the magnetization is determined by the spin components (), which are calculated with the help of the spectral theorem. The knowledge of the orientation angle allows a non-perturbative determination of the temperature dependence of the effective second-order anisotropy coefficient. Results for the Green's function theory are compared with those obtained with mean-field theory (MFT). We find significant differences between these approaches. Received 6 April 1999 and Received in final form 9 July 1999     

Quantum spin model of a cubic ferromagnet in a magnetic field

The zero temperature phase diagram of a one-dimensional ferromagnet with cubic single ion anisotropy in an external magnetic field is studied. The mean-field approximation and the density-matrix renormalization group method are applied. Two phases at finite magnetic fields are identified: a canted phase with spontaneously broken symmetry and a phase with magnetization along the magnetic field. Both methods predict that the canted phase exists even for the single-ion anisotropy strong enough to destroy the magnetic order at zero magnetic field. In contrast to the mean-field theory, the density-matrix renormalization group predicts a reentrant behavior for the model. The character of the phase transition at finite magnetic field has also been considered and the critical index has been found. Received 9 May 2000 and Received in final form 5 July 2000     

Many-body Green's function theory for thin ferromagnetic anisotropic Heisenberg films: treatment of the exchange anisotropy

The many-body Green's function theory developed in our previous work for treating the reorientation of the magnetization of thin ferromagnetic films is extended to include the exchange anisotropy. This leads to additional momentum dependencies which require some non-trivial changes in the formalism. The theory is developed for arbitrary spin values S and for multilayers. The effects of the exchange anisotropy and the single-ion anisotropy, which was treated in our earlier work, on the magnetic properties of thin ferromagnetic films are compared. Received 31 October 2002 Published online 7 May 2003     

Magnetization and magnetic susceptibility of the Ising ferromagnetic/antiferromagnetic superlattice

A linear cluster mean-field approximation is used to study the magnetic properties of the Ising ferromagnetic/antiferromagnetic superlattice, which is composed of a spin-1/2 ferromagnetic monolayer and a spin-1 antiferromagnetic monolayer with a single-ion anisotropy alternatively. By using the transfer matrix method, we calculate the magnetization and the initial magnetic susceptibility as functions of temperature for different interlayer coupling, single-ion anisotropy. We summarize the changing behaviors of the spin structure in ferromagnetic and antiferromagnetic layers and the characteristics of the corresponding magnetic susceptibilities, give the transition temperature as a function of the interlayer exchange coupling for different single-ion anisotropy, and analyze the features of the magnetization and the magnetic susceptibility.     

Many‐body Green's function theory for thin ferromagnetic films: exact treatment of the single‐ion anisotropy

A theory for the magnetization of ferromagnetic films is formulated within the framework of many‐body Green's function theory which considers all components of the magnetization. The model Hamiltonian includes a Heisenberg term, an external magnetic field, a second‐ and fourth‐order uniaxial single‐ion anisotropy, and the magnetic dipole‐dipole coupling. The single‐ion anisotropy terms can be treated exactlyby introducing higher‐order Green's functions and subsequently taking advantage of relations between products of spin operators which leads to an automatic closure of the hierarchy of the equations of motion for the Green's functions with respect to the anisotropy terms. This is an improvement on the method of our previous work, which treated the corresponding terms only approximately by decoupling them at the level of the lowest‐order Green's functions. RPA‐like approximations are used to decouple the exchange interaction terms in both the low‐order and higher‐order Green's functions. As a first numerical example we apply the theory to a monolayer for spin S = 1 in order to demonstrate the superiority of the present treatment of the anisotropy terms over the previous approximate decouplings.     

Magnetic-roughness-induced magnetostatic interactions in magnetic tunnel junctions

Magnetostatic ferromagnetic coupling in magnetic tunnel junctions was selectively analyzed. We have shown that in samples involving polycrystalline magnetic films, beyond the orange-peel coupling, an important class of interaction is related to the dispersion fields associated to magnetic inhomogeneities. These magnetization fluctuations were described in terms of magnetic roughness arising from the local anisotropy fluctuations. Therefore, using roughness data extracted from atomic/ magnetic force microscopy analysis, the amplitude and the variation with distance of the magnetostatic interactions were selectively quantified. Received 7 December 2001     

Vertex correction of the anisotropic magnetic impurities to the spin polarization of 2D electron gas

In terms of Kubo's formula and Green's function method, for the two-dimensional electron gas (2DEG) with Rashba spin-orbit coupling (SOC), we study the spin polarization due to the effect from magnetic impurities with anisotropic spin dependent delta type coupling to electrons when an external dc electric field in plane is applied. The vertex correction of impurities in ladder approximation is carried out in the limit of EF?1/τ, Δ. We find that the strength of spin polarization can be significantly modified by vertex correction and the spin polarization is relevant to the anisotropy coefficient γ, but the direction of net spin polarization cannot be changed.     

Calculations of ferromagnetic surface dynamics using the Green's functions theory and matching procedure

A Heisenberg model is employed to study the spin fluctuation dynamics on a (001) ferromagnetic surface using a new theoretical formalism. The solution of the full magnetic problem arising from the absence of magnetic translation symmetry in one dimension due to the presence of a magnetic surface is presented. The calculations are described using simultaneously a closed form of the spin-wave Green's function and the matching procedure in the random-phase approximation. Analytic expressions for the Green's functions are also derived in a low-temperature spin-wave approximation. The theoretical approach determines the bulk and evanescent spin fluctuation fields in the two dimensional plane normal to the surface. The results are used to calculate the localised modes of magnons associated with the surface. Numerical examples of the modes are given and they are found to exhibit various effects due to the interplay between the bulk and surface modes. It is shown that there may be surface spin-waves that decay in amplitude with distance into the bulk domain. Also the bulk spin fluctuations field as well as the magnons localised at the surface depend on the nature of the bulk-surface coupling exchange. The unstable surface magnetic configurations are illustrated and discussed. The results derived from the dynamic correlation functions between a pair of spin operators at any two sites are employed to evaluate the spin deviation in the ferromagnet due to localised surface modes obtained by the matching procedure as a function of temperature. Received 21 April 2002 / Received in final form 25 October 2002 Published online 14 March 2003     

Spin kinetic Monte Carlo method for nanoferromagnetism and magnetization dynamics of nanomagnets with large magnetic anisotropy

The Kinetic Monte Carlo (KMC) method based on the transition-state theory, powerful and famous for simulating atomic epitaxial growth of thin films and nanostructures, was used recently to simulate the nanoferromagnetism and magnetization dynamics of nanomagnets with giant magnetic anisotropy. We present a brief introduction to the KMC method and show how to reformulate it for nanoscale spin systems. Large enough magnetic anisotropy, observed experimentally and shown theoretically in terms of first-principle calculation, is not only essential to stabilize spin orientation but also necessary in making the transition-state barriers during spin reversals for spin KMC simulation. We show two applications of the spin KMC method to monatomic spin chains and spin-polarized-current controlled composite nanomagnets with giant magnetic anisotropy. This spin KMC method can be applied to other anisotropic nanomagnets and composite nanomagnets as long as their magnetic anisotropy energies are large enough.      

Laser induced ultrafast demagnetization in diluted magnetic semiconductor nanostructures

We present a dynamical model that reproduces the observed time evolution of the magnetization in diluted magnetic semiconductor films after weak laser excitation. Based on a many-particle expansion of the exact p–d exchange interaction, our approach goes beyond the usual mean-field approximation. Numerical results demonstrate that the hole spin relaxation plays a crucial role for explaining the ultrafast demagnetization processes observed experimentally. The influence of the laser power on the magnetization dynamics is also investigated.     

Temperature dependence of surface magnetization in local-moment systems

We present a theory to study the temperature-dependent behavior of surface magnetization in a ferromagnetic semi-infinite crystal. Our approach is based on the single-site approximation for the s-f model. The effect of the semi-infinite nature of the crystal is taken into account by a localized perturbation method. Using the mean-field theory for the layer-dependent magnetization, the local density of states and the electron-spin polarization are investigated at different temperatures for ordinary and surface transition cases. The results show that the surface magnetic properties may differ strongly from those in the bulk and the coupling constant of atoms plays a decisive role in the degree of spin polarization. In particular, for the case in which the exchange coupling constant on the surface and between atoms in the first and second layer is higher than the corresponding in the bulk, an enhancement of surface Curie temperature and hence the spin polarization can be obtained.     

Magnetic Properties of Spin-1/2 Quantum Heisenberg Ferromagnet with Spatially Anisotropy

The spin-1/2 quantum Heisenberg ferromagnet with anisotropic spin exchange interactions in three dimensions are investigated by means of the Green's function method. In the Tyablikov approximation, the correlation functions, the magnetization, and the susceptibilities are computed. The magnetic properties of this model are found to be dependent of anisotropy.     

Spin-liquid state for two-dimensional Heisenberg antiferromagnets on a kagomé lattice

The magnetic properties of the spin liquid state of the antiferromagnetic Heisenberg model on the kagomé lattice are investigated within the self-consistent mean-field theory. The results show that the spin liquid ground-state energy per site is , which is in very good agreement with the best numerical estimates. The spin structure factor and spin susceptibility are also discussed. Received 1 December 1998 and Received in final form 12 April 1999     

Spin dynamics in (III,Mn)V ferromagnetic semiconductors: the role of correlations

We address the role of correlations between spin and charge degrees of freedom on the dynamical properties of ferromagnetic systems governed by the magnetic exchange interaction between itinerant and localized spins. For this we introduce a general theory that treats quantum fluctuations beyond the random phase approximation based on a correlation expansion of the Green's function equations of motion. We calculate the spin susceptibility, spin-wave excitation spectrum, and magnetization precession damping. We find that correlations strongly affect the magnitude and carrier concentration dependence of the spin stiffness and magnetization Gilbert damping.     

Magnetic properties of undoped YBa 2 Cu 3 O 6 + x system

In the present paper, we study the magnetic properties of bilayer cuprate antiferromagnets. In order to evaluate the expressions for spin-wave dispersion, sublattice magnetization, Néel temperature and the magnetic contribution to the specific heat, the double time Green's function technique has been employed in the random phase approximation (RPA). The spin wave dispersion curve for a bilayer antiferromagnetic system is found to consist of one acoustic and one optic branch. The “optical magnon gap” has been attributed solely to the intra-bilayer exchange coupling (J _⊥ ) as its magnitude does not change significantly with the inter-bilayer exchange coupling (J_z). However J_z is essential to obtain the acoustic mode contribution to the magnetization. The numerical calculations show that the Néel temperature (T _N ) of the bilayer antiferromagnetic system increases with the J_z and a small change in J_z gives rise to a large change in the Néel temperature of the system. The magnetic specific heat of the system follows a T² behaviour but in the presence of J_z it varies faster than T². Received 13 July 2000 and Received in final form 14 May 2001     

On the competition between magnetic order and local Kondo effect in Kondo lattice

We investigate the competition between magnetic order and local Kondo effect in a Kondo lattice model (i.e. the Coqblin-Schrieffer Hamiltonian extended to a lattice) in a mean-field approximation, taking account of the spin-orbit degeneracy of each localized f level. This leads to the definition of a dependent Kondo temperature. We study the Kondo phase and compare its energy with the energies of magnetic phases, when the number of the conduction band electron per site is near one. We present a phase diagram which shows the occurrence of three phases: Kondo, antiferromagnetic and paramagnetic phases. Our model in the mean-field approximation also shows a somewhat flat Kondo temperature, for large values of , as a function of the exchange coupling J between conduction and localized f electrons. Finally we show some scaling effects between and J and we define a corresponding Kondo temperature. Received 21 September 1998 and Received in final form 8 February 1999     

Orbital contribution to the magnetic properties of nanowires: is the orbital polarization ansatz justified?

We show that considerable orbital magnetic moments and magneto-crystalline anisotropy energies are obtained for a Fe monatomic wire described in a tight-binding method with intra-atomic electronic interactions treated in a full Hartree Fock (HF) decoupling scheme. Even though the use of the orbital polarization ansatz with simplified Hamiltonians leads to fairly good results when the spin magnetization is saturated this is not the case of unsaturated systems. We conclude that the full HF scheme is necessary to investigate low dimensional systems.     

Magnetoconductance of a two-dimensional metal in the presence of spin-orbit coupling

We show that in the metallic phase of a two dimensional electron gas the spin-orbit coupling due to structure inversion asymmetry leads to a characteristic anisotropy in the magnetoconductance. Within the assumption that the metallic phase can be described by a Fermi liquid, we compute the conductivity in the presence of an in-plane magnetic field. Both the spin-orbit coupling and the Zeeman coupling with the magnetic field give rise to two spin subbands, in terms of which most of the transport properties can be discussed. The strongest conductivity anisotropy occurs for Zeeman energies of the order of the Fermi energy corresponding to the depopulation of the upper spin subband. The energy scale associated with the spin-orbit coupling controls the strength of the effect. More in particular, we find that the detailed behavior and the sign of the anisotropy depends on the underlying scattering mechanism. Assuming small angle scattering to be the dominant scattering mechanism our results agree with recent measurement on Si-MOSFET's in the vicinity of the metal-insulator transition. Received 11 July 2001     

三维Ising模型的Green函数方法处理

本文利用Creen函数方法,对三维Ising模型进行严格处理,得到一组可以递推的关于体系自旋系综平均值的线性方程。通过对体系自旋集团作切断近似,从而使得对体系转变温度,磁化强度等问题的求解,变成对一组代数方程的求解。本文表明,对较小的自旋集团,就可得到精度较高的结果。 关键词：     

单相ABO3型多铁材料的磁电耦合及磁电性质研究

实验发现多铁性钙钛矿物质YMnO₃和BiMnO₃在接近磁有序相变温度时,其介电常数和正切损失会出现异常,这些现象说明在物质的磁性和介电性质之间存在耦合.通过对系统磁性和铁电性之间可能磁电耦合方式的分析,考虑在系统哈密顿量中加入与自旋关联和极化相关的耦合项,对铁电子系统应用软模理论,对磁性运用基于海森伯模型的量子平均场近似,研究了外磁场诱导的极化、介电的变化和外电场诱导的磁化的变化等,并将以上结果与实验进行了比较和分析,较为合理地解释了一些多铁钙钛矿物质中的磁电现 关键词： 多铁 磁电耦合 铁电 铁磁