Optimization of highly efficient terahertz generation in lithium niobate driven by Ti:sapphire laser pulses with 30 fs pulse duration

We systematically study the optimization of highly efficient terahertz(THz) generation in lithium niobate(LN)crystal pumped by 800 nm laser pulses with 30 fs pulse duration. At room temperature, we obtain a record optical-to-THz energy conversion efficiency of 0.43% by chirping the pump laser pulses. Our method provides a new technique for producing millijoule THz radiation in LN via optical rectification driven by joule-level Ti:sapphire laser systems, which deliver sub-50-fs pulse durations.     

Toward generation of μJ range sub-ps THz pulses by optical rectification

Recently the possibility of scaling up the energy of sub-ps THz pulses generated in lithium-niobate by tilted pulse front excitation was demonstrated. Using 500 μJ energy pump pulses at 780 nm center wavelength, we achieved THz pulses with energy up to 240 nJ. In this article, results of calculations using a simple model predict the possibility of increasing the THz pulse energy above 1 μJ and the quantum efficiency up to 50% by decreasing the temperature. The dependence of the THz pulse energy and the maximum achievable electric field on the crystal length and the pump pulse duration is also presented. According to the calculations, generation of the maximum THz energy needs a specific pump pulse duration, because of increasing dispersion and absorption with increasing frequency. Not only longer, but also shorter pulses lead to a degradation of the THz energy. Results of calculations for GaSe, GaP and ZnTe are also presented. PACS 07.57.Hm; 42.65.Ky; 42.79.Nv     

Femtosecond parametric generation in ZnGeP(2)

We report traveling-wave optical parametric generation in short (2-mm) ZnGeP(2) samples with reduced anomalous absorption, using femtosecond pump pulses near 2 mum . The signal and the idler waves generated could be tuned from 2.5 to 10 mum , and they extend the tunability of the beta-barium borate optical parametric generator used as a pump source to the mid-infrared. At a single-pass internal conversion efficiency of 2.5% we estimate pulse durations of 75 fs (signal near 3 mum) and 200 fs (idler near 6 mum).     

Compact and high-power broadband terahertz source based on femtosecond photonic crystal fiber amplifier

We present a review of the development of a compact and high-power broadband terahertz (THz) source optically excited by a femtosecond photonic crystal fiber (PCF) amplifier.The large mode area of the PCF and the stretcher-free configuration make the pump source compact and very efficient.Broadband THz pulses of 150 μW extending from 0.1 to 3.5 THz are generated from a 3-mm-thick GaP crystal through optical rectification of 12-W pump pulses with duration of 66 fs and a repetition rate of 52 MHz.A strong saturation effect is observed,which is attributed to pump pulse absorption;a Z-scan measurement shows that three-photon absorption dominates the nonlinear absorption when the crystal is pumped by femtosecond pulses at 1 040 nm.A further scale-up of the THz source power is expected to find important applications in THz nonlinear optics and nonlinear THz spectroscopy.     

Femtosecond optical parametric converter in the 168–182-nm range

Femtosecond pulses continuously tunable in the vacuum ultraviolet (VUV) spectral range between 168 and 182 nm were generated using four-wave frequency mixing in an argon-filled capillary. The pulse energy reached 200 nJ at a pump-to-VUV conversion efficiency of 1%. The bandwidth at 181 nm was up to 27 THz corresponding to a transform limited duration of 17 fs. The upper limit in the shortest measured pulse duration was 75 fs.     

Generation of single-cycle THz transients with high electric-field amplitudes

Single-cycle terahertz (THz) transients in the frequency range 0.3-7 THz with electric-field amplitudes of more than 400 kV/cm are generated by four-wave mixing of the fundamental and the second harmonic of 25 fs pulses from a Ti:sapphire amplifier in ionized air. These transients are fully characterized by electro-optic sampling with ZnTe and GaP crystals. One can tune the center frequency of the THz transients by varying the length of the incident pulse. The electric-field amplitude increases linearly with the incident pulse energy.     

Generation of high average power 1 kHz shaped THz pulses via optical rectification

Generation of near single-cycle THz pulses from lithium niobate with 3.3 μJ energy, 3.3 mW average power, 1.2 THz central frequency and 4 MW peak power was demonstrated by tilting the intensity front of the pump pulses from a 1 kHz Ti:sapphire laser. THz pulse intensity as high as 200 MW/cm² was achieved. The energy conversion efficiency was 7 × 10⁻⁴. The capability of the present scheme to generate high energy shaped THz pulses was also demonstrated by using a sequence of optical pump pulses.     

飞秒超强激光驱动太赫兹辐射特性的实验研究

强太赫兹源是太赫兹科学技术发展的关键,其中大能量强场太赫兹脉冲源在超快物态调控、新型电子加速器等领域具有重要的应用前景.超快超强激光与等离子体相互作用是近年来发展起来的一种新型的强场太赫兹辐射产生途径.本文报道了利用超强飞秒激光脉冲与金属薄膜靶作用产生太赫兹辐射的实验结果,研究了激光能量和离焦量对靶后太赫兹辐射能量的影响,并通过监测激光背向散射光谱,定性揭示了其变化规律与不同光强下的电子加热机制的相关性.实验表征了太赫兹辐射的频谱、偏振及聚焦光斑情况.测量结果表明,实验产生了脉冲能量达458μJ、聚焦场强高达GV/m量级的超宽带太赫兹辐射,为开展极端太赫兹脉冲与物质相互作用研究提供了一种新的强场太赫兹光源.     

Scaling submillimeter single-cycle transients toward megavolts per centimeter field strength via optical rectification in the organic crystal OH1

We present the generation of high-power single-cycle terahertz (THz) pulses in the organic salt crystal 2-[3-(4-hydroxystyryl)-5.5-dimethylcyclohex-2-enylidene]malononitrile or OH1. Broadband THz radiation with a central frequency of 1.5 THz (λ(c)=200 μm) and high electric field strength of 440 kV/cm is produced by optical rectification driven by the signal of a powerful femtosecond optical parametric amplifier. A 1.5% pump to THz energy conversion efficiency is reported, and pulse energy stability better than 1% RMS is achieved. An approach toward the realization of higher field strength is discussed.     

Stable mode-locked fiber laser using 49 cm long bismuth oxide based erbium doped fiber and slow saturable absorber

A stable mode-locked fiber laser employing a 49 cm long bismuth oxide based erbium doped fiber (Bi-EDF) by using a slow saturable absorber is demonstrated. Near transform limited short pulses with a repetition rate of 8.27 MHz are obtained at a wavelength of 1560 nm with a maximum spectral width of 15 nm. Results indicate that pulse characteristics are strongly dependent on pump power rather than spectral width. Moreover the Time-Bandwidth products (TBWP), pulse duration, the energy fluctuation and timing jitter decrease with increasing pump power. The pulse width is continuously varied from 1.2 ps to less than 300 fs. It produces stable mode locking with a maximum spectral width of 15 nm, minimum timing jitter of 4 ps and energy fluctuations of 2.5%. The pulse train was amplified using a two-stage amplifier up to 447 mW average power corresponding to peak powers of 177.3 kW.     

基于大基模体积的10mJ飞秒钛宝石激光再生放大器

文章报导了基于大基模体积的高能量飞秒钛宝石激光再生放大器的设计与实验研究,在重复频率10 Hz、抽运能量60 mJ的激励下,得到了单脉冲能量17.4 mJ的种子脉冲放大结果,压缩后的脉冲宽度为40.6 fs,能量为13.9 mJ.借助于此大基模体积再生腔,仅增加一级多通放大,实现了峰值功率达1.9 TW飞秒激光脉冲输出.结果表明,大模体积再生放大不仅降低了后续放大对抽运能量的要求,也可以单独压缩实现再生腔直接输出10 mJ量级的飞秒激光脉冲,是大能量高峰值功率飞秒激光系统的优质前端.     

Dissociation and ionization of H+2 by ultrashort intense laser pulses probed by coincidence 3D momentum imaging

Laser-induced dissociation and ionization of H(+)(2) were simultaneously measured using coincidence 3D momentum imaging, allowing direct separation of the two processes, even where the fragment kinetic energy is the same for both processes. The results for 45 and 135 fs 790 nm pulses with an intensity of approximately 2.5 x 10(14) W/cm(2) differ from each other much more than one would expect from previous measurements with longer pulses. Ionization was negligible for the longer pulse and was strongly aligned along the laser polarization for the shorter pulse, but showed no structure in its kinetic energy distribution. In addition, the ionization to dissociation ratio was found to be much smaller than theoretically predicted for H(+)(2).     

Temperature dependent narrow-band terahertz pulse generation in periodically poled crystals via difference frequency generation

Femtosecond optical pulse is used to generate narrow-band terahertz pulses depending on a quasi-phase-matched condition in periodically poled lithium niobate (PPLN) and stoichiometric lithium tantalate (PPSLT) crystals by difference frequency generation. The origin of narrow-band THz generation proved that the two frequency components of the fs pulse contribute to the frequency mixing. By cryogenic cooling, the absorption of THz waves in the crystal is significantly reduced which results in efficient THz generation. Simultaneously generated forward and backward THz pulses were 1.38 and 0.65 THz with as narrow as the bandwidth of 32 GHz in the PPSLT sample. Temperature dependence of the generated THz waveforms had good agreement with the simulation result using one dimensional plane-wave propagation model.     

20-50-fs pulses tunable across the near infrared from a blue-pumped noncollinear parametric amplifier

A two-stage blue-pumped noncollinearly phase matched optical parametric amplifier was used to generate near-infrared pulses that were continuously tunable from 865 to 1600 nm. The pulse lengths scaled from 20 fs at the shorter wavelengths to below 50 fs at 1600 nm, with a nearly Fourier-transform-limited bandwidth. From 200 muJ of 775-nm pump light at a 1-kHz repetition rate and a 130-fs duration, 7-2.5-muJ pulse energies were generated, corresponding to a typical quantum efficiency of 25% from blue to near-infrared light.     

High-power output from a compact OPCPA laser system

With a tabletop hybrid Nd:YAG-Nd:glass laser as pump source, a compact optical parametric chirpedpulse amplification(OPCPA)laser system with a peak output power of 16.7 TW and a pulse duration of120 fs has been demonstrated.Chirped pulses are amplified from 50 pJ to more than 3.1 J with an energygain of above 6×10~(10)by three LBO optical parametric amplifiers with a pump energy of 12.4 J at 532nm.After compression, a final output of 2.0-J/120-fs pulse is obtained. To the best of our knowledge,itis the highest peak output power from an OPCPA laser so far.In addition, a practical design of 1-PWlaser system based on the technique of OPCPA is also proposed.     

Generation of 2.5 μJ vacuum ultraviolet pulses with sub-50 fs duration by noncollinear four-wave mixing in argon

Generation of sub-50fs vacuum UV pulses with more than 2.5μJ energy at a 1kHz repetition rate is reported. The pulses at 160nm are produced using noncollinear difference-frequency four-wave mixing between the fundamental and third harmonics of an amplified Ti:sapphire laser in argon. While the pulse duration is maintained by increasing the phase-matching pressure, noncollinear interaction improves the conversion efficiency by 1 order of magnitude in comparison with the previous results in collinear geometry.     

Degenerate parametric frequency conversion of phase-modulated femtosecond laser pulses in crystals with a regular and chirped domain structure

A systematic theoretical analysis of the degenerate parametric frequency conversion in a LiNbO₃ crystal with a regular domain structure and a linearly varying domain thickness (chirped crystal) is presented for the pulses of a titanium-sapphire laser with a wavelength of 0.8 μm and durations of 100 and 50 fs in the presence and in the absence of phase modulation. The results are obtained with regard to the difference in the group velocities of interacting pulses and the group velocity dispersion. For an effective frequency conversion of the phase-modulated (PM) pump pulse, it is expedient to employ chirped crystals in which the domain thickness decreases from the entrance to the exit of the crystal. The pump energy is effectively converted into subharmonic energy when the pump carrier frequency decreases with time. It is demonstrated that the efficiency of the energy conversion to a subharmonic of 80% can be realized for PM pumping with a pulse duration of 100 fs in the chirped LiNbO₃ crystal. The efficiency of the parametric frequency conversion depends on the pump intensity as well as on the phase modulation of the pulse and the chirp of the crystal. Note that a variation in one of these parameters causes variations in the remaining parameters needed for the maximum efficiency of the parametric frequency conversion.     

Diode-pumped, high-average-power femtosecond Cr3+ :LiCAF laser

We demonstrate a high-average-power continuous wave (cw) and cw mode-locked Cr3+ :LiCAF laser pumped by broad-area laser diodes. In cw lasing experiments, up to 580 mW of output was obtained with 4.35 W of incident pump. A semiconductor saturable absorber mirror was used to initiate stable, self-starting, mode locking. In the cw mode-locked regime, the Cr3+ :LiCAF laser produced nearly transform-limited, 67 fs long pulses near 800 nm with an average output power of 300 mW. The pulse repetition rate was 120 MHz, with a pulse energy of 2.5 nJ.     

多脉冲激光增强太赫兹辐射的PIC模拟

 模拟了强激光和稀薄非均匀等离子体相互作用在界面辐射超强太赫兹波的物理过程,提出了利用多脉冲激光增强太赫兹辐射的方案,详细研究了多脉冲激光的脉冲个数（取１～４个）、脉冲间距等因素对太赫兹辐射功率和频率的影响。当入射激光包含4个脉冲时,辐射最强,此时的辐射功率是相同条件下单脉冲的6倍,可达到7.16 MW,辐射的太赫兹波的脉宽约为330 fs,总能量约为1 μJ。研究结果表明:多脉冲激光可以显著增强太赫兹辐射,且随着脉冲个数的增加,激起的电子静电波振幅变大,辐射功率也随之变大,直到尾流场饱和;当脉冲间距等于入射激光脉宽时辐射最强。     

Heating of Nanosized Liquid Water in High-Intensity Terahertz Pulses

Non-equilibrium molecular dynamics simulations of liquid water in picosecond high-power terahertz pulses are performed by using a non-polarizable potential model.Numerical results show that the energy absorption of water molecules exhibits a pronounced resonance with THz pulses in the frequency range of 14-17 THz.With the THz pulse at resonant frequencies,the maximum temperature is about 562 K by heating the water at room temperature.Further investigation indicates that the results are independent of the size of the nanoscale water box.The efficiency of energy transfer by resonant absorption is more than seven times of microwave heating.These studies show promising applications of ultrashort THz pulses.