载波相位对超短正弦高斯脉冲的影响

在时间域中研究了载波相位对超短正弦高斯脉冲的影响.给出了超短正弦高斯脉冲的脉冲能量和时间重心的解析表达式和数值模拟结果.结果表明载波相位和正弦函数的参数对超短正弦高斯脉冲的脉冲能量和时间重心有很大的影响.当载波相位等于nπ和2n+1π/2时,超短正弦高斯脉冲的脉冲能量分别达到最小和最大值;当载波相位等于2n+1π/4时,载波相位对超短正弦高斯脉冲的脉冲能量没有影响.当载波相位等于4n+3π/4和4n+1π/4时,超短正弦高斯脉冲的时间重心分别达到最小和最大值;当载波相位等于nπ/2时,超短正弦高斯脉冲的时间重心不发生变化.     

铷原子低次谐波产生中的载波拉比振荡特征

本文通过数值求解三维含时薛定谔方程,研究了铷原子在ω=E_5p-E_5s共振激光及非共振激光驱动下的三次谐波发射特性.结果表明,在共振波长驱动下,当脉冲面积为2π时,三次谐波展示了一个正常的峰值结构,通过分析5s态和5p态的布居分布,发现这种峰值结构源于拉比振荡;随着脉冲面积的增大,三次谐波结构变得更加复杂,其与载波拉比振荡相关,此时面积定理不再适用.在非共振波长驱动下,无论脉冲面积为2π或者大于2π,三次谐波都展示出正常的峰值结构,通过布居分析,发现非共振波长驱动下,不能满足拉比振荡及载波拉比振荡的条件.     

不同激光脉冲宽度下甲苯的光学非线性特性的研究

在不同激光脉冲激发下,用Z 扫描法测量了甲苯的三阶光学非线性,发现其非线性折射率随着脉冲宽度增加而增大（从150 fs时的3.7×10－16 cm2/W到4 ns时的2.6×10－14 cm2/W）.在波长532 nm、光强4.73×1014 W/m2 和21 ps的脉冲作用下,甲苯溶液呈现反饱和吸收现象.结果表明,该吸收效应主要来自于导致该分子中苯环结构π－π电子跃迁的双光子吸收的贡献.     

相位变形组合π脉冲NMR

描述了相位变形组合π脉冲序列核磁共振,进行了理论分析. 对脉冲角和相位角进行优化,在优化过程中使用了Wigner矩阵元Z₂₂（函数）及函数对脉冲角、相位角的一阶导数. 利用自编子程序DBSLSJ和SOLEQJ代替“IMSL”程序库DBCLSJ进行非线性最小二乘法求极小值点. 计算是在PⅢ PC机上进行,其优化结果和IBM/3600大型计算机计算结果吻合,并优于文献报道的其它组合π脉冲.     

Ladder型三能级介质中传播的少周期激光脉冲的空间分布

利用由时域有限差分法和预估校正法求得全波Maxwell-Bloch方程的数值解,研究少周期超短激光脉冲在Ladder型三能级原子介质中传播时脉冲及介质粒子布居的空间分布.结果表明,脉冲及介质粒子布居的空间分布规律随脉冲面积的改变而发生明显的变化.当脉冲面积较小时,脉冲形状不规则,振荡次数较多;当脉冲面积较大时,脉冲形状变得较为规则,振荡次数明显减少.随着脉冲面积的增大,脉冲振幅和传播速度逐渐增大,各能级粒子布居振荡次数增多,不同时刻的脉冲和粒子布居空间分布的变化明显减小.粒子布居的空间分布与脉冲的空间分布密切相关.     

掺镱光纤放大器泵浦脉宽优化

为抑制低重复频率高能脉冲光纤主振荡功率放大(MOPA)系统的放大自发辐射(ASE)效应,达到脉冲泵浦的最佳放大效果,需要对泵浦脉宽进行优化。基于求解速率方程和功率传输方程,理论研究了脉冲泵浦下掺镱光纤放大器上能级粒子数密度、光纤内存储能量、正反向放大自发辐射的瞬态响应。在给定的泵浦功率、光纤长度、纤芯面积和掺杂数密度等参数下,数值计算得到的优化泵浦脉宽为793 s。此外,实验测定了ASE的建立时间; 通过调节泵浦脉宽,测定了脉冲泵浦下掺镱光纤放大器的放大效果,实验中得到的泵浦脉宽的优化值为800 s,证明了数值模拟的正确性。     

二能级原子各态几率随脉冲面积变化的2π准周期衰减振荡

二能级原子各态几率随脉冲面积的变化过程将呈现2π准周期衰减振荡,这一结果可为研究任意强激光脉冲作用下的原子行为提供很好的普遍演变图象.     

基于密度泛函理论下多肽光谱性质研究

多肽类物质在生物医药等领域是一种重要的生物大分子,而紫外-可见吸收光谱和荧光光谱是研究生物分子精细结构的重要手段。采用密度泛函理论（DFT/RI）计算了生长激素释放肽（GHRP-6）和催产素（Oxytocin）两种多肽的结构模型和分子前线轨道;在含时密度泛函理论（TDDFT）的基础上,引入了TDA等近似,建立了多肽类物质的紫外-可见吸收光谱和荧光光谱的理论模型。结果表明,实验测得到GHRP-6的紫外-可见吸收光谱最大吸收波长为279 nm,计算得到的最大吸收波长为282 nm,误差为3 nm,误差百分比约为1%;Oxytocin紫外-可见吸收光谱的实验值为275 nm,计算值为269 nm,误差百分比约为2%。GHRP-6荧光光谱计算值为368 nm,实验值为360 nm,误差百分比约为2%;Oxytocin荧光光谱计算值为305 nm,实验值为312 nm,误差百分比约为2%。GHRP-6产生荧光的发射波长与色氨酸产生的荧光波长范围相近,说明GHRP-6产生荧光的主要贡献为色氨酸残基上的π→π*轨道跃迁,Oxytocin荧光峰位置与酪氨酸产生的荧光波长范围相近,Oxytocin产生荧光的主要贡献为酪氨酸残基上的π→π*轨道跃迁。根据该模型计算得到的光谱与实验结果吻合度较高,表明该模型能够准确计算多肽类物质紫外-可见吸收光谱和荧光光谱,为实验提供可靠的理论依据。     

亚毫微秒脉冲染料激光器的瞬态过程的研究

本文报导一种N_2激光器泵浦的亚毫微秒弛豫振荡脉冲染料激光器.用实验观测了其弛豫振荡及亚毫微秒脉冲的形成过程,并根据振荡的瞬态过程不同阶段,采取分别求速率方程组近似解的方法,对其工作过程进行了理论分析.将有关参量和实验测量值代入这些解,所估算的脉冲宽度数量级与实验显示值能较好地相符合.     

低强度周期量级脉冲驱动排列分子的非次序双电离

本文利用三维经典系综模型研究了低强度周期量级脉冲驱动排列分子的非次序双电离. 结果表明, 电子对的关联特性强烈地依赖于分子的排列方向和激光脉冲的载波包络相位; 垂直分子反关联电子对的比例总是高于平行分子反关联电子对的比例; 当载波包络相位从0到π 逐渐增加时, 反关联电子对的数目先增加再减少; 对于平行分子, 电子对的释放总是以正关联为主; 而垂直分子的主导关联模式则依赖于激光脉冲的载波包络相位, 当载波包络相位为0.3π-0.7π之间时, 电子对以反关联释放为主, 其他相位下以正关联为主. 本文利用分子势能曲线和电子返回能量很好地解释了电子关联特性对分子排列方向和载波包络相位的依赖关系.     

非均匀展宽对超短激光脉冲传播特性的影响

用建立的"预报校正-四阶龙格库塔"数值算法研究了非均匀展宽二能级体系中超短激光脉冲的传播特性。计算结果表明,非均匀展宽线型的线宽对光脉冲传播会产生调制作用。当线宽大于脉冲的频谱宽度时,脉冲面积演化与面积定理相符且脉冲传播平稳;但随着线宽的减小,脉冲面积演化会越来越偏离面积定理,脉冲传播不再平稳并出现"拖尾"振荡。脉冲主峰的峰值和脉冲的传播速度也受到线宽的影响。     

The effect of the homogeneous broadening on the propagation of the light pulses

The propagation of resonant pulses in a two-level homogeneously broadened atomic medium is analyzed. The pulses with the duration comparable with the atomic coherence relaxation time are considered. The effects of the long pulse area stabilization and destabilization are reported. The numerical simulation is performed.     

光学Maxwell-Bloch方程的数值算法研究及其应用

建立了高准确度快速求解均匀展宽二能级体系光学Maxwell-Bloch耦合方程的数值算法.通过与特定条件得到的解析解的比较,验证了算法所具有的高收敛性和稳定性,并可保持算法的误差阶数,因此算法是可靠并实用的.应用该算法数值求解了一般条件下的MB方程,并由计算结果分析了失谐量、弛豫时间、初始光强对光脉冲在介质中的传播及对Bloch矢量演化的影响.所建立的数值算法对MB方程以及修正的这类偏微分方程组具有普适性.     

Acoustic self-induced transparency for transverse waves in a system with resonant and quasi-resonant transitions

A theoretical analysis of acoustic self-induced transparency is presented for transverse elastic waves propagating perpendicular to an applied magnetic field through a crystal with spin-3/2 paramagnetic impurities. The interaction between an acoustic pulse and magnetic field is described by Maxwell-Bloch-type equations for a system with transitions inhomogeneously broadened because of a quadrupole Stark shift. If the pulse carrier frequency is resonant with one transition and quasi-resonant with another transition, then the evolution of a one-dimensional pulse is described by an integrable Konno-Kameyama-Sanuki (KKS) equation. The underlying physics of its soliton solution and the corresponding behavior of the medium are analyzed. Self-focusing and self-trapping conditions are found for a pulse of finite transverse size. In the latter regime, the pulse stretches along the propagation direction, transforming into a “hollow bullet,” while its transverse size remains constant.     

周期量级激光脉冲在不同密度的原子介质中传播行为的比较(英文)

利用不含慢变包络近似和旋波近似的全波Maxwell-Bloch方程组的数值解,研究了周期量级超短激光脉冲在Ladder型三能级原子介质中的传播行为并与在相应的稀疏介质中的情况进行了比较.我们发现,在传播过程中,超短脉冲在稠密介质中的时间演化规律与在稀疏介质中明显不同,而且这种差别将随初始脉冲面积的增大而加大.当初始脉冲面积较小时,在传播过程中,脉冲形状在稀疏介质中只有小的改变而在稠密介质中却有显著的变化.当初始脉冲面积足够大时,在稠密介质中在不同的传播距离处脉冲分裂为不同数量和形状的亚脉冲;在稀疏介质中脉冲形状在传播过程中仍然只有小的改变。产生以上差别的原因在于稠密原子介质中近偶极-偶极(NDD)相互作用导致的局域场修正(LFC)及比稀疏原子介质更强的极化电场的影响.其中,更强的极化电场的影响起着主要的作用,但局域场修正的作用也不能忽略,而极化电场的增强是由于原子密度的增加.     

周期量级激光脉冲在不同密度的原子介质中传播行为的比较

利用不含慢变包络近似和旋波近似的全波Maxwell-Bloch方程组的数值解,研究了周期量级超短激光脉冲在Ladder型三能级原子介质中的传播行为并与在相应的稀疏介质中的情况进行了比较.我们发现,在传播过程中,超短脉冲在稠密介质中的时间演化规律与在稀疏介质中明显不同,而且这种差别将随初始脉冲面积的增大而加大.当初始脉冲面积较小时,在传播过程中,脉冲形状在稀疏介质中只有小的改变而在稠密介质中却有显著的变化.当初始脉冲面积足够大时,在稠密介质中在不同的传播距离处脉冲分裂为不同数量和形状的亚脉冲|在稀疏介质中脉冲形状在传播过程中仍然只有小的改变。产生以上差别的原因在于稠密原子介质中近偶极-偶极(NDD)相互作用导致的局域场修正(LFC) 及比稀疏原子介质更强的极化电场的影响.其中,更强的极化电场的影响起着主要的作用,但局域场修正的作用也不能忽略,而极化电场的增强是由于原子密度的增加.     

Spectrum and wave shape of intense laser pulse propagating through Raman active medium

Results of the analytical solution of non-linear equations describing the propagation of an ultra-short intense laser pulse through a Raman-active medium are presented. The pulse passing through the medium generates a large number of high-order harmonics if the pulse intensity is close to some thresholds. The medium is described by the density matrix for two-level systems. The laser pulse duration was much shorter than both the period of oscillation and the relaxation times of an oscillator. Using this solution, the spectrum of such a pulse was expressed in terms of integrals of the initial field. The solution allows the harmonic spectrum dependence on the pulse intensity and effects of propagation to be investigated. Estimations of the conversion efficiency of the initial pumping frequency into high-order harmonics are given. The evolution of the pulse shape as a function of the distance passed by the pulse through the media was investigated. This revised version was published online in November 2006 with corrections to the Cover Date.     

Steady pulse propagation in an inhomogeneously broadened resonant medium

Steady propagation of a single pulse in an inhomogeneously broadened resonant medium is studied. 2π-pulse solutions which are slightly different from those given in the literature are reported and it is shown that π-pulse solutions do not exist.     

Area of ultimately short light pulses

The evolution of the area of a pulse of optical radiation propagating in a nonlinear medium is analyzed. The role played by the medium relaxation and the correctness of the formulation of the problem on the propagation of short pulses are discussed.     

Quantum theory of light propagation in a fluctuating laser-active medium

The basic equations are derived which describe the propagation of an electromagnetic field in a fluctuating laser-active medium. The well-known methods of Langevinequations and master-equation for a few discrete modes are generalized to meet also the case of a radiation field with continuous spectrum. The medium is described by two-level atoms which are embedded in a merely passive solid matrix and homogeneously distributed over space. They have an inversion which is kept constant by an externally applied pump. The atomic line may be homogeneously or inhomogeneously broadened. We obtain a complete set of partial differential equations for the field operators with damping terms and fluctuating forces homogeneously distributed over the material. The telegraph equation with a fluctuating force occurs as a special case. After the exact elimination of the atomic variables we obtain a nonlinear field equation for the radiation field alone. By means of a pseudo-Hamiltonian and by a simple one-dimensional example we show that in a certain sense there exists a close formal analogy between the present theory and the theory of an interacting Bose gas. The characteristic differences between the two theories are also discussed. We find, that there occurs a phase transition of the radiation field because above a certain threshold of the pump the photons condense into a single mode and establish an “offdiagonal-long-range order”. The amplitude fluctuations and the phase fluctuations, which restore the broken phase symmetry, are calculated in detail. A new condition for the occurrence of undamped spiking (pulse formation) for a continuum of modes is derived.