14MeV中子引起的Pb(n,x)203Hg, W(n,x)182Ta和W(n,x)183Ta的核反应截面测量

利用活化方法测量了14MeV中子引起的Pb(n,x)²⁰³Hg,W(n,x)¹⁸²Ta和W(n,x)¹⁸³Ta的反应截面.中子注量由监督反应⁹³Nb(n,2n)^92mNb给出,中子能量利用⁹⁰Zr(n,2n)^89m+gZr和⁹³Nb(n,2n)^92mNb反应的截面比来确定.     

光子穿透系数及同质异能态俘获截面的研究

合理地给出了复合核反应光子穿透系数及同质异能态俘获截面的计算公式,其中包括统计和非统计过程.通过求解级联γ退激过程计算光子穿透系数,既合理地扣除(n,γn)过程,又包括首次γ跃迁至中子分离能B_n以上能级的贡献.以4MeV以下中子和⁵⁹Co及¹⁰³Rh的反应为例,比较用不同方法计算的光子穿透系数,计算同质异能态俘获截面并和实验数据进行比较,最后对结果进行了分析和讨论.     

用基态特征γ射线计算同质异能态反应截面的公式及其应用

根据人工放射性的生长与衰变规律, 推导出一个在特殊情况下用基态特征γ射线计算同质异能态反应截面的公式, 并据此公式用活化法以⁹³Nb(n,2n)^92mNb反应截面为中子注量标准对¹²⁸Te(n,2n)^127mTe反应截面进行了测量. 由能量为(14.1±0.2)和(14.6±0.3)MeV的中子引发的¹²⁸Te(n,2n)^127mTe反应截面值分别为(737±69)和(853±82)mb. 单能中子用T(d,n)⁴He反应获得, 其能量用铌锆截面比法测定. 为减小热中子的(n, γ)反应的影响, 在辐照过程中对样品进行了包镉处理.     

Ba(n,x)134Cs,134Ba(n,2n)133Ba,140Ce(n,2n)139Ce,142Ce(n,2n)141)Ce和23Na(n,2n)22Na反应截面的测量

用中子活化法相对于⁵⁴Fe(n,P)⁵⁴Mn反应,在13.50—14.80MeV中子能区测量了Ba(n,x)¹³⁴Cs,¹³⁴Ba(n,2n)¹³³Ba,¹⁴⁰Ce(n,2n)¹³⁹Ce,¹⁴²Ce(n,2n)¹⁴¹Ce和²³Na(n,2n)²²Na的反应截面.并将所测的结果和其他作者的结果进行了比较,中子能量是用⁹⁰Zr(n,2n)^89m+gZr反应和⁹³Nb(n,2n)^92mNb反应截面比法测定的.     

197Au（n,2n）反应中同质异能素截面比

用活化法测量了15MeV中子引起¹⁹⁷Au（n,2n）反应的同质异能素截面比。使用Huizenga-Vandenbosch描述的方法计算了该反应的同质异能截面比,根据实验值同理论值的比较,确定了产物核的自旋切割因子和核有效转动惯量的值。     

85Rb(n, 2n)84Rb反应中同质异能态截面比

在14.7MeV中子能量下, 测量了⁸⁵Rb(n,2n)反应同质异能态截面及其比值. 实验比值与Vandenbosh-Huizenga方法算出的理论值做了比较, 定出了自旋切割因子σ值.     

近垒及垒下12C+93Nb的蒸发剩余核截面

使用离线γ测量技术在实验室系28.3MeV至45.7MeV的能区首次测量了¹²C+⁹³Nb反应产生的8个核素及同质异能态的激发函数.使用包括非弹性激发和α转移道的简单耦合道模型,结合统计蒸发程序对实验结果进行拟合.计算结果能较好地重现强截面的中子蒸发道(xn)的激发函数.而对于弱的质子(xpyn)特别是α粒子(xαyn)蒸发道的截面,实验测量明显高于模型计算结果.α转移道与入射道耦合作为熔合反应的门庭态使垒下能区重离子熔合截面有很大的加强,实验测量与理论计算的比较表明对于¹²C+⁹³Nb反应系统在垒下能区可能存在着很强的α转移截面.     

143Nd中高自旋同质异能态的识别与研究

利用能量为80MeV的18O束流,通过¹³⁰Te(¹⁸O,5n)反应研究了¹⁴³Nd的高自旋态能级结构.基于γγ延迟符合、γ射线的角分布及线性极化测量,首次发现了¹⁴³Nd的一个半寿命为(35±8)ns,自旋和宇称为49/2⁺的同质异能态.用形变独立粒子模型探讨了此同质异能态的形成机制.     

产生长寿命核的几个(n,2n)反应截面的测量

本文报道了E_n=13.5—14.8MeV中子能区几个长寿命生成核的(n,2n)反应截面的测量.测量方法是以⁹³Nb(n,2n)^92mNb反应截面为中子注量标准的相对活化法.测量的几个反应为:¹⁵¹Eu(n,2n)^150mEu、¹⁵³Eu(n,2n)¹⁵²Eu、¹⁵⁹Tb(n,2n)¹⁵⁸Tb和¹⁰⁹Ag(n,2n)^108mAg.中子能量是用铌锆截面比法测定的.本文的结果和已收集到的测量结果进行了比较.     

中子反应同质异能态截面比的系统学

提出了中子反应同质异能态截面比的半经验公式.该公式含有一系统学参数,适应于产物核质量数44≤A≤197、同质异能态自旋0≤J_m≤12和基态自旋0.5≤J_g≤8的中子反应.在入射中子能量E_n<20MeV能区,对该系统学参数进行了系统学研究.通过获得的半经验公式和系统学参数,可以很好地再现已有实验数据,也可较好地预言无实验数据的同质异能态截面比或同质异能态截面.     

ISOMERIC CROSS SECTION RATIO IN THE 197Au(n,2n)196Au REACTION

Isomeric cross section ratio for the ¹⁹⁷Au (n, 2n) reaction at 15 MeV is measured by the activation method. Using the Huizenga and Vandenbosch method, the isomeric ratio is calculated for the reaction. From the comparison of the measured and theoretically calculated isomeric ratio, the values of the spin cut-off factor and nuclear moment of inertia are determined.     

Measurement of Cross Sections for Pb(n,x)203Hg,W(n,x)182Ta and W(n,x)183Ta Reactions Induced by 14 MeV Neutrons

The cross sections for Pb(n,x)²⁰³Hg,W(n,x)^l82Ta and W(n,x)¹⁸³Ta reactions have been measured by the activation method. The neutron fluences were determined by the cross sections of ⁹³Nb (n,2n)^92mNb reaction. The neutron energies in the measurements were determined by the cross section ratios of Zr(n,2n)^89m+gZr and Nb(n,2n)^92mNb reactions.     

DETERMINATION OF THE AVERAGE NEUTRON ENERGY USING CROSS SECTION RATIO OF 58Ni(n,p)58m+gCo and 58Ni(n,2n)57Ni REACTIONS

The method of determination for average neutron energy from D-T reaction by using two silicon semiconductor detectors and the cross section ratios of ⁵⁸Ni(n,p)^58m+gCo and ⁵⁸Ni(n,2n)⁵⁷Ni reactions is described.The plot of the cross section ratio against the neutron energy has been obtained.The results have been compared with existing data.     

Isomeric cross sections for the (n, 2n) reaction on 82Se, 81Br,and 45Sc at 15.1 MeV

Activation techniques have been used to measure the cross sections at 15.1 MeV neutron energy for the following reactions: ⁸²Se(n, 2n)^81m+gSe, ⁸¹Br(n, 2n)^80m+gBr, and ⁴⁵Sc(n, 2n) ^44m+gSc. Isomeric cross-section ratios were evaluated by applying the method of least squares to the time behavior of γ-ray activity following the ground-state decay of each isomeric pair. The absolute cross section σ_m for the formation of the metastable state was measured by the mixed-powder method with the ²⁷Al(n, α)²⁴Na reaction as the monitor. The cross section σ_g for the formation of the ground state was then determined by using the isomeric cross-section ratio. The sum of σ_m and σ_g for each reaction is compared with the theoretical value obtained from calculations based on the statistical model for the formation of a compound nucleus and its subsequent emission of neutrons.     

THE SYSTEMATIC CALCULATIONS OF (n,2n) AND (n,3n) REACTION CROSS SECTIONS FOR MEDIUM-HEAVY NUCLEI AT 14.5MeV

The (n,2n) and (n,3n) reaction processes have been studied by mechanism analysis of the neutron-induced nuclear reactions,formulae for evaluating the reduced cross section have been given.The cross sections of 14.5MeV (n,2n),(n,3n) reactions have been calculated according to the systematic method for Z=58—83 about 53 nuclei.A good agreement between the results of the systematic calculations and the experimental data has been reached.     

Ba（n，x）~（134）Cs，~（134）Ba（n，2n）~（133）Ba，

用中子活化法相对于５４Ｆｅ（ｎ，Ｐ）５４Ｍｎ反应，在１３．５０—１４．８０ＭｅＶ中子能区测量了Ｂａ（ｎ，ｘ）１３４Ｃｓ，１３４Ｂａ（ｎ，２ｎ）１３３Ｂａ，１４０Ｃｅ（ｎ，２ｎ）１３９Ｃｅ，１４２Ｃｅ（ｎ，２ｎ）１４１Ｃｅ和２３Ｎａ（ｎ，２ｎ）２２Ｎａ的反应截面．并将所测的结果和其他作者的结果进行了比较，中子能量是用９０Ｚｒ（ｎ，２ｎ）８９ｍ＋ｇＺｒ反应和９３Ｎｂ（ｎ，２ｎ）９２ｍＮｂ反应截面比法测定的。     

Cross-section measurement for Ni(n,x)58(m+g)Co,Ni(n,x)60mCo,Ni(n,x)61Co and Ni(n,x)62mCo reactions induced by neutrons around 14MeV

The cross sections of Ni(n,x)58(m+g)CO,Ni(n,x)80mCo,Ni(n,x)61Co and Ni(n,x)62mCo reactions induced by neutrons around [14]MeV were measured in this work and calculated by a previously developed formula in this work.The neutron flux was determined using the monitor reaction 27Al(n,α)24Na and the neutron energies were measured with the method of cross-section ratios for 89Zr(n,2n)89Zr to 93Nb(n,2n)92mNbreactions.     

替代反应法测量锕系核(n,f)和(n,xn)截面

对于某些中子反应截面,在直接测量上存在困难。为了获得那些对核能发展极其重要的核数据,人们提出替代反应法,即利用带电粒子代替中子进行反应,从而实现中子反应截面间接测量的方法。现有替代反应一般采用非弹激发、转移等周边反应,涉及的角动量远比中子反应的大,需要理论修正,这造成了一定的困难。有鉴于此,提出利用轻带电离子的俘获反应作为替代反应,其复合核自旋与中子反应的相当,有效避免了自旋修正的困难。根据这个思路,采用236U的（α,f）和（α,2n）反应作为替代反应,成功提取了239Pu的（n,f）和（n,2n）反应截面,与ENDFB7评价库数据在误差范围内符合较好,表明了替代反应法的优越性,可以在核数据测量中推广应用。There are always difficulties in the direct measurement of reactions induced by neutron, in order to obtain the neutron induced nuclear reaction data which are extremely important for nuclear power development, the surrogate reaction method, which uses charged particles instead of neutron, was proposed. The existing surrogate reaction method generally chooses peripheral reaction as the surrogate reaction, such as inelastic scattering excitation or transfer reaction. As a result, the angular momentum involved is always far larger than the neutron induced reaction, which causes difficulties in the theoretical calculation. Because of this, we proposed to use light-ion capture reaction as the surrogate reaction, the compound nuclei spin is similar with that of the neutron induced reaction, so that the difficulties in spin correction can be effectively avoided. Based on this idea, the 239Pu(n, f) and (n, 2n) reaction cross sections were successfully extracted using 236U(α,f) and (α,2n) reactions as the surrogate reaction. The results coincide well with the data of ENDFB7 within the error range, which shows that the surrogate reaction method has its own superiority, and it can be applied in the measurement of nuclear data.     

Cross-sections for the formation of isomeric pair Ge through (n, 2n), (n, p) and (n, α) reactions measured over 13.73 MeV to 14.77 MeV and calculated from near threshold to 20 MeV neutron energies

The cross-sections for formation of isomeric pair, ⁷⁵Ge^m(σ_m) and ⁷⁵Ge^g(σ_g), through ⁷⁶Ge(n, 2n), ⁷⁵As(n, p) and ⁷⁸Se(n, α) reactions were measured at 13.73 MeV, 14.42 MeV and 14.77 MeV neutrons and also estimated using EMPIRE-II and TALYS codes over neutron energies from near threshold to 20 MeV. For each (n, 2n), (n, p) and (n, α) reaction, the cross-section initially increases with neutron energy, but starts decreasing as the neutron energy exceeds the respective threshold of (n, 3n), (n, pn) and (n, αn) reactions. The higher values of σ_m relative to σ_g reveal that the transitions of the excited ⁷⁵Ge from higher energy levels to metastable state (7⁺/2) are favored as compared to unstable ground state (1⁻/2). The present values of cross sections for formation of ⁷⁵Ge^m,g through (n, 2n) and (n, α) reactions are lower, and that of (n, p) reaction are higher compared to most of the corresponding literature cross-sections.