Evidence of non-statistical structures in the elastic and inelastic scattering of58Ni+58Ni and58Ni+62Ni and intermediate dinuclear states

Excitation functions and angular distributions of⁵⁸Ni+⁵⁸Ni and⁵⁸Ni+⁶²Ni scattering at energies just above the Coulomb barrier have been measured aroundθ _cm=90° in energy stepsΔE _cm=0.25 MeV fromE _cm ? 110 MeV toE _cm ? 120 MeV for⁵⁸Ni+⁵⁸Ni and fromE _cm ? 110 MeV toE _cm ? 118 MeV for⁵⁸Ni+⁶²Ni. Evidence for structure of non-statistical character has been found in the angle-summed excitation functions; this evidence is corroborated by the analysis of the angular distributions. This is the first time that non-statistical structure in elastic and inelastic scattering is reported with high confidence level for this mass and excitation energy ranges. Attempts are presented to understand the nature of this structure, including the presence of intermediate dinuclear states and virtual states in a potential well.     

Multiple-source analysis of inclusive proton spectra from58Ni +60Ni Collisions at 876.5 MeV

Experimental inclusive proton spectra of⁵⁸Ni+⁶⁰Ni at 15.1 MeV/u have been decomposed using three moving sources associated with, respectively, equilibrium, deep-inelastic, and preequilibrium processes. For the last, a new expression, taking into account the anisotropy of preequilibrium particles in the source system, has been applied. The high-energy part of the obtained angle-integrated proton spectrum has been compared with predictions of the diabatic dissipation model.     

CO vibrations on a stepped Ni surface

Electron energy loss spectra (ELS) have been measured after CO adsorption on the stepped Ni[5(111) × (11̄0)] surface as function of substrate temperature and CO exposure. At 150 K and exposures below 0.5 L, only adsorption sites close to the step edges are occupied. Pronounced rearrangements of CO molecules over terrace sites occur by increasing the temperature to 300 K. The occupation of special step sites gives rise to an exceptionally low frequency C-O stretching vibration of 1520 cm⁻¹. This frequency indicative of a weakened C-O bond is correlated with the previously found tendency for CO decomposition to occur on this surface during a flash desorption experiment.     

Instability of C 60 + on Ni (100) in surface collisions

Collisions of C ₆₀ ⁺ -ions with a nickel (100) surface in ultra high vacuum have been studied. Fullerene ions emerging from the surface after impact were not observed. Auger spectroscopy reveals an increasing carbon coverage of the surface as the exposure dose of C ₆₀ ⁺ increased until saturation is reached. Low energy electron diffraction shows formation of ac(2×2) carbon superstructure ofp4g-symmetry. There is strong evidence, that the observed instability of C₆₀ is induced by a chemical reaction at the surface and that the Ni–C bonds formed lead to the superstructure.     

Damped oscillations in the energy autocorrelation functions of the 58Ni+46Ti elastic and 58Ni+62Ni elastic and inelastic scattering cross sections

Structures of non-statistical character, recently observed in ⁵⁸ Ni +⁴⁶ Ti elastic and ⁵⁸ Ni +⁶² Ni elastic and inelastic excitation functions, produce damped oscillations in the cross section energy autocorrelation functions. The analysis of these damped oscillations in terms of S-matrix spin and parity decoherence indicates, as a possible interpretation, damping of the coherent rotational motion of the intermediate dinuclear system formed in the reaction.     

Influence of chemisorbed oxygen on nickel surface vibrations

We calculate the lattice vibration spectra near free and oxygen covered nickel surfaces. The phonon frequencies are deduced from the surface band structure using a simple band scheme for the nickel d and oxygen p states. Comparison is made with recent measurements obtained by electron loss spectroscopy.     

Multifragmentation study on 30 AMeV32S+58Ni

In a multidetector experiment on 26 or 30 AMeV³²S+⁵⁸Ni, up to four coincident heavier or intermediate-mass fragments were observed. One of these occasionally has the characteristics of a projectile-like fragment, up to three may be attributed to the decay of the heavy reaction product. Taking the velocity of the fragments as a measure of the heavy-product excitation energy, one finds evaporation, fission and multifragmentation to follow one another with rising excitation. Model simulations of sequential decay with up to two binary fissions and, alternatively, of simultaneous statistical multifragmentation were performed for comparison with experimental distributions of mass, velocity and (for events with three slow intermediate-mass fragments) relative azimuthal angle. Though in the three-fragment events indications of simultaneous multifragmentation are present, the sequential binary decay predominates. Evaporated protons and α particles detected in coincidence have a mean multiplicity growing with excitation energy, while the temperature governing the spectra has a plateau with a value of about 5.5 MeV.     

Calculation of the 0+ and 2+ giant resonances in Ni58

Estimates of the excitation energy, width and sum rule fraction of the collective monopole and quadrupole vibrations indicate that the peak in the 62A ^?1/3 MeV region is a superposition of the 0⁺ and 2⁺ modes.     

Clustering states in the62Ni(58Ni,58Ni)62Ni reaction

Excitation function and angular distributions of the⁶²Ni(⁵⁸Ni,⁵⁸Ni)⁶²Ni elastic scattering have been measured at incident⁵⁸Ni energies from 220.0 to 230.0 MeV in steps of 0.5 MeV. Evidence of two structures was found in the excitation function; a statistical analysis suggests a possible nuclear cluster quasi-molecular nature for these structures.     

The study of neutral pion azimuthal distribution in 58Ni+58Ni reaction at 2 GeV/nucleon

In order to study the anisotropic azimuthal emission of mesons in heavy ion collisions we measured the neutral pions emitted in the Ni+Ni collisions at 2 GeV/u with respect to the reaction plane. We studied the strength of the azimuthal anisotropy for neutral pions in dependence of the transverse momentum and impact parameter. The preliminary results and their comparison with previous experimental data are reported.     

Influence of packing on the vibrations of homogeneous bundles of C60 peapods

The non-resonant Raman spectra of homogeneous bundles of C₆₀ peapods (C₆₀ inserted in single-walled carbon nanotubes) are calculated in the framework of spectral moment method, together with a bond-polarizability model. The evolutions of the low wavenumber range of the Raman spectrum of homogeneous bundles of C₆₀ peapods as a function of the nanotube diameter and the size of bundles are discussed. The effect of the C₆₀ filling factor is investigated in detail. The results are compared to experimental Raman data measured on various samples of C₆₀ peapods.     

Fusion excitation function measurements for the 16O+58Ni and 16O+62Ni systems

High precision fusion excitation functions have been measured for the ¹⁶O+⁵⁸Ni and ¹⁶O+⁶²Ni systems from which fusion barrier distributions have been evaluated. Coupled-reaction-channels (CRC) calculations, which describe elastic and quasi-elastic scattering, also satisfactorily reproduce the fusion cross sections and barrier distributions. The small value of Z₁Z₂ in this case leads to barrier distributions with relatively little structure. However, in conjunction with the detailed elastic scattering data for these systems, this allows us to elucidate the role of previously ignored states in ¹⁶O in pushing the entire distribution to lower energies. These shifts are consistent with derived magnitudes of polarization potentials for both systems.     

Sub-barrier fusion of35, 37Cl+58, 64Ni evidence of effects of proton transfer channels

Sub-barrier fusion excitation functions of^35,37Cl+^58,64Ni have been measured. They are discussed in comparison to similar data of^34,36S+^58,64Ni with the aim of revealing the influence of coupled proton transfer channels. Using the simplified coupled channel code CCFUS, differences in the effects of inelastic channels are eliminated in an approximative manner to stress the differences in the effects of transfer channels. Signatures of positiveQ-value transfer channels coupled to fusion are clearly identified.     

Near-barrier fusion of Sn + Ni and Te + Ni systems: examining the correlation between nucleon transfer and fusion enhancement

The fusion excitation functions for radioactive (132)Sn + (58)Ni and stable (130)Te + (58,64)Ni were measured at energies near the Coulomb barrier. The coupling of transfer channels in heavy-ion fusion was examined through a comparison of Sn + Ni and Te + Ni systems, which have large variations in the number of positive Q-value nucleon transfer channels. In contrast with previous experimental comparisons, where increased sub-barrier fusion cross sections were observed in systems with positive Q-value neutron transfer channels, the reduced excitation functions were equivalent for the different Sn + Ni and Te + Ni systems. The present results suggest a dramatically different influence of positive Q-value transfer channels on the fusion process for the Sn + Ni and Te + Ni systems.     

Elastic and inelastic scattering of 58Ni +90,94Zr

Pure elastic and inelastic scattering cross sections have been measured for the systems ⁵⁸Ni +^90,94Zr at energies near the Coulomb barrier where not only quasi-elastic and fusion but also deep-inelastic process come into play. Coupled channels calculations including both projectile and target inelastic excitations can successfully explain the elastic and inelastic scattering angular distributions with an energy-independent semi-empirical bare potential. The calculation reproduces also the sum of the total quasi-elastic, fusion and deep-inelastic cross sections. Received: 14 September 1998 / Revised version: 21 October 1998     

Self-consistent analysis of sub-barrier fusion enhancement effect in Ca+Ca and Ni+Ni

The fusion dynamic mechanism of heavy ions at energies near the Coulomb barrier is complicated and still not very clear up to now. Accordingly, a self-consistent method based on the CCFULL calculations has been developed and applied for an ongoing study of the effect of the positive Q-value neutron transfer (PQNT) channels in this work. The typical experimental fusion data of Ca+Ca and Ni+Ni is analyzed within the unified calculation scheme. The PQNT effect in near-barrier fusion is further confirmed based on the self-consistent analysis and extracted quantitatively.     

Inelastic proton scattering to the lowest 1+ state in58Ni

A microscopic, antisymmetrized Distorted Wave approximation is used in an analysis of the inelastic scattering of 17.8 MeV protons from⁵⁸Ni in which the 1⁺ (2.90 MeV) state is excited. Two step resonance amplitudes complement the usual direct reaction transition amplitudes in this analysis. In particular, resonance amplitudes associated with the virtual excitation of a giant dipole and of a giant octupole resonances are considered, and are essential for the model to fully explain the experimental data.