Properties of the ν7/2-[503]（f7/2） band in 185Pt

High-spin states in ¹⁸⁵Pt have been reinvestigated via the reaction ¹⁷³Yb(¹⁶O, 4n) at a beam energy of 90 MeV. The previously known band based on the ν7/2^-[503](f_7/2) Nilsson orbital has been extended to higher spin states. Properties of the ν7/2^-[503](f_7/2) band have been discussed with an emphasis on the evolution of configuration while increasing the spin.     

Spin splittings in the ν3 band of NO2

Spin splittings for several important atmospheric lines in the ν₃ band of NO₂ have been measured by diode laser. An improved spin-splitting program has been developed which takes into account the asymmetry effects in the lower K_a splittings. The measured spin splittings and the derived spin-rotational constants are reported in this study to a much higher accuracy than previously achieved.     

Properties of the πh 9/2 ⊗ νi 13/2 band in odd-odd 188Au

A new rotational band has been identified and assigned to ¹⁸⁸Au for the first time using the ¹⁷³Yb(¹⁹F,4nγ) reaction at the beam energies of 86 and 90 MeV. This band is proposed to be built on the πh _9/2 ⊗ νi _13/2 configuration by comparing the band properties with known bands in neighboring nuclei. The prolate-to-oblate shape transition through triaxial shape has been proposed to occur around ¹⁸⁸Au for the ηh _9/2 ⊗ νi _13/2 bands in odd-odd Au isotopes on the basis of total Routhian surface (TRS) calculations.

     

Intensities of two-photon transitions in the 2ν2 band of NH3

We determine theoretically all the coincidences between the ¹⁴NH₃ν₂= 0−2 band and the spectrum of two CO₂ lasers; they can be induced either by a small frequency tuning of lasers or by a Stark tuning of molecular levels. For each two-photon transition we report the line intensity, the preferred laser lines and the necessary Stark field or laser tuning. The theoretical line intensities are compared to the results of an optoacoustic Doppler-free experiment.     

Properties of the ν7/2-[503](f7/2) band in 185pt

High-spin states in 185pt have been reinvestigated via the reaction 173Yb(<'16>O, 4n) at a beam energy of 90 MeV. The previously known band based on the ν7/2<'->[503](f<,7/2>) Nilsson orbital has been extended to higher spin states. Properties of the ν7/2<'->[503](f<,7/2>) band have been discussed with an emphasis on the evolution of configuration while increasing the spin.     

Description of the Properties of nuclei far from βstability line in relativistic Hartree approach

In the usual relativistic mean field(RMF) calculation of stable nuclei, the tensor coupling of ρ meson is not taken into account. It is necessary to clarify thecontribution of the tensor coupling of ρ meson when the RMF is extended to nucleifar from β stability line. The tensor coupling of ρ meson is included and its effectis discussed in the present work.     

Analysis of the hot bands in the 2ν9 band region of propyne-d3

The rovibrational spectrum of 2ν₉ band of CD₃CCH is overlapped by two prominent hot bands identified as (2ν₉⁰+ν₁₀^±1)(E)←ν₁₀^±1(E) and 3ν₉^±1(E)←ν₉^±1(E), where ν₁₀ and ν₉ are the degenerate CCC and CCH bending fundamental vibrations, respectively. Assignment of lines to the transitions of these hot bands were carried out with the help of the high-resolution spectra recorded at ∼195 K and at room temperature. Molecular parameters for these hot bands have been obtained from the rotational analysis of the partially resolved K-structure lines. Only Q-head of the third hot band , originating from the lower 2ν₁₀ state could be identified.     

Properties of the πh_(9/2)  νi_(13/2) band in odd-odd ~(188)Au

A new rotational band has been identified and assigned to 188Au for the first time using the 173Yb(19F,4nγ) reaction at the beam energies of 86 and 90 MeV. This band is proposed to be built on the πh9/2  νi13/2 configuration by comparing the band properties with known bands in neighboring nuclei. The prolate-to-oblate shape transition through triaxial shape has been proposed to occur around 188Au for the πh9/2  νi13/2 bands in odd-odd Au isotopes on the basis of total Routhian surface (TRS) calculations.     

Role of 8Be → 2 α intermediate nuclei in the fragmentation of 16O relativistic nuclei in nuclear track emulsions

In searches along a track in the chamber irradiated at the Laboratory of High Energies at the Joint Institute for Nuclear Research (JINR, Dubna) with oxygen ions accelerated to a momentum of 4.5 GeV/c per nucleon, 215 events containing two or more doubly charged fragments of the primary nucleus were found. Emission angles in the track-emulsion plane were measured in these events. Their distribution is consistent with that which alpha particles are expected to have in an oxygen nucleus prior to its interaction with a track-emulsion nucleus. Events of the ¹⁶O ?? 2⁸Be ?? 4?? type were discovered for the first time. They are treated as events of the coherent electromagnetic dissociation of an oxygen nucleus. Among all events, about 14% of the ⁸Be ?? 2?? decays proceed through the ground state of spin-parity 0⁺; an approximately the same fraction of such decays proceed through the first excited state of spin-parity 2⁺.     

Laser stark spectroscopy of the ν2 fundamental band of 15NH3

The ν₂ fundamental band of ¹⁵NH₃ has been observed with a laser Stark spectrometer in Doppler-limited resolution. A set of 38 band constants including the electric dipole moment and its rotational dependence are determined from 416 Stark resonances observed in the present work and three submillimeter lines reported in the literature. The ν₂-band absorption line frequencies in the region 800–1160 cm⁻¹ and their relative absorption intensities are estimated from the band constants.     

High-resolution spectrum of the ν9 band and reinvestigation of the ν8 band of cis-CH3ONO

The infrared spectrum of methyl nitrite CH₃ONO has been recorded at a spectral resolution of 0.003 cm^?1 using a Fourier-transform spectrometer Bruker IFS125HR. The ν₈ band of the cis isomer has been reinvestigated in the 780–880 cm^?1 spectral range to complete the study made by Goss et al. (2004) [3] and to fit the internal rotor splittings. The BELGI-IR program, which enables us to treat an isolated infrared band for asymmetric molecules containing one internal methyl rotor has been used for the analysis and predictions of spectra. Finally 1036 lines (913 A-type and 123 E-type lines for J≤50 and K_a≤28) have been assigned for the cis isomer and fitted with a standard deviation of 0.00047 cm^?1.Furthermore, for the first time, the ν₉ band of cis-CH₃ONO was investigated in the 540–660 cm^?1 spectral range and rather large internal rotation splittings were also observed at higher J values. For the ν₉ band, the effective approach performed with the BELGI-IR program allowed us to analyze and reproduce 682 lines up to J=50 and K_a=18 with a standard deviation of 0.00051 cm^?1. The multiple vibration–rotation–torsion interactions, which are likely to occur between the excited v₉=1 and v₈=1 states and the torsional manifolds are discussed.     

Diode-laser measurements and calculations of H2-broadening coefficients in the ν3 band of CH3D

Using a tunable diode-laser spectrometer, we have measured at room temperature the H₂-broadening coefficients of for 36 lines belonging to QP and QR branches in the ν₃ parallel band. The recorded lines with J values ranging from 1 to 15 and K from 0 to 9 (K?J) are located between 1196 and 1412 cm⁻¹. The H₂-broadening coefficients were determined by fitting each spectral line with Voigt, Rautian, and Galatry profiles. They were also calculated on the basis of a semiclassical model of interacting linear molecules performed by considering in addition to the weak electrostatic contributions the atom-atom Lennard-Jones potential. The theoretical results are in reasonable agreement with the experimental data, except for high J transitions where they are overestimated and for K approaching or equal to J with J?3 where they are underestimated. The latter discrepancy may be caused by the assumption to consider only ΔK=0 collision-induced transitions, associated with |ΔJ| transitions up to 4.     

Rotational analysis of the ν2 band of NH2D

High-resolution diode laser spectra and medium-resolution F-T spectra of deuterated ammonia have been obtained in the 700- to 1030-cm⁻¹ region. Out of about 800 lines measured by diode laser spectroscopy, approximately 500 lines have been assigned to the ν₂ transitions of NH₂D. The parameters for the ground and ν₂ states of NH₂D have been derived by the simultaneous analysis of the infrared and microwave data. The standard deviation for the IR data is ∼8 × 10⁻⁴ cm⁻¹. It is shown that the energy levels of NH₂D in the ν₂ state are heavily perturbed by inversion-rotation interaction and that it is necessary to include higher order inversion-rotation interaction terms to obtain a satisfactory fit of the observed data.     

Signature splitting of the πh11/2 band and high-spin structures in 155Tb

Seven experimentally observed bands of 155Tb are analyzed in detail, using the particle-number-conserving method for treating the cranked shell model with monopole and quadrupole pairing interactions. We satisfactorily reproduce the experimental alignments and especially focus on the microscopic mechanism of the second back-bending and the influence of pair interaction on ultrahigh spins. Our calculated results show that the πi13/2 orbitals are too high to give a contribution to the moment of inertia below hω≈0.7 MeV. Instead, the crossing between the π[541]l/2 and other proton orbitals is responsible for the second back-bending. We assign a possible configuration to the decoupled band found in 155Tb and predict eleven bands which are experimentally unobserved.     

Spectral-Luminescent Properties of Yb3+ in SOCl2–GaCl3

Optics and Spectroscopy - The absorption and luminescence spectra and the excited state lifetime of Yb3+ in SOCl2–GaCl3–Yb3+ solutions are measured. Information on the Stark splitting...     

Nonclassical Properties of Superposition of Two Coherent States Shifted in Phase by 3π/2

We consider the quantum superposition of two coherent states shifted in phase by 3π/2 ｜α〉 and ｜ -iα〉, as well as special states that are characterized solely with respect to amplitude α. According to analysis of nonclassical properties such as oscillatory and sub-Poissonian distribution of photon numbers, photon antibunching, quadrature squeezing, and negativity of Wigner function, it is concluded that the considered superposition state is a nonclassical state. Also, the special state is found to exhibit even stronger nonclassical features when relative phase φ of the superposition is equal to the average photon number ｜α｜^2.     

Infrared diode laser spectroscopy of the ν2 fundamental band of SH3+

The high-resolution absorption spectrum of the ν₂ fundamental band of SH₃⁺ has been observed with the magnetic field modulation technique. The ions were generated in a hollow cathode discharge through a mixture of H₂ and H₂S. The molecular constants in the excited vibrational state are determined through a least-squares fit of the data to a standard symmetric top energy level expression. The anomalous sign of the centrifugal distortion constants is explained by the Coriolis interaction between the v₂ = 1 and v₄ = 1 states.     

Collisional parameters of N2 broadened methane lines in the R9 multiplet of the 2ν3 band. Multispectrum fittings of the overlapping spectral lines

A high-sensitive two-channel photo-acoustic (PA) spectrometer with a near infrared diode laser was used to make precise measurements of N₂-broadened methane spectra in the R9 multiplet of 2ν₃ band. For the accurate retrieval of spectroscopic line parameters (intensities, positions at zero pressure, pressure-shifting and -broadening, collisional narrowing and line mixing coefficients) from the methane PA spectra, a program based on a multispectrum fitting procedure has been used. The multispectrum least squares fitting procedure is based on a relatively simple line profile model and on the linear pressure dependences of the line profile parameters. The line parameters were determined for 11 lines of the methane 2ν₃ R9 multiplet. The results have been compared with other available data.