超强激光超热电子激发的Kα X射线发射研究

建立了无色散型X射线谱仪. 利用SILEX-I激光装置的超强激光辐照固体物质,分别在靶前、后定量测量了Cu和Mo物质在不同激光功率密度时的X射线谱和Kα光子产额,推导了不同激光强度时的Kα X射线光子转换效率. 实验发现,打靶激光能量越高,靶后出射的Kα产额越高,100μm Mo靶可获得10^-5量级转换效率. 关键词： X射线发射 激光-物质相互作用 Kα谱仪')" href="#">Kα谱仪     

Al2O3X(X=H,D, T)的电子振动近似理论方法研究

用密度泛函理论(DFT)方法在6-311++G(d,p)水平上对Al₂O₃X(X=H, D, T)分子较低能量的几何构型进行了优化. 计算结果表明该分子有两个可能基态, 即Al₂O₃X(X=H,D,T)(²A′)C_s和Al₂O₃X 关键词： 2O₃X(X=H;D;T)分子团簇')" href="#">Al₂O₃X(X=H;D;T)分子团簇 热力学函数 氢同位素效应 吉布斯自由能改变     

晶体NiF2的吸收光谱和电子顺磁共振谱的一种完全对角化计算

采用半自洽场(semi-SCF)自由Ni²⁺的d轨道波函数、点电荷-偶极子模型和Ni²⁺-6X^-(X=F,Cl,Br,I)络合物的μ-κ-α模型,建立结构参数与光谱、电子顺磁共振(EPR)谱(零场分裂D,E和顺磁g因子)之间的定量关系.利用能量矩阵完全对角化方法(CDP)和高阶微扰方法,统一解释NiF₂晶体的局部结构、吸收光谱和电子顺磁共振谱(EPR).比较两种方法计算得到的零场分裂D,E和顺磁g因子.结果表明:①高阶微扰方法算出的D,E值误差大;②能量矩阵完全对角化方法(CDP)算出的D,E值、光谱、顺磁g因子的值都与实验符合很好.     

XF3 (X=N,P,As)价层电离势的运动方程耦合团簇理论计算

采用运动方程单双取代耦合团簇理论(EOM-CCSD)对XF₃(X=N,P,As)的价层垂直离势(VIP)进行了系统计算,同时对称匹配团簇组态相互作用(SAC-CI)、外价层格林函数(OVGF)以及部分三阶近似(P3)方法也被应用到目前计算.与已有的实验结果比较表明:EOM-CCSD计算的价层垂直电离势整体上与SAC-CI结果相近,而优于OVGF和P3理论结果,在整个价层上,EOM-CCSD结果与实验值总体差距约0.2 eV, 在外价层这种差距相对较小,在内 关键词： XF₃(X=N;P;As)')" href="#">XF₃(X=N;P;As) 垂直电离势 运动方程耦合团簇理论     

BaTi2Bi2O的电子结构与磁性

采用第一性原理方法,对BaTi₂Bi₂O的电子结构和磁性进行计算.非磁性态的计算结果显示:费米能级处的态密度主要来自d_z²,d_x²-y²和d_xy三个轨道,同时费米面也主要有三部分组成,并且将其沿着矢量q₁=(π/a,0,0)和q₂=(0,π/a,0)平移时,第三部分费米面(沿着X-R连线)与第一部分费米面(M-A连线)嵌套明显,计算得出磁化系数χ₀(q)在X点出现峰值,与峰值出现在M点的FeAs基超导体不同.上述磁化率峰值可以诱导产生自旋密度波,使得BaTi₂Bi₂O材料的磁性基态是bi-collinear antiferromagnetism(AF3)与blocked checkerboard antiferromagnetism(AF4)的二度简并态.随着空穴掺杂,χ₀(q)的峰值降低,而电子掺杂则导致峰值变大.当自旋涨落被完全压制时,超导出现,这可以解释为什么超导只出现在空穴掺杂型化合物而非电子掺杂型.     

激光-电子康普顿散射物理特性研究

对激光-电子康普顿散射物理特性即能量特性和微分截面角分布进行了仔细的研究.计算结果显示出光子能量和微分截面角分布的简单结构.康普顿散射X射线光源具有散射光子的能量易调节、方向性好等特点.在入射电子束能量很高时,X射线近乎单向出射.光源色散度较大,但实验上可以获得色散（带宽）小的X射线.对于各种波长的激光,在很宽的电子束能量范围（1 MeV—10 GeV）内,散射X射线光子的总截面和前向发射圆锥内（半圆锥角1/γ,其中γ=E/m₀ 关键词： 康普顿散射 能量特性 微分截面 角分布     

AuZn和AuAl分子基态与低激发态的势能函数与热力学性质

用密度泛函理论B3LYP方法计算研究AuZn和AuAl分子基态与低激发态的结构与势能函数,导出分子的光谱数据.结果表明,AuZn和AuAl分子基态分别为X²Σ和X¹Σ,基态与低激发态的势能函数均可用Murrell-Sorbie函数来表达.AuZn分子低激发态a⁴Σ的绝热激发能为43529kJ/mol,AuAl分子低激发态a³Σ的绝热激发能为19991kJ/mol.计算固体AuZn和AuAl的内能和熵时,近似以气体分子的电子能和振动能代替固体分子的内能,用电子熵和振动熵代替固体分子的熵.在此近似下,计算得到AuZn和AuAl基态与低激发态固态分子生成反应热力学性质与温度的关系. 关键词： AuZn和AuAl B3LYP 热力学性质 势能函数     

光子晶体微腔中高偏振单偶极模的研究

三角晶格排列的光子晶体微腔中的偶极模式是简并的,通过改变其晶格的对称性可以消除模式简并.晶格的整体形变破坏了晶格对称性从而影响光场的分布,同时还改变了电磁场的偏振分布.晶格整体形变使得简并的偶极模式分离成x极和y极偶极模式.通过计算分析发现分离后的模式具有良好的偏振特性,从而为实现单偏振光子晶体激光器提供了一种很好的途径.文中针对光子晶体薄板结构的微腔,主要计算了偶极模中x极偶极模式在不同拉伸时以及不同填充因子情况下的Q值,并分别计算了x关键词： 光子晶体 偶极模 品质因子 偏振度     

差分法求解时空分布的激光动力学模型

利用速率方程理论和差分法数值计算,建立了描述激光器内部粒子数密度和光子数密度的时间演化和空间分布的动力学模型.该方法完善了普通的激光速率方程理论,为了解激光能量的时间演化和空间分布提供了较好的理论模型. 关键词： 速率方程 差分法 动力学模型 铜激光     

Analysis of characteristic X-ray generation induced by laser plasma electrons accelerated by an electric field

The results of experiments devoted to the study of spectral, spatial, and time characteristics of a spectrally bright point x-ray source based on a vacuum diode with a laser-plasma cathode and a titanium needle anode with a photon energy approximately equal to 4.5 keV are presented. The experimental results revealed a considerable difference between the electron emission from laser plasma in a strong electric field and the explosive electron emission and demonstrated the effectiveness of laser plasma as an electron source. The optimization of the laser radiation power density, the accelerating voltage, and the interelectrode spacing made it possible to create a point x-ray source whose spectral brightness exceeds available sources in the class of small-size pulse x-ray instruments (tubes with explosive cathodes). It has been proved experimentally that the maximum contrast of the characteristic lines of the anode material is attained in the case of an optimal choice of accelerating voltage. The x-ray source has the following parameters: (1) spectral brightness of the K-lines of titanium of the order of 10²¹ photons/cm² s sr keV; (2) emitting region size of 250 mm; and (3) laser pulse duration less than 20 ns.     

Spatial distributions of electron density in microplasmas produced by laser ablation of solids

The spatial distribution of electron density in argon microplasmas produced by laser ablation of solids has been investigated by time-resolved emission spectroscopy. The electron density was derived from Stark broadening and shift of spectral lines. It was found that the radial gradient of the electron density is much smaller than the gradient of the atomic number density of atoms ablated by the laser into the plasma. The almost homogeneous plasma conditions in the centre of the microplasmas are essential for quantitative element analysis of solid samples by laser ablation. On the other hand, because of the homogeneous conditions microplasmas are excellent sources for measurements of reliable Stark broadening and shift parameters of atomic and ionic spectral lines of all elements which can be ablated by lasers from solid samples.     

The enhancement effect in K-shell radiative recombination of \mbox{\sffamily\bfseries U}^{\hbox{\sffamily\bfseries\fontsize{10}{12}\selectfont 92+}} ions with cooling electrons

We report the results of the x-ray radiative recombination (RR) experiment at the electron cooler of the ESR storage ring performed, for the first time, for detuned (off-cooling) electron energies. In this experiment the recombination of stored, decelerated bare uranium ions with electrons in the energy range 0–1000 meV was studied by observing K-RR x-ray photons emitted from direct radiative recombination to the lowest n=1 state. In this way the RR process was studied in a state selective manner for several off-cooling electron energies. The measured dependency of the recombination rate on the relative electron energies for K-shell RR x-ray photons are compared with the predictions of both nonrelativistic and fully relativistic calculations for the radiative recombination. A role of the relativistic effects, which contribute substantially for higher relative electron energies, are discussed. Strong enhancement of the recombination rate is observed for the the zero relative electron energy (cooling condition) for the K-shell.     

高能闪光射线源空间位置抖动实验测量

高能闪光照相中光子散射会导致接收图像清晰度降低,影响照相客体界面和密度的分辨精度。使用网栅相机可显著降低散射光子影响,提高图像分辨能力,但同时要求X射线源空间位置更加稳定以减少信号光子在网栅结构中的损失。采用小孔成像的方法测量神龙一号直线感应加速器X射线源焦斑分布,计算焦斑的质心位置和半高全宽大小,分析电子束聚焦状态改变对X射线源空间位置和大小的影响。实验结果表明,电子束聚焦状态改变会导致射线源质心位置及尺寸大小发生明显变化。在恒定聚焦状态下,源质心抖动及大小变化均可稳定在较小范围。 ;     

Diffraction and channeling in nanotubes

A theory of the interaction of fast charged particles and gamma rays with nanotubes with different helicity is developed. Analytical expressions are obtained for the potential and the electron density of a nanotube taking account of the anisotropic thermal vibrations of the atoms. A system of equations determining the quantum states of the transverse motion of relativistic electrons, positrons, and x-ray photons in a superlattice consisting of nanotubes is formulated, and methods for solving this system are developed. Calculations of the soft x-ray Bragg reflection coefficients of a superlattice are performed in the two-wave approximation of the dynamical theory of diffraction.     

X-Ray Tube Voltage Dependence of Wiener Spectra of Screen Structure Mottle Recorded on Front and Back Emulsions

A low-speed screen/film system was used to investigate structure mottle, i.e., the density fluctuation of an x-ray film due to inhomogeneous screen structure. The tube voltage dependence of the Wiener spectra of the structure mottle was separately determined for front and back film emulsions. The Wiener spectral values of the structure mottle of the front emulsion were greater than those of the back emulsion at lower tube voltages. The spectral values of the structure mottle of the front emulsion decreased with tube voltage, while those of the back emulsion increased. We explain these phenomena by the behavior of the Wiener spectra of the relative spatial fluctuation of fluorescence intensity due to following reasons: (1) spatial thickness fluctuation of the screen produces a relative spatial fluctuation of x-ray energy absorbed in the screen, and (2) as the distance between the emulsion of the film and the average position of the x-ray absorption in the screen lengthens, the number of random scattering and absorption of light photons increase.Presented at the International Commission for Optics Topical Meeting, Kyoto, 1994.     

X-ray scattering measurements of radiative heating and cooling dynamics

Spectrally and time-resolved x-ray scattering is used to extract the temperature and charge state evolution in a near solid density carbon foam driven by a supersonic soft x-ray heat wave. The measurements show a rapid heating of the foam material (approximately 200 eV/ns) followed by a similarly fast decline in the electron temperature as the foam cools. The results are compared to an analytic power balance model and to results from radiation-hydrodynamics simulations. Finally, the combination of charge state and temperature extracted from this known density isochorically heated plasma is used to distinguish between dense plasma ionization balance models.     

On the absence of oxygen spectral lines in sputtering

It is well established that atomic oxygen spectral lines are normally not observed in optical studies of sputtering processes. We suggest that this can be explained in terms of local variations in the electron density along the solid surface. The model outlined is in accordance with the finding that the yields of secondary ions, secondary electrons, and secondary photons are normally enhanced by presence of oxygen at the target surface.     

Single-pulse coherent diffraction imaging using soft x-ray laser

We report a coherent diffraction imaging (CDI) using a single 8 ps soft x-ray laser pulse at a wavelength of 13.9 nm. The soft x-ray pulse was generated by a laboratory-scale intense pumping laser providing coherent x-ray pulses up to the level of 10(11) photons/pulse. A spatial resolution below 194 nm was achieved with a single pulse, and it was shown that a resolution below 55 nm is feasible with improved detector capability. The single-pulse CDI might provide a way to investigate dynamics of nanoscale molecules or particles.     

金等离子体M带谱强度的定量测量

在"神光II"多束高功率激光装置上利用列阵透镜匀滑钕玻璃波长0.53μm的强激光幅照平面金(Au)靶时产生X射线,本文给出了X射线绝对转换效率ξx。研究了多束倍频激光叠加驱动靶形成X射线背景光源辐射金M壳层1.8—3.1Kev带谱的特性,获得了不同激光功率密度及不同角度驱动靶面等几种条件下X射线能谱的定量测量结果和能谱分布。