The influence of fractal size distribution of covers on radon exhalation from uranium mill tailings

Tailings produced during mining and milling of uranium ores represent potentially large volumes of low level radioactive materials. A typical environmental problem associated with mill tailings is radon emanation. Covering tailings is widely applied to reduce radon exhalation rate. In this paper, the fractal theories and field covering tests are used to study the fractal characters of size distribution of six types of covering materials, including waste rock, sand, laterite, kaolin, mixture of sand and laterite, and mixture of waste rock and laterite, and their influences on radon exhalation. The size distributions of uranium tailings and the six aforementioned covering materials all exhibit a good fractal structure. The contents of fine grain increase with the increasing value of fractal dimension. The results of field radon measurement show that the radon emanation rate of tailings without covers is 14.7–18.6 Bq/m² s. Covering tests were carried out of the six abovementioned covering materials with thickness of 0.4 m, 0.8 m, 1.2 m, 1.6 m and 2.0 m. The results indicate that the application of these materials for cover layers can decrease the radon exhalation rate markedly. The effectiveness of a cover layer in reducing radon exhalation is related to its fractal texture of size distribution. Under the same thickness conditions, the attenuation coefficient of radon exhalation rate increases with the increasing fractal dimension of size distribution of covers. The empirical expressions of the attenuation coefficients in relation to fractal dimension D of size distribution and thickness x of covers is obtained for evaluating the effectiveness of final covers for uranium tailings impoundments.     

A new method for studying the transport of radon and thoron in various building materials using CR-39 and LR-115 solid state nuclear track detectors

Radon (²²²Rn) and thoron (²²⁰Rn) α-activities per unit volume were measured inside and outside different building materials by using two types of solid state nuclear track detectors (SSNTD) (CR-39 and LR-115 type II). In addition, the radon and thoron emanation coefficients of the studied materials were evaluated. Based on these data, the transport of radon and thoron across parallelepipedic blocks of the building materials could be investigated and radon and thoron global α-activities per unit volume outside different building material blocks were determined. Moreover, the diffusion length and the effective diffusion coefficient of radon in the building materials were evaluated and the total alpha activity due to radon in the atmospheres of different rooms consisting of different building materials was studied.     

An experimental method for measuring the radon-222 emanation factor in rocks

An experimental method, based on a 21-day accumulation technique, is proposed for measuring the radon-222 emanation factor in undisturbed consolidated materials. The leakage rate is determined from the form of the radon growth curve in the measurement chamber. It was comparable to the radon decay. In order to obtain the “true” radon emanation factor, the thickness of the sample must be less than the radon diffusion length in the porous material. The method was used to measure the radon emanation factor in water-saturated claystones (argillites). The radon emanation factor, determined from experiments on a rock sample with a thickness of 5 mm, was 15%, a value typical for this kind of material.     

Correlation between radon exhalation and radium content in granite samples used as construction material in Saudi Arabia

Measurements of radon exhalation for a total of 205 selected samples of construction materials used in Saudi Arabia were carried out using an active radon gas analyzer with an emanation container. It was found that granite samples were the main source of radon exhalation. The radon exhalation rates per unit area from these granite samples varied from below the minimum detection limit up to with an average of 1.5 . The radium contents of 27 granite samples were measured using an HPGe-based γ spectroscopy setup. The ²²⁶Ra content of the granites varied from below the minimum detection limit up to , with an average of . The linear correlation coefficient between exhaled radon and radium content was found to be 0.90.     

An approach to discriminatively determine thoron and radon emanation rates for a granular material with a scintillation cell

A powder sandwich technique was applied to determine thoron (²²⁰Rn) and radon (²²²Rn) emanation rates for a granular material. The feature of this technique is the sample preparation, in which a granular material is put and fixed between two membrane filters. Airflow is directly given to this sandwich sample, will include thoron and radon emanated from the material, and then is transferred to the detector. This method makes sure that thoron and radon emanated are not retained in pore space within the sample volume, which is crucial for the appropriate emanation test. This technique was first introduced by Kanse et al. (2013) with the intention to measure the emanation of thoron - but not of radon - from materials having much higher ²²⁴Ra activity than ²²⁶Ra. In the present study, the methodology for the discriminative determination of thoron and radon emanation rates from a granular material has been examined using a flow-through scintillation cell and sandwich sample. The mathematical model was developed to differentiate total alpha counts into thoron- and radon-associated counts. With a sample of uranium ore, this model was experimentally validated by comparison between the scintillation cell and a reference detector that can discriminatively measure thoron and radon concentrations. Furthermore, the detection limits and uncertainties were evaluated to discuss the characteristics of this method. Key parameters for improving the determination of thoron and radon emanations were found to be the background radon concentration and the leakage of radon from the measurement system, respectively. It was concluded that the present method is advantageous to a sample that has much higher ²²⁶Ra activity than ²²⁴Ra.     

Experimental and modeling studies of grain size and moisture content effects on radon emanation

Some models have already been developed to explain the effect of moisture content on the radon emanation fraction of soil. For this purpose, “microscopic” soil models, which are easy to deal with mathematically but cannot take grain size into consideration, have been designed. These previous models consist basically of two opposite grain surfaces and pores between the grains. In the present study, in order to study the effect of not only moisture content but also grain size, we present a simple modeling approach based on two “macroscopic” soil models: (1) a single-grain model and (2) a multiple-grain model. The latter model represents a configuration of spherical grains packed in a simple cubic structure. Based on these soil models and general assumptions, the radon emanation fraction was calculated as a function of grain size or moisture content by Monte Carlo simulation. The results for the multiple-grain model show that the radon emanation fraction is markedly increased with grain sizes ranging from 10 to 100 μm and reaches a constant value of 50% when moisture content is 0% and the radium is uniformly distributed on the grain surface. Moreover, a drastic increase is seen at smaller grain sizes with increasing moisture content. From these results, we concluded that the calculation of radon emanation depends greatly on the pore size between a Ra-bearing grain and a neighboring grain. The validity of the model was also evaluated by comparison to experimental data.     

Calculation of radon diffusion coefficient and diffusion length for different building construction materials

The diffusion of radon in dwellings is a process determined by the radon concentration gradient across the building material structure between the radon source and the surrounding air, and can be a significant contributor to indoor radon inflow. Radon can originate from the deeply buried deposit beneath homes and can migrate to the surface of earth. Radon emanates to the surfaces mainly by diffusion processes from the point of origin following α-decay of ²²⁶Ra in underground soil and building materials used, in the construction of floors, walls, and ceilings. In the present study radon diffusion through some building materials viz. coarse sand and stone dust of different grain size has been carried out using LR-115 type II solid-state nuclear track detectors (SSNTDs). The radon diffusion coefficients and diffusion lengths through these building construction materials have been calculated. The effect of grain size on radon diffusion through these building materials shows the decrease in radon diffusion with decrease in grain size.     

Radon exhalation studies in an Indian uranium tailings pile

A study was taken up to quantify the source term arising due to radon exhalation from Uranium(U) tailings pile at Singbhum shear zone in Jharkhand state of India. In-situ experiments were conducted at 40 locations of the U tailings pile in three seasons namely summer, rainy and winter to measure the radon fluxes. The fluxes were also predicted by a diffusion model using the measured parameters such as Ra-226 content, bulk density, diffusion coefficient, radon emanation factor, moisture content and temperature in the U tailings. It was observed that the predicted fluxes using the in-situ diffusion length and emanation factor were closer to measured values by accumulator technique than that predicted using empirically estimated diffusion coefficient and emanation factor. A conversion factor has been established between radon fluxes and Ra-226 content in U tailings for Jaduguda. The source term arising due to the radon exhalation from U tailings pile at Jaduguda has determined using the measured data of radon fluxes.     

Study of radon transport through concrete modified with silica fume

The concentration of radon in soil usually varies between a few kBq/m³ and tens or hundreds of kBq/m³ depending upon the geographical region. This causes the transport of radon from the soil to indoor environments by diffusion and advection through the pore space of concrete. To reduce indoor radon levels, the use of concrete with low porosity and a low radon diffusion coefficient is recommended. A method of reducing the radon diffusion coefficient through concrete and hence the indoor radon concentration by using silica fume to replace an optimum level of cement was studied. The diffusion coefficient of the concrete was reduced from (1.63 ± 0.3) × 10⁻⁷ to (0.65 ± 0.01) × 10⁻⁸ m²/s using 30% substitution of cement with silica fume. The compressive strength of the concrete increased as the silica-fume content increased, while radon exhalation rate and porosity of the concrete decreased. This study suggests a cost-effective method of reducing indoor radon levels.     

Seasonal indoor radon concentration in FYR of Macedonia

This paper presents the results of the seasonal indoor radon concentration measurements in dwellings in all regions of the Former Yugoslav Republic (FYR) of Macedonia. The measurements were made in 437 dwellings using CR-39 track detectors over four successive three-month periods (winter, spring, summer and autumn) throughout 2009. The results of analysis of variance showed statistically significant differences between indoor radon concentrations in different seasons. The geometric mean values and geometric standard deviations of indoor radon concentrations in winter, spring, summer and autumn were obtained to be: 115 Bq m^?3 (2.02), 72 Bq m^?3 (1.97), 46 Bq m^?3 (1.95), 92 Bq m^?3 (2.02), respectively. The geometric mean values of spring, summer and autumn to winter ratios were found to be: 0.63 (1.50), 0.40 (1.81), and 0.80 (1.58), respectively. The results of the analysis of the variance showed statistically significant differences among the indoor radon measurements for the regions in different seasons. The influence of the factors linked to building characteristics in relation to radon measurements in different seasons was examined. The factors which enable a differentiation into subgroups (significance level p < 0.05) are the floor level, basement and building materials.     

Simulation of radon emanation from free-flowing mineral raw materials

A mathematical model has been constructed which describes the radon emanation from free-flowing mineral raw materials in relation to the physical-mechanical properties of the materials. __________ Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 7, pp. 34–36, July, 2007.     

An intercomparison of indoor radon data using NTD and different dynamic recording systems

Indoor radon data monitored with several different recording systems in a controlled cellar were analyzed. The one-room cellar is carved into volcanic rock and presents an almost constant radon emanation throughout the year. Measurements were performed using the AlphaGUARD^®, Sun Nuclear^® 1027, DOSEman^® and RAD7^® radon monitors, and CR-39 Lantrack^® in a passive integrating detector. The radon concentrations measured by the active detection systems and averaged over the three-month measurement period ranged from 533 to 805 Bq m⁻³. The response of the passive detector system was a linear function for exposure times of one, two and three months. The data are discussed as a function of changes in the distribution of radon within the cellar and the response characteristics of the detection devices.     

The use of nuclear prospecting measurements for characterizing the radioactive status of Al-Bayyarat and Sabkhet Mouh areas,southern Palmyrides,Syria

Al-Bayyarat and Sabkhet Mouh areas in southern Palmyride have been radioactively characterized by using different nuclear prospecting measurements. Those measurements include the application of airborne, carborne spectrometric gamma, radon emanation and borehole techniques. The merging of airborne, carborne spectrometric gamma data enables to establish the normalized eU, eTh, and K% maps in the study area. Radon emanation and spectrometric gamma measurements have been applied only in Al- Bayyarat area, where radioactive anomalous zone has been observed. The radioactive characteristics of the study area has been explained through studying and analyzing a profile of 30 Km long, where a plausible geo-radioactive model has been proposed for the uranium leaching and its transport.     

Radon exhalation studies in building materials using solid-state nuclear track detectors

Indoor radon has been recognized as one of the health hazards for mankind. Building materials constitute the second most important source of radon in dwellings. The common building materials used in the construction of dwellings are studied for radon exhalation rate. The ‘Can’ technique using LR-115 type-II solid-state nuclear track detector has been used for these measurements. The radon exhalation rate in these samples varies from 4.75 m Bq m⁻² h⁻¹ (0.14 m Bq kg⁻¹ h⁻¹) for limestone to 506.76 m Bq m⁻² h⁻¹ (15.24 m Bq kg⁻¹ h⁻¹) for soil.     

Radon emanation from soil samples

The soil or bedrock beneath a building is one of the sources of radon gas in the indoor air. The ²³⁸U content of samples of the soil or the bedrock can be measured by gamma ray spectrometry and is of interest because the uranium content in the soil is a precursor of the presence of the radon gas in the soil. The emanation of radon gas from different types of material can be estimated to some extent if the content of ²³⁸U of a sample is known and the ²²⁶Ra content is only minorly affected. The true emanation is, however, affected by various parameters. One of these parameters is the possibility or not for the gas to come out from the grains into the air in the space between the grains of the sample.

In this study we report the results from measurements of radon gas emanating from samples of soil frequent in the Lund region in Sweden and in the Barcelona region in Spain. As soils have different grain size it is important to know the type of soil. The ²³⁸U content of the soil is measured with gamma ray spectrometry. The radon measurements are made by Kodak plastic film in closed cans, filled with the soil according to a technique, developed for radon measurements in water samples.

The result shows, that the combination of grain size and uranium content is important for the emanation of the radon gas from the grains of the soil.     

Indoor radon measurement via Nuclear Track Methodology: A comparative study

Indoor radon concentration represents an important public health challenge, for simple and inexpensive measurement devices and methods, suitable for large-scale indoors radon measurements, are required. Nuclear Track Methodology, by using a closed-end cup device as a radon chamber is an attractive option for such large-scale indoor radon measurements. A comparative analysis of the detection efficiency of four different (one commercial and 3 specially designed) passive closed-end cup devices for the measurement of indoor radon concentrations is presented. CR-39 (Lantrack®) polycarbonate was the detector material. The four devices were simultaneously exposed to a mean radon concentration of 860 ± 60 Bq m⁻³ inside a closed room for periods of one, two and three months. An AlphaGUARD^® radon monitoring system was used to continuously monitor the radon concentration within the room. The chemical etching and reading procedures were carried out following a well-established protocol for indoor radon surveys. The detection efficiency and the exposure-time-response relationship of each of the devices were determined.     

Emanations and “induced” radioactivity: From mystery to (mis)use

Radon, Rn; atomic number Z=85; is a (gaseous) chemical element of which no stable but only radioactive isotopes exist. Three of them, namely actinon (²¹⁹Rn), thoron (²²⁰Rn) and radon (²²²Rn) are the decay products of naturally occurring radioisotopes of radium:²²³Ra,²²⁴Ra and²²⁶Ra, respectively. The natural Rn isotopes were discovered within the period 1899–1902 and at that time referred to as emanations because they came out (emanated) of sources/materials containing actinium, thorium and radium, respectively. The (somewhat mysterious) emanations appeared to disintegrate into radioactive decay products which by depositing at solid surfaces gave rise to “induced” radioactivity i.e. radioactive substances with various half-lives. Following the discovery of the emanations the volume of the research involving them and their disintegration products grew steeply. The identity of a number of these radioactive products was soon established. Radium- emanation was soon used as a source of RaD (²¹⁰Pb) to be applied as an “indicator” (radiotracer) for lead in a study on the solubility of lead sulphide and lead chromate. Moreover, radium and its emanation were introduced into the medical practice. Inhaling radon and drinking radon-containing water became an accepted medicinal use (or misuse?) of that gas. Shortly after the turn of the century, the healing (?) action of natural springs (spas) was attributed to their radium emanation i.e. radon. Bathing in radioactive spring water and drinking it became very popular. Even today, bathing in radon-containing water is still a common medical treatment in Jáchymov, Czech Republic.     

Seasonal variation on radon emission from soil and water

Radon is being measured continuously in spring water and soil-gas at Badshahi Thaul Campus, Tehri Garhwal in Himalayan region by using radon Emanometer since December 2002. An effort was made to correlate the variance of radon concentrations in spring water and soil-gas with meteorological parameters at the same location. The main meteorological parameters that affect the radon emanation from host material is surrounding temperature, barometric pressure, wind velocity, rain fall and water level of the spring. The correlation coefficient between radon concentration in spring water and different atmospheric parameters was computed. The correlation coefficient between radon concentration in spring water and the maximum atmospheric temperature was 0.3, while it was 0.4 for minimum atmospheric temperature at the monitoring site. The correlation coefficient for radon concentration in spring water with minimum and maximum relative humidity was 0.4. Spring water radon concentration was found positively correlated (0.6) with water discharge rate of the spring. A weak correlation (0.09) was observed between the radon concentration in spring water and rain fall during the measurement period. As temperature of near surface soil increases, the radon emanation coefficient from the soil surface also increases. The possible effects due to global warming and other climatic changes on environment radiation level were also discussed in detail.      

Observation and removal of daily quasi-periodic components in soil radon data

We report (quasi) periodic oscillations observed in soil radon emanation data especially during summer period. Soil radon has been continuously monitored in the Marmara region of Turkey over the past nine years to reveal possible relationships between soil radon and seismic activities. This long term monitoring has clearly demonstrated that soil radon concentrations are affected by various parameters such as seasonal and daily changes in atmospheric parameters (temperature, pressure, precipitation). Sometimes, soil temperature variations as well as barometric pressure and precipitation may dominantly influence the soil radon concentration; leading to seemingly complex radon time series. One may need to remove such components for better analysis of the possible relationships between soil radon emanation and seismic activities. Here, we suggest using an algorithm to detect and remove daily-oscillations from the raw data. The detection and separation (extraction) algorithm is based on Empirical Mode Decomposition method which is a signal-adaptive method that automatically decompose the signal into its characteristic modes. The algorithm is applied to the data collected from three different soil radon monitoring stations (Bal?kesir, Gönen, and Armutlu) in Marmara region of Turkey and the results are provided.     

On the uncertainty of building acoustic measurements – Case study of a cross-laminated timber construction

If variations and uncertainty in building acoustic measurements can be controlled, construction costs can potentially be reduced since the building will not have to be acoustically over-designed. Field measurements of impact and airborne sound insulation were carried out for an industrially prefabricated cross-laminated timber (CLT) system of plate elements. The results from 18 rooms, forming three groups with respect to size, were compared to a similar study dealing with a prefabricated Volume Based Building (VBB) system. Large variations were found at frequencies below 100 Hz which is crucial for the low frequency adaptation terms connected to the weighted sound insulation indices. The measurement uncertainty was investigated by analysing the repeatability, measurement direction and the time dependence of the sound source. The variations due to the measurement procedure were found to be small compared to the total variations. It was also indicated that the variations in sound insulation are smaller with a prefabricated system compared to on-site production, since less work is required at the building site.