原子核的大质量转移反应和丰中子超重核的产生(英文)

迄今为止,人们合成的超重核都是缺中子的,无论是熔合-裂变反应还是碎化过程都无法使产物达到周期表的“东北区域”。而重核之间(如U核之间) 的近垒大质量转移反应则可能是目前生成丰中子超重核和达到未知丰中子重核区域的唯一途径。在改进的量子分子动力学(ImQMD) 模型结合统计模型框架内,研究了U+U等反应体系的大质量转移反应,计算了反应产生的初生态碎片的质量和电荷分布,并成功再现了产物的终态质量和电荷分布。通过比较3 个反应136Xe+248Cm,48Ca+248Cm和238U+248Cm 产生的106号元素的截面大小,揭示了U+U等重核大质量转移反应对产生丰中子超重核是非常有利的。For elements with Z > 100 only neutron deficient isotopes have been synthesized so far. The “northeast area” of the nuclear map can be reached neither in fusion-fission reactions nor in fragmentation processes.The large mass transfer reactions in near barrier collisions of heavy (U-like) ions seem to be the only reaction mechanism allowing us to produce neutron rich heavy nuclei including those located at the superheavy(SH) island of stability and unexplored area of heavy neutron-rich nuclides. This study is extremely important for nuclear astrophysical investigations and, in particular, for the understanding of the r process. In this paper within the Improved Quantum Molecular Dynamics (ImQMD) model combining with the statistical-evaporation model, the large mass transfer reactions, like 238U+238U have been studied. The charge and mass distributions of transiently formed primary fragments are investigated within the ImQMD model and de-excitation processes of those primary fragments are described by the statistical decay model. The mass distribution of the final products in 238U+238U collisions is obtained and compared with the recent experimental data. Through compared the formation cross sections of transfermium element 106 by three reactions of 136Xe+248Cm, 48Ca+248Cm and 238U+248Cm, it is explored that the large mass transfer reactions, like U+U are very benefit for the production of SH nuclei.     

Gas-cell-based setup for the production and study of neutron rich heavy nuclei

The present limits of the upper part of the nuclear map are very close to stability while the unexplored area of heavy neutron-rich nuclides along the neutron closed shell N = 126 is extremely important for nuclear astrophysics investigations and, in particular, for the understanding of the r-process of astrophysical nucleosynthesis. This area of the nuclear map can be reached neither in fusion–fission reactions nor in fragmentation processes widely used nowadays for the production of exotic nuclei. A new way was recently proposed for the production of these nuclei via low-energy multi-nucleon transfer reactions. The estimated yields of neutron-rich nuclei are found to be significantly high in such reactions and several tens of new nuclides can be produced, for example, in the near-barrier collision of ¹³⁶Xe with ²⁰⁸Pb. A new setup is proposed to produce and study heavy neutron-rich nuclei located along the neutron closed shell N = 126.     

Production and study of heavy neutron rich nuclei formed in multi-nucleon transfer reactions

A new setup is proposed to produce and investigate heavy neutron-rich nuclei located along the neutron closed shell N = 126. This “blank spot” of the nuclear map can be reached neither in fusion–fission reactions nor in fragmentation processes widely used nowadays for the production of exotic nuclei. The present limits of the upper part of the nuclear map are very close to stability while the unexplored area of heavy neutron-rich nuclides along the neutron closed shell N = 126 is extremely important for nuclear astrophysics investigations and, in particular, for the understanding of the r-process of astrophysical nucleosynthesis. A new way was recently proposed for the production of these nuclei via low-energy multi-nucleon transfer reactions. The estimated yields of neutron-rich nuclei are found to be rather high in such reactions and several tens of new nuclides can be produced, for example, in the near-barrier collision of 136Xe with 208Pb. This setup could definitely open a new opportunity in the studies at heavy-ion facilities and will have significant impact on future experiments.     

Production of new heavy isotopes in low-energy multinucleon transfer reactions

It is shown that the multinucleon transfer reactions in low-energy collisions of heavy ions may be used for production of new neutron-rich nuclei at the "northeast" part of the nuclear map along the neutron closed shell N=126 which plays an important role in the r process of nucleosynthesis. More than 50 unknown nuclei might be produced in such reactions (in particular, in collision of 136Xe with 208Pb) with cross sections of not less than 1 microb.     

Experimental nuclear astrophysics with radioactive ion beams

Reactions involving unstable nuclei play an important role in many astrophysical sites. Radioactive ion beams provide a unique tool to investigate the structure of such unstable nuclei as well as the cross sections for many reactions of astrophysical relevance. This paper provides a brief survey of some recent results in experimental nuclear astrophysics with Radioactive Ion Beams, particularly for processes which take place during explosive hydrogen burning in novae and X-ray bursts. Some prospects for future studies at next generation facilities are also briefly discussed.     

Dispersion theory of nucleon transfer reactions induced by heavy ions

A new approach, the distorted wave pole approximation (DWPA) with the three-body Coulomb effects, is developed by combining the dispersion method and DWBA to analyse the heavy ion-induced neutron transfer reactions. The influence of the three-body Coulomb dynamics on the peripheral partial wave amplitudes is investigated. Differential cross sections of the neutron transfer reactions are calculated to compare the proposed model with the conventional DWBA. The values of nuclear vertex constants for virtual separation of neutron from various nuclei are obtained. The results of the calculations show that DWPA can be applied to analyse the heavy ion-induced neutron transfer reactions and that the three-body Coulomb effects are taken into account with acceptable accuracy in DWBA.     

Nuclear Physics Programs for the Future RIBs Facility in Korea

We present nuclear physics programs based on the planned experiments using rare isotope beams (RIBs) for the future Korean Rare Isotope Beams Accelerator facility(KRIA). This ambitious facility has both an Isotope Separation On Line (ISOL) and fragmentation capability for producing RIBs and accelerating beams of wide range mass of nuclides with energies of a few to hundreds MeV per nucleon. Low energy RIBs at Elab = 5 to 20 MeV per nucleon are for the study of nuclear structure and nuclear astrophysics toward and beyond the drip lines while higher energy RIBs produced by inflight fragmentation with the reaccelerated ions from the ISOL enable to explore the neutron drip lines in intermediate mass regions. The planned programs have goals for investigating internal structures of the exotic nuclei toward and beyond the nucleon drip lines by addressing the following issues: how the shell structure evolves in areas of extreme proton to neutron imbalance; whether the isospin symmetry maintains in isobaric mirror nuclei at and beyond the drip lines; how two-proton radioactivity affects abundances of the elements; what the role of the continuum states including resonant states above protondecay threshold in exotic nuclei is in astrophysical nuclear reaction processes, and how the nuclear reaction rates triggered by unbound proton-rich nuclei make an effect on rapid proton capture processes in a very hot stellar plasma.     

Neutron-induced reaction rates for the <Emphasis Type="Italic">r</Emphasis>-process

Neutron-induced reaction rates for the formation of heavy and superheavy nuclei in the astrophysical r-process are presented. Neutron-induced reactions, including fission and neutron capture, at astrophysical temperatures are treated within the framework of the statistical model and calculated for targets with the atomic number 84 < Z < 118, using different mass and fission barrier predictions. The dependence of heavy element yields from nuclear explosions on the target nuclei, nuclear reactions, and nuclear models is discussed.     

Fusion and transfer reactions in beams of light loosely bound nuclei at energies in the vicinity of the Coulomb barrier

Experiments devoted to studying cross sections for fusion and transfer reactions induced by the interaction of beams of halo-like (⁶He), cluster (⁶Li and ⁷Li), and loosely bound (³He) nuclei with nuclei of light and heavy elements are described. The cross sections obtained experimentally for such reactions are analyzed. Special features in the behavior of the cross sections for the formation of evaporation residues and products of transfer reactions at energies in the vicinity of the Coulomb barrier are revealed. In particular, an increase in the cross sections for fusion and transfer reactions involving halo-like nuclei and proceeding at energies in the subbarrier region is observed. The cross sections for neutron-transfer and light-cluster-transfer reactions reachmaximum values at an energy in the vicinity of the Coulomb barrier for the reaction being considered.     

间接测量天体物理S因子的特洛伊木马方法

天体环境下的核反应速率是各种关于天体核合成理论模型所需的输入量,对于了解天体核合成过程,以及宇宙的演化很重要。但是在天体温度下,核反应是在很低的能量上发生的。由于库仑位垒的作用,反应截面非常低,直接测量很难进行。通过测量合适的三体反应截面,特洛伊木马方法提供了一种提取感兴趣的低能两体反应截面的方法;而且,采用一系列近似可得到便于计算的理论公式。本文介绍特洛伊木马方法的原理及其在天体核反应中的应用。     

Total Nuclear Reaction Cross Section Induced by Halo Nuclei and Stable Nuclei

We develop a method for calculation of the total reaction cross sections induced by the halo nuclei and stable nuclei. This approach is based on the Glauber theory, which is valid for nuclear reactions at high energies. It is extended for nuclear reactions at low energies and intermediate energies by including both the quantum correction and Coulomb correction under the assumption of the effective nuclear density distribution. The calculated results of the total reaction cross section induced by stable nuclei agree well with 30 experimental data within 10 percent accuracy.The comparison between the numerical results and 20 experimental data for the total nuclear reaction cross section induced by the neutron halo nuclei and the proton halo nuclei indicates a satisfactory agreement after considering the halo structure of these nuclei, which implies quite digerent mean fields for the nuclear reactions induced by halo nuclei and stable nuclei. The halo nucleon distributions and the root-mean-square radii of these nuclei can be extracted from the above comparison based on the improved Glauber model, which indicates clearly the halo structures of these nuclei. Especially,it is clear to see that the medium correction of the nucleon-nucleon collision has little effect on the total reaction cross sections, induced by the halo nuclei due to the very weak binding and the very extended density distribution.     

Total Nuclear Reaction Cross Section Induced by Halo Nuclei and Stable Nuclei

We develop a method for calculation of the total reaction cross sections induced by the halo nuclei and stable. nuclei. This approach is based on the Glauber theory, which is valid for nuclear reactions at high energies. It is extended for nuclear reactions at low energies and intermediate energies by including both the quantum correction and Coulomb correction under the assumption of the effective nuclear density distribution. The calculated results of the total reaction cross section induced by stable nuclei agree well with 30 experimental data within 10 percent accuracy. The comparison between the numerical results and 20 experimental data for the total nuclear reaction cross section induced by the neutron halo nuclei and the proton halo nuclei indicates a satisfactory agreement after considering the halo structure of these nuclei, which implies quite different mean fields for the nuclear reactions induced by halo nuclei and stable nuclei. The halo nucleon distributions and the root-mean-square radii of these nuclei can be extracted from the above comparison based on the improved Glauber model, which indicates clearly the halo structures of these nuclei. Especially,it is clear to see that the medium correction of the nucleon-nucleon collision has little effect on the total reaction cross sections induced by the halo nuclei due to the very weak binding and the very extended density distribution.     

Production cross sections for exotic nuclei with multinucleon transfer reactions

The main progresses in the multinucleon transfer reactions at energies close to the Coulomb barrier are reviewed. After a short presentation of the experimental progress and theoretical progress, the predicted production cross sections for unknown neutron-rich heavy nuclei and the trans-uranium nuclei are presented.     

MEND——-—个计算250 MeV以下中重核数据的程序(英文)

基于球型光学模型、 预平衡发射和Hauser Feshbach统计等理论, 编制了MEND程序（Medium Energy Nuclear Data）, 该程序适用于中重原子核在入射粒子能量低于250 MeV的中低能区的全套核数据计算。对于中子和质子在250 MeV以下诱发的核反应, 其全截面、 反应截面、 弹性散射微分截面、 双微分截面和能谱等理论计算值与相应的实验值基本一致。MEND是计算中低能核反应的基础程序, 在我国已被广泛用于核数据计算及建立中能核数据库Based on the spherical optical model, pre equilibrium statistical theory, and Hauser Feshbach theory, etc., the code MEND (Medium Energy Nuclear Data) is written for calculating the complete set of nuclear data of medium heavy nuclei in medium low energy region (≤250 MeV). For the reactions induced by neutron and proton below 250 MeV, the total cross sections, reaction cross sections, elastic scattering differential cross sections, double differential cross sections and energy spectra, etc. calculated by the code MEND, generally agree with those corresponding experimental data. MEND is a foundational program for nuclear reaction in medium low energy region and is wildely used for nuclear data calculation and establishing ENDF/B6 format files of medium low energy region in China.     

Theoretical study on production cross sections of exotic actinide nuclei in multinucleon transfer reactions

Within the dinuclear system(DNS) model, the multinucleon transfer reactions ~(129,136)Xe +~(248)Cm,~(112)Sn+~(238)U, and ~(144)Xe +~(248)Cm are investigated. The production cross sections of primary fragments are calculated with the DNS model. By using a statistical model, we investigate the influence of charged particle evaporation channels on production cross sections of exotic nuclei. It is found that for excited neutron-deficient nuclei the charged particle evaporation competes with neutron emission and plays an important role in the cooling process. The production cross sections of several exotic actinide nuclei are predicted in the reactions ~(112)Sn +~(238)U and ~(136,144)Xe +~(248)Cm.Considering the beam intensities, the collisions of ~(136,144)Xe projectiles with a ~(248)Cm target for producing neutron-rich nuclei with Z =92-96 are investigated.     

Production mechanism of neutron-rich nuclei around N =126 in the multi-nucleon transfer reaction ~(132)Sn+~(208)Pb

The time-dependent Hartree-Fock approach in three dimensions is employed to study the multi-nucleon transfer reaction~(132) Sn +~(208) Pb at various incident energies above the Coulomb barrier. Probabilities for different transfer channels are calculated by using the particle-number projection method. The results indicate that neutron stripping(transfer from the projectile to the target) and proton pick-up(transfer from the target to the projectile)are favored. De-excitation of the primary fragments is treated by using the state-of-art statistical code GEMINI++.Primary and final production cross sections of the target-like fragments(with Z =77 to Z =87) are investigated. The results reveal that fission decay of heavy nuclei plays an important role in the de-excitation process of nuclei with Z 82. It is also found that the final production cross sections of neutron-rich nuclei depend only slightly on the incident energy, while those of neutron-deficient nuclei depend strongly on the incident energy.     

Nuclear physics aspects of the astrophysical <Emphasis Type="Italic">p</Emphasis>-process

An overview is given on the experimental nuclear physics aspects of the astrophysical p-process that is responsible for the production of the heavy proton-rich nuclei known as p-nuclei. The nuclear physics input of the p-process scenario involves the knowledge of radiative capture cross sections, mostly calculated by the Hauser-Feshbach statistical model. Our experiments test the reliability of the model calculations in the proton-rich region as well as provide experimental information on the cross sections relevant to the p-process.     

Deformation effects in heavy-ion scattering

Many experiments on the scattering of heavy ions confirm that the elastic cross sections display characteristics of Fresnel diffraction. Recent experiments on the scattering of very heavy ions, however, show marked deviations from the expected Fresnel shapes and an analysis of these experiments using the “quarter-point-recipe” of the Fresnel cross section yields a larger radius for ²⁰⁸Pb than for ²³²Th. It is shown that the deviations may be described in terms of the ground state deformations of the nuclei involved. Taking the deformations into account removes the above anomaly in the radii. The actual fit to the experimental cross sections is not very good and suggests that the real part of the nuclear potential may have an appreciable effect on the orbits of nuclei which are elastically scattered below the Coulomb barrier.     

Theoretical Analysis of Neutron Double-Differential Cross Section of n+11B at 14.2 MeV

A new reaction model for light nuclei is proposed to analyze the measured data, especially for the doubledifferential cross sections. In this paper the calculation with this model is employed to analyze measurements of the total outgoing neutron double-differential cross sections for n+11B reactions at En = 14.2 MeV. The representation of the double-differential cross sections of the second emitted particles is given in detail. The calculation results indicate that the recoil effect in light nuclear reaction is essentially important. The reaction channels are discussed in detail.     

Special features of nuclear reactions induced by loosely bound <Superscript>6</Superscript>He and <Superscript>6,7</Superscript>Li nuclei in the vicinity of the Coulomb barrier height

Excitation functions are measured for complete-fusion and transfer reactions induced by the interaction of ⁶He and ⁶Li with ²⁰⁶Pb, ²⁰⁹Bi, and Pt. Data obtained for fusion reactions induced by ⁶He ions deviate from the predictions of the statistical model of compound-nucleus decay at projectile energies in the vicinity of the Coulomb barrier height. A strong enhancement of cross sections for fusion reactions induced by the interaction of ⁶He with target nuclei is observed. The cross sections for reactions of cluster transfer, neutron transfer from ⁶He, and deuteron transfer from ⁶Li at deep-subbarrier energies are also found to be enhanced. These results are discussed from the point of view of the effect of the cluster structure of nuclei on the interaction probability at energies in the vicinity of the Coulomb barrier height.