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采用三维粒子动力学模拟方法研究了甲烷团簇在超短强激光脉冲激励下的爆炸动力学行为,重点讨论了几种典型的内电离机理对团簇爆炸过程中离子的价态和动能的影响.研究表明,在激光脉冲强度比较小的情况下,团簇中的原子主要是在光场作用下通过隧道电离的方式发生电离.当激光场进一步增强时,势垒压低电离是电离的主要方式.在相同的较高激光强度下,团簇更容易通过势垒压低电离达到高的电离价态.团簇发生电离后,其内部库仑电场的点火电离效应和内部滞留自由电子的碰撞电离效应也将增强团簇的再次电离过程.
关键词:
超短强激光脉冲
甲烷团簇
内电离 相似文献
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Three-dimensional simulation on explosions of hydrogen atomic clusters irradiated by an intense femtosecond laser pulse 下载免费PDF全文
Using classic particle dynamics simulations, the interaction process between an intense femtosecond laser pulse and icosahedral hydrogen atomic clusters H_{13}, H_{55} and H_{147} has been studied. It is revealed that with increasing number of atoms in the cluster, the kinetic energy of ions generated in the Coulomb explosion of the ionized hydrogen clusters increases. The expansion process of the clusters after laser irradiation has also been examined, showing that the expansion scale decreases with increasing cluster size. 相似文献
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Nuclear fusion from Coulomb explosions of deuterated methane clusters subjected to ultraintense femtosecond laser pulses 下载免费PDF全文
This paper reports that Coulomb explosions taken place in the
experiment of heteronuclear deuterated methane clusters
((CD4)2) in a gas jet subjected to intense femtosecond
laser pulses (170mJ, 70fs) have led to table-top laser driven DD
nuclear fusion. The clusters produced in supersonic expansion had an
average size of about 5nm in radius and the laser intensity used
was 3×1017W/cm2.The measured maximum and average
energies of deuterons produced in the laser--cluster interaction were
60 and 13.5keV, respectively. From DD collisions of energetic
deuterons, a yield of 2.5(±0.4)×104 fusion neutrons
of 2.45MeV per shot was realized, giving rise to a neutron
production efficiency of about 1.5×105 per joule of
incident laser pulse energy. Theoretical calculations were performed
and a fairly good agreement of the calculated neutron yield with
that obtained from the present experiment was found. 相似文献
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Under classical particle dynamics, the interaction process between intense femtosecond laser pulses and icosahedral noble-gas atomic clusters was studied. Our calculated results show that ionization proceeds mainly through tunnel ionization in the combined field from ions, electrons and laser, rather than the electron-impact ionization. With increasing cluster size, the average and maximum kinetic energy of the product ion increases. According to our calculation, the expansion process of the clusters after laser irradiation is dominated by Coulomb explosion and the expansion scale increases with increasing cluster size. The dependence of average kinetic energy and average charge state of the product ions on laser wavelength is also presented and discussed. The dependence of average kinetic energy on the number of atoms inside the cluster was studied and compared with the experimental data. Our results agree with the experimental results reasonably well. 相似文献
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靶室腔体谐振产生的电磁辐射是超短超强激光与靶相互作用实验中生成的电磁脉冲(EMP)来源之一。基于有限元分析方法,对靶室腔谐振产生电磁脉冲和电磁脉冲通过窗口向外传播这两个过程进行仿真模拟。前者模拟获得空腔和含结构模型谐振时特征磁场,结果显示内部结构对电磁场强度分布和谐振频率有显著影响;后者模拟结果显示,窗口外侧电场强度比窗口内侧高约40%,而且电磁脉冲传播到靶室外后呈球面波形式扩散并衰减。对电磁脉冲的强度衰减规律进行了分析,得到该衰减曲线的拟合函数。 相似文献
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用一维相对论粒子模拟研究了相对论超短强激光脉冲在等离子体中传播时激发的尾波场,初步获得了近共振区尾波场的峰值幅度随激光脉冲宽度变化的特点,发现在近共振区等离子体波激发出现增强。通过准静态近似下尾波激发的一维非线性方程数值求解,并与粒子模拟结果比较,得到了该非线性方程的适用范围:当激光脉冲宽度小于等离子体波波长的4倍时,该方程所得结果与粒子模拟结果一致;而当激光脉冲宽度大于该数值时,该方程不再适用。 相似文献
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The interaction between intense femtosecond laser pulses
and hydrogen atomic clusters is studied by a simplified Coulomb
explosion model. The dependences of average proton kinetic energy on
cluster size, pulse duration, laser intensity and wavelength are
studied respectively. The calculated results indicate that the
irradiation of a femtosecond laser of longer wavelength on hydrogen
atomic clusters may be a simple, economical way to produce highly
kinetic hydrogen ions. The phenomenon suggests that the irradiation
of femtosecond laser of longer wavelength on deuterium atomic
clusters may be easier than that of shorter wavelength to drive
nuclear fusion reactions. The product of the laser intensity and the
squared laser wavelength needed to make proton energy saturated as a
function of the squared cluster radius is also investigated. The
proton energy distribution calculated is also shown and compared
with the experimental data. Our results are in agreement with the
experimental results fairly well. 相似文献
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利用飞行时间谱,研究了在飞秒强激光场(60 fs,2×1016 W/cm2)作用下,大尺寸氩原子团簇Arn(n—=3×103—3×106原子/每团簇)的电离爆炸过程,测量了 团簇爆炸所产生的氩离子的平均能量与团簇尺寸(气体背压)的关系.实验发现,随着气体 背压的升高(团簇尺寸增大),氩离子的平均能量也相应升高.通过分析两个不同几何尺寸 锥形超声喷嘴所产生团簇爆炸后的离子能量,结合Hagena团簇尺寸规律,发现在激光参数保 持不变的情况下,离子的平均能量由团簇尺寸唯一确定.分析表明,团簇尺寸在3×105原 子/每团簇以下时,团簇膨胀的主要机理是库仑爆炸.随着团簇尺寸的进一步增大,团簇膨胀 机理将由库仑爆炸向流体动力学膨胀过渡,在3×105关键词:
原子团簇
飞秒强激光
库仑爆炸
流体动力学膨胀 相似文献
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采用简化库仑爆炸模型对强激光脉冲照射氘代乙烷团簇发生的库仑爆炸过程进行数值模拟,研究了氘代乙烷团簇爆炸产生的氘核动能、中子产额与团簇尺寸的关系,且与氘代甲烷团簇产生的氘核动能及中子产额进行了比较.研究表明,尺寸为5 nm的氘代乙烷团簇在发生库仑爆炸后氘核的最大动能为20.96 keV,获得的中子产额为6.31×105,比同尺寸氘代甲烷团簇产生的氘核最大动能及中子产额更大.因此相对于氘代甲烷团簇,大尺寸的氘代乙烷团簇更适合作为激光驱动团簇库仑爆炸获得高额中子的靶材,这与报道的实验推论相一致. 相似文献
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用二维粒子模拟程序研究了超短脉冲强激光与等离子体相互作用中局域低频电磁场的产生现象.这种低频电磁场在超短脉冲激光激发尾波场、脉冲后沿产生频率下移的过程中形成.通常它们的振荡频率接近于或低于电子等离子体振荡频率,因而被捕获在等离子体中(即传播速度接近于零).在演化过程中,通常它们以孤子场的形式出现.这种孤子波的形成及其演化与离子运动有极大关系.用相对论强激光脉冲可以产生达到相对论振幅的电磁场孤子波,后者可以把离子加速到非常高的能量.研究还表明,在二维几何位形下,孤子波产生与入射光的偏振态有很大关系. 相似文献
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We experimentally demonstrate the Coulomb explosion process of CS_2 molecule under a near-infrared(800 nm)intense femtosecond laser field by a DC-sliced ion imaging technique. We obtain the DC-sliced images of these fragment ions S~+, S~(2+), CS~+, and CS~(2+)by breaking one C–S bond, and assign their Coulomb explosion channels by considering their kinetic energy release and angular distribution. We also numerically simulate the dissociation dynamics of parent ions CS_2~(k+)(k = 2–4) by a Coulomb potential approximation, and obtain the time evolution of Coulomb energy and kinetic energy release, which indicates that the dissociation time of parent ions CS_2~(k+) decreases with the increase of the charge number k.These experimental and theoretical results can serve as a useful benchmark for those researchers who work in the related area. 相似文献
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High-order harmonic generation spectrum of an excited one-dimensional Coulomb atom in an intense laser field 下载免费PDF全文
Response of the wave packet of a one-dimensional Coulomb atom
to an intense laser field is calculated using the symmetrized
split operator fast Fourier method. The high-order harmonic
generation (HHG) of the initial state separately being the ground and excited states
is presented. When the hardness parameter \alpha in the soft
Coulomb potential V(x)=-1/\sqrt{x^2+\alpha} is chosen to be small
enough, the so-called hard Coulomb potential
V(x)=-1/|x| can be obtained. It is well known that the hard one-dimensional Coulomb atom
has an unstable ground
state with an energy eigenvalue of $\sim0.5$ and it
has no states corresponding to physical states in the true atoms, and
has the first and second excited states being degenerate. The parity effects on the HHG
can be seen from the first and second excited states of the hard
one-dimensional Coulomb atom. The HHG spectra of the excited states
from both the soft and hard Coulomb atom models are shown to have more
complex structures and to be much stronger than the corresponding
HHG spectrum of the ground state of the soft Coulomb model with
$\alpha=2$ in the same laser field. Laser-induced non-resonant
one-photon emission is also observed. 相似文献
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陈基根 《原子与分子物理学报》2008,25(5):1431-1434
采用强短激光脉冲辐照叠加态原子提高孤立阿秒脉冲的强度。数值研究表明,与强短脉冲
(脉冲宽度只有几个光学周期的超短脉冲)辐照基态原子获得孤立阿秒脉冲相比,采用叠加
态原子的方案不仅同样可以获得孤立的阿秒脉冲,而且阿秒脉冲的强度得到显著增强。 相似文献
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利用低温脉冲气阀获得了平均含有3×103氘原子的氘团簇。在飞秒激光装置上实现了氘团簇聚变,每发中子产额为1×103。中子产额对激光功率密度敏感,保持激光能量不变,随着激光焦斑的变大,DD聚变中子产额逐渐增加,最大值出现在激光焦斑为470 mm时;继续增大激光焦斑,没有观察到中子信号。实验结果还表明激光氘团簇聚变发生的区域主要是激光辐照的等离子体热区,此区域内邻近氘团簇库仑爆炸发射的高能氘离子碰撞引发聚变反应。 相似文献