Probable Decay Modes at Limits of Nuclear Stability of the Superheavy Nuclei

The modes of decay for the even–even isotopes of superheavy nuclei of Z = 118 and 120 with neutron number 160 ≤ N ≤ 204 are investigated in the framework of the axially deformed relativistic mean field model. The asymmetry parameter η and the relative neutron–proton asymmetry of the surface to the center (R _η ) are estimated from the ground state density distributions of the nucleus. We analyze the resulting asymmetry parameter η and the relative neutron–proton asymmetry R _η of the density play a crucial role in the mode(s) of decay and its half-life. Moreover, the excess neutron richness on the surface, facets a superheavy nucleus for β^? decays.     

Effect of properties of superheavy nuclei on their production and decay

Properties and stability of superheavy nuclei resulting from hot fusion are discussed. It is shown that the microscopic–macroscopic approach allows obtaining the closed proton shell at Z ≥ 120. Isotopic trends of K-isomeric states in superheavy nuclei are predicted. Evaporation residue cross sections in hot fusion reactions are calculated using the predicted properties of superheavy nuclei. Interruption of α decay chains by spontaneous fission is analyzed. Alpha decay chains through isomeric states are considered. Internal level densities in superheavy nuclei are microscopically calculated.     

Dynamical screening of AMM and QED effects for large-<Emphasis Type="Italic">Z</Emphasis> hydrogen-like atoms

The effective interaction ΔU_AMM of the anomalous magnetic moment (AMM) of an electron with the Coulomb field of an extended nucleus is analyzed. As soon as the q² dependence of the electron formfactor F₂(q²)is taken into account from the beginning, the AMM is found to be dynamically screened at small distances of r ? 1/m. The ΔU_AMM effects on the low-lying electronic levels of a superheavy extended nucleus with Zα > 1are analyzed using the nonperturbative approach. The growth rate of the ΔU_AMM contribution with increasing Z is shown to be essentially nonmonotonic. At the same time, the energy shifts of electronic levels in the vicinity of the threshold of the lower continuum monotonically decrease in the region Z ?Z_cr,1s. The latter result is generalized to the whole self-energy contribution to energy shifts of electronic levels, thus also referring to the possible behavior of QED radiative effects with virtual-photon exchange, considered beyond the framework of the perturbative expansion in Zα.     

Energy scan of cross sections for <Emphasis Type="Italic">e</Emphasis><Superscript>+</Superscript><Emphasis Type="Italic">e</Emphasis><Superscript>–</Superscript> annihilation into quarkonia and light hadrons in the Belle experiment

The cross sections of the reactions e⁺e^– → ?(nS)π⁺π^? (n = 1, 2,3) and e⁺e^– → h _b (nP)π⁺π^? (n = 1, 2) are measured as a function of the cms collision energy from their thresholds up to 11.02 GeV using the data of the Belle experiment operating at the KEKB e⁺e^– collider. The peaks of the ?(10 860) and ?(11020) resonances are observed in the cross sections with an insignificant contribution of the continuum. The decay ?(11020) → h _b (nP)π⁺π^? is found to fully proceed through intermediate isovector states Z _b (10610) and Z _b (10650).     

Collective excitations of the element <Emphasis Type="Italic">Z</Emphasis> = 120

The low-lying vibrational excitations of superheavy even-even nuclei around Z=120 and N=172, predicted to be spherical by the relativistic mean-field (RMF) model, are studied within a phenomenological collective approach. In the framework of the macroscopic model for giant resonances, we compute the transition densities of the isoscalar monopole, quadrupole, and octupole and isovector dipole modes for the superheavy nucleus ²⁹²120, whose ground-state density is determined from the RMF model. The results are also compared to those for²⁰⁸Pb.     

The study of superheavy elements at SHIP: Results and plans

The nuclear shell model predicts that the next doubly magic shell closure beyond ²⁰⁸Pb is at a proton number between Z=114 and 126 and at a neutron number N=184. The outstanding aim of experimental investigations is the exploration of this region of spherical “superheavy elements.” This article describes the experiments that were performed at the GSI SHIP. They resulted in an unambiguous identification of elements 107 to 112. They were negative thus far in searching for elements 113, 116, and 118. The measured decay data are compared with theoretical predictions. Some aspects concerning the reaction mechanism are also presented.     

Optical and x-ray diffraction studies of the symmetry of distorted phases of the (NH<Subscript>4</Subscript>)<Subscript>3</Subscript>ZrF<Subscript>7</Subscript> crystal

(NH₄)₃ZrF₇ single crystals were grown, and polarization-optical and x-ray diffraction studies were performed on powders and crystalline plates of various cuts over a wide temperature range. Phase transitions are revealed at temperatures T _1↑ = 280 K, T _2↑ = 279.6 K, T _3↑ = 260–265 K, and T _4↑ = 238 K on heating and at T _1↓ = 280 K, T _2↓ = 269–270 K, T _3↓ = 246 K, and T _4↓ = 235 K on cooling. The sequence of changes in symmetry is established to be as follows: O _h ⁵ (Z = 4) ? D _2h ²⁵ (Z = 2) ? C _2h ³ (Z = 2) ? C _i ¹ (Z = 108) ? monoclinic²(Z = 216).     

On search and identification of relatively short-lived superheavy nuclei (<Emphasis Type="Italic">Z</Emphasis> ≥ 110) by fossil track studies of meteoritic and lunar olivine crystals

The main goal of the present work is the search for and identification of relatively stable nuclei of superheavy elements (SHE) (Z>110) in galactic matter by fossil track study of nonconducting crystals from the surface of meteorites and rocks from the lunar regolith. Nuclei of SHE are thought to be the products of nucleosynthesis in explosive processes in our Galaxy (supernova r-process nucleosynthesis and, especially, neutron-star formation, etc.). When accelerated to relativistic energies in the Galaxy, they can produce extended trails of damage in nonconducting extraterrestrial crystals. The lifetime of such SHE in galactic cosmic rays will range from 10³ to 10⁷ yr to be registered in extraterrestrial crystals. To search for and to identify the superheavy nuclei in the galactic cosmic rays, it was proposed to use the ability of nonconducting extraterrestrial crystals such as olivines, pyroxenes, and feldspars to detect and to store for many millions of years the trails of damage produced by fast Z≥23 nuclei coming to rest in the crystalline lattice. The track lengths of fast Z≥23 nuclei are directly proportional to Z² of these nuclei. The nuclei of SHE produce, when coming to rest in a crystal volume, tracks that are a factor of 1.6–1.8 longer than the tracks due to cosmic-ray Th and U nuclei. To identify the tracks due to superheavy nuclei, calibrations of the same crystals were performed with accelerated Au, Pb, and U nuclei. For visualization of these tracks inside the crystal volume, proper controlled annealing and chemical etching procedures were developed. Since 1980, fossil tracks due to Th and U nuclei have observed and unambiguously identified (1988) by subsequent calibrations of the olivine crystals with accelerated U, Au, and Pb ions. The number of tracks of Th and U nuclei measured in olivine crystals totaled more than 1600, as compared with the prior 30 events. The other approach to identifying SHE in nature is to search for tracks in phosphate crystals from spontaneous fission of Z ≥ 110 nuclei; these produce two-prong and three-prong fission fragment tracks and differ significantly from the tracks from spontaneous fission of ²³⁸U and ²⁴⁴Pu nuclei. Extraterrestrial phosphate crystals of lunar and meteoritic origin will be investigated. Such SHE nuclei can survive in crystals of extraterrestrial rocks and produce spontaneous fission tracks, if the lifetime is more than 5×10⁷ yr.     

Special features of the structure of the beta-stability line for nuclei

The mass-number (A) dependence Z _β(A) for nuclei lying on the beta-stability line (BSL) is calculated for A and Z values in the ranges of A = 2–258 and Z = 1–100, respectively. The calculated values are compared with experimental data. The deviations ΔZ = Z _expt ? Z _β are analyzed. This analysis of ΔZ reveals that there are three regions of A values in which the A dependence of ΔZ is parabolic. The possible forms of the A dependence of ΔZ are analyzed, and it is shown that the majority of nuclei belong to several parabolas simultaneously.     

On the Possibility of Delayed Fission of Nuclei in the Region of Superheavy Transuranium Elements

Delayed fission of atomic nuclei was discovered in 1966. It is observed primarily in odd–odd nuclei for which the energy released in beta decay (K capture) is commensurate with the fission barrier in the nucleus formed after this process. Delayed fission was found in four nuclide regions: neutrondeficient isotopes in the Pb region, neutron-deficient isotopes in the Ac and Pa regions, and neutrondeficient and neutron-rich isotopes of transuranium elements. In the wake of investigations into the properties of isotopes of superheavy transuranium elements, numerous calculations were performed in order to determine the masses of new nuclei and to predict their decay properties. Explored and predicted properties of superheavy-element nuclides, where, for some odd–odd nuclei of transuranium elements, the K-capture energy is commensurate with the fission barriers in the corresponding daughter nuclei formed after K capture, are analyzed. Estimates of the delayed-fission probability are presented for some isotopes of elements whose charge number Z ranges from 103 to 107.     

New outlook on the possible existence of superheavy elements in nature

A consistent interpretation is given to some previously unexplained phenomena seen in nature in terms of the recently discovered long-lived high-spin super-and hyperdeformed isomeric states. The Po halos seen in mica are interpreted as being due to the existence of such isomeric states in corresponding Po or nearby nuclei that eventually decay by γ or β decay to the ground states of ²¹⁰Po, ²¹⁴Po, and ²¹⁸Po nuclei. The low-energy 4.5-MeV α-particle group observed in several minerals is interpreted as being due to a very enhanced α transition from the third minimum of the potential-energy surface in a superheavy nucleus with atomic number Z=108 (Hs) and atomic mass number around 271 to the corresponding minimum in the daughter.     

Electron gas induced in SrTiO<Subscript>3</Subscript>

This mini-review is dedicated to the 85th birthday of Prof. L.V. Keldysh, from whom we have learned so much. In this paper, we study the potential and electron density depth profiles in surface accumulation layers in crystals with a large and nonlinear dielectric response such as SrTiO₃ (STO) in the cases of planar, spherical, and cylindrical geometries. The electron gas can be created by applying an induction D₀ to the STO surface. We describe the lattice dielectric response of STO using the Landau–Ginzburg free energy expansion and employ the Thomas–Fermi (TF) approximation for the electron gas. For the planar geometry, we arrive at the electron density profile n(x) ∝ (x + d)^–12/7, where d ∝ D₀^–12/7. We extend our results to overlapping electron gases in GTO/STO/GTO heterojunctions and electron gases created by spill-out from NSTO (heavily n-type doped STO) layers into STO. Generalization of our approach to a spherical donor cluster creating a big TF atom with electrons in STO brings us to the problem of supercharged nuclei. It is known that for an atom with a nuclear charge Ze where Z > 170, electrons collapse onto the nucleus, resulting in a net charge Zn < Z. Here, instead of relativistic physics, the collapse is caused by the nonlinear dielectric response. Electrons collapse into the charged spherical donor cluster with radius R when its total charge number Z exceeds the critical value Z_c ≈ R/a, where a is the lattice constant. The net charge eZ_n grows with Z until Z exceeds Z* ≈ (R/a)^9/7. After this point, the charge number of the compact core Z_n remains ≈ Z*, with the rest Z* electrons forming a sparse TF atom with it. We extend our studies of collapse to the case of long cylindrical clusters as well.     

<Emphasis Type="Italic">Z</Emphasis><Superscript>0</Superscript>-boson decays in a strong electromagnetic field

The probability of Z ⁰-boson decay to a pair of charged fermions in a strong electromagnetic field, Z ⁰ → \(\bar f\) f, is calculated. On the basis of a method that employs exact solutions to relativistic wave equations for charged particles, an analytic expression for the partial decay width Γ(?) = Γ(Z ⁰ → \(\bar f\) f) is obtained at an arbitrary value of the parameter ? = \(eM_Z^{ - 3} \sqrt { - (F_{\mu \nu } q^\nu )^2 } \), which characterizes the external-field strength. The total Z ⁰-boson decay width in an intense electromagnetic field, Γ _Z (?), is calculated by summing these results over all known generations of charged leptons and quarks. It is found that, in the region of relatively weak fields (? < 0.06), the field-induced corrections to the standard Z ⁰-boson decay width in a vacuum do not exceed 2%. As ? increases, the total decay width Γ _Z (?) develops oscillations against the background of its gradual decrease to the absolute-minimum point. At ?_min = 0.445, the total Z ⁰-boson decay width reaches the minimum value of Γ _Z (?_min) = 2.164 GeV, which is smaller than the Z ⁰-boson decay width in a vacuum by more than 10%. In the region of superstrong fields (? > 1), Γ _Z (?) grows monotonically with increasing external-field strength. In the region ? > 5, the t-quark-production process Z ⁰ → \(\bar t\) t, which is forbidden in the absence of an external field, begins contributing significantly to the total decay width of the Z ⁰ boson.     

Description of quasifission reactions in the dinuclear system model

The formation and evolution of dinuclear systems in quasifission reactions are investigated. The process of formation of reaction products is analyzed based on the concept of a dinuclear system. Isotopic trends of cross sections of production of superheavy nuclei in quasifission reactions are discussed. The yields of new neutron-rich isotopes of nuclei with Z = 64–80 in quasifission reactions are predicted. The mechanism of production of complex fragments in complete fusion and quasifission reactions is analyzed.     

Probing of <Emphasis Type="Italic">Z</Emphasis>γγ production sensitivity to anomalous quartic gauge couplings at LHC experiments with √ <Emphasis Type="Italic">s</Emphasis> =13 TeV

Sensitivity to anomalous ZZγγ and Zγγγ couplings in Zγγ production was probed for the ATLAS experiment at Large Hadron Collider. Zγγ process with anomalous couplings simulation in ppcollisions with √ s = 13 TeV was performed using VBFNLO MC generator. The expected limits on the Effective Field Theory parameters f _T0/Λ4, f _T5/Λ4, f _T9/Λ4, f _M2/Λ4, f _M3/Λ4 were extracted for 5 fb^?1 integral luminosity using the distribution on the invariant mass of Zγγ from the combination of charged leptonic decay channels of Z boson (Zγγ → μ⁺μ^?γγ and Zγγ → e⁺e^?γγ).     

The 3–3–1 Model with RH Neutrinos and Associated ZH Production at High-Energy ${\bf \textit{e}}^{+}{\bf \textit{e}}^{-}$ Collider

In the context of SU(3) _C ?? SU(3) _L ?? U(1) _X (3–3–1) model with right-handed neutrinos, we study the Higgsstrahlung process e ^?+? e ^???→ZH and calculate the cross section of this process at leading order. Our numerical results showed that the production cross sections for this process can be significantly large as \(M_{Z'}\approx \sqrt{s}\). With reasonable values of the Z′ mass M _Z′, Z′ exchange can generate large corrections to the cross sections of this process, which might be detected in the future high-energy linear e ^?+? e ^??? collider experiments.     

Elastic scattering of 0.5 MeV gamma rays by heavy elements

The absolute differential cross sections for the elastic scattering of 0.511 MeV gamma rays were measured in the angular range 0.5? to 10? for the elements withZ=72 toZ=92. The experimental method, employing annihilation radiation in coincidence, permits the investigation at very small momentum transfer. In general the results obtained are in very good agreement with the predictionZ ² r ₀ ² for the differential Rayleigh cross section atθ=0? and with the form factor theory, using Hartree-Fock-Slater wave functions, for the investigated angular range. However, for the elements lead, bismuth and thorium we found marked deviations from the form factor predictions, occurring at very small scattering angles. This is attributed to an outer atomic charge distribution different from the other investigated elements, which is also indicated by considerably greater metallic radii. Also effects due to the crystalline structure cannot be excluded. — Further, an elastic, resonance-like andZ-dependent scattering effect by bound electrons is discussed which is due to the formation of an intermediate, bound positronium state by electron-positron pairs.     

New Bounds on the Maximum Ionization of Atoms

We prove that the maximum number N _c of non-relativistic electrons that a nucleus of charge Z can bind is less than 1.22Z + 3Z ^1/3. This improves Lieb’s upper bound N _c  < 2Z + 1 Lieb (Phys Rev A 29:3018–3028, 1984) when Z ≥ 6. Our method also applies to non-relativistic atoms in magnetic field and to pseudo-relativistic atoms. We show that in these cases, under appropriate conditions, \({\limsup_{Z \to \infty}N_c/Z \le 1.22}\).     

New neutron magic number <Emphasis Type="Italic">N</Emphasis> = 16 for neutron-rich nuclei

A survey of experimental results obtained at GANIL (Caen, France) on the study of the properties of very neutron-rich nuclei (Z=6–20, A=20–60) near the neutron drip line and resulting in an appearance of further evidence for the new magic number N=16 is presented. Very recent data on mass measurements of neutron-rich nuclei at GANIL and some characteristics of binding energies in this region are discussed. Nuclear binding energies are very sensitive to the existence of nuclear shells, and together with the measurements of instability of doubly magic nuclei ¹⁰He and ²⁸O, they provide information on changes in neutron shell closures of very neutron-rich isotopes. The behavior of the two-neutron separation energies S_2n derived from mass measurements gives very clear evidence for the existence of the new shell closure N=16 for Z=9 and 10 appearing between the 2s_1/2 and 1d_3/2 orbitals. This fact, strongly supported by the instability of C, N, and O isotopes with N>16, confirms the magic character of N=16 for the region from carbon up to neon, while the shell closure at N=20 tends to disappear for Z≤13. Decay studies of these hardly accessible short-lived neutron-rich nuclei from oxygen to silicon using in-beam γ-ray spectroscopy are also reported.