Study of semiconductors using solid state nuclear track detectors

Uranium trace characterization of crystalline GeS, sputtered thin films of GeS and amorphous SiH on quartz substrates, and crystalline p-type Si using the technique of solid state nuclear track detectors is reported. Concentration and distribution of uranium in these materials studied are presented. Using uranium as microprobe, it is observed that uranium prefers to be in the cleavage planes of GeS crystals. There seems to be a link between uranium concentration and the thermally induced defects in Si.     

Gamma and neutron dose measurements with solid state nuclear track detectors

An attempt has been made to explore the possibility of using solid state nuclear track detectors for the estimation of gamma and neutron doses based on the use of changes in activation energy of degradation of these detectors, due to irradiation (gamma-neutron), as a means of dosimetry. Thermogravimetry (TG) has been applied as a tool for these studies carried out on Lexan and CR-39 track detectors. A linear relationship observed between the decrease in activation energy and the dose (gamma-neutron) received by the detectors suggests the possibility of the use of these detectors as gamma and neutron dosimeters.      

Time-resolved photoluminescence study of AgCl:Cd solid state nuclear track detectors

Crystalline AgCl:Cd²⁺ thin foils (Cd²⁺ concentration 62.5 – 5000 ppm) were studied by time-resolved photoluminescence spectroscopy in temperature range 20 – 80K using a mechanical phoroscope. Simple method is presented how to use the photoluminescence behaviour to check suitability of AgCl:Cd²⁺ foils to record high-energy particles tracks.     

Ferrofluidic masking of solid state nuclear track detectors during etching

This work presents a novel method for determining bulk etch rate of CR-39 during prolonged etching by masking the surface with a ferrofluidic film held in position by magnetostatic forces. The CR-39 etching conditions were 6.25 M NaOH solution for 24 h at temperatures ranging from 50 to 80 °C. After etching, the heights of the resulting un-etched plateaus were measured using a Talyscan 150 profilometer. The removed layer thicknesses ranged from 12 to 85 μm, giving corresponding bulk etch rates in the range 0.5–3.54 μm/h.     

Radon epidemiology and nuclear track detectors: Methods, results and perspectives

An important achievement of nuclear track detectors is that they render it possible to measure a large number of radon concentrations. These are necessary for epidemiological studies aimed to estimate the lung cancer risk due to exposure to radon and its decay products in dwellings. Many case–control studies were conducted in the last 15 years in Europe, North America and China, in order to avoid the uncertainties associated with the risk extrapolation from epidemiological studies on miners exposed in underground mines. In this review paper, the main methodological issues of these studies are introduced: confounding factors, the impact of radon exposure uncertainties on the estimated risk, the retrospective assessment of radon exposure through the measurement of surface concentration on glass objects, the interaction between radon and smoking, statistical methods to analyze data and combine studies, etc. As regards the estimated risk of lung cancer, the main characteristics and results of each study are reported and discussed, together with the results of meta-analyses and, most importantly, of the three recently published analyses that pool 2 Chinese, 7 North American, and 13 European studies. Finally, some conclusions are given and a brief reference is made to ongoing studies.     

Single-sheet identification method of heavy charged particles using solid state nuclear track detectors

The theoretical and experimental investigations of the penetration of charged particles in matter played a very important role in the development of modern physics. Solid state nuclear track detectors have become one of the most important tools for many branches of science and technology. An attempt has been made to examine the suitability of the single-sheet particle identification technique in CR-39 and CN-85 polycarbonate by plotting track cone length vs. residual range for different heavy ions in these detectors. So, the maximum etchable ranges of heavy ions such as ⁹³Nb, ⁸⁶Kr and ⁴He in CR-39 and ⁴He and ¹³²Xe in CN-85 polycarbonate have been determined. The ranges of these ions in these detectors have also been computed theoretically using the Henke-Benton program. A reasonably good agreement has been observed between the experimentally and theoretically computed values.      

Uranium analysis by neutron induced fissionography method using solid state nuclear track detectors

In this study total twenty samples (eight reference materials and twelve sediment samples) were analysed for their uranium content which is in the range of 1–17 μg/g, by neutron induced fissionography (NIF) method using solid state nuclear track detectors (SSNTDs) in comparison with the results of neutron activation analysis (NAA), delayed neutron counting (DNC) technique or fluorometric method. It is found that NIF method using SSNTDs is very sensitive for analysis of uranium.     

Factors affecting the registration and counting of alpha tracks in solid state nuclear track detectors

In view of the fact that the radon progeny contribute the highest to the natural radiation dose to general populations, large scale and long-term measurements of radon and its progeny in the houses have been receiving considerable attention. Solid State Nuclear Track Detector (SSNTD) based systems, being the best suited for large scale passive monitoring, have been widely used for the radon gas (using a cup closed with a semi-permeable membrane) and to a limited extent, for the measurement of radon progeny (using bare mode in conjunction with the cup). These have been employed for radon mapping and indoor radon epidemiological studies with good results. In this technique, alpha tracks recorded on SSNTD films are converted to radon/thoron concentrations using corresponding conversion factors obtained from calibration experiments carried out in controlled environments. The detector response to alpha particles depends mainly on the registration efficiency of the alpha tracks on the detector films and the subsequent counting efficiency. While the former depends on the exposure design, the latter depends on the protocols followed for developing and counting of the tracks. The paper discusses on parameters like etchant temperature, stirring of the etchant and duration of etching and their influence on the etching rates on LR-115 films. Concept of break down thickness of the SSNTD film in spark counting technique is discussed with experimental results. Error estimates on measurement results as a function of background tracks of the films are also discussed in the paper.      

Direct determination of bulk etching rate for LR-115-II solid state nuclear track detectors

The thickness of the removed layer of the LR-115-II solid state nuclear track detector during etching is measured directly with a rather precise instrument. Dependence of bulk etching rate on temperature of the etching solution is investigated. It has been found that the bulk etching rate is 3.2 μm/h at 60°C in 2.5 N NaOH of water solution. It is also found that the track density in detectors exposed to soil samples increases linearly with the removed layer.     

Investigation of uranium dioxide distribution dissolved in silicate compositions using solid state nuclear track detectors

The method of solid state nuclear track detectors (SSNTD) has been used for the determination of uranium dioxide distribution in silicate compositions. The method of -radiography based on registration of - particles at the contact of SSNTD CR-39 with the specimen has been used here. An initial uranium dioxide applied for studying the dissolving process used as the standard. The results of the measurements of distribution of uranium dioxide concentration obtained with the help of this technique have been used for the estimation of diffusion and solubility of UO₂ in silicate melts.     

Measurement of indoor radon levels in Erbil capital by using solid state nuclear track detectors

Radon alpha activity concentration has been measured in 28 homes in the Erbil Capital-Iraqi Kurdistan region during the autumn season by using time-integrated passive radon dosimeters containing CR-39 solid state nuclear track detectors “SSNTDs”. The radon activity concentrations in these homes range from (10.33–90.34) with an average of . The average absorption effective dose equivalent for a person living in homes for which the investigation were done was found to be , obtained by using an equilibrium factor of 0.5 and an occupancy factor of 0.8. The average lung cancer cases per year per 10⁶ person was found to be 23±12.     

Plastics as nuclear track detectors for thermal neutron dosimetry

An attempt is made to determine the response of CR-39 and cellulose nitrate plastic track detectors subjected to thermal neutrons. The α-particles are produced from (n, α) reactions in lithium tetraborate convertor placed in contact with different plastics and are recorded in the detectors. The corrected track density gives a fluence sensitivity and dose sensitivity of the order of 10^?4 tracks per neutron and 10² tracks/cm² mrem respectively. A linear relationship is observed between track density and neutron fluence.     

Radiator effect on plastic nuclear track detectors for high-energy neutrons

The effect of radiators supplying charged particles to plastic nuclear track detectors has been investigated both experimentally and theoretically in order to apply them to personal dosimeters for high-energy neutrons. Performance of four types of radiator materials, CH₂, CD₂ (deuterized hydrocarbon), LiF (lithium fluoride) and C (graphite), was checked in a quasi-monoenergetic neutron field generated by p-Li reactions. The efficiency has been numerically calculated based on a model with a special attention to the angular dependence of cross sections and data of characteristic response to light ions. The effect of respective radiator candidates has been evaluated as a function of the neutron energy. A two-layer radiator has also been proposed to adjust the energy dependence of the relative sensitivity to conversion factor for dose-equivalent.     

The method of simultaneous size and activity measurement of alpha emitting hot particles using multiple track analysis of solid state nuclear track detectors

Current work is concentrated upon the detection and analysis of hot particles from contaminated ground. Simultaneous measurement of parameters as activity and size of radioactive particle would have immense value for many applications in radiation protection and control of the environment. The algorithm and performance of multiple alpha track analysis is discussed.     

The applications of nuclear track detectors in transuranic contamination problems

Nuclear Track Methodology (NTM) is very well known for its possibilities in applications in a wide variety of fields. The appearance of the polycarbonate as alpha radiation detector material, established a very confident monitoring surface alpha contamination, soil and water alpha activity. The purpose of the study is to investigate the utility of the CR-39 (Allyl Diglycol Carbonate) in fast semi-quantitative transuranic contaminant evaluation, including the distribution in underground contaminated soils, hot spots and transuranic material accumulations.     

A joint UAB-IReS-IPNO neutron comparison exercise with nuclear track detectors

The response of PN3 and CR-39 personal dosemeters with different configurations, developed by the IReS (Strasbourg), the IPNO (Orsay) and the UAB (Barcelona) groups, is investigated in this study. Both dosemeters were mounted on a water-filled phantom and were simultaneously exposed under different incidence angles (0, 30 and 60) to the following: (i) three ISO neutron sources (²⁴¹Am-Be, bare ²⁵²Cf and moderated ²⁵²Cf with Cd shielding), and (ii) two realistic neutron sources (SIGMA and moderated ²⁵²Cf) at the IRSN (Cadarache) facilities. After irradiation, the plastic detectors were etched and evaluated according to local routine procedures and corrections for the effect of source-to-detector distance were taken into account. A comparison of the average background, the minimum detectable dose equivalent and the field calibration factor is performed as well.     

New results from exposures of CR-39 nuclear track detectors

Six stacks of nuclear track detectors were exposed in December 1994 to ²⁰⁷Pb⁸²⁺ ions of 158 A GeV at the CERN-SPS. Each stack was made of CR39 sheets placed after a target. The CR39 was manufactured by the Intercast Europe Co. of Parma (Italy). The exposures were carried out at normal incidence to an average density of 400 ions/cm². The main purpose of the exposures was the calibration of the CR39 nuclear track detector used in a large area detector to search for magnetic monopoles (experiment MACRO at the Gran Sasso Laboratory). We compare the response of CR39 of different production batches in different etching conditions. The results indicate no relevant aging effect for the CR39 made more than 5 years ago. The first result of a “long period” investigation of possible fading effects for the CR39 is also presented.     

Calibration of PM-355 nuclear track detectors; comparison of track diameter diagrams with track depth characteristics

The calibration diagrams, i.e. track diameters and track depths versus ion energy and etching time, as obtained for PM-355 track detector irradiated with He-ions are presented. The both detector characteristics are compared. The track etch rate is determined by two methods, as a function of the etch pit depth and the ion energy loss.     

Low-energy ion measurements by means of CR-39 nuclear track detectors

The paper presents an additional acceleration system, used to shift up an ion energy spectrum by 20 keV, and some examples of the ion parabolas registered by means of a Thomson-type spectrometer within the rod plasma injector (RPI-60) facility, designed for plasma physics and application studies. The use of the described acceleration system and CR-39 track detectors has enabled the registration of ions of energy above 20 keV to be performed. It made possible to measure the ion (e.g. deuteron) energy spectrum more exactly in the low-energy range, what is important for the determination of ion emission characteristics.     

Radon exhalation studies in building materials using solid-state nuclear track detectors

Indoor radon has been recognized as one of the health hazards for mankind. Building materials constitute the second most important source of radon in dwellings. The common building materials used in the construction of dwellings are studied for radon exhalation rate. The ‘Can’ technique using LR-115 type-II solid-state nuclear track detector has been used for these measurements. The radon exhalation rate in these samples varies from 4.75 m Bq m⁻² h⁻¹ (0.14 m Bq kg⁻¹ h⁻¹) for limestone to 506.76 m Bq m⁻² h⁻¹ (15.24 m Bq kg⁻¹ h⁻¹) for soil.