Angular distributions and anisotropy of the fragments from neutron-induced fission of <Superscript>233</Superscript>U and <Superscript>209</Superscript>Bi in the intermediate energy range of 1–200 MeV

New results of the neutron-induced fission experiments carried out at the neutron time-of-flight spectrometer GNEIS of the PNPI are given. Angular distributions of fission fragments from the neutron-induced fission of ²³³U and ²⁰⁹Bi nuclei have been measured in the energy range 1–200 MeV using position sensitive multiwire proportional counters as fission fragment detector. The recent improvements of the measurement and data processing procedures are described. The data on anisotropy of fission fragments deduced from the measured angular distributions are presented in comparison with the experimental data of other authors.     

Study of the πn → π<Superscript>{-}</Superscript>π<Superscript>{-}</Superscript>p reaction at 430 MeV energy

The total cross-section for the ^{-}n ^{-}{-}p reaction has been measured at a pion kinetic energy of 430MeV in a deuterium bubble chamber. The cross-section value was found to be 0.197±0.016mb that is much smaller than the predictions of the chiral perturbation theory. The differential spectra are compared with calculations made in the framework of the model of Bolokhov et al. 13.60.LeMeson production [:AND:]13.85.LgTotal cross-sections     

Comparison of the Effects of Different <Superscript>19</Superscript>F <Emphasis Type="Italic">π</Emphasis> Pulses on the Sensitivity and Phaseability of the <Superscript>19</Superscript>F-<Superscript>13</Superscript>C HSQC

The ¹⁹F-¹³C heteronuclear single quantum coherence (HSQC) experiment is vital for the structural elucidation of polyfluorinated organic species, yet its sensitivity and phaseability are limited by difficulties in uniform excitation of the widely disperse ¹⁹F spectral window. Adiabatic pulses of different types have previously been employed to generate effective π pulses for inversion and refocussing, but a systematic comparison of various adiabatic and other inversion pulses has not been published. In this work, it was observed that the use of a broadband inversion pulse (BIP) during the t ₁ evolution period resulted in properly phaseable spectra for experiments optimized to detect ¹ J _CF, in contrast to CHIRP or WURST adiabatic pulses. For the INEPT and reverse-INEPT transfer segments of the HSQC, optimal sensitivity for resonances distant from the transmitter frequency was afforded by optimized universal rotation (BURBOP) or CHIRP pulses. In HSQC experiments with delays optimized for two-bond correlations, only the use of BURBOP pulses in INEPT and reverse-INEPT sequences afforded spectra cleanly phaseable across the F ₂ and F ₁ spectral windows. This observation is supported by off-resonance pulsed field gradient spin-echo experiments.     

Cross sections for the photofission of <Superscript>243</Superscript>Cm, <Superscript>245</Superscript>Cm, <Superscript>249</Superscript>Bk,and <Superscript>249</Superscript>Cf isotopes in the energy range from the threshold to 10–12 MeV

The relative method was used to measure the photofission cross sections for ²⁴³Cm and ²⁴⁹Cf isotopes in the energy range from 6 to 12 MeV, for ²⁴⁵Cm in the energy range from 5 to 10 MeV, and for ²⁴⁹Bk in the energy range from 5.5 to 10 MeV. The measurements were performed with an energy step of 50 to 200 keV by using the microtron installed at the Institute of Physics and Power Engineering (Obninsk). The cross section for ²³⁸U photofission was used as a reference in these measurements. Data on the cross sections for ²⁴³Cm, ²⁴⁵Cm, and ²⁴⁹Bk photofission were obtained for the first time, while data on the cross section for ²⁴⁹Cf photofission were obtained for the first time only in the energyregion E<10 MeV. The data on the ²⁴⁵Cm nucleus suggest that, in the energy region around 6 MeV, the cross section for its photofission has a maximum, which is likely to be due to the low-energy resonance structure of the dipole-photoabsorption cross section. For ²⁴⁹Cf, an anomalously large value of the photo fission cross section is observed in the region of the first maximum of the giant dipole resonance (E≈11 MeV). By comparing the energy dependences obtained for the fissilities of the ²⁴³Cm and ²⁴⁹Bk isotopes from photofission data with the fissilities from direct-reaction data, it is found that the observed fission thresholds agree and that there is a plateau-like dependence at energies above 7.5 MeV. For the ²⁴⁵Cm and ²⁴⁹Cf nuclei, there are no similar data for performing such a comparison. Data on the fissilities as obtained from the present series of relative measurements that employ the microtron bremsstrahlung spectrum are analyzed.     

The resonance-like structure observed in the <Superscript>25</Superscript>Mg(p, γ)<Superscript>26</Superscript>Al reaction

The gamma decay of resonance-like structure (RLS) observed in the ²⁵Mg(p, γ)²⁶Al reaction in the region of excitation energies of 7–9 MeV is studied, and the excitation function of this reaction is measured. The resonance transition strengths of states in the 1.4–2.0 MeV range of accelerated proton energies are determined. The resulting strength distributions of M1 transitions between the resonance states and the low-lying bound states in ²⁶Al are of a resonance nature. The position of the center of gravity of magnetic dipole resonance for the ground state in ²⁶Al is 7.92 MeV, and the total MDR transition strength is 5.7 MeV × μ _N ² .     

Investigation of the reaction D(<Superscript>4</Superscript>He, γ)<Superscript>6</Superscript>Li at ultralow energies

The cross section of the reaction D(⁴He, γ)⁶Li with titanium and zirconium deuterides as targets is measured for incident ⁴He⁺ ion energies of 30 and 36 keV, respectively. The ion beam is generated by a Hall pulsed plasma accelerator. For the first time, upper limits on the cross section of the reaction D(⁴He, γ)⁶Li at ultralow energies are imposed (at 90% confidence level): σ ≤ 1.2 × 10^?35 cm² for the TiD₂ target and E(⁴He⁺) = 30 keV, and σ ≤ 7 × 10^?36 cm² for the ZrD₂ target and E(⁴He⁺) = 36 keV     

On the energy of the 8<Stack><Subscript>2</Subscript><Superscript>−</Superscript></Stack> 1479-keV level in <Superscript>178</Superscript>Hf

The difference in the 332-and 326-keV transition energies from ¹⁷⁸Ta decay is measured with a magnetic β spectrometer and a γ spectrometer. The energy of the 332-keV transition (E(332) = 331 607 ± 4 eV) and the energy of the 8 ₂ ^? 1479-keV level in ¹⁷⁸Hf (E(1479) = 1479001 ± 6 eV) are determined with high accuracy.     

Induction and repair of DNA double-strand breaks in rat cerebellar cortex exposed to <Superscript>60</Superscript>Co γ-rays

The induction and repair of DNA double-strand breaks are studied using the immunohistochemical staining procedure of paraffin-embedded rat cerebellum tissues after exposure to γ-rays of ⁶⁰Co. The dose dependence of radiation-induced colocalized γH2AX/53BP1 foci is studied and its linear character is established. It is shown that these foci are efficiently eliminated 24 h after irradiation.     

Angular Distributions and Anisotropy of the Fragments from Neutron-Induced Fission of <Superscript>239</Superscript>Pu and <Superscript>nat</Superscript>Pb in the Energy Range of 1–200 MeV

The angular distributions of fragments from the neutron-induced fission of ^natPb and ²³⁹Pu nuclei have been measured in the energy of range 1–200 MeV using the neutron time-of-flight spectrometer GNEIS. Fission fragments have been detected by position sensitive multiwire proportional counters. The results for the anisotropy of fission fragments deduced from the measured angular distributions have been presented. The results have been compared with the experimental data of other authors.     

Low energy α+<Superscript>16</Superscript>O scattering in the orthogonality condition model

The orthogonality condition model (OCM) is used to describe α+¹⁶O scattering at low energies. A double folding potential with density-dependent effective NN interactions is used as the local potential of the model. The energies and widths of α-cluster resonances and differential cross sections are calculated. The results are compared to one obtained using the standard potential approach, without the nonlocal interaction of the OCM.     

Radiation widths of resonances in the <Superscript>40</Superscript>Ar(pγ)<Superscript>41</Superscript>K reaction

The excitation function for the ⁴⁰Ar(pγ)⁴¹K reaction at the accelerated proton energy E _p= 450–2700 keV is studied. Positions of 168 resonances identified as levels of the ⁴¹K nucleus are observed in this energy range. The data for the proton energy E _p < 1 MeV and E _p > 2 MeV are obtained for the first time. Relative yields of γ rays observed in the decay of the resonances are calculated from a comparison with the yield of the calibrating resonance at E _p= 1102 keV. Total radiation widths of the resonances are calculated on the basis of the data obtained.     

Emission of γ-quanta,electrons, and positrons upon the decay of <Superscript>12</Superscript>N and <Superscript>12</Superscript>B produced in characteristic targets

The emission of γ-quanta, electrons, and positrons upon the decay of ¹²N and ¹²B produced in characteristic targets is calculated within radiation–matter interaction models generated using the GEANT and MCNP simulation software.     

Measurement of the cross section for the reaction <Superscript>20</Superscript>Ne(<Emphasis Type="Italic">n,α</Emphasis>)<Superscript>17</Superscript>O in the neutron-energy between 4 and 7 MeV

The cross section for the reaction ²⁰Ne(n, α)¹⁷O was measured in the neutron-energy range 4–7 MeV. An ionization chamber equipped with a Frisch grid combined with a pulse-shape digitizer was used as a detector. Gaseous neon that served as a target on which the reaction being studied proceeded was added to the gas filling the ionization chamber. The partial cross sections for the α ₀, α ₁, α ₂, and α ₃ channels of the reaction ²⁰Ne(n, α)¹⁷O were obtained for the first time.     

Narrow α + <Superscript>28</Superscript>Si elastic-scattering states at high excitation in <Superscript>32</Superscript>S

The excitation function and angular distributions of elastic α-particle scattering on ²⁸Si have been measured in the laboratory energy range 6-28 MeV using a backscattering technique on a thick target, yielding a continuous energy distribution. More than 200 narrow states are observed, with widths in the range ∼ 30-100 keV at excitation energies E ^* = 13-32 MeV. Angular distributions at backward angles were measured, and angular momentum values of more than 83 states have been deduced. The analysis gives spin-parities J ^π, α-partial widths Γ_α and reduced widths of the narrow high-lying resonant states in ³²S. The experimentally observed states display both the negative- and the positive-parity rotational-like sequences with seemingly no parity splitting, a finding which is at variance with most potential-model predictions. The deduced effective moment of inertia indicates a more extended structure than the ground-state configuration. The observed strength of each ℓ-value is analyzed in terms of an underlying split doorway state of Lorentzian form, which yields an interpretation as fragmented rotational α + ²⁸Si states. Received: 26 June 2000 / Accepted: 16 September 2002 / Published online: 4 February 2003 RID="a" ID="a"e-mail: kkallman@abo.fi RID="b" ID="b"Present address: Swedish Polytechnic, FIN-65200 Vasa, Finland. Communicated by D. Guerreau     

Potential energy of <Superscript>∞</Superscript>H<Stack><Subscript>2</Subscript><Superscript>-</Superscript></Stack>(<Superscript>2</Superscript>∑<Stack><Subscript>u</Subscript><Superscript>+</Superscript></Stack> in the bound-state region

An accurate calculation of the lowest negative electronic state of H ₂ ^- (fixed nuclei) is reported using the CCSD(T) method and doubly augmented cc-pv5z basis set. Comparison has been made with the reference data by Senekowitsch et al. [Chem. Phys. Lett. 111 (1984) 211]. Owing to larger size of the basisset and inclusion of triple excitations, no vertical shift in this work is necessary to reproduce the asymptotics of H + H ^-. In addition, the effect of basis-set truncation is estimated, based on the complete-basis-set extrapolation method. The contribution of correlated electron-proton motion to the electron-energy curve for H₂ ^– dynamics is pointed out.Dedicated to Prof. Jií Horáek on the occasion of his 60th birthday.     

Stereodynamics of the reaction He+H<Stack><Subscript>2</Subscript><Superscript>+</Superscript></Stack> → HeH<Superscript>+</Superscript> + H: a theoretical study

Quasiclassical trajectory method for the title reaction He +H₂⁺ → HeH⁺ + H was carried out on the potential energy surface which was revised by Aquilanti et al. [Chem. Phys. Lett. 469, 26 (2009)]. The initial vibrational quantum number of reactant was set as v=1, v=2 and v=3. Stereodynamics information of the reaction was obtained, such as the distributions of product angular momentum P(θ _r ), P(ϕ _r ),p(ϕ _r , θ _r ) and the two commonly used polarization-dependent differential cross sections (PDDCSs) (2π/σ)(dσ ₀₀/dω _t ) and (2π/σ)(dσ ₂₀/dω _t ), to get the alignment and orientation of product molecules. The results show that the influence of both the collision energy and vibrational quantum number (v) to the reaction are highly sensitive.     

Role of various mechanisms in the formation of a <Superscript>12</Superscript>C nucleus in the reaction <Superscript>13</Superscript>C(<Superscript>3</Superscript>He, <Emphasis Type="Italic">α</Emphasis>)<Superscript>12</Superscript>C

The contributions of various mechanisms to the production of the final nucleus ¹²C in the reaction ¹³C(³He, α)¹²C are estimated. These are neutron stripping and the transfer of the heavy cluster ⁹Be in the pole approximation or via a sequential transfer of virtual ⁸Be and a neutron. It is shown that the sequential mechanism of heavy-cluster transfer must be taken into account in order to describe correctly experimental data over the whole angular range.     

Investigation of the influence of incomplete fusion on complete fusion of <Superscript>12</Superscript>C-induced reactions at ≈ 4–7.2 MeV/nucleon

In this paper, we present the results of our investigation of reaction dynamics leading to incomplete fusion of heavy ions at moderate excitation energies, especially the influence of incomplete fusion on complete fusion of ¹²C -induced reactions at specific energies ≈ 4–7.2M eV/nucleon. Excitation functions of various reaction products populated via complete and/or incomplete fusions of a ¹²C projectile with ⁹³Nb, ⁵⁹Co and ⁵²Cr targets were measured at several specific energies ≈ 4–7.2 MeV/nucleon, using a recoil catcher technique, followed by off-line γ-ray spectrometry. The measured excitation functions were compared with theoretical values obtained using the PACE4 statistical model code. For representative non-α-emitting channels in the ¹²C + ⁹³Nb system, the experimentally measured excitation functions were, in general, found to be in good agreement with the theoretical predictions. However, for α-emitting channels in the ¹²C + ⁹³Nb, ¹²C + ⁵⁹Co, and ¹²C + ⁵²Cr systems, the measured excitation functions were higher than the predictions of the theoretical model code, which may be credited to incomplete fusion reactions at these energies. An attempt was made to estimate the incomplete fusion fraction for the present systems, which revealed that the fraction was sensitive to the projectile energy and mass asymmetry of the entrance channel.     

Study of the energy spectrum and mass composition of primary cosmic rays in the energy range of 10<Superscript>18</Superscript>–10<Superscript>20</Superscript> eV using a balloon setup in antarctica (SPHERE-antarctica project)

An Antarctic balloon experiment for measuring the energy spectrum and elemental composition of cosmic rays in the ultrahigh-energy range (10¹⁸–10²⁰) eV is proposed. Scientific equipment will measure fluorescence caused by an extensive air shower formed in the atmosphere by an ultrahigh energy particle and Cherenkov light of this shower reflected from a snow surface. It is assumed that the balloon will fly in the circumpolar orbit in Antarctica at a height of ~25 km for (2–3) winter (in the Southern Hemisphere)months. For this time, ~3000 events caused by particles with energies above 10¹⁸ eV and (200–300) events caused by particles with energies above 10¹⁹ eV will be detected.     

(EC + β<Superscript>+</Superscript>) decays of the 11/2<Superscript>-</Superscript> isomer and 1/2<Superscript>+</Superscript> ground state of <Superscript>143</Superscript>Dy

The 1/2⁺ ground state and a 11/2^- isomer of very neutron-deficient isotope ¹⁴³Dy were produced by irradiation of an enriched target of ¹⁰⁶Cd with ⁴⁰Ca and studied by using a helium-jet fast tape-transport system in combination with proton-γ, X-γ and γ-γ coincidence measurements. A simple ( EC + β⁺) decay scheme of ^143mDy with a half-life of 3.0(3) s and a tentative ( EC + β⁺) decay scheme of ^143gDy with a half-life of 5.6(10) s are proposed. As a by-product, the 347- and 545-keV γ transitions in ¹³⁸Sm following the β-delayed proton emission of ¹³⁹Gd decay and the 323-keV γ transition in ¹³⁹Eu following the β-delayed proton emission of ¹⁴⁰Tb decay could be observed for the first time. Received: 20 August 2002 / Accepted: 28 October 2002 / Published online: 11 February 2003 RID="a" ID="a"e-mail: xsw@ns.lzb.ac.cn Communicated by D. Schwalm