Velocity tuned resonances as multi-doppleron processes

We consider multi-photon processes for a Doppler broadened two-level system. Alternative absorption and emission from two oppositely travelling waves is interpreted as a multi-quantum absorption (or emission) process with quanta $\text{h}\text{?}$kv. These are called Dopplerons and the analogy with the RF work is established. The calculations also display a resonance caused by slow atoms.     

Angular resonances in the light emission from atoms near a grating

A two step light emission process becomes possible when atoms are placed near a metallic grating. The atoms can excite surface plasmons in the grating. The surface plasmons can then emit light. This light is emitted at certain angles determined by momentum conservation in the plane of the grating. Thus, the angles depend on the spacing of the grating. Our measurements on light from nitrogen atoms at distances, d, ranging from 10 to 100 nm from a silver grating are in agreement with a recent theory of Aravind, Hood and Metiu. We also report the effect of a nonsinusoidal grating profile and the emission of light at angles which can be predicted from a straightforward extension of the theory.     

Influence of cesium atoms on the field electron emission from multi-walled carbon nanotubes

It has been shown that the deposition of cesium atoms on multi-wall carbon nanotubes abruptly increases the current of the field electron emission, decreases the threshold electric field by a factor of three (to 0.8 V/m), and decreases the work function to 2.1–2.3 eV. It has been found that the flowing of the large emission current I ≥ 2 × 10^?6 A leads to a change in the current-voltage characteristics and a decrease in the emission current. This effect has been explained by escape of cesium atoms from the tips of most nanotubes into the nanotube depth due to desorption or intercalation. At the same time, the low work function is retained for some nanotubes, probably, due to the stronger bonding of Cs atoms with these nanotubes.     

Influence of the symmetry on the circular dichroism in angular resolved core-level photoemission

The model for angular resolved photoemission from adsorbed atoms is extended to account for the non-axial symmetry of atoms in a crystal field. In particular, circular dichroism in the angular distribution (CDAD) is theoretically investigated. A special emphasis is put on the case when incident photons are propagating along the principal axis of an atom in C_nv symmetry. The model, although mainly developed for adsorbates, may also be used as a base for emission from solid surfaces. An extension to simple bulk symmetries, like D_6h for hexagonal or O_h for cubic crystals, is included. The CDAD for normal incidence does not vanish in the extended model and reflects the symmetry of the adsorption site. Scattering induced final state effects are discussed for alkali metal adsorption. A numerical calculation of the emission from the shallow 4p core level of Rb atoms adsorbed in a (√3×√3)−R30° structure on a Pt(111) surface is presented. In this case even the extended photoemission model predicts the absence of CDAD. The appearance of CDAD is only possible due to the scattering of photoelectrons from the neighbouring atoms of the solid.     

Robust scheme to generate N-atom W state in two distant cavities

We propose a scheme to realize W states for N-atoms trapped in two distant cavities connected by an optical fiber. In the scheme, the cavity modes and fiber mode are not excited during the process. The quantum information is encoded in two degenerate ground states, so the atom's spontaneous emission can be omitted approximately. Moreover, the operation speed increases with the number of the atoms without a limitation and thus the scheme is extremely robust against decoherence.     

Quantum gate operation with non-instantaneous unitary kicks

A two-qubit controlled-z gate is presented based on the non-instantaneous unitary kicks. Instead of putting two atoms through the cavity simultaneously, we make the atoms cross the cavity sequentially. The interaction between the second atom and the cavity plays the role for kicking the evolution of the system consisting of the first atom and cavity. By repeating the whole process N times, we obtain the controlled-z gate with a high fidelity. The effects of decoherence such as spontaneous emission and the loss of cavity on the average gate fidelity are investigated in virtue of master equation. Furthermore the method for achieving the multi-qubit controlled-z gate is also proposed.     

Cooperative effects in the two atom resonance fluorescence spectrum

We consider the resonance fluorescence spectrum of two similar interacting atoms in the limit of high photon densities. The excitation spectrum of the symmetric modes contains two sidebands in addition to the usual three peaks which are analogous to those of the isolated atom. These two new sidebands are due entirely to the cooperative behaviour of the two atoms and vanish when the atoms are far apart. The energy shifts and spectral widths for these two sidebands are two and five times larger than those for the isolated atom respectively. The probability of occurrence of these sidebands depends on the parameters V_AB/Ω and γ²₀/Ω², where V_AB is the dipole-dipole interaction energy, γ₀ is the spontaneous emission probability and Ω is the Rabi frequency. The asymmetric broadening of both sidebands depends on the parameter γ₀/Ω. The possibility to measure the dipole-dipole energy through the observation of these sidebands is discussed.     

X-ray absorption and emission spectroscopy at the Hf L1 edge of hafnium-(silicon)-oxide ultra-thin films

X-ray absorption and emission spectroscopic study at the Hf L₁ edge was applied to investigate the local structure around hafnium atoms in Hf(Si)O_x ultra-thin films, which are the most promising candidates for the high-k gate dielectric material of next generation CMOS devices. HfSiO_x showed an extra absorption above the Hf-L₁ threshold, which is not seen in HfO_x. HfSiO_x also had stronger Compton scattering peak in Hf-Lγ emission region, and smaller Hf-Lγ₂/Lγ₃ ratio, compared with those of HfO_x. These differences should be caused by partial replacements of hafnium atoms by silicon atoms as the second nearest neighbors of a hafnium atom.     

Time-dependent directionality of cooperative emission after short pulse excitation

Cooperative emission from a sphere of N two-level atoms excited by a short pulse is shown to have a time-dependent angular distribution, with the possibility of reversal in the dominant direction of emission. This is a result of the different values of the frequency shifts and decay rates associated with the various collective eigenmodes of the atomic system obtained in a scalar photon model.     

Tripartite entanglement of atoms trapped in coupled cavities via quantum Zeno dynamics

A scheme is proposed for the generation of a W state for three atoms trapped in spatially separated cavities connected by optical fibers via quantum Zeno dynamics. Our scheme is based on the resulting effective dynamics induced by continuous coupling between the atoms and cavities. The effects of decoherence such as atomic spontaneous emission and the fiber and cavity losses are considered. Numerical results show that the scheme is very robust against the cavity decay due to a tiny excitation probability of the cavity fields during the operation.     

Effect of the optical orientation of spin angular momenta of sodium atoms in the 32 S 1/2 state and metastable helium atoms in the 23 S 1 state on the Na-He gas-discharge plasma conduction

The observation of the effect of mutual orientation of spin angular momenta of sodium atoms in the 3² S _1/2 state and helium atoms in the 2³ S ₁ state on the electrical conduction of a Na-He gas-discharge plasma is reported. In the experiments, a simultaneous optical orientation of atoms by the optical emission of sodium and helium lamps was carried out. The influence of the mutual orientation on the conduction was observed as a change in the high-frequency voltage across electrodes of a gas-discharge camera caused by the destruction of orientation of sodium atoms. The effect is explained by the dependence of Penning ionization in the interaction of sodium and helium atoms on the mutual orientation of spin angular momenta of partners.     

Shifts of X-ray characteristic L lines of free atoms of rare-earth metals

Results of the study of X-ray characteristic spectra of free atoms of a number of rare-earth metals from Ce to Ho are reported. L _α1 and L _β1 lines were studied, and the shifts of the peaks of emission lines of free atoms relative to their positions in the case of emission by the solid aggregate state were measured. The data obtained enable one to use the corresponding X-ray characteristic lines as references with the accuracy Δλ/λ≈10^?5. The Z-dependences of shifts are plotted.     

Experimental and theoretical radiative properties of odd-parity highly excited levels in Mo II

Investigations are made for the collective spontaneous emission of a Bose-Einstein condensate consisting of N two-level atoms when s atoms are initially excited in a multi-photon q-deformed Dicke model. The model is based on the generalized deformed oscillator algebra in which the field radiation operators are deformed by an operator-valued function $f\left( {\hat n} \right)$ of the photon number operator $\hat n$ . The time evolution of the expectation value of the atomic inversion is calculated for s = 1, s = 2 and s = 3. When s = 3 its spectra are characterized by nonequidistant eigenvalues, and the phenomenon of the quantum collapse and revival is demonstrated. In particular, the influences of photon multiplicity and q-deformation on the spontaneous emission of the system are discussed. The results show that the nonlinearities due to the photon multiplicity and q-deformation may lead to the inhibition of collective spontaneous emission.     

X-ray emission and X-ray photoelectron spectroscopic studies of fullerene fluoride C<Subscript>60</Subscript>F<Subscript>24</Subscript>

The structure of the fullerence fluoride C₆₀F₂₄ of the T _h symmetry contains two types of chemically different carbon atoms, namely, atoms of isolated double bonds and atoms of CF groups. X-ray photoelectron and x-ray emission spectroscopic studies of C₆₀F₂₄ revealed a difference in the widths of the x-ray bands corresponding to these types of atoms. Nonempirical quantum-chemical calculations performed for C₅₉NF ₂₄ ⁺ ions with a hole in the C 1s core level of the fullerence fluoride showed that the difference in the bandwidths may be due to the fact that the vibrational states of the system are different when 1s electrons are removed from chemically nonequivalent atoms.     

两个双能级原子与双模腔场的拉曼相互作用

研究了两个双能级原子与双模辐射腔场的拉曼相互作用，计算了两个原子与腔场具有相同耦合常数但同时考虑原子间偶极一偶极相互作用情形下的辐射谱．讨论了双模腔场处于不同数态时辐射谱的新特点．     

Coherence-controlled stationary entanglement between two atoms embedded in a bad cavity injected with squeezed vacuum

We investigate the entanglement between two atoms in an overdamped cavity injected with squeezed vacuum when these two atoms are initially prepared in coherent states. It is shown that the stationary entanglement exhibits a strong dependence on the initial state of the two atoms when the spontaneous emission rate of each atom is equal to the collective spontaneous emission rate, corresponding to the case where the two atoms are close together. It is found that the stationary entanglement of two atoms increases with decreasing effective atomic cooperativity parameter. The squeezed vacuum can enhance the entanglement of two atoms when the atoms are initially in coherent states. Valuably, this provides us with a feasible way to manipulate and control the entanglement, by changing the relative phases and the amplitudes of the polarized atoms and by varying the effective atomic cooperativity parameter of the system, even though the cavity is a bad one. When the spontaneous emission rate of each atom is not equal to the collective spontaneous emission rate, the steady-state entanglement of two atoms always maintains the same value, as the amplitudes of the polarized atoms varies. Moreover, the larger the degree of two-photon correlation, the stronger the steady-state entanglement between the atoms.     

The temperature distributions of the electrons,atoms and ions in aerodynamic radiative transfer

The time-dependent individual specie equations specifying conservation of mass, energy and linear momentum for electrons, atoms and ions are solved, together with the transfer equation for continuum radiation, for several specific situations. We assume the temperature of the atoms and ions to be equal, but different to the electron temperature. An ionising disturbance is propagated through a physically idealistic radiating medium and it is shown that the time-development of the differences in temperature distributions are such as to sufficiently affect the absorption and emission properties of the gas, and thus, the emergent flux intensities.     

Dipole emission of a nanostructure system composed of two atoms and dimensional resonances

A stationary solution is obtained for the joint system of equations for atomic and field variables for two different atoms with dipole-dipole interaction in the radiation field taking into account the common radiative friction. The atoms are treated as an Lorentz oscillator with one isolated resonance. The interaction of atoms in the radiation field forms four dimensional resonances at frequencies that are substantially different from the natural frequencies of isolated atoms. Two of the four dimensional resonances are characterized by negative dispersion, and the intensity of dipole emission at these frequencies may be increased with respect to the intensity of emission at the frequencies of natural atomic resonances by a factor of about 10¹².     

Field emission properties of linear carbon clusters

The field emission of linear carbon clusters in a constant electric field is studied both numerically and analytically. It is found that for fields of the order of 0.6 V/Å, a chain of 10 carbon atoms can yield currents as large as aμA. Such an ‘electron gun’ is expected to be highly monoenergetic.     

Hydrogen passivation effect on the yellow-green emission band and bound exciton in n - ZnO

Photoluminescence (PL) measurements performed on as-grown, hydrogenated, and annealed n-type ZnO bulk samples investigated the origins of their yellow (2.10 eV) and green (2.43 eV) emission bands. After hydrogenation, the defect-related peak at 2.10 eV was no longer present in the room temperature PL spectrum, the peak intensity at 2.43 eV was unchanged, and the intensity of the emission peak at 3.27 eV increased significantly. These results indicate that yellow band emission is due to oxygen vacancies, as the emission peak at 2.10 eV disappears when hydrogen atoms passivate these vacancies. The emission peak at 2.43 eV originates from complexes between oxygen vacancies and other crystal defects. We discuss the shallow donor impurities arising due to these hydrogen atoms in the ZnO bulk sample.